Articles | Volume 20, issue 10
https://doi.org/10.5194/acp-20-6037-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-6037-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 May 2020
Research article |
| 25 May 2020
| 25 May 2020
Solar UV radiation measurements in Marambio, Antarctica, during years 2017–2019
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
Tartu Observatory, University of Tartu, Tõravere, Estonia
Kaisa Lakkala
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
Space and Earth Observation Centre, Finnish Meteorological Institute, Sodankylä, Finland
Ricardo Sanchez
Servicio Meteorológico Nacional, Buenos Aires, Argentina
Eija Asmi
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
Servicio Meteorológico Nacional, Buenos Aires, Argentina
Fernando Nollas
Servicio Meteorológico Nacional, Buenos Aires, Argentina
Outi Meinander
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
Larisa Sogacheva
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
Veerle De Bock
Royal Meteorological Institute of Belgium, Brussels, Belgium
Antti Arola
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
Gerrit de Leeuw
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
currently at: R&D Satellite Observations, Royal Netherlands Meteorological Institute (KNMI), De Bilt, the Netherlands
Veijo Aaltonen
Climate Research Programme, Finnish Meteorological Institute, Helsinki, Finland
David Bolsée
Royal Belgian Institute for Space Aeronomy, Brussels, Belgium
Klara Cizkova
Solar and Ozone Observatory, Czech Hydrometeorological Institute, Hradec Králové, Czech Republic
Institute of Geography, Masaryk University, Brno, Czech Republic
Alexander Mangold
Royal Meteorological Institute of Belgium, Brussels, Belgium
Ladislav Metelka
Solar and Ozone Observatory, Czech Hydrometeorological Institute, Hradec Králové, Czech Republic
Erko Jakobson
Tartu Observatory, University of Tartu, Tõravere, Estonia
Tove Svendby
NILU – Norwegian Institute for Air Research, Kjeller, Norway
Didier Gillotay
Royal Belgian Institute for Space Aeronomy, Brussels, Belgium
Bert Van Opstal
Royal Belgian Institute for Space Aeronomy, Brussels, Belgium
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Antti Lipponen, Jaakko Reinvall, Arttu Väisänen, Henri Taskinen, Timo Lähivaara, Larisa Sogacheva, Pekka Kolmonen, Kari Lehtinen, Antti Arola, and Ville Kolehmainen
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Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-26, https://doi.org/10.5194/amt-2022-26, 2022
Publication in AMT not foreseen
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Aeolus is the first satellite mission to directly observe wind profile information on a global scale. However, Aeolus wind products over China were thus far not evaluated by in-situ comparison. This work is the comparison of wind speed on a large scale between the Aeolus, ERA5 and RS , shedding important light on the data application of Aeolus wind products.
Jutta Kesti, John Backman, Ewan J. O'Connor, Anne Hirsikko, Eija Asmi, Minna Aurela, Ulla Makkonen, Maria Filioglou, Mika Komppula, Hannele Korhonen, and Heikki Lihavainen
Atmos. Chem. Phys., 22, 481–503, https://doi.org/10.5194/acp-22-481-2022, https://doi.org/10.5194/acp-22-481-2022, 2022
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In this study we combined aerosol particle measurements at the surface with a scanning Doppler lidar providing vertical profiles of the atmosphere to study the effect of different boundary layer conditions on aerosol particle properties in the understudied Arabian Peninsula region. The instrumentation used in this study enabled us to identify periods when pollution from remote sources was mixed down to the surface and initiated new particle formation in the growing boundary layer.
Anu Kauppi, Antti Kukkurainen, Antti Lipponen, Marko Laine, Antti Arola, Hannakaisa Lindqvist, and Johanna Tamminen
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-328, https://doi.org/10.5194/amt-2021-328, 2021
Revised manuscript not accepted
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We present a methodology in Bayesian framework for retrieving atmospheric aerosol optical depth and aerosol type from the pre-computed look-up tables (LUTs). Especially, we consider Bayesian model averaging and uncertainty originating from aerosol model selection and imperfect forward modelling. Our aim is to get more realistic uncertainty estimates. We have applied the methodology to TROPOMI/S5P satellite observations and evaluated the results against ground-based data from the AERONET.
Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Konstantinos Eleftheriadis, Stergios Vratolis, Radovan Krejci, Paul Zieger, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Yutaka Tobo, Junji Matsushita, and Naga Oshima
Atmos. Meas. Tech., 14, 6723–6748, https://doi.org/10.5194/amt-14-6723-2021, https://doi.org/10.5194/amt-14-6723-2021, 2021
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Reliable values of mass absorption cross sections (MACs) of black carbon (BC) are required to determine mass concentrations of BC at Arctic sites using different types of filter-based absorption photometers. We successfully estimated MAC values for these instruments through comparison with independent measurements of BC by a continuous soot monitoring system called COSMOS. These MAC values are consistent with each other and applicable to study spatial and temporal variation in BC in the Arctic.
Xiaoxia Shang, Tero Mielonen, Antti Lipponen, Elina Giannakaki, Ari Leskinen, Virginie Buchard, Anton S. Darmenov, Antti Kukkurainen, Antti Arola, Ewan O'Connor, Anne Hirsikko, and Mika Komppula
Atmos. Meas. Tech., 14, 6159–6179, https://doi.org/10.5194/amt-14-6159-2021, https://doi.org/10.5194/amt-14-6159-2021, 2021
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The long-range-transported smoke particles from a Canadian wildfire event were observed with a multi-wavelength Raman polarization lidar and a ceilometer over Kuopio, Finland, in June 2019. The optical properties and the mass concentration estimations were reported for such aged smoke aerosols over northern Europe.
Kevin Lamy, Thierry Portafaix, Colette Brogniez, Kaisa Lakkala, Mikko R. A. Pitkänen, Antti Arola, Jean-Baptiste Forestier, Vincent Amelie, Mohamed Abdoulwahab Toihir, and Solofoarisoa Rakotoniaina
Earth Syst. Sci. Data, 13, 4275–4301, https://doi.org/10.5194/essd-13-4275-2021, https://doi.org/10.5194/essd-13-4275-2021, 2021
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This paper is about the presentation of the UV-Indien measurement network. This network measures the ultraviolet radiation emitted by the Sun received at the Earth's surface and the clouding above each station. It has been deployed at several sites in the Indian Ocean region representing different environmental conditions. A description of the instruments and their calibration, maintenance, and data processing is presented in this paper along with a valuation of the data quality.
Panagiotis G. Kosmopoulos, Stelios Kazadzis, Alois W. Schmalwieser, Panagiotis I. Raptis, Kyriakoula Papachristopoulou, Ilias Fountoulakis, Akriti Masoom, Alkiviadis F. Bais, Julia Bilbao, Mario Blumthaler, Axel Kreuter, Anna Maria Siani, Kostas Eleftheratos, Chrysanthi Topaloglou, Julian Gröbner, Bjørn Johnsen, Tove M. Svendby, Jose Manuel Vilaplana, Lionel Doppler, Ann R. Webb, Marina Khazova, Hugo De Backer, Anu Heikkilä, Kaisa Lakkala, Janusz Jaroslawski, Charikleia Meleti, Henri Diémoz, Gregor Hülsen, Barbara Klotz, John Rimmer, and Charalampos Kontoes
Atmos. Meas. Tech., 14, 5657–5699, https://doi.org/10.5194/amt-14-5657-2021, https://doi.org/10.5194/amt-14-5657-2021, 2021
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Large-scale retrievals of the ultraviolet index (UVI) in real time by exploiting the modern Earth observation data and techniques are capable of forming operational early warning systems that raise awareness among citizens of the health implications of high UVI doses. In this direction a novel UVI operating system, the so-called UVIOS, was introduced for massive outputs, while its performance was tested against ground-based measurements revealing a dependence on the input quality and resolution.
Yuqin Liu, Tao Lin, Juan Hong, Yonghong Wang, Lamei Shi, Yiyi Huang, Xian Wu, Hao Zhou, Jiahua Zhang, and Gerrit de Leeuw
Atmos. Chem. Phys., 21, 12331–12358, https://doi.org/10.5194/acp-21-12331-2021, https://doi.org/10.5194/acp-21-12331-2021, 2021
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The four-dimensional variation of aerosol properties over the BTH, YRD and PRD (east China) were investigated using satellite observations from 2007 to 2020. Distinct differences between the aerosol optical depth and vertical distribution of the occurrence of aerosol types over these regions depend on season, aerosol loading and meteorological conditions. Day–night differences between the vertical distribution of aerosol types suggest effects of boundary layer dynamics and aerosol transport.
Eija Asmi, John Backman, Henri Servomaa, Aki Virkkula, Maria I. Gini, Konstantinos Eleftheriadis, Thomas Müller, Sho Ohata, Yutaka Kondo, and Antti Hyvärinen
Atmos. Meas. Tech., 14, 5397–5413, https://doi.org/10.5194/amt-14-5397-2021, https://doi.org/10.5194/amt-14-5397-2021, 2021
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Absorbing aerosols are warming the planet and accurate measurements of their concentrations in pristine environments are needed. We applied eight different absorbing-aerosol measurement methods in a field campaign at the Arctic Pallas station. The filter-based techniques were found to be the most sensitive to detect the minuscule amounts of black carbon present, showing a 40 % agreement between them. Our results help to reduce uncertainties in absorbing aerosol measurements.
Antti Arola, William Wandji Nyamsi, Antti Lipponen, Stelios Kazadzis, Nickolay A. Krotkov, and Johanna Tamminen
Atmos. Meas. Tech., 14, 4947–4957, https://doi.org/10.5194/amt-14-4947-2021, https://doi.org/10.5194/amt-14-4947-2021, 2021
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Methods to estimate surface UV radiation from satellite measurements offer the only means to obtain global coverage, and the development of satellite-based UV algorithms has been ongoing since the early 1990s. One of the main challenges in this development has been how to account for the overall effect of absorption by atmospheric aerosols. One such method was suggested roughly a decade ago, and in this study we propose further improvements for this kind of approach.
Evelyn Freney, Karine Sellegri, Alessia Nicosia, Leah R. Williams, Matteo Rinaldi, Jonathan T. Trueblood, André S. H. Prévôt, Melilotus Thyssen, Gérald Grégori, Nils Haëntjens, Julie Dinasquet, Ingrid Obernosterer, France Van Wambeke, Anja Engel, Birthe Zäncker, Karine Desboeufs, Eija Asmi, Hilkka Timonen, and Cécile Guieu
Atmos. Chem. Phys., 21, 10625–10641, https://doi.org/10.5194/acp-21-10625-2021, https://doi.org/10.5194/acp-21-10625-2021, 2021
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In this work, we present observations of the organic aerosol content in primary sea spray aerosols (SSAs) continuously generated along a 5-week cruise in the Mediterranean. This information is combined with seawater biogeochemical properties also measured continuously along the ship track to develop a number of parametrizations that can be used in models to determine SSA organic content in oligotrophic waters that represent 60 % of the oceans from commonly measured seawater variables.
Tove M. Svendby, Bjørn Johnsen, Arve Kylling, Arne Dahlback, Germar H. Bernhard, Georg H. Hansen, Boyan Petkov, and Vito Vitale
Atmos. Chem. Phys., 21, 7881–7899, https://doi.org/10.5194/acp-21-7881-2021, https://doi.org/10.5194/acp-21-7881-2021, 2021
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Measurements of total ozone and effective cloud transmittance (eCLT) have been performed since 1995 at three Norwegian sites with GUV multi-filter instruments. The unique data sets of high-time-resolution measurements can be used for a broad range of studies. Data analyses reveal an increase in total ozone above Norway from 1995 to 2019. Measurements of GUV eCLT indicate changes in albedo in Ny-Ålesund (Svalbard) during the past 25 years, most likely resulting from increased Arctic ice melt.
Cheng Fan, Zhengqiang Li, Ying Li, Jiantao Dong, Ronald van der A, and Gerrit de Leeuw
Atmos. Chem. Phys., 21, 7723–7748, https://doi.org/10.5194/acp-21-7723-2021, https://doi.org/10.5194/acp-21-7723-2021, 2021
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Emission control policy in China has resulted in the decrease of nitrogen dioxide concentrations, which however leveled off and stabilized in recent years, as shown from satellite data. The effects of the further emission reduction during the COVID-19 lockdown in 2020 resulted in an initial improvement of air quality, which, however, was offset by chemical and meteorological effects. The study shows the regional dependence over east China, and results have a wider application than China only.
Nick Schutgens, Oleg Dubovik, Otto Hasekamp, Omar Torres, Hiren Jethva, Peter J. T. Leonard, Pavel Litvinov, Jens Redemann, Yohei Shinozuka, Gerrit de Leeuw, Stefan Kinne, Thomas Popp, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 21, 6895–6917, https://doi.org/10.5194/acp-21-6895-2021, https://doi.org/10.5194/acp-21-6895-2021, 2021
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Absorptive aerosol has a potentially large impact on climate change. We evaluate and intercompare four global satellite datasets of absorptive aerosol optical depth (AAOD) and single-scattering albedo (SSA). We show that these datasets show reasonable correlations with the AErosol RObotic NETwork (AERONET) reference, although significant biases remain. In a follow-up paper we show that these observations nevertheless can be used for model evaluation.
Antti Lipponen, Ville Kolehmainen, Pekka Kolmonen, Antti Kukkurainen, Tero Mielonen, Neus Sabater, Larisa Sogacheva, Timo H. Virtanen, and Antti Arola
Atmos. Meas. Tech., 14, 2981–2992, https://doi.org/10.5194/amt-14-2981-2021, https://doi.org/10.5194/amt-14-2981-2021, 2021
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We have developed a new computational method to post-process-correct the satellite aerosol retrievals. The proposed method combines the conventional satellite aerosol retrievals relying on physics-based models and machine learning. The results show significantly improved accuracy in the aerosol data over the operational satellite data products. The correction can be applied to the existing satellite aerosol datasets with no need to fully reprocess the much larger original radiance data.
Johan Ström, Jonas Svensson, Henri Honkanen, Eija Asmi, Nathaniel B. Dkhar, Shresth Tayal, Ved P. Sharma, Rakesh Hooda, Outi Meinander, Matti Leppäranta, Hans-Werner Jacobi, Heikki Lihavainen, and Antti Hyvärinen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-158, https://doi.org/10.5194/acp-2021-158, 2021
Revised manuscript not accepted
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Snow darkening in the Himalaya results from the deposition of different particles. Here we assess the change in the seasonal snow cover duration due to the presence of mineral dust and black carbon particles in the snow of Sunderdhunga valley, Central Himalaya, India. With the use of in situ weather station data, the snow melt-out date is estimated to be shifted ~13 days earlier due to the presence of the particles in the snow.
