Articles | Volume 20, issue 12
https://doi.org/10.5194/acp-20-7531-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-7531-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
30 Jun 2020
Research article |
| 30 Jun 2020
| 30 Jun 2020
Strong anthropogenic control of secondary organic aerosol formation from isoprene in Beijing
Daniel J. Bryant
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
William J. Dixon
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
James R. Hopkins
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
National Centre for Atmospheric Science, University of York, York, UK
Rachel E. Dunmore
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
Kelly L. Pereira
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
Marvin Shaw
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
National Centre for Atmospheric Science, University of York, York, UK
Freya A. Squires
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
Thomas J. Bannan
School of Earth and Environmental Sciences, The University of
Manchester, Manchester, UK
Archit Mehra
School of Earth and Environmental Sciences, The University of
Manchester, Manchester, UK
Stephen D. Worrall
School of Earth and Environmental Sciences, The University of
Manchester, Manchester, UK
now at: Chemical Engineering and Applied Chemistry, School of
Engineering and Applied Science, Aston University, Birmingham, UK
Asan Bacak
School of Earth and Environmental Sciences, The University of
Manchester, Manchester, UK
now at: Turkish Accelerator and Radiation Laboratory, Ankara University
Institute of Accelerator Technologies, Ankara, Turkey
School of Earth and Environmental Sciences, The University of
Manchester, Manchester, UK
Carl J. Percival
School of Earth and Environmental Sciences, The University of
Manchester, Manchester, UK
now at: Jet Propulsion Laboratory, California Institute of
Technology, 4800 Oak Grove Drive, Pasadena, CA, USA
Lisa K. Whalley
School of Chemistry, University of Leeds, Leeds, UK
National Centre for Atmospheric Science, University of Leeds, Leeds,
UK
Dwayne E. Heard
School of Chemistry, University of Leeds, Leeds, UK
Eloise J. Slater
School of Chemistry, University of Leeds, Leeds, UK
Bin Ouyang
Lancaster Environment Centre, Lancaster University, Lancaster, UK
Department of Chemistry, University of Cambridge, Cambridge, UK
Tianqu Cui
Department of Environmental Sciences and Engineering, Gillings School
of Global Health, University of North Carolina, Chapel Hill, USA
now at: Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
5232 Villigen, Switzerland
Jason D. Surratt
Department of Environmental Sciences and Engineering, Gillings School
of Global Health, University of North Carolina, Chapel Hill, USA
Di Liu
School of Geography, Earth and Environmental Sciences, the University
of Birmingham, Birmingham, UK
now at: State Key Laboratory of Organic Geochemistry and Guangdong
Provincial Key Laboratory of Environmental Protection and Resources
Utilization, Guangzhou Institute of Geochemistry, Chinese Academy of
Sciences, Guangzhou 510640, PR China
Zongbo Shi
School of Geography, Earth and Environmental Sciences, the University
of Birmingham, Birmingham, UK
Institute of Surface-Earth System Science, Tianjin University,
Tianjin, China
Roy Harrison
School of Geography, Earth and Environmental Sciences, the University
of Birmingham, Birmingham, UK
Yele Sun
Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, PR China
Weiqi Xu
Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, PR China
Alastair C. Lewis
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
National Centre for Atmospheric Science, University of York, York, UK
James D. Lee
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
National Centre for Atmospheric Science, University of York, York, UK
Andrew R. Rickard
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
National Centre for Atmospheric Science, University of York, York, UK
Jacqueline F. Hamilton
CORRESPONDING AUTHOR
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry,
University of York, York, UK
Data sets
Dataset for "Strong anthropogenic control of Isoprene SOA" J. Hamilton and D. Bryant https://doi.org/10.15124/7c1a54dd-ce72-4b1a-bed1-812cf25bc407
Short summary
Using the chemical composition of offline filter samples, we report that a large share of oxidized organic aerosol in Beijing during summer is due to isoprene secondary organic aerosol (iSOA). iSOA organosulfates showed a strong correlation with the product of ozone and particulate sulfate. This highlights the role of both photochemistry and the availability of particulate sulfate in heterogeneous reactions and further demonstrates that iSOA formation is controlled by anthropogenic emissions.
Using the chemical composition of offline filter samples, we report that a large share of...
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