Thomas Thorp, Stephen R. Arnold, Richard J. Pope, Dominick V. Spracklen, Luke Conibear, Christoph Knote, Mikhail Arshinov, Boris Belan, Eija Asmi, Tuomas Laurila, Andrei I. Skorokhod, Tuomo Nieminen, and Tuukka Petäjä
Atmos. Chem. Phys., 21, 4677–4697, https://doi.org/10.5194/acp-21-4677-2021, https://doi.org/10.5194/acp-21-4677-2021, 2021
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We compare modelled near-surface pollutants with surface and satellite observations to better understand the controls on the regional concentrations of pollution in western Siberia for late spring and summer in 2011. We find two commonly used emission inventories underestimate human emissions when compared to observations. Transport emissions are the main source of pollutants within the region during this period, whilst fire emissions peak during June and are only significant south of 60° N.
Nicola Zoppetti, Simone Ceccherini, Bruno Carli, Samuele Del Bianco, Marco Gai, Cecilia Tirelli, Flavio Barbara, Rossana Dragani, Antti Arola, Jukka Kujanpää, Jacob C. A. van Peet, Ronald van der A, and Ugo Cortesi
Atmos. Meas. Tech., 14, 2041–2053, https://doi.org/10.5194/amt-14-2041-2021, https://doi.org/10.5194/amt-14-2041-2021, 2021
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The new platforms for Earth observation from space will provide an enormous amount of data that can be hard to exploit as a whole. The Complete Data Fusion algorithm can reduce the data volume while retaining the information of the full dataset. In this work, we applied the Complete Data Fusion algorithm to simulated ozone profiles, and the results show that the fused products are characterized by higher information content compared to individual L2 products.
Jianping Guo, Boming Liu, Wei Gong, Lijuan Shi, Yong Zhang, Yingying Ma, Jian Zhang, Tianmeng Chen, Kaixu Bai, Ad Stoffelen, Gerrit de Leeuw, and Xiaofeng Xu
Atmos. Chem. Phys., 21, 2945–2958, https://doi.org/10.5194/acp-21-2945-2021, https://doi.org/10.5194/acp-21-2945-2021, 2021
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Vertical wind profiles are crucial to a wide range of atmospheric disciplines. Aeolus is the first satellite mission to directly observe wind profile information on a global scale. However, Aeolus wind products over China have thus far not been evaluated by in situ comparison. This work is expected to let the public and science community better know the Aeolus wind products and to encourage use of these valuable data in future research and applications.
Jonas Svensson, Johan Ström, Henri Honkanen, Eija Asmi, Nathaniel B. Dkhar, Shresth Tayal, Ved P. Sharma, Rakesh Hooda, Matti Leppäranta, Hans-Werner Jacobi, Heikki Lihavainen, and Antti Hyvärinen
Atmos. Chem. Phys., 21, 2931–2943, https://doi.org/10.5194/acp-21-2931-2021, https://doi.org/10.5194/acp-21-2931-2021, 2021
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Light-absorbing particles specifically affect snowmelt in the Himalayas. Through measurements of the constituents in glacier snow pits from the Indian Himalayas our investigations show that different snow layers display striking similarities. These similarities can be characterized by a deposition constant. Our results further indicate that mineral dust can be responsible for the majority of light absorption in the snow in this part of the Himalayas.
Terhikki Manninen, Kati Anttila, Emmihenna Jääskeläinen, Aku Riihelä, Jouni Peltoniemi, Petri Räisänen, Panu Lahtinen, Niilo Siljamo, Laura Thölix, Outi Meinander, Anna Kontu, Hanne Suokanerva, Roberta Pirazzini, Juha Suomalainen, Teemu Hakala, Sanna Kaasalainen, Harri Kaartinen, Antero Kukko, Olivier Hautecoeur, and Jean-Louis Roujean
The Cryosphere, 15, 793–820, https://doi.org/10.5194/tc-15-793-2021, https://doi.org/10.5194/tc-15-793-2021, 2021
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The primary goal of this paper is to present a model of snow surface albedo (brightness) accounting for small-scale surface roughness effects. It can be combined with any volume scattering model. The results indicate that surface roughness may decrease the albedo by about 1–3 % in midwinter and even more than 10 % during the late melting season. The effect is largest for low solar zenith angle values and lower bulk snow albedo values.
Boming Liu, Jianping Guo, Wei Gong, Yong Zhang, Lijuan Shi, Yingying Ma, Jian Li, Xiaoran Guo, Ad Stoffelen, Gerrit de Leeuw, and Xiaofeng Xu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-41, https://doi.org/10.5194/acp-2021-41, 2021
Revised manuscript not accepted
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Vertical wind profiles are crucial to a wide range of atmospheric disciplines. Aeolus is the first satellite mission to directly observe wind profile information on a global scale. However, Aeolus wind products over China were thus far not evaluated by in-situ comparison. This work is expected to let the public and science community better know the Aeolus wind products and to encourage use of these valuable data in future researches and applications.
Antti Ruuskanen, Sami Romakkaniemi, Harri Kokkola, Antti Arola, Santtu Mikkonen, Harri Portin, Annele Virtanen, Kari E. J. Lehtinen, Mika Komppula, and Ari Leskinen
Atmos. Chem. Phys., 21, 1683–1695, https://doi.org/10.5194/acp-21-1683-2021, https://doi.org/10.5194/acp-21-1683-2021, 2021
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The study focuses mainly on cloud-scavenging efficiency of absorbing particulate matter (mainly black carbon) but additionally covers cloud-scavenging efficiency of scattering particles and statistics of cloud condensation nuclei. The main findings give insight into how black carbon is distributed in different particle sizes and the sensitivity to cloud scavenged. The main findings are useful for large-scale modelling for evaluating cloud scavenging.
Jonas Gliß, Augustin Mortier, Michael Schulz, Elisabeth Andrews, Yves Balkanski, Susanne E. Bauer, Anna M. K. Benedictow, Huisheng Bian, Ramiro Checa-Garcia, Mian Chin, Paul Ginoux, Jan J. Griesfeller, Andreas Heckel, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Paolo Laj, Philippe Le Sager, Marianne Tronstad Lund, Cathrine Lund Myhre, Hitoshi Matsui, Gunnar Myhre, David Neubauer, Twan van Noije, Peter North, Dirk J. L. Olivié, Samuel Rémy, Larisa Sogacheva, Toshihiko Takemura, Kostas Tsigaridis, and Svetlana G. Tsyro
Atmos. Chem. Phys., 21, 87–128, https://doi.org/10.5194/acp-21-87-2021, https://doi.org/10.5194/acp-21-87-2021, 2021
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Simulated aerosol optical properties as well as the aerosol life cycle are investigated for 14 global models participating in the AeroCom initiative. Considerable diversity is found in the simulated aerosol species emissions and lifetimes, also resulting in a large diversity in the simulated aerosol mass, composition, and optical properties. A comparison with observations suggests that, on average, current models underestimate the direct effect of aerosol on the atmosphere radiation budget.
Kaisa Lakkala, Jukka Kujanpää, Colette Brogniez, Nicolas Henriot, Antti Arola, Margit Aun, Frédérique Auriol, Alkiviadis F. Bais, Germar Bernhard, Veerle De Bock, Maxime Catalfamo, Christine Deroo, Henri Diémoz, Luca Egli, Jean-Baptiste Forestier, Ilias Fountoulakis, Katerina Garane, Rosa Delia Garcia, Julian Gröbner, Seppo Hassinen, Anu Heikkilä, Stuart Henderson, Gregor Hülsen, Bjørn Johnsen, Niilo Kalakoski, Angelos Karanikolas, Tomi Karppinen, Kevin Lamy, Sergio F. León-Luis, Anders V. Lindfors, Jean-Marc Metzger, Fanny Minvielle, Harel B. Muskatel, Thierry Portafaix, Alberto Redondas, Ricardo Sanchez, Anna Maria Siani, Tove Svendby, and Johanna Tamminen
Atmos. Meas. Tech., 13, 6999–7024, https://doi.org/10.5194/amt-13-6999-2020, https://doi.org/10.5194/amt-13-6999-2020, 2020
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The TROPOspheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5 Precursor (S5P) satellite was launched on 13 October 2017 to provide the atmospheric composition for atmosphere and climate research. Ground-based data from 25 sites located in Arctic, subarctic, temperate, equatorial and Antarctic
areas were used for the validation of the TROPOMI surface ultraviolet (UV) radiation product. For most sites 60 %–80 % of TROPOMI data was within ± 20 % of ground-based data.
Veerle De Bock, Alexander Mangold, L. Gijsbert Tilstra, Olaf N. E. Tuinder, and Andy Delcloo
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-425, https://doi.org/10.5194/amt-2020-425, 2020
Revised manuscript not accepted
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The Absorbing Aerosol Height (AAH) is a new GOME-2 product representing the height of absorbing aerosol layers. In this paper the AAH is validated against the layer height detected by CALIOP. We concluded that the AAH often underestimates the height of volcanic layers, so it should be handled with care when using it for aviation safety purposes. Taking into account the uncertainties, the product can be considered as an important added value for near-real time monitoring of volcanic ash layers.
Sho Ohata, Tatsuhiro Mori, Yutaka Kondo, Sangeeta Sharma, Antti Hyvärinen, Elisabeth Andrews, Peter Tunved, Eija Asmi, John Backman, Henri Servomaa, Daniel Veber, Makoto Koike, Yugo Kanaya, Atsushi Yoshida, Nobuhiro Moteki, Yongjing Zhao, Junji Matsushita, and Naga Oshima
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1190, https://doi.org/10.5194/acp-2020-1190, 2020
Preprint withdrawn
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Reliable values of mass absorption cross sections (MAC) of black carbon (BC) are required to determine mass concentrations of BC at Arctic sites using different types of filter-based absorption photometers. We successfully estimated MAC values for these instruments through comparison with independent measurements of BC by continuous soot monitoring system called COSMOS. These MAC values are consistent with each other and applicable to study spatial and temporal variation of BC in the Arctic.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Ying Zhang, Zhengqiang Li, Yu Chen, Gerrit de Leeuw, Chi Zhang, Yisong Xie, and Kaitao Li
Atmos. Chem. Phys., 20, 12795–12811, https://doi.org/10.5194/acp-20-12795-2020, https://doi.org/10.5194/acp-20-12795-2020, 2020
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Observation of atmospheric aerosol components plays an important role in reducing uncertainty in climate assessment. In this study, an improved remote sensing method which can better distinguish scattering components is developed, and the aerosol components in the atmospheric column over China are retrieved based on the Sun–sky radiometer Observation NETwork (SONET). The component distribution shows there could be a sea salt component in northwest China from a paleomarine source in desert land.
Nick Schutgens, Andrew M. Sayer, Andreas Heckel, Christina Hsu, Hiren Jethva, Gerrit de Leeuw, Peter J. T. Leonard, Robert C. Levy, Antti Lipponen, Alexei Lyapustin, Peter North, Thomas Popp, Caroline Poulsen, Virginia Sawyer, Larisa Sogacheva, Gareth Thomas, Omar Torres, Yujie Wang, Stefan Kinne, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 20, 12431–12457, https://doi.org/10.5194/acp-20-12431-2020, https://doi.org/10.5194/acp-20-12431-2020, 2020
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We intercompare 14 different datasets of satellite observations of aerosol. Such measurements are challenging but also provide the best opportunity to globally observe an atmospheric component strongly related to air pollution and climate change. Our study shows that most datasets perform similarly well on a global scale but that locally errors can be quite different. We develop a technique to estimate satellite errors everywhere, even in the absence of surface reference data.
Piia Post and Margit Aun
Adv. Sci. Res., 17, 219–225, https://doi.org/10.5194/asr-17-219-2020, https://doi.org/10.5194/asr-17-219-2020, 2020
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The satellite-based fractional cloud cover and cloud top height from CLARA-A2 data record has been used to analyse trends in the Baltic Sea region, 1982–2015. Cloud observations from the Tartu-Tõravere meteorological station were used as reference data for the same period. A downward trend in fractional cloud cover in March over the 1982–2015 period was found. For cloud top heights summer and spring regional averages showed opposite signs of the trend: for June positive and for March negative.
Ilann Bourgeois, Jeff Peischl, Chelsea R. Thompson, Kenneth C. Aikin, Teresa Campos, Hannah Clark, Róisín Commane, Bruce Daube, Glenn W. Diskin, James W. Elkins, Ru-Shan Gao, Audrey Gaudel, Eric J. Hintsa, Bryan J. Johnson, Rigel Kivi, Kathryn McKain, Fred L. Moore, David D. Parrish, Richard Querel, Eric Ray, Ricardo Sánchez, Colm Sweeney, David W. Tarasick, Anne M. Thompson, Valérie Thouret, Jacquelyn C. Witte, Steve C. Wofsy, and Thomas B. Ryerson
Atmos. Chem. Phys., 20, 10611–10635, https://doi.org/10.5194/acp-20-10611-2020, https://doi.org/10.5194/acp-20-10611-2020, 2020
Paolo Laj, Alessandro Bigi, Clémence Rose, Elisabeth Andrews, Cathrine Lund Myhre, Martine Collaud Coen, Yong Lin, Alfred Wiedensohler, Michael Schulz, John A. Ogren, Markus Fiebig, Jonas Gliß, Augustin Mortier, Marco Pandolfi, Tuukka Petäja, Sang-Woo Kim, Wenche Aas, Jean-Philippe Putaud, Olga Mayol-Bracero, Melita Keywood, Lorenzo Labrador, Pasi Aalto, Erik Ahlberg, Lucas Alados Arboledas, Andrés Alastuey, Marcos Andrade, Begoña Artíñano, Stina Ausmeel, Todor Arsov, Eija Asmi, John Backman, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Sébastien Conil, Cedric Couret, Derek Day, Wan Dayantolis, Anna Degorska, Konstantinos Eleftheriadis, Prodromos Fetfatzis, Olivier Favez, Harald Flentje, Maria I. Gini, Asta Gregorič, Martin Gysel-Beer, A. Gannet Hallar, Jenny Hand, Andras Hoffer, Christoph Hueglin, Rakesh K. Hooda, Antti Hyvärinen, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Jeong Eun Kim, Giorgos Kouvarakis, Irena Kranjc, Radovan Krejci, Markku Kulmala, Casper Labuschagne, Hae-Jung Lee, Heikki Lihavainen, Neng-Huei Lin, Gunter Löschau, Krista Luoma, Angela Marinoni, Sebastiao Martins Dos Santos, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Nhat Anh Nguyen, Jakub Ondracek, Noemi Pérez, Maria Rita Perrone, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Natalia Prats, Anthony Prenni, Fabienne Reisen, Salvatore Romano, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Maik Schütze, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Martin Steinbacher, Junying Sun, Gloria Titos, Barbara Toczko, Thomas Tuch, Pierre Tulet, Peter Tunved, Ville Vakkari, Fernando Velarde, Patricio Velasquez, Paolo Villani, Sterios Vratolis, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Jesus Yus-Diez, Vladimir Zdimal, Paul Zieger, and Nadezda Zikova
Atmos. Meas. Tech., 13, 4353–4392, https://doi.org/10.5194/amt-13-4353-2020, https://doi.org/10.5194/amt-13-4353-2020, 2020
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The paper establishes the fiducial reference of the GAW aerosol network providing the fully characterized value chain to the provision of four climate-relevant aerosol properties from ground-based sites. Data from almost 90 stations worldwide are reported for a reference year, 2017, providing a unique and very robust view of the variability of these variables worldwide. Current gaps in the GAW network are analysed and requirements for the Global Climate Monitoring System are proposed.
Jill S. Johnson, Leighton A. Regayre, Masaru Yoshioka, Kirsty J. Pringle, Steven T. Turnock, Jo Browse, David M. H. Sexton, John W. Rostron, Nick A. J. Schutgens, Daniel G. Partridge, Dantong Liu, James D. Allan, Hugh Coe, Aijun Ding, David D. Cohen, Armand Atanacio, Ville Vakkari, Eija Asmi, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 9491–9524, https://doi.org/10.5194/acp-20-9491-2020, https://doi.org/10.5194/acp-20-9491-2020, 2020
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We use over 9000 monthly aggregated grid-box measurements of aerosol to constrain the uncertainty in the HadGEM3-UKCA climate model. Measurements of AOD, PM2.5, particle number concentrations, sulfate and organic mass concentrations are compared to 1 million
variantsof the model using an implausibility metric. Despite many compensating effects in the model, the procedure constrains the probability distributions of many parameters, and direct radiative forcing uncertainty is reduced by 34 %.
William Wandji Nyamsi, Antti Lipponen, Arturo Sanchez-Lorenzo, Martin Wild, and Antti Arola
Atmos. Meas. Tech., 13, 3061–3079, https://doi.org/10.5194/amt-13-3061-2020, https://doi.org/10.5194/amt-13-3061-2020, 2020
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This paper proposes a novel and accurate method for estimating and reconstructing aerosol optical depth from sunshine duration measurements under cloud-free conditions at any place and time since the late 19th century. The method performs very well when compared to AErosol RObotic NETwork measurements and operates an efficient detection of signals from massive volcanic eruptions. Reconstructed long-term aerosol optical depths are in agreement with the dimming/brightening phenomenon.
Kaisa Lakkala, Margit Aun, Ricardo Sanchez, Germar Bernhard, Eija Asmi, Outi Meinander, Fernando Nollas, Gregor Hülsen, Tomi Karppinen, Veijo Aaltonen, Antti Arola, and Gerrit de Leeuw
Earth Syst. Sci. Data, 12, 947–960, https://doi.org/10.5194/essd-12-947-2020, https://doi.org/10.5194/essd-12-947-2020, 2020
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A GUV multi-filter radiometer was set up at Marambio, 64° S, 56° W, Antarctica, in 2017. The instrument continuously measures ultraviolet (UV) radiation, visible (VIS) radiation and photosynthetically active radiation (PAR). The measurements are designed for providing high-quality long-term time series that can be used to assess the impact of global climate change in the Antarctic region. The data from the last 5 d are plotted and updated daily.
Larisa Sogacheva, Thomas Popp, Andrew M. Sayer, Oleg Dubovik, Michael J. Garay, Andreas Heckel, N. Christina Hsu, Hiren Jethva, Ralph A. Kahn, Pekka Kolmonen, Miriam Kosmale, Gerrit de Leeuw, Robert C. Levy, Pavel Litvinov, Alexei Lyapustin, Peter North, Omar Torres, and Antti Arola
Atmos. Chem. Phys., 20, 2031–2056, https://doi.org/10.5194/acp-20-2031-2020, https://doi.org/10.5194/acp-20-2031-2020, 2020
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The typical lifetime of a single satellite platform is on the order of 5–15 years; thus, for climate studies the usage of multiple satellite sensors should be considered.
Here we introduce and evaluate a monthly AOD merged product and AOD global and regional time series for the period 1995–2017 created from 12 individual satellite AOD products, which provide a long-term perspective on AOD changes over different regions of the globe.
Giulia Saponaro, Moa K. Sporre, David Neubauer, Harri Kokkola, Pekka Kolmonen, Larisa Sogacheva, Antti Arola, Gerrit de Leeuw, Inger H. H. Karset, Ari Laaksonen, and Ulrike Lohmann
Atmos. Chem. Phys., 20, 1607–1626, https://doi.org/10.5194/acp-20-1607-2020, https://doi.org/10.5194/acp-20-1607-2020, 2020
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The understanding of cloud processes is based on the quality of the representation of cloud properties. We compared cloud parameters from three models with satellite observations. We report on the performance of each data source, highlighting strengths and deficiencies, which should be considered when deriving the effect of aerosols on cloud properties.
Santtu Mikkonen, Mikko R. A. Pitkänen, Tuomo Nieminen, Antti Lipponen, Sini Isokääntä, Antti Arola, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 19, 12531–12543, https://doi.org/10.5194/acp-19-12531-2019, https://doi.org/10.5194/acp-19-12531-2019, 2019
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Atmospheric measurement data never come without measurement error. Too often, these errors are neglected when researchers make inferences from their data. We applied multiple line-fitting methods to simulated data mimicking two central variables in aerosol research. Our results show that an ordinary least squares fit, typically used to describe relationships, underestimates the slope of the fit and that methods taking the measurement uncertainty into account performed significantly better.
Yahui Che, Jie Guang, Gerrit de Leeuw, Yong Xue, Ling Sun, and Huizheng Che
Atmos. Meas. Tech., 12, 4091–4112, https://doi.org/10.5194/amt-12-4091-2019, https://doi.org/10.5194/amt-12-4091-2019, 2019
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The use of AOD data retrieved from ATSR-2, AATSR and AVHRR to produce a very long time series is investigated. The study is made over a small area in northern China with a large variation of AOD values. Sun photometer data from AERONET and CARSNET and radiance-derived AOD are used as reference. The results show that all data sets compare well. However, AVHRR underestimates high AOD (mainly occurring in summer) but performs better than (A)ATSR in winter.
Michael Boy, Erik S. Thomson, Juan-C. Acosta Navarro, Olafur Arnalds, Ekaterina Batchvarova, Jaana Bäck, Frank Berninger, Merete Bilde, Zoé Brasseur, Pavla Dagsson-Waldhauserova, Dimitri Castarède, Maryam Dalirian, Gerrit de Leeuw, Monika Dragosics, Ella-Maria Duplissy, Jonathan Duplissy, Annica M. L. Ekman, Keyan Fang, Jean-Charles Gallet, Marianne Glasius, Sven-Erik Gryning, Henrik Grythe, Hans-Christen Hansson, Margareta Hansson, Elisabeth Isaksson, Trond Iversen, Ingibjorg Jonsdottir, Ville Kasurinen, Alf Kirkevåg, Atte Korhola, Radovan Krejci, Jon Egill Kristjansson, Hanna K. Lappalainen, Antti Lauri, Matti Leppäranta, Heikki Lihavainen, Risto Makkonen, Andreas Massling, Outi Meinander, E. Douglas Nilsson, Haraldur Olafsson, Jan B. C. Pettersson, Nønne L. Prisle, Ilona Riipinen, Pontus Roldin, Meri Ruppel, Matthew Salter, Maria Sand, Øyvind Seland, Heikki Seppä, Henrik Skov, Joana Soares, Andreas Stohl, Johan Ström, Jonas Svensson, Erik Swietlicki, Ksenia Tabakova, Throstur Thorsteinsson, Aki Virkkula, Gesa A. Weyhenmeyer, Yusheng Wu, Paul Zieger, and Markku Kulmala
Atmos. Chem. Phys., 19, 2015–2061, https://doi.org/10.5194/acp-19-2015-2019, https://doi.org/10.5194/acp-19-2015-2019, 2019
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The Nordic Centre of Excellence CRAICC (Cryosphere–Atmosphere Interactions in a Changing Arctic Climate), funded by NordForsk in the years 2011–2016, is the largest joint Nordic research and innovation initiative to date and aimed to strengthen research and innovation regarding climate change issues in the Nordic region. The paper presents an overview of the main scientific topics investigated and provides a state-of-the-art comprehensive summary of what has been achieved in CRAICC.
Yuqin Liu, Jiahua Zhang, Putian Zhou, Tao Lin, Juan Hong, Lamei Shi, Fengmei Yao, Jun Wu, Huadong Guo, and Gerrit de Leeuw
Atmos. Chem. Phys., 18, 18187–18202, https://doi.org/10.5194/acp-18-18187-2018, https://doi.org/10.5194/acp-18-18187-2018, 2018
Nuno Pereira, David Bolsée, Peter Sperfeld, Sven Pape, Dominique Sluse, and Gaël Cessateur
Atmos. Meas. Tech., 11, 6605–6615, https://doi.org/10.5194/amt-11-6605-2018, https://doi.org/10.5194/amt-11-6605-2018, 2018
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The knowledge of the solar spectrum at the top of Earth's atmosphere is of great importance for climatic studies. Satellite instruments allow direct measurements; however, their calibration presents issues. It is possible to determine this spectrum precisely from Earth-based measurements as well, using the Langley plot technique and accurate calibration techniques. We present an infrared spectrum using these techniques for measurements made at the reference Mauna Loa Observatory.
Stephen M. Platt, Sabine Eckhardt, Benedicte Ferré, Rebecca E. Fisher, Ove Hermansen, Pär Jansson, David Lowry, Euan G. Nisbet, Ignacio Pisso, Norbert Schmidbauer, Anna Silyakova, Andreas Stohl, Tove M. Svendby, Sunil Vadakkepuliyambatta, Jürgen Mienert, and Cathrine Lund Myhre
Atmos. Chem. Phys., 18, 17207–17224, https://doi.org/10.5194/acp-18-17207-2018, https://doi.org/10.5194/acp-18-17207-2018, 2018
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We measured atmospheric mixing ratios of methane over the Arctic Ocean around Svalbard and compared observed variations to inventories for anthropogenic, wetland, and biomass burning methane emissions and an atmospheric transport model. With knowledge of where variations were expected due to the aforementioned land-based emissions, we were able to identify and quantify a methane source from the ocean north of Svalbard, likely from sub-sea hydrocarbon seeps and/or gas hydrate decomposition.
Larisa Sogacheva, Edith Rodriguez, Pekka Kolmonen, Timo H. Virtanen, Giulia Saponaro, Gerrit de Leeuw, Aristeidis K. Georgoulias, Georgia Alexandri, Konstantinos Kourtidis, and Ronald J. van der A
Atmos. Chem. Phys., 18, 16631–16652, https://doi.org/10.5194/acp-18-16631-2018, https://doi.org/10.5194/acp-18-16631-2018, 2018
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Understanding long-term trends in aerosol optical density (AOD) is essential for evaluating health and climate effects and the effectiveness of pollution control policies. A method to construct a combined AOD long time series (1995-2017) using ATSR and MODIS spaceborne instruments is introduced. The effect of changes in the emission regulation policy in China is seen in a gradual AOD decrease after 2011. The effect is more visible in highly populated and industrialized areas in southeast China.
Kaisa Lakkala, Alberto Redondas, Outi Meinander, Laura Thölix, Britta Hamari, Antonio Fernando Almansa, Virgilio Carreno, Rosa Delia García, Carlos Torres, Guillermo Deferrari, Hector Ochoa, Germar Bernhard, Ricardo Sanchez, and Gerrit de Leeuw
Atmos. Chem. Phys., 18, 16019–16031, https://doi.org/10.5194/acp-18-16019-2018, https://doi.org/10.5194/acp-18-16019-2018, 2018
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Solar UV irradiances were measured at Ushuaia (54° S) and Marambio (64° S) during 2000–2013. The measurements were part of the Antarctic NILU-UV network, which was maintained as a cooperation between Spain, Argentina and Finland. The time series of the network were analysed for the first time in this study. At both stations maximum UV indices and daily doses were measured when spring-time ozone loss episodes occurred. The maximum UV index was 13 and 12 in Ushuaia and Marambio, respectively.
Tuomo Nieminen, Veli-Matti Kerminen, Tuukka Petäjä, Pasi P. Aalto, Mikhail Arshinov, Eija Asmi, Urs Baltensperger, David C. S. Beddows, Johan Paul Beukes, Don Collins, Aijun Ding, Roy M. Harrison, Bas Henzing, Rakesh Hooda, Min Hu, Urmas Hõrrak, Niku Kivekäs, Kaupo Komsaare, Radovan Krejci, Adam Kristensson, Lauri Laakso, Ari Laaksonen, W. Richard Leaitch, Heikki Lihavainen, Nikolaos Mihalopoulos, Zoltán Németh, Wei Nie, Colin O'Dowd, Imre Salma, Karine Sellegri, Birgitta Svenningsson, Erik Swietlicki, Peter Tunved, Vidmantas Ulevicius, Ville Vakkari, Marko Vana, Alfred Wiedensohler, Zhijun Wu, Annele Virtanen, and Markku Kulmala
Atmos. Chem. Phys., 18, 14737–14756, https://doi.org/10.5194/acp-18-14737-2018, https://doi.org/10.5194/acp-18-14737-2018, 2018
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Atmospheric aerosols have diverse effects on air quality, human health, and global climate. One important source of aerosols is their formation via nucleation and growth in the atmosphere. We have analyzed long-term observations of regional new particle formation events around the globe and provide a comprehensive view on the characteristics of this phenomenon in diverse environments. The results are useful in developing more realistic representation of atmospheric aerosols in global models.
Harri Kokkola, Thomas Kühn, Anton Laakso, Tommi Bergman, Kari E. J. Lehtinen, Tero Mielonen, Antti Arola, Scarlet Stadtler, Hannele Korhonen, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Ina Tegen, Colombe Siegenthaler-Le Drian, Martin G. Schultz, Isabelle Bey, Philip Stier, Nikos Daskalakis, Colette L. Heald, and Sami Romakkaniemi
Geosci. Model Dev., 11, 3833–3863, https://doi.org/10.5194/gmd-11-3833-2018, https://doi.org/10.5194/gmd-11-3833-2018, 2018
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In this paper we present a global aerosol–chemistry–climate model with the focus on its representation for atmospheric aerosol particles. In the model, aerosols are simulated using the aerosol module SALSA2.0, which in this paper is compared to satellite, ground, and aircraft-based observations of the properties of atmospheric aerosol. Based on this study, the model simulated aerosol properties compare well with the observations.
Kaisa Lakkala, Antti Arola, Julian Gröbner, Sergio Fabian León-Luis, Alberto Redondas, Stelios Kazadzis, Tomi Karppinen, Juha Matti Karhu, Luca Egli, Anu Heikkilä, Tapani Koskela, Antonio Serrano, and José Manuel Vilaplana
Atmos. Meas. Tech., 11, 5167–5180, https://doi.org/10.5194/amt-11-5167-2018, https://doi.org/10.5194/amt-11-5167-2018, 2018
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The performance of the cosine error correction method for correcting spectral UV measurements of the Brewer spectroradiometer was studied. The correction depends on the sky radiation distribution, which can change during one spectral scan. The results showed that the correction varied between 4 and 14 %, and that the relative differences between the reference and the Brewer diminished by 10 %. The method is applicable to other instruments as long as the required input parameters are available.
Lauren Schmeisser, John Backman, John A. Ogren, Elisabeth Andrews, Eija Asmi, Sandra Starkweather, Taneil Uttal, Markus Fiebig, Sangeeta Sharma, Kostas Eleftheriadis, Stergios Vratolis, Michael Bergin, Peter Tunved, and Anne Jefferson
Atmos. Chem. Phys., 18, 11599–11622, https://doi.org/10.5194/acp-18-11599-2018, https://doi.org/10.5194/acp-18-11599-2018, 2018
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This paper presents pan-Arctic seasonality of in-situ-measured aerosol optical properties from six surface monitoring sites. The analysis provides insight into aerosol annual variability throughout the region – something that is not possible using only measurements from satellite or temporary aircraft campaigns. This paper shows that the large spatiotemporal variability in aerosol optical properties needs to be taken into account in order to properly represent Arctic climate.
Larisa Sogacheva, Gerrit de Leeuw, Edith Rodriguez, Pekka Kolmonen, Aristeidis K. Georgoulias, Georgia Alexandri, Konstantinos Kourtidis, Emmanouil Proestakis, Eleni Marinou, Vassilis Amiridis, Yong Xue, and Ronald J. van der A
Atmos. Chem. Phys., 18, 11389–11407, https://doi.org/10.5194/acp-18-11389-2018, https://doi.org/10.5194/acp-18-11389-2018, 2018
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Using AATSR ADV (1995–2011) and MODIS C6.1 (2000–2017) annual and seasonal aerosol optical depth (AOD) aggregates, we obtained information regarding the occurrence of aerosols and their spatial and temporal variation over China. We specifically focused on regional differences in annual and seasonal AOD behavior for selected regions. AOD dataset comparisons, validation results and AOD tendencies during the overlapping period (2000–2011) are discussed.
Niels Souverijns, Alexandra Gossart, Irina V. Gorodetskaya, Stef Lhermitte, Alexander Mangold, Quentin Laffineur, Andy Delcloo, and Nicole P. M. van Lipzig
The Cryosphere, 12, 1987–2003, https://doi.org/10.5194/tc-12-1987-2018, https://doi.org/10.5194/tc-12-1987-2018, 2018
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This work is the first to gain insight into the local surface mass balance over Antarctica using accurate long-term snowfall observations. A non-linear relationship between accumulation and snowfall is discovered, indicating that total surface mass balance measurements are not a good proxy for snowfall over Antarctica. Furthermore, the meteorological drivers causing changes in the local SMB are identified.
Pieternel F. Levelt, Joanna Joiner, Johanna Tamminen, J. Pepijn Veefkind, Pawan K. Bhartia, Deborah C. Stein Zweers, Bryan N. Duncan, David G. Streets, Henk Eskes, Ronald van der A, Chris McLinden, Vitali Fioletov, Simon Carn, Jos de Laat, Matthew DeLand, Sergey Marchenko, Richard McPeters, Jerald Ziemke, Dejian Fu, Xiong Liu, Kenneth Pickering, Arnoud Apituley, Gonzalo González Abad, Antti Arola, Folkert Boersma, Christopher Chan Miller, Kelly Chance, Martin de Graaf, Janne Hakkarainen, Seppo Hassinen, Iolanda Ialongo, Quintus Kleipool, Nickolay Krotkov, Can Li, Lok Lamsal, Paul Newman, Caroline Nowlan, Raid Suleiman, Lieuwe Gijsbert Tilstra, Omar Torres, Huiqun Wang, and Krzysztof Wargan
Atmos. Chem. Phys., 18, 5699–5745, https://doi.org/10.5194/acp-18-5699-2018, https://doi.org/10.5194/acp-18-5699-2018, 2018
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The aim of this paper is to highlight the many successes of the Ozone Monitoring Instrument (OMI) spanning more than 13 years. Data from OMI have been used in a wide range of applications. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. OMI data continue to be used for new research and applications.
Antti Lipponen, Tero Mielonen, Mikko R. A. Pitkänen, Robert C. Levy, Virginia R. Sawyer, Sami Romakkaniemi, Ville Kolehmainen, and Antti Arola
Atmos. Meas. Tech., 11, 1529–1547, https://doi.org/10.5194/amt-11-1529-2018, https://doi.org/10.5194/amt-11-1529-2018, 2018
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Atmospheric aerosols are small solid or liquid particles suspended in the atmosphere and they have a significant effect on the climate. Satellite data are used to get global estimates of atmospheric aerosols. In this work, a statistics-based Bayesian aerosol retrieval algorithm was developed to improve the accuracy and quantify the uncertainties related to the aerosol estimates. The algorithm is tested with NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) satellite data.
Jonas Svensson, Johan Ström, Niku Kivekäs, Nathaniel B. Dkhar, Shresth Tayal, Ved P. Sharma, Arttu Jutila, John Backman, Aki Virkkula, Meri Ruppel, Antti Hyvärinen, Anna Kontu, Henna-Reetta Hannula, Matti Leppäranta, Rakesh K. Hooda, Atte Korhola, Eija Asmi, and Heikki Lihavainen
Atmos. Meas. Tech., 11, 1403–1416, https://doi.org/10.5194/amt-11-1403-2018, https://doi.org/10.5194/amt-11-1403-2018, 2018
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Receding glaciers in the Himalayas are of concern. Here we present measurements of light-absorbing impurities, known to contribute to the ongoing glacier decrease, in snow from Indian Himalayas and compare them to snow samples from the Finnish Arctic. The soot particles in the snow are shown to have lower light absorbing efficiency, possibly affecting their radiative forcing potential in the snow. Further, dust influences the snow in the Himalayas to a much greater extent than in Finland.
Anders V. Lindfors, Jukka Kujanpää, Niilo Kalakoski, Anu Heikkilä, Kaisa Lakkala, Tero Mielonen, Maarten Sneep, Nickolay A. Krotkov, Antti Arola, and Johanna Tamminen
Atmos. Meas. Tech., 11, 997–1008, https://doi.org/10.5194/amt-11-997-2018, https://doi.org/10.5194/amt-11-997-2018, 2018
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This paper describes the algorithm that will be used for estimating surface UV radiation from TROPOMI (TROPOspheric Monitoring Instrument) measurements. TROPOMI is the only payload of the Sentinel-5 Precursor (S5P), which is a polar-orbiting satellite mission of the European Space Agency (ESA). The presented algorithm has been tested using input based on previous satellite measurements. These preliminary results indicate that the algorithm is functioning according to expectations.
Timo H. Virtanen, Pekka Kolmonen, Larisa Sogacheva, Edith Rodríguez, Giulia Saponaro, and Gerrit de Leeuw
Atmos. Meas. Tech., 11, 925–938, https://doi.org/10.5194/amt-11-925-2018, https://doi.org/10.5194/amt-11-925-2018, 2018
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We study the collocation mismatch uncertainty related to validating coarse-resolution satellite-based aerosol data against point-like ground based measurements. We use the spatial variability in the satellite data to estimate the upper limit for the uncertainty and study the effect of sampling parameters in the validation. We find that accounting for the collocation mismatch uncertainty increases the fraction of consistent data in the validation.
Klára Čížková, Kamil Láska, Ladislav Metelka, and Martin Staněk
Atmos. Chem. Phys., 18, 1805–1818, https://doi.org/10.5194/acp-18-1805-2018, https://doi.org/10.5194/acp-18-1805-2018, 2018
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In order to broaden the knowledge of long-term UV radiation variability, we have reconstructed and analyzed a 50-year-long UV radiation time series from Hradec Králové, Czech Republic. The UV radiation intensities increased greatly following the decline of ozone amounts in the 1980s and 1990s. High UV radiation doses were observed in days with low ozone amounts, clear or partly cloudy skies, or snow cover.
Gerrit de Leeuw, Larisa Sogacheva, Edith Rodriguez, Konstantinos Kourtidis, Aristeidis K. Georgoulias, Georgia Alexandri, Vassilis Amiridis, Emmanouil Proestakis, Eleni Marinou, Yong Xue, and Ronald van der A
Atmos. Chem. Phys., 18, 1573–1592, https://doi.org/10.5194/acp-18-1573-2018, https://doi.org/10.5194/acp-18-1573-2018, 2018
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The complementary use of two sensors, ATSR and MODIS, to provide aerosol information over two decades (1995–2015) is described. To this end, the AOD retrieved from both instruments had to be compared, showing that ATSR slightly underestimates and MODIS overestimates by a similar amount. Results show the increase of aerosols over the years, with an indication of the onset of a decrease in recent years. The AOD spatial distribution shows seasonal variations across China.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Aristeidis K. Georgoulias, Stavros Solomos, Stelios Kazadzis, Julien Chimot, Huizheng Che, Georgia Alexandri, Ioannis Binietoglou, Vasiliki Daskalopoulou, Konstantinos A. Kourtidis, Gerrit de Leeuw, and Ronald J. van der A
Atmos. Chem. Phys., 18, 1337–1362, https://doi.org/10.5194/acp-18-1337-2018, https://doi.org/10.5194/acp-18-1337-2018, 2018
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We provide a 3-D climatology of desert dust aerosols over South and East Asia, based on 9 years of CALIPSO observations and an EARLINET methodology. The results provide the horizontal, vertical and seasonal distribution of dust aerosols over SE Asia along with the change in dust transport pathways. The dataset is unique for its potential applications, including evaluation and assimilation activities in atmospheric simulations and the estimation of the climatic impact of dust aerosols.
William Wandji Nyamsi, Phillipe Blanc, John A. Augustine, Antti Arola, and Lucien Wald
Biogeosciences Discuss., https://doi.org/10.5194/bg-2017-512, https://doi.org/10.5194/bg-2017-512, 2018
Manuscript not accepted for further review
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This paper proposes a new, fast and accurate method for estimating photosynthetically active radiation at ground level in cloud-free conditions at any place and time. The method performs very well with the Copernicus Atmosphere Monitoring Service products as inputs describing the state of the atmosphere. An accuracy that is close to the uncertainty of the measurements themselves is reached. We believe that our research will be widely used in the near future.
John Backman, Lauren Schmeisser, Aki Virkkula, John A. Ogren, Eija Asmi, Sandra Starkweather, Sangeeta Sharma, Konstantinos Eleftheriadis, Taneil Uttal, Anne Jefferson, Michael Bergin, Alexander Makshtas, Peter Tunved, and Markus Fiebig
Atmos. Meas. Tech., 10, 5039–5062, https://doi.org/10.5194/amt-10-5039-2017, https://doi.org/10.5194/amt-10-5039-2017, 2017
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Light absorption by aerosol particles is of climatic importance. A widely used means to measure aerosol light absorption is a filter-based measurement technique. In remote areas, such as the Arctic, filter-based instruments operate close to their detection limit. The study presents how a lower detection limit can be achieved for one such instrument, the Aethalometer. Additionally, the Aethalometer is compared to similar instruments, thus improving measurement inter-comparability in the Arctic.
William Wandji Nyamsi, Mikko R. A. Pitkänen, Youva Aoun, Philippe Blanc, Anu Heikkilä, Kaisa Lakkala, Germar Bernhard, Tapani Koskela, Anders V. Lindfors, Antti Arola, and Lucien Wald
Atmos. Meas. Tech., 10, 4965–4978, https://doi.org/10.5194/amt-10-4965-2017, https://doi.org/10.5194/amt-10-4965-2017, 2017
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This paper proposes a new, fast and accurate method for estimating UV fluxes at ground level in cloud-free conditions at any place and time. The method performs very well with the Copernicus Atmosphere Monitoring Service products as inputs describing the state of the atmosphere. An accuracy that is close to the uncertainty of the measurements themselves is reached. We believe that our research will be widely used in the near future.
Ilias Fountoulakis, Alberto Redondas, Kaisa Lakkala, Alberto Berjon, Alkiviadis F. Bais, Lionel Doppler, Uwe Feister, Anu Heikkila, Tomi Karppinen, Juha M. Karhu, Tapani Koskela, Katerina Garane, Konstantinos Fragkos, and Volodya Savastiouk
Atmos. Meas. Tech., 10, 4491–4505, https://doi.org/10.5194/amt-10-4491-2017, https://doi.org/10.5194/amt-10-4491-2017, 2017
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Results of the temperature characterization of the global UV spectral measurements of eight different Brewer spectrophotometers operating in Greece, Finland, Germany and Spain are presented. Different temperature characterization methods are evaluated and an improved methodology for the correction of the measurements for the effects of temperature is presented.
Liisi Jakobson, Erko Jakobson, Piia Post, and Jaak Jaagus
Earth Syst. Dynam., 8, 1019–1030, https://doi.org/10.5194/esd-8-1019-2017, https://doi.org/10.5194/esd-8-1019-2017, 2017
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Relationships between meteorological parameters between Arctic and the Baltic Sea regions were investigated using NCEP-CFSR reanalysis for 1979–2015. The Greenland and Baffin Bay regions climate have the most significant teleconnections with the Baltic Sea region temperature, specific humidity and wind speed. These relationships can be explained by the AO/NAO index variability only in winter. The results are valuable for selecting Arctic regions with the largest effect on the Baltic Sea region.
Peter W. Thorne, Fabio Madonna, Joerg Schulz, Tim Oakley, Bruce Ingleby, Marco Rosoldi, Emanuele Tramutola, Antti Arola, Matthias Buschmann, Anna C. Mikalsen, Richard Davy, Corinne Voces, Karin Kreher, Martine De Maziere, and Gelsomina Pappalardo
Geosci. Instrum. Method. Data Syst., 6, 453–472, https://doi.org/10.5194/gi-6-453-2017, https://doi.org/10.5194/gi-6-453-2017, 2017
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The term system-of-systems with respect to observational capabilities is frequently used, but what does it mean and how can it be assessed? Here, we define one possible interpretation of a system-of-systems architecture that is based upon demonstrable aspects of observing capabilities. We develop a set of assessment strands and then apply these to a set of atmospheric observational networks to decide which observations may be suitable for characterising satellite platforms in future work.
Christopher J. Merchant, Frank Paul, Thomas Popp, Michael Ablain, Sophie Bontemps, Pierre Defourny, Rainer Hollmann, Thomas Lavergne, Alexandra Laeng, Gerrit de Leeuw, Jonathan Mittaz, Caroline Poulsen, Adam C. Povey, Max Reuter, Shubha Sathyendranath, Stein Sandven, Viktoria F. Sofieva, and Wolfgang Wagner
Earth Syst. Sci. Data, 9, 511–527, https://doi.org/10.5194/essd-9-511-2017, https://doi.org/10.5194/essd-9-511-2017, 2017
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Climate data records (CDRs) contain data describing Earth's climate and should address uncertainty in the data to communicate what is known about climate variability or change and what range of doubt exists. This paper discusses good practice for including uncertainty information in CDRs for the essential climate variables (ECVs) derived from satellite data. Recommendations emerge from the shared experience of diverse ECV projects within the European Space Agency Climate Change Initiative.
Antti Arola, Thomas F. Eck, Harri Kokkola, Mikko R. A. Pitkänen, and Sami Romakkaniemi
Atmos. Chem. Phys., 17, 5991–6001, https://doi.org/10.5194/acp-17-5991-2017, https://doi.org/10.5194/acp-17-5991-2017, 2017
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One of the issues that hinder the measurement-based assessment of aerosol–cloud interactions by remote sensing methods is that typically aerosols and clouds cannot be measured simultaneously by passive remote sensing methods. AERONET includes the SDA product that provides the fine-mode AOD also in mixed cloud–aerosol observations. These measurements have not yet been fully exploited in studies of aerosol–cloud interactions. We applied SDA for this kind of analysis.
Yuqin Liu, Gerrit de Leeuw, Veli-Matti Kerminen, Jiahua Zhang, Putian Zhou, Wei Nie, Ximeng Qi, Juan Hong, Yonghong Wang, Aijun Ding, Huadong Guo, Olaf Krüger, Markku Kulmala, and Tuukka Petäjä
Atmos. Chem. Phys., 17, 5623–5641, https://doi.org/10.5194/acp-17-5623-2017, https://doi.org/10.5194/acp-17-5623-2017, 2017
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The aerosol effects on warm cloud parameters over the Yangtze River Delta are systematically examined using multi-sensor retrievals. This study shows that the COT–CDR and CWP–CDR relationships are not unique, but are affected by atmospheric aerosol loading. CDR and cloud fraction show different behaviours for low and high AOD. Aerosol–cloud interaction (ACI) is stronger for clouds mixed with smoke aerosol than for clouds mixed with dust. Meteorological conditions play an important role in ACI.
Giulia Saponaro, Pekka Kolmonen, Larisa Sogacheva, Edith Rodriguez, Timo Virtanen, and Gerrit de Leeuw
Atmos. Chem. Phys., 17, 3133–3143, https://doi.org/10.5194/acp-17-3133-2017, https://doi.org/10.5194/acp-17-3133-2017, 2017
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The effect of aerosol upon cloud properties is studied over the Baltic Sea region, which presents a distinct contrast of aerosol loading between the clean Fennoscandia and the polluted area of central–eastern Europe. Statistically significant positive values are found over the Baltic Sea and Fennoscandia, while negative values are found over central–eastern Europe, contradicting the theory of aerosol indirect effect on clouds.
Larisa Sogacheva, Pekka Kolmonen, Timo H. Virtanen, Edith Rodriguez, Giulia Saponaro, and Gerrit de Leeuw
Atmos. Meas. Tech., 10, 491–505, https://doi.org/10.5194/amt-10-491-2017, https://doi.org/10.5194/amt-10-491-2017, 2017
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Clouds reflect solar light much more strongly than aerosol particles. Therefore, the retrieval of aerosol optical depth is usually only attempted over cloud-free areas. A very strict cloud detection scheme has to be applied to remove all cloudy pixels. However, often not all clouds are detected. To remove possibly cloud-contaminated pixels, a cloud post-processing algorithm has been designed, which effectively solves the problem and results in smoother AOD maps and improved validation results.
Christos S. Zerefos, Kostas Eleftheratos, John Kapsomenakis, Stavros Solomos, Antje Inness, Dimitris Balis, Alberto Redondas, Henk Eskes, Marc Allaart, Vassilis Amiridis, Arne Dahlback, Veerle De Bock, Henri Diémoz, Ronny Engelmann, Paul Eriksen, Vitali Fioletov, Julian Gröbner, Anu Heikkilä, Irina Petropavlovskikh, Janusz Jarosławski, Weine Josefsson, Tomi Karppinen, Ulf Köhler, Charoula Meleti, Christos Repapis, John Rimmer, Vladimir Savinykh, Vadim Shirotov, Anna Maria Siani, Andrew R. D. Smedley, Martin Stanek, and René Stübi
Atmos. Chem. Phys., 17, 551–574, https://doi.org/10.5194/acp-17-551-2017, https://doi.org/10.5194/acp-17-551-2017, 2017
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The paper makes a convincing case that the Brewer network is capable of detecting enhanced SO2 columns, as observed, e.g., after volcanic eruptions. For this reason, large volcanic eruptions of the past decade have been used to detect and forecast SO2 plumes of volcanic origin using the Brewer and other ground-based networks, aided by satellite, trajectory analysis calculations and modelling.
Tomi Raatikainen, David Brus, Rakesh K. Hooda, Antti-Pekka Hyvärinen, Eija Asmi, Ved P. Sharma, Antti Arola, and Heikki Lihavainen
Atmos. Chem. Phys., 17, 371–383, https://doi.org/10.5194/acp-17-371-2017, https://doi.org/10.5194/acp-17-371-2017, 2017
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We have measured black carbon aerosol properties in northern India at two sites: the first site is located at the polluted Indo-Gangetic Plain, while the second site is at the Himalayan foothills in a significantly cleaner environment. The observations show a clear difference in black carbon concentrations, but individual aerosol particles seem to be similar in both sites. Indirect evidence suggests that the particles are highly irregular resembling freshly emitted soot.
Emmanuel Dekemper, Jurgen Vanhamel, Bert Van Opstal, and Didier Fussen
Atmos. Meas. Tech., 9, 6025–6034, https://doi.org/10.5194/amt-9-6025-2016, https://doi.org/10.5194/amt-9-6025-2016, 2016
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We present a spectral imager capable of measuring the 2-D distribution of NO2 above well-delimited emission sources (power plant, city, etc.) with an unprecedent spatiotemporal resolution. Tests at a coal-fired power plant demonstrated its capability to observe dynamic processes such as the conversion from NO to NO2 in the early plume. Potential applications are pollution sources monitoring, reactive plume chemistry models validation, ships and volcanic emissions tracking, etc.
Stelios Kazadzis, Panagiotis Raptis, Natalia Kouremeti, Vassilis Amiridis, Antti Arola, Evangelos Gerasopoulos, and Gregory L. Schuster
Atmos. Meas. Tech., 9, 5997–6011, https://doi.org/10.5194/amt-9-5997-2016, https://doi.org/10.5194/amt-9-5997-2016, 2016
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Aerosols play an important role in the Earth's climate. One of the main aerosol properties is the single scattering albedo which is a measure of the aerosol absorption. In this work we have presented a method to retrieve this aerosol property in the ultraviolet and we presented the results for measurements at the urban environment of Athens, Greece. We show that the spectral dependence of the aerosol absorption in the VIS–IR and the UV range depends on the aerosol composition and type.
Colette Brogniez, Frédérique Auriol, Christine Deroo, Antti Arola, Jukka Kujanpää, Béatrice Sauvage, Niilo Kalakoski, Mikko Riku Aleksi Pitkänen, Maxime Catalfamo, Jean-Marc Metzger, Guy Tournois, and Pierre Da Conceicao
Atmos. Chem. Phys., 16, 15049–15074, https://doi.org/10.5194/acp-16-15049-2016, https://doi.org/10.5194/acp-16-15049-2016, 2016
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The atmospheric ozone layer is changing, thus the UV radiation at the surface is changing. Due to both beneficial and adverse effects of UV on the biosphere, monitoring of UV is essential. Satellite sensors provide estimates of UV at the surface with a global coverage. Validation of satellite-sensor UV is therefore needed and this can be done by comparison with ground-based measurements. The present validation in three sites (midlatitude, tropical) shows that OMI and GOME-2 provide reliable UV.
Anu Heikkilä, Jakke Sakari Mäkelä, Kaisa Lakkala, Outi Meinander, Jussi Kaurola, Tapani Koskela, Juha Matti Karhu, Tomi Karppinen, Esko Kyrö, and Gerrit de Leeuw
Geosci. Instrum. Method. Data Syst., 5, 531–540, https://doi.org/10.5194/gi-5-531-2016, https://doi.org/10.5194/gi-5-531-2016, 2016
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Lamp measurements used for the UV irradiance calibration of two Brewer spectrophotometers operated for 20 years in Jokioinen and Sodankylä, Finland, were examined. Temporal development of the responsivity after fixing the irradiance measurements into a specific scale was studied. Both long-term gradual decrease and abrupt changes in responsiveness were detected. Frequent-enough measurements of working standard lamps were found necessary to detect the short-term variations in responsiveness.
Hanna K. Lappalainen, Veli-Matti Kerminen, Tuukka Petäjä, Theo Kurten, Aleksander Baklanov, Anatoly Shvidenko, Jaana Bäck, Timo Vihma, Pavel Alekseychik, Meinrat O. Andreae, Stephen R. Arnold, Mikhail Arshinov, Eija Asmi, Boris Belan, Leonid Bobylev, Sergey Chalov, Yafang Cheng, Natalia Chubarova, Gerrit de Leeuw, Aijun Ding, Sergey Dobrolyubov, Sergei Dubtsov, Egor Dyukarev, Nikolai Elansky, Kostas Eleftheriadis, Igor Esau, Nikolay Filatov, Mikhail Flint, Congbin Fu, Olga Glezer, Aleksander Gliko, Martin Heimann, Albert A. M. Holtslag, Urmas Hõrrak, Juha Janhunen, Sirkku Juhola, Leena Järvi, Heikki Järvinen, Anna Kanukhina, Pavel Konstantinov, Vladimir Kotlyakov, Antti-Jussi Kieloaho, Alexander S. Komarov, Joni Kujansuu, Ilmo Kukkonen, Ella-Maria Duplissy, Ari Laaksonen, Tuomas Laurila, Heikki Lihavainen, Alexander Lisitzin, Alexsander Mahura, Alexander Makshtas, Evgeny Mareev, Stephany Mazon, Dmitry Matishov, Vladimir Melnikov, Eugene Mikhailov, Dmitri Moisseev, Robert Nigmatulin, Steffen M. Noe, Anne Ojala, Mari Pihlatie, Olga Popovicheva, Jukka Pumpanen, Tatjana Regerand, Irina Repina, Aleksei Shcherbinin, Vladimir Shevchenko, Mikko Sipilä, Andrey Skorokhod, Dominick V. Spracklen, Hang Su, Dmitry A. Subetto, Junying Sun, Arkady Y. Terzhevik, Yuri Timofeyev, Yuliya Troitskaya, Veli-Pekka Tynkkynen, Viacheslav I. Kharuk, Nina Zaytseva, Jiahua Zhang, Yrjö Viisanen, Timo Vesala, Pertti Hari, Hans Christen Hansson, Gennady G. Matvienko, Nikolai S. Kasimov, Huadong Guo, Valery Bondur, Sergej Zilitinkevich, and Markku Kulmala
Atmos. Chem. Phys., 16, 14421–14461, https://doi.org/10.5194/acp-16-14421-2016, https://doi.org/10.5194/acp-16-14421-2016, 2016
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After kick off in 2012, the Pan-Eurasian Experiment (PEEX) program has expanded fast and today the multi-disciplinary research community covers ca. 80 institutes and a network of ca. 500 scientists from Europe, Russia, and China. Here we introduce scientific topics relevant in this context. This is one of the first multi-disciplinary overviews crossing scientific boundaries, from atmospheric sciences to socio-economics and social sciences.
Laura Riuttanen, Marja Bister, Veli-Matti Kerminen, Viju O. John, Anu-Maija Sundström, Miikka Dal Maso, Jouni Räisänen, Victoria A. Sinclair, Risto Makkonen, Filippo Xausa, Gerrit de Leeuw, and Markku Kulmala
Atmos. Chem. Phys., 16, 14331–14342, https://doi.org/10.5194/acp-16-14331-2016, https://doi.org/10.5194/acp-16-14331-2016, 2016
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Here we show observational evidence that aerosols increase upper tropospheric humidity (UTH) via changes in the microphysics of deep convection. Using remote sensing data over the ocean east of China in summer, we show that increased aerosol loads are associated with an UTH increase of 2.2 ± 1.5 in units of relative humidity. We show that humidification of aerosols or other meteorological covariation is very unlikely to be the cause for this result indicating relevance for the global climate.
Monique F. M. A. Albert, Magdalena D. Anguelova, Astrid M. M. Manders, Martijn Schaap, and Gerrit de Leeuw
Atmos. Chem. Phys., 16, 13725–13751, https://doi.org/10.5194/acp-16-13725-2016, https://doi.org/10.5194/acp-16-13725-2016, 2016
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Sea spray source functions (SSSFs) predict production of sea salt aerosol, important for climate. Sea spray originates from bubble bursting within whitecaps, mainly formed by wind speed (U). Using satellite-based whitecap fraction (W) data analyzed on global and regional scale and explicitly accounting for sea surface temperature (T) we derive a new W(U, T) parameterization. We use it to evaluate influence of secondary factors on a SSSF via W.
Elham Baranizadeh, Benjamin N. Murphy, Jan Julin, Saeed Falahat, Carly L. Reddington, Antti Arola, Lars Ahlm, Santtu Mikkonen, Christos Fountoukis, David Patoulias, Andreas Minikin, Thomas Hamburger, Ari Laaksonen, Spyros N. Pandis, Hanna Vehkamäki, Kari E. J. Lehtinen, and Ilona Riipinen
Geosci. Model Dev., 9, 2741–2754, https://doi.org/10.5194/gmd-9-2741-2016, https://doi.org/10.5194/gmd-9-2741-2016, 2016
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The molecular mechanisms through which new ultrafine (< 100 nm) aerosol particles are formed in the atmosphere have puzzled the scientific community for decades. In the past few years, however, significant progress has been made in unraveling these processes through laboratory studies and computational efforts. In this work we have implemented these new developments to an air quality model and study the implications of anthropogenically driven particle formation for European air quality.
Anu Heikkilä, Jussi Kaurola, Kaisa Lakkala, Juha Matti Karhu, Esko Kyrö, Tapani Koskela, Ola Engelsen, Harry Slaper, and Gunther Seckmeyer
Geosci. Instrum. Method. Data Syst., 5, 333–345, https://doi.org/10.5194/gi-5-333-2016, https://doi.org/10.5194/gi-5-333-2016, 2016
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Solar spectral UV irradiance data measured by the Brewer #037 spectroradiometer in Sodankylä, Finland, in 1990–2014 were examined for their quality flags given by the quality assurance (QA) tools of the European UV DataBase (EUVDB). Statistical analysis on the flags was performed, and five cases were investigated in detail. The results can be used in further development of the quality control/QA tools and selection of cases of exceptional atmospheric conditions for process studies.
Kaisa Lakkala, Hanne Suokanerva, Juha Matti Karhu, Antti Aarva, Antti Poikonen, Tomi Karppinen, Markku Ahponen, Henna-Reetta Hannula, Anna Kontu, and Esko Kyrö
Geosci. Instrum. Method. Data Syst., 5, 315–320, https://doi.org/10.5194/gi-5-315-2016, https://doi.org/10.5194/gi-5-315-2016, 2016
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This paper describes the laboratory facilities at the Finnish Meteorological Institute – Arctic Research Centre (FMI-ARC). They comprise an optical laboratory, a facility for biological studies, and an office. The facilities are ideal for responding to the needs of international multidisciplinary research, giving the possibility to calibrate and characterize the research instruments as well as handle and store samples.
U. Frieß, H. Klein Baltink, S. Beirle, K. Clémer, F. Hendrick, B. Henzing, H. Irie, G. de Leeuw, A. Li, M. M. Moerman, M. van Roozendael, R. Shaiganfar, T. Wagner, Y. Wang, P. Xie, S. Yilmaz, and P. Zieger
Atmos. Meas. Tech., 9, 3205–3222, https://doi.org/10.5194/amt-9-3205-2016, https://doi.org/10.5194/amt-9-3205-2016, 2016
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This article describes the first direct comparison of aerosol extinction profiles from Multi-Axis DOAS measurements of the oxygen collision complex using five different retrieval algorithms. A comparison of the retrieved profiles with co-located aerosol measurements shows good agreement with respect to profile shape and aerosol optical thickness. This study shows that MAX-DOAS is a simple, versatile and cost-effective method for the measurement of aerosol properties in the lower troposphere.
Tero Mielonen, Anca Hienola, Thomas Kühn, Joonas Merikanto, Antti Lipponen, Tommi Bergman, Hannele Korhonen, Pekka Kolmonen, Larisa Sogacheva, Darren Ghent, Antti Arola, Gerrit de Leeuw, and Harri Kokkola
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-625, https://doi.org/10.5194/acp-2016-625, 2016
Revised manuscript not accepted
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We studied the temperature dependence of AOD and its radiative effects over the southeastern US. We used spaceborne observations of AOD, LST and tropospheric NO2 with simulations of ECHAM-HAMMOZ. The level of AOD in this region is governed by anthropogenic emissions but the temperature dependency is most likely caused by BVOC emissions. According to the observations and simulations, the regional clear-sky DRE for biogenic aerosols is −0.43 ± 0.88 W/m2/K and −0.86 ± 0.06 W/m2/K, respectively.
Jani Huttunen, Harri Kokkola, Tero Mielonen, Mika Esa Juhani Mononen, Antti Lipponen, Juha Reunanen, Anders Vilhelm Lindfors, Santtu Mikkonen, Kari Erkki Juhani Lehtinen, Natalia Kouremeti, Alkiviadis Bais, Harri Niska, and Antti Arola
Atmos. Chem. Phys., 16, 8181–8191, https://doi.org/10.5194/acp-16-8181-2016, https://doi.org/10.5194/acp-16-8181-2016, 2016
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For a good estimate of the current forcing by anthropogenic aerosols, knowledge in past is needed. One option to lengthen time series is to retrieve aerosol optical depth from solar radiation measurements. We have evaluated several methods for this task. Most of the methods produce aerosol optical depth estimates with a good accuracy. However, machine learning methods seem to be the most applicable not to produce any systematic biases, since they do not need constrain the aerosol properties.
Tomi Karppinen, Kaisa Lakkala, Juha M. Karhu, Pauli Heikkinen, Rigel Kivi, and Esko Kyrö
Geosci. Instrum. Method. Data Syst., 5, 229–239, https://doi.org/10.5194/gi-5-229-2016, https://doi.org/10.5194/gi-5-229-2016, 2016
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In this paper, a 26-year-long time series of total ozone column above Arctic Research Center in Sodankylä is presented. The time series is produced using a uniform method, presented in the paper, for retrieving the ozone column from the measurements. The data are checked for obvious errors and filtered automatically and manually to ensure that only good-quality data are delivered to public databases. Some features of the time series are highlighted and availability of the measurements is presented.
Fanni Mylläri, Eija Asmi, Tatu Anttila, Erkka Saukko, Ville Vakkari, Liisa Pirjola, Risto Hillamo, Tuomas Laurila, Anna Häyrinen, Jani Rautiainen, Heikki Lihavainen, Ewan O'Connor, Ville Niemelä, Jorma Keskinen, Miikka Dal Maso, and Topi Rönkkö
Atmos. Chem. Phys., 16, 7485–7496, https://doi.org/10.5194/acp-16-7485-2016, https://doi.org/10.5194/acp-16-7485-2016, 2016
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The primary emissions of a coal-fired power plant were highly affected by the flue-gas cleaning technologies. The primary emission results were used as input values for a Gaussian plume model and the model correlated well with the atmospheric measurements from the flue-gas plume. Concentrations of newly formed particles in the flue gas plume were higher than the primary particle concentration, and thus the source of particle-forming precursors should be characterized in more detail.
Jakke Sakari Mäkelä, Kaisa Lakkala, Tapani Koskela, Tomi Karppinen, Juha Matti Karhu, Vladimir Savastiouk, Hanne Suokanerva, Jussi Kaurola, Antti Arola, Anders Vilhelm Lindfors, Outi Meinander, Gerrit de Leeuw, and Anu Heikkilä
Geosci. Instrum. Method. Data Syst., 5, 193–203, https://doi.org/10.5194/gi-5-193-2016, https://doi.org/10.5194/gi-5-193-2016, 2016
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We describe the steps that are used at the Finnish Meteorological Institute (FMI) to process spectral ultraviolet (UV) radiation measurements made with its three Brewer spectrophotometers, located in Sodankylä (67° N) and Jokioinen (61° N). Multiple corrections are made to the data in near-real time and quality control is also performed automatically. Several data products are produced, including the near-real-time UV index and various daily dosages, and submitted to databases.
G. L. Schuster, O. Dubovik, and A. Arola
Atmos. Chem. Phys., 16, 1565–1585, https://doi.org/10.5194/acp-16-1565-2016, https://doi.org/10.5194/acp-16-1565-2016, 2016
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We describe a method of using remote sensing of the refractive index to determine the relative contribution of carbonaceous aerosols and absorbing iron minerals. Monthly climatologies of fine mode soot carbon are low for West Africa and the Middle East, but the southern Africa and South America biomass burning sites have peak values that are much higher; this is consistent with expectations. Hence, refractive index is a practical parameter for quantifying soot carbon in the atmosphere.
G. L. Schuster, O. Dubovik, A. Arola, T. F. Eck, and B. N. Holben
Atmos. Chem. Phys., 16, 1587–1602, https://doi.org/10.5194/acp-16-1587-2016, https://doi.org/10.5194/acp-16-1587-2016, 2016
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Some authors have recently suggested that the spectral dependence of aerosol absorption may be used to separate soot carbon absorption from the aerosol absorption associated with organic carbon and dust. We demonstrate that this approach is inconsistent with the underlying assumptions that are required to infer aerosol absorption through remote sensing techniques, and that carbonaceous aerosols can not be differentiated from dust by exclusively using spectral absorption signatures.
E. Asmi, V. Kondratyev, D. Brus, T. Laurila, H. Lihavainen, J. Backman, V. Vakkari, M. Aurela, J. Hatakka, Y. Viisanen, T. Uttal, V. Ivakhov, and A. Makshtas
Atmos. Chem. Phys., 16, 1271–1287, https://doi.org/10.5194/acp-16-1271-2016, https://doi.org/10.5194/acp-16-1271-2016, 2016
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Aerosol number size distributions were measured in Arctic Russia continuously during 4 years. The particles' seasonal characteristics and sources were identified based on these data. In early spring, elevated concentrations were detected during episodes of Arctic haze and during days of secondary particle formation. In summer, Siberian forests biogenic emissions had a significant impact on particle number and mass. These are the first such results obtained from the region.
O. Meinander, A. Aarva, A. Poikonen, A. Kontu, H. Suokanerva, E. Asmi, K. Neitola, E. Rodriguez, R. Sanchez, M. Mei, G. de Leeuw, and E. Kyrö
Geosci. Instrum. Method. Data Syst. Discuss., https://doi.org/10.5194/gi-2015-31, https://doi.org/10.5194/gi-2015-31, 2016
Revised manuscript not accepted
J. I. Peltoniemi, M. Gritsevich, T. Hakala, P. Dagsson-Waldhauserová, Ó. Arnalds, K. Anttila, H.-R. Hannula, N. Kivekäs, H. Lihavainen, O. Meinander, J. Svensson, A. Virkkula, and G. de Leeuw
The Cryosphere, 9, 2323–2337, https://doi.org/10.5194/tc-9-2323-2015, https://doi.org/10.5194/tc-9-2323-2015, 2015
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Light-absorbing impurities change the reflectance of snow in different ways. Some particles are heated by the Sun and they sink out of sight. During the process, snow may look darker than pure snow when observed by nadir, but at larger view zenith angles the snow may look as white as clean snow. Thus an observer on the ground may overestimate the albedo, while a satellite underestimates the albedo. Climate studies need to examine how the contaminants behave in snow, not only their total amounts.
A. Arola, G. L. Schuster, M. R. A. Pitkänen, O. Dubovik, H. Kokkola, A. V. Lindfors, T. Mielonen, T. Raatikainen, S. Romakkaniemi, S. N. Tripathi, and H. Lihavainen
Atmos. Chem. Phys., 15, 12731–12740, https://doi.org/10.5194/acp-15-12731-2015, https://doi.org/10.5194/acp-15-12731-2015, 2015
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There have been relatively few measurement-based estimates for the direct radiative effect of brown carbon so far. This is first time that the direct radiative effect of brown carbon is estimated by exploiting the AERONET-retrieved imaginary indices. We estimated it for four sites in the Indo-Gangetic Plain: Karachi, Lahore,
Kanpur and Gandhi College.
H. Eskes, V. Huijnen, A. Arola, A. Benedictow, A.-M. Blechschmidt, E. Botek, O. Boucher, I. Bouarar, S. Chabrillat, E. Cuevas, R. Engelen, H. Flentje, A. Gaudel, J. Griesfeller, L. Jones, J. Kapsomenakis, E. Katragkou, S. Kinne, B. Langerock, M. Razinger, A. Richter, M. Schultz, M. Schulz, N. Sudarchikova, V. Thouret, M. Vrekoussis, A. Wagner, and C. Zerefos
Geosci. Model Dev., 8, 3523–3543, https://doi.org/10.5194/gmd-8-3523-2015, https://doi.org/10.5194/gmd-8-3523-2015, 2015
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The MACC project is preparing the operational atmosphere service of the European Copernicus Programme, and uses data assimilation to combine atmospheric models with available observations. Our paper provides an overview of the aerosol and trace gas validation activity of MACC. Topics are the validation requirements, the measurement data, the assimilation systems, the upgrade procedure, operational aspects and the scoring methods. A summary is provided of recent results, including special events.
M. Paramonov, V.-M. Kerminen, M. Gysel, P. P. Aalto, M. O. Andreae, E. Asmi, U. Baltensperger, A. Bougiatioti, D. Brus, G. P. Frank, N. Good, S. S. Gunthe, L. Hao, M. Irwin, A. Jaatinen, Z. Jurányi, S. M. King, A. Kortelainen, A. Kristensson, H. Lihavainen, M. Kulmala, U. Lohmann, S. T. Martin, G. McFiggans, N. Mihalopoulos, A. Nenes, C. D. O'Dowd, J. Ovadnevaite, T. Petäjä, U. Pöschl, G. C. Roberts, D. Rose, B. Svenningsson, E. Swietlicki, E. Weingartner, J. Whitehead, A. Wiedensohler, C. Wittbom, and B. Sierau
Atmos. Chem. Phys., 15, 12211–12229, https://doi.org/10.5194/acp-15-12211-2015, https://doi.org/10.5194/acp-15-12211-2015, 2015
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The research paper presents the first comprehensive overview of field measurements with the CCN Counter performed at a large number of locations around the world within the EUCAARI framework. The paper sheds light on the CCN number concentrations and activated fractions around the world and their dependence on the water vapour supersaturation ratio, the dependence of aerosol hygroscopicity on particle size, and seasonal and diurnal variation of CCN activation and hygroscopic properties.
J. Joutsensaari, P. Yli-Pirilä, H. Korhonen, A. Arola, J. D. Blande, J. Heijari, M. Kivimäenpää, S. Mikkonen, L. Hao, P. Miettinen, P. Lyytikäinen-Saarenmaa, C. L. Faiola, A. Laaksonen, and J. K. Holopainen
Atmos. Chem. Phys., 15, 12139–12157, https://doi.org/10.5194/acp-15-12139-2015, https://doi.org/10.5194/acp-15-12139-2015, 2015
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Global warming will induce large-scale insect outbreaks in boreal forests. Our results from field and laboratory experiments, satellite observations and global-scale modelling suggest that more frequent insect outbreaks, in addition to temperature-dependent increases in VOC emissions, could result in substantial increases in biogenic SOA formation and therefore affect both aerosol direct and indirect forcing of climate at regional scales. This should be considered in future climate predictions.
K. Atlaskina, F. Berninger, and G. de Leeuw
The Cryosphere, 9, 1879–1893, https://doi.org/10.5194/tc-9-1879-2015, https://doi.org/10.5194/tc-9-1879-2015, 2015
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Snow cover explained most of the spring surface albedo changes in the Northern Hemisphere in the years 2000−2012. However, there are vast areas where albedo changed up to ±0.2 under full snow-covered conditions. We found that if in these areas, the mean monthly air temperature exceeds a value between -15°C and -10°C, depending on the region, albedo decreases with an increase of the temperature. The complexity of processes involved in surface albedo changes is discussed.
T. Raatikainen, D. Brus, A.-P. Hyvärinen, J. Svensson, E. Asmi, and H. Lihavainen
Atmos. Chem. Phys., 15, 10057–10070, https://doi.org/10.5194/acp-15-10057-2015, https://doi.org/10.5194/acp-15-10057-2015, 2015
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We have measured atmospheric aerosol composition by using a Single Particle Soot Photometer (SP2) in the Finnish Arctic during winter 2011-2012. SP2 can give detailed information about mass distributions and mixing state of refractory black carbon (rBC). The measurements showed varying rBC mass concentrations, but relatively constant rBC core size distributions and mixing state parameters. On average, 24% of all particles contain rBC and the observed rBC cores are always thickly coated.
E. Rodríguez, P. Kolmonen, T. H. Virtanen, L. Sogacheva, A.-M. Sundström, and G. de Leeuw
Atmos. Meas. Tech., 8, 3075–3085, https://doi.org/10.5194/amt-8-3075-2015, https://doi.org/10.5194/amt-8-3075-2015, 2015
A. N. Schwier, C. Rose, E. Asmi, A. M. Ebling, W. M. Landing, S. Marro, M.-L. Pedrotti, A. Sallon, F. Iuculano, S. Agusti, A. Tsiola, P. Pitta, J. Louis, C. Guieu, F. Gazeau, and K. Sellegri
Atmos. Chem. Phys., 15, 7961–7976, https://doi.org/10.5194/acp-15-7961-2015, https://doi.org/10.5194/acp-15-7961-2015, 2015
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The effect of ocean acidification and changing water conditions on primary (and secondary) marine aerosol emissions is not well understood on a regional or a global scale. To investigate this effect, we deployed mesocosms in the Mediterranean Sea for several weeks during both winter pre-bloom and summer oligotrophic conditions and subjected them to various levels of CO2. We observed larger effects due to the differences between a pre-bloom and oligotrophic environment than due to CO2 levels.
W. Wandji Nyamsi, A. Arola, P. Blanc, A. V. Lindfors, V. Cesnulyte, M. R. A. Pitkänen, and L. Wald
Atmos. Chem. Phys., 15, 7449–7456, https://doi.org/10.5194/acp-15-7449-2015, https://doi.org/10.5194/acp-15-7449-2015, 2015
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A novel model of the absorption of radiation by ozone in the UV bands [283, 307]nm and [307, 328]nm yields improvements in the modeling of the transmissivity in these bands. This model is faster than detailed spectral calculations and is as accurate with maximum errors of respectively 0.0006 and 0.0143. How to practically implement this new parameterization in a radiative transfer model is discussed for the case of libRadtran.
G. Bernhard, A. Arola, A. Dahlback, V. Fioletov, A. Heikkilä, B. Johnsen, T. Koskela, K. Lakkala, T. Svendby, and J. Tamminen
Atmos. Chem. Phys., 15, 7391–7412, https://doi.org/10.5194/acp-15-7391-2015, https://doi.org/10.5194/acp-15-7391-2015, 2015
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Surface erythemal UV data from the Ozone Monitoring Instrument (OMI) are validated for high northern latitudes (Arctic and Scandinavia) using ground-based measurements. The bias in OMI data caused by incorrect assumptions of the surface albedo are quantified and the mechanism that causes this bias is discussed. Methods to improve the accuracy of OMI data products are presented.
P. Zieger, P. P. Aalto, V. Aaltonen, M. Äijälä, J. Backman, J. Hong, M. Komppula, R. Krejci, M. Laborde, J. Lampilahti, G. de Leeuw, A. Pfüller, B. Rosati, M. Tesche, P. Tunved, R. Väänänen, and T. Petäjä
Atmos. Chem. Phys., 15, 7247–7267, https://doi.org/10.5194/acp-15-7247-2015, https://doi.org/10.5194/acp-15-7247-2015, 2015
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The effect of water uptake (hygroscopicity) on aerosol light scattering properties is generally lower for boreal aerosol due to the dominance of organic substances. A columnar optical closure study using ground-based and airborne measurements of aerosol optical, chemical and microphysical properties was conducted and the implications and limitations are discussed.
A.-M. Sundström, A. Nikandrova, K. Atlaskina, T. Nieminen, V. Vakkari, L. Laakso, J. P. Beukes, A. Arola, P. G. van Zyl, M. Josipovic, A. D. Venter, K. Jaars, J. J. Pienaar, S. Piketh, A. Wiedensohler, E. K. Chiloane, G. de Leeuw, and M. Kulmala
Atmos. Chem. Phys., 15, 4983–4996, https://doi.org/10.5194/acp-15-4983-2015, https://doi.org/10.5194/acp-15-4983-2015, 2015
C. Rose, K. Sellegri, E. Asmi, M. Hervo, E. Freney, A. Colomb, H. Junninen, J. Duplissy, M. Sipilä, J. Kontkanen, K. Lehtipalo, and M. Kulmala
Atmos. Chem. Phys., 15, 3413–3428, https://doi.org/10.5194/acp-15-3413-2015, https://doi.org/10.5194/acp-15-3413-2015, 2015
J. Svensson, A. Virkkula, O. Meinander, N. Kivekäs, H.-R. Hannula, O. Järvinen, J. I. Peltoniemi, M. Gritsevich, A. Heikkilä, A. Kontu, A.-P. Hyvärinen, K. Neitola, D. Brus, P. Dagsson-Waldhauserova, K. Anttila, T. Hakala, H. Kaartinen, M. Vehkamäki, G. de Leeuw, and H. Lihavainen
The Cryosphere Discuss., https://doi.org/10.5194/tcd-9-1227-2015, https://doi.org/10.5194/tcd-9-1227-2015, 2015
Revised manuscript not accepted
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Soot's (including black carbon and organics) negative effect on a natural snow pack is experimentally addressed in this paper through a series of experiments. Soot concentrations in the snow in the range of 200-200 000 ppb verify the negative effects on the albedo, the physical snow characteristics, as well as increasing the melt rate of the snow pack. Our experimental data generally agrees when compared with the Snow, Ice and Aerosol Radiation model.
L. Sogacheva, P. Kolmonen, T. H. Virtanen, E. Rodriguez, A.-M. Sundström, and G. de Leeuw
Atmos. Meas. Tech., 8, 891–906, https://doi.org/10.5194/amt-8-891-2015, https://doi.org/10.5194/amt-8-891-2015, 2015
A.-M. Sundström, A. Arola, P. Kolmonen, Y. Xue, G. de Leeuw, and M. Kulmala
Atmos. Chem. Phys., 15, 505–518, https://doi.org/10.5194/acp-15-505-2015, https://doi.org/10.5194/acp-15-505-2015, 2015
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In this work, a satellite-based approach to derive the aerosol direct shortwave (SW) radiative effect (ADRE) is studied. The method is based on using coincident satellite observations of SW fluxes and aerosol optical depths (AODs). The key findings of this study are that using normalized values of observed fluxes improves the estimates of ADRE and aerosol-free TOA fluxes as compared to a model. The method was applied over eastern China where the satellite-based mean ADRE of -5Wm-2 was obtained.
M. R. A. Pitkänen, A. Arola, K. Lakkala, T. Koskela, and A. V. Lindfors
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-8-487-2015, https://doi.org/10.5194/amtd-8-487-2015, 2015
Revised manuscript not accepted
A.-I. Partanen, E. M. Dunne, T. Bergman, A. Laakso, H. Kokkola, J. Ovadnevaite, L. Sogacheva, D. Baisnée, J. Sciare, A. Manders, C. O'Dowd, G. de Leeuw, and H. Korhonen
Atmos. Chem. Phys., 14, 11731–11752, https://doi.org/10.5194/acp-14-11731-2014, https://doi.org/10.5194/acp-14-11731-2014, 2014
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New parameterizations for the sea spray aerosol source flux and its organic fraction were incorporated into a global aerosol-climate model. The emissions of sea salt were considerably less than previous estimates. This study demonstrates that sea spray aerosol may actually decrease the number of cloud droplets, which has a warming effect on climate. Overall, sea spray aerosol was predicted to have a global cooling effect due to the scattering of solar radiation from sea spray aerosol particles.
T. F. Eck, B. N. Holben, J. S. Reid, A. Arola, R. A. Ferrare, C. A. Hostetler, S. N. Crumeyrolle, T. A. Berkoff, E. J. Welton, S. Lolli, A. Lyapustin, Y. Wang, J. S. Schafer, D. M. Giles, B. E. Anderson, K. L. Thornhill, P. Minnis, K. E. Pickering, C. P. Loughner, A. Smirnov, and A. Sinyuk
Atmos. Chem. Phys., 14, 11633–11656, https://doi.org/10.5194/acp-14-11633-2014, https://doi.org/10.5194/acp-14-11633-2014, 2014
C. Gielen, M. Van Roozendael, F. Hendrick, G. Pinardi, T. Vlemmix, V. De Bock, H. De Backer, C. Fayt, C. Hermans, D. Gillotay, and P. Wang
Atmos. Meas. Tech., 7, 3509–3527, https://doi.org/10.5194/amt-7-3509-2014, https://doi.org/10.5194/amt-7-3509-2014, 2014
M. Karl, N. Castell, D. Simpson, S. Solberg, J. Starrfelt, T. Svendby, S.-E. Walker, and R. F. Wright
Atmos. Chem. Phys., 14, 8533–8557, https://doi.org/10.5194/acp-14-8533-2014, https://doi.org/10.5194/acp-14-8533-2014, 2014
L. L. Mei, Y. Xue, A. A. Kokhanovsky, W. von Hoyningen-Huene, G. de Leeuw, and J. P. Burrows
Atmos. Meas. Tech., 7, 2411–2420, https://doi.org/10.5194/amt-7-2411-2014, https://doi.org/10.5194/amt-7-2411-2014, 2014
T. H. Virtanen, P. Kolmonen, E. Rodríguez, L. Sogacheva, A.-M. Sundström, and G. de Leeuw
Atmos. Meas. Tech., 7, 2437–2456, https://doi.org/10.5194/amt-7-2437-2014, https://doi.org/10.5194/amt-7-2437-2014, 2014
J. Huttunen, A. Arola, G. Myhre, A. V. Lindfors, T. Mielonen, S. Mikkonen, J. S. Schafer, S. N. Tripathi, M. Wild, M. Komppula, and K. E. J. Lehtinen
Atmos. Chem. Phys., 14, 6103–6110, https://doi.org/10.5194/acp-14-6103-2014, https://doi.org/10.5194/acp-14-6103-2014, 2014
O. Meinander, A. Kontu, A. Virkkula, A. Arola, L. Backman, P. Dagsson-Waldhauserová, O. Järvinen, T. Manninen, J. Svensson, G. de Leeuw, and M. Leppäranta
The Cryosphere, 8, 991–995, https://doi.org/10.5194/tc-8-991-2014, https://doi.org/10.5194/tc-8-991-2014, 2014
A. Hirsikko, E. J. O'Connor, M. Komppula, K. Korhonen, A. Pfüller, E. Giannakaki, C. R. Wood, M. Bauer-Pfundstein, A. Poikonen, T. Karppinen, H. Lonka, M. Kurri, J. Heinonen, D. Moisseev, E. Asmi, V. Aaltonen, A. Nordbo, E. Rodriguez, H. Lihavainen, A. Laaksonen, K. E. J. Lehtinen, T. Laurila, T. Petäjä, M. Kulmala, and Y. Viisanen
Atmos. Meas. Tech., 7, 1351–1375, https://doi.org/10.5194/amt-7-1351-2014, https://doi.org/10.5194/amt-7-1351-2014, 2014
A. Virkkula, J. Levula, T. Pohja, P. P. Aalto, P. Keronen, S. Schobesberger, C. B. Clements, L. Pirjola, A.-J. Kieloaho, L. Kulmala, H. Aaltonen, J. Patokoski, J. Pumpanen, J. Rinne, T. Ruuskanen, M. Pihlatie, H. E. Manninen, V. Aaltonen, H. Junninen, T. Petäjä, J. Backman, M. Dal Maso, T. Nieminen, T. Olsson, T. Grönholm, J. Aalto, T. H. Virtanen, M. Kajos, V.-M. Kerminen, D. M. Schultz, J. Kukkonen, M. Sofiev, G. De Leeuw, J. Bäck, P. Hari, and M. Kulmala
Atmos. Chem. Phys., 14, 4473–4502, https://doi.org/10.5194/acp-14-4473-2014, https://doi.org/10.5194/acp-14-4473-2014, 2014
D. C. S. Beddows, M. Dall'Osto, R. M. Harrison, M. Kulmala, A. Asmi, A. Wiedensohler, P. Laj, A.M. Fjaeraa, K. Sellegri, W. Birmili, N. Bukowiecki, E. Weingartner, U. Baltensperger, V. Zdimal, N. Zikova, J.-P. Putaud, A. Marinoni, P. Tunved, H.-C. Hansson, M. Fiebig, N. Kivekäs, E. Swietlicki, H. Lihavainen, E. Asmi, V. Ulevicius, P. P. Aalto, N. Mihalopoulos, N. Kalivitis, I. Kalapov, G. Kiss, G. de Leeuw, B. Henzing, C. O'Dowd, S. G. Jennings, H. Flentje, F. Meinhardt, L. Ries, H. A. C. Denier van der Gon, and A. J. H. Visschedijk
Atmos. Chem. Phys., 14, 4327–4348, https://doi.org/10.5194/acp-14-4327-2014, https://doi.org/10.5194/acp-14-4327-2014, 2014
M. Tjernström, C. Leck, C. E. Birch, J. W. Bottenheim, B. J. Brooks, I. M. Brooks, L. Bäcklin, R. Y.-W. Chang, G. de Leeuw, L. Di Liberto, S. de la Rosa, E. Granath, M. Graus, A. Hansel, J. Heintzenberg, A. Held, A. Hind, P. Johnston, J. Knulst, M. Martin, P. A. Matrai, T. Mauritsen, M. Müller, S. J. Norris, M. V. Orellana, D. A. Orsini, J. Paatero, P. O. G. Persson, Q. Gao, C. Rauschenberg, Z. Ristovski, J. Sedlar, M. D. Shupe, B. Sierau, A. Sirevaag, S. Sjogren, O. Stetzer, E. Swietlicki, M. Szczodrak, P. Vaattovaara, N. Wahlberg, M. Westberg, and C. R. Wheeler
Atmos. Chem. Phys., 14, 2823–2869, https://doi.org/10.5194/acp-14-2823-2014, https://doi.org/10.5194/acp-14-2823-2014, 2014
J. Ovadnevaite, A. Manders, G. de Leeuw, D. Ceburnis, C. Monahan, A.-I. Partanen, H. Korhonen, and C. D. O'Dowd
Atmos. Chem. Phys., 14, 1837–1852, https://doi.org/10.5194/acp-14-1837-2014, https://doi.org/10.5194/acp-14-1837-2014, 2014
V. Cesnulyte, A. V. Lindfors, M. R. A. Pitkänen, K. E. J. Lehtinen, J.-J. Morcrette, and A. Arola
Atmos. Chem. Phys., 14, 593–608, https://doi.org/10.5194/acp-14-593-2014, https://doi.org/10.5194/acp-14-593-2014, 2014
C. Rose, J. Boulon, M. Hervo, H. Holmgren, E. Asmi, M. Ramonet, P. Laj, and K. Sellegri
Atmos. Chem. Phys., 13, 11573–11594, https://doi.org/10.5194/acp-13-11573-2013, https://doi.org/10.5194/acp-13-11573-2013, 2013
G. Bernhard, A. Dahlback, V. Fioletov, A. Heikkilä, B. Johnsen, T. Koskela, K. Lakkala, and T. Svendby
Atmos. Chem. Phys., 13, 10573–10590, https://doi.org/10.5194/acp-13-10573-2013, https://doi.org/10.5194/acp-13-10573-2013, 2013
M. Lefèvre, A. Oumbe, P. Blanc, B. Espinar, B. Gschwind, Z. Qu, L. Wald, M. Schroedter-Homscheidt, C. Hoyer-Klick, A. Arola, A. Benedetti, J. W. Kaiser, and J.-J. Morcrette
Atmos. Meas. Tech., 6, 2403–2418, https://doi.org/10.5194/amt-6-2403-2013, https://doi.org/10.5194/amt-6-2403-2013, 2013
G. Saponaro, P. Kolmonen, J. Karhunen, J. Tamminen, and G. de Leeuw
Atmos. Meas. Tech., 6, 2301–2309, https://doi.org/10.5194/amt-6-2301-2013, https://doi.org/10.5194/amt-6-2301-2013, 2013
A. Arola, T. F. Eck, J. Huttunen, K. E. J. Lehtinen, A. V. Lindfors, G. Myhre, A. Smirnov, S. N. Tripathi, and H. Yu
Atmos. Chem. Phys., 13, 7895–7901, https://doi.org/10.5194/acp-13-7895-2013, https://doi.org/10.5194/acp-13-7895-2013, 2013
T. Holzer-Popp, G. de Leeuw, J. Griesfeller, D. Martynenko, L. Klüser, S. Bevan, W. Davies, F. Ducos, J. L. Deuzé, R. G. Graigner, A. Heckel, W. von Hoyningen-Hüne, P. Kolmonen, P. Litvinov, P. North, C. A. Poulsen, D. Ramon, R. Siddans, L. Sogacheva, D. Tanre, G. E. Thomas, M. Vountas, J. Descloitres, J. Griesfeller, S. Kinne, M. Schulz, and S. Pinnock
Atmos. Meas. Tech., 6, 1919–1957, https://doi.org/10.5194/amt-6-1919-2013, https://doi.org/10.5194/amt-6-1919-2013, 2013
E. Järvinen, A. Virkkula, T. Nieminen, P. P. Aalto, E. Asmi, C. Lanconelli, M. Busetto, A. Lupi, R. Schioppo, V. Vitale, M. Mazzola, T. Petäjä, V.-M. Kerminen, and M. Kulmala
Atmos. Chem. Phys., 13, 7473–7487, https://doi.org/10.5194/acp-13-7473-2013, https://doi.org/10.5194/acp-13-7473-2013, 2013
P. Kolmonen, A.-M. Sundström, L. Sogacheva, E. Rodriguez, T. Virtanen, and G. de Leeuw
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-6-4039-2013, https://doi.org/10.5194/amtd-6-4039-2013, 2013
Revised manuscript has not been submitted
A. V. Lindfors, N. Kouremeti, A. Arola, S. Kazadzis, A. F. Bais, and A. Laaksonen
Atmos. Chem. Phys., 13, 3733–3741, https://doi.org/10.5194/acp-13-3733-2013, https://doi.org/10.5194/acp-13-3733-2013, 2013
S. J. Norris, I. M. Brooks, B. I. Moat, M. J. Yelland, G. de Leeuw, R. W. Pascal, and B. Brooks
Ocean Sci., 9, 133–145, https://doi.org/10.5194/os-9-133-2013, https://doi.org/10.5194/os-9-133-2013, 2013
L. Riuttanen, M. Dal Maso, G. de Leeuw, I. Riipinen, L. Sogacheva, V. Vakkari, L. Laakso, and M. Kulmala
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-4289-2013, https://doi.org/10.5194/acpd-13-4289-2013, 2013
Revised manuscript has not been submitted
A. Asmi, M. Collaud Coen, J. A. Ogren, E. Andrews, P. Sheridan, A. Jefferson, E. Weingartner, U. Baltensperger, N. Bukowiecki, H. Lihavainen, N. Kivekäs, E. Asmi, P. P. Aalto, M. Kulmala, A. Wiedensohler, W. Birmili, A. Hamed, C. O'Dowd, S. G Jennings, R. Weller, H. Flentje, A. M. Fjaeraa, M. Fiebig, C. L. Myhre, A. G. Hallar, E. Swietlicki, A. Kristensson, and P. Laj
Atmos. Chem. Phys., 13, 895–916, https://doi.org/10.5194/acp-13-895-2013, https://doi.org/10.5194/acp-13-895-2013, 2013
V.-M. Kerminen, M. Paramonov, T. Anttila, I. Riipinen, C. Fountoukis, H. Korhonen, E. Asmi, L. Laakso, H. Lihavainen, E. Swietlicki, B. Svenningsson, A. Asmi, S. N. Pandis, M. Kulmala, and T. Petäjä
Atmos. Chem. Phys., 12, 12037–12059, https://doi.org/10.5194/acp-12-12037-2012, https://doi.org/10.5194/acp-12-12037-2012, 2012
T. Viskari, E. Asmi, P. Kolmonen, H. Vuollekoski, T. Petäjä, and H. Järvinen
Atmos. Chem. Phys., 12, 11767–11779, https://doi.org/10.5194/acp-12-11767-2012, https://doi.org/10.5194/acp-12-11767-2012, 2012
T. Viskari, E. Asmi, A. Virkkula, P. Kolmonen, T. Petäjä, and H. Järvinen
Atmos. Chem. Phys., 12, 11781–11793, https://doi.org/10.5194/acp-12-11781-2012, https://doi.org/10.5194/acp-12-11781-2012, 2012
E. Asmi, E. Freney, M. Hervo, D. Picard, C. Rose, A. Colomb, and K. Sellegri
Atmos. Chem. Phys., 12, 11589–11607, https://doi.org/10.5194/acp-12-11589-2012, https://doi.org/10.5194/acp-12-11589-2012, 2012
Related subject area
Subject: Radiation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Tethered balloon-borne observations of thermal-infrared irradiance and cooling rate profiles in the Arctic atmospheric boundary layer
Assessing the cloud radiative bias at Macquarie Island in the ACCESS-AM2 model
Surface energy balance fluxes in a suburban area of Beijing: energy partitioning variability
Effects of variable ice–ocean surface properties and air mass transformation on the Arctic radiative energy budget
Broadband and filter radiometers at Ross Island, Antarctica: Detection of cloud ice phase versus liquid water influences on shortwave and longwave radiation
Airborne observations of the surface cloud radiative effect during different seasons over sea ice and open ocean in the Fram Strait
Assessment of spectral UV radiation at Marambio Base, Antarctic Peninsula
Parameterization of downward long-wave radiation based on long-term baseline surface radiation measurements in China
An assessment of land energy balance over East Asia from multiple lines of evidence and the roles of the Tibet Plateau, aerosols, and clouds
Ozone, DNA-active UV radiation, and cloud changes for the near-global mean and at high latitudes due to enhanced greenhouse gas concentrations
In situ observation of warm atmospheric layer and the heat contribution of suspended dust over the Tarim Basin
Eight-year variations in atmospheric radiocesium in Fukushima city
Variability and trends in surface solar spectral ultraviolet irradiance in Italy: on the influence of geopotential height and lower-stratospheric ozone
Fifty-six years of surface solar radiation and sunshine duration over São Paulo, Brazil: 1961–2016
Changes in the surface broadband shortwave radiation budget during the 2017 eclipse
Reassessment of shortwave surface cloud radiative forcing in the Arctic: consideration of surface-albedo–cloud interactions
Deposition of brown carbon onto snow: changes in snow optical and radiative properties
A revisiting of the parametrization of downward longwave radiation in summer over the Tibetan Plateau based on high-temporal-resolution measurements
Trends in surface radiation and cloud radiative effect at four Swiss sites for the 1996–2015 period
Can downwelling far-infrared radiances over Antarctica be estimated from mid-infrared information?
Measurements of spectral irradiance during the solar eclipse of 21 August 2017: reassessment of the effect of solar limb darkening and of changes in total ozone
UV measurements at Marambio and Ushuaia during 2000–2010
On the suitability of current atmospheric reanalyses for regional warming studies over China
A long-term time series of global and diffuse photosynthetically active radiation in the Mediterranean: interannual variability and cloud effects
Long-term series and trends in surface solar radiation in Athens, Greece
Reconstruction and analysis of erythemal UV radiation time series from Hradec Králové (Czech Republic) over the past 50 years
Trends in erythemal doses at the Polish Polar Station, Hornsund, Svalbard based on the homogenized measurements (1996–2016) and reconstructed data (1983–1995)
Effects of vernal equinox solar eclipse on temperature and wind direction in Switzerland
Sky radiance at a coastline and effects of land and ocean reflectivities
Impact of aerosols and clouds on decadal trends in all-sky solar radiation over the Netherlands (1966–2015)
Contributions of surface solar radiation and precipitation to the spatiotemporal patterns of surface and air warming in China from 1960 to 2003
Multiresolution analysis of the spatiotemporal variability in global radiation observed by a dense network of 99 pyranometers
Validation of satellite-based noontime UVI with NDACC ground-based instruments: influence of topography, environment and satellite overpass time
Is global dimming and brightening in Japan limited to urban areas?
The climatology of planetary boundary layer height in China derived from radiosonde and reanalysis data
Detection of dimming/brightening in Italy from homogenized all-sky and clear-sky surface solar radiation records and underlying causes (1959–2013)
Comparison of land–atmosphere interaction at different surface types in the mid- to lower reaches of the Yangtze River valley
Spectral optical layer properties of cirrus from collocated airborne measurements and simulations
Local short-term variability in solar irradiance
The contrasting roles of water and dust in controlling daily variations in radiative heating of the summertime Saharan heat low
Global dimming and urbanization: did stronger negative SSR trends collocate with regions of population growth?
Short- and long-term variability of spectral solar UV irradiance at Thessaloniki, Greece: effects of changes in aerosols, total ozone and clouds
On the progress of the 2015–2016 El Niño event
Role of radiatively forced temperature changes in enhanced semi-arid warming in the cold season over east Asia
Assessment of long-term WRF–CMAQ simulations for understanding direct aerosol effects on radiation "brightening" in the United States
Comparison of OMI UV observations with ground-based measurements at high northern latitudes
Characterisation of J(O1D) at Cape Grim 2000–2005
On the scaling of the solar incident flux
Analysis of actinic flux profiles measured from an ozonesonde balloon
Relations between erythemal UV dose, global solar radiation, total ozone column and aerosol optical depth at Uccle, Belgium
Michael Lonardi, Elisa F. Akansu, André Ehrlich, Mauro Mazzola, Christian Pilz, Matthew D. Shupe, Holger Siebert, and Manfred Wendisch
Atmos. Chem. Phys., 24, 1961–1978, https://doi.org/10.5194/acp-24-1961-2024, https://doi.org/10.5194/acp-24-1961-2024, 2024
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Profiles of thermal-infrared irradiance were measured at two Arctic sites. The presence or lack of clouds influences the vertical structure of these observations. In particular, the cloud top region is a source of radiative energy that can promote cooling and mixing in the cloud layer. Simulations are used to further characterize how the amount of water in the cloud modifies this forcing. A case study additionally showcases the evolution of the radiation profiles in a dynamic atmosphere.
Zhangcheng Pei, Sonya L. Fiddes, W. John R. French, Simon P. Alexander, Marc D. Mallet, Peter Kuma, and Adrian McDonald
Atmos. Chem. Phys., 23, 14691–14714, https://doi.org/10.5194/acp-23-14691-2023, https://doi.org/10.5194/acp-23-14691-2023, 2023
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In this paper, we use ground-based observations to evaluate a climate model and a satellite product in simulating surface radiation and investigate how radiation biases are influenced by cloud properties over the Southern Ocean. We find that significant radiation biases exist in both the model and satellite. The cloud fraction and cloud occurrence play an important role in affecting radiation biases. We suggest further development for the model and satellite using ground-based observations.
Junxia Dou, Sue Grimmond, Shiguang Miao, Bei Huang, Huimin Lei, and Mingshui Liao
Atmos. Chem. Phys., 23, 13143–13166, https://doi.org/10.5194/acp-23-13143-2023, https://doi.org/10.5194/acp-23-13143-2023, 2023
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Multi-timescale variations in surface energy fluxes in a suburb of Beijing are analyzed using 16-month observations. Compared to previous suburban areas, this study site has larger seasonal variability in energy partitioning, and summer and winter Bowen ratios are at the lower and higher end of those at other suburban sites, respectively. Our analysis indicates that precipitation, irrigation, crop/vegetation growth activity, and land use/cover all play critical roles in energy partitioning.
Manfred Wendisch, Johannes Stapf, Sebastian Becker, André Ehrlich, Evelyn Jäkel, Marcus Klingebiel, Christof Lüpkes, Michael Schäfer, and Matthew D. Shupe
Atmos. Chem. Phys., 23, 9647–9667, https://doi.org/10.5194/acp-23-9647-2023, https://doi.org/10.5194/acp-23-9647-2023, 2023
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Atmospheric radiation measurements have been conducted during two field campaigns using research aircraft. The data are analyzed to see if the near-surface air in the Arctic is warmed or cooled if warm–humid air masses from the south enter the Arctic or cold–dry air moves from the north from the Arctic to mid-latitude areas. It is important to study these processes and to check if climate models represent them well. Otherwise it is not possible to reliably forecast the future Arctic climate.
Kristopher Scarci, Ryan Scott, Madison Ghiz, Andrew Vogelmann, and Dan Lubin
EGUsphere, https://doi.org/10.5194/egusphere-2023-1665, https://doi.org/10.5194/egusphere-2023-1665, 2023
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We demonstrate what can be learned about an Antarctic region's climate from basic atmospheric irradiance measurements made by broadband and filter radiometers, instruments suitable for deployment at very remote sites, assisted by meteorological reanalysis and satellite remote sensing. Analysis of shortwave and longwave irradiance reveals subtle contrasts between meteorological regimes favoring cloud ice versus liquid water, relevant to onset versus inhibition of surface melt over ice shelves.
Sebastian Becker, André Ehrlich, Michael Schäfer, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7015–7031, https://doi.org/10.5194/acp-23-7015-2023, https://doi.org/10.5194/acp-23-7015-2023, 2023
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This study analyses the variability of the warming or cooling effect of clouds on the Arctic surface. Therefore, aircraft radiation measurements were performed over sea ice and open ocean during three seasonally different campaigns. It is found that clouds cool the open-ocean surface most strongly in summer. Over sea ice, clouds warm the surface in spring but have a neutral effect in summer. Due to the variable sea ice extent, clouds warm the surface during spring but cool it during late summer.
Klára Čížková, Kamil Láska, Ladislav Metelka, and Martin Staněk
Atmos. Chem. Phys., 23, 4617–4636, https://doi.org/10.5194/acp-23-4617-2023, https://doi.org/10.5194/acp-23-4617-2023, 2023
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The study deals with ultraviolet (UV) radiation in southern polar conditions, where ozone depletion occurs each spring. A 10-year-long time series of UV spectra from Marambio Base, Antarctic Peninsula, has been studied, with a focus on the changes of UV radiation at different wavelengths and the effects of atmospheric and terrestrial variables like ozone, solar elevation, or cloudiness. At the very short wavelengths, the effect of ozone and its deficiency was clearly observed.
Junli Yang, Jianglin Hu, Qiying Chen, and Weijun Quan
Atmos. Chem. Phys., 23, 4419–4430, https://doi.org/10.5194/acp-23-4419-2023, https://doi.org/10.5194/acp-23-4419-2023, 2023
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Downward long-wave radiation (DLR) affects energy exchange between the land surface and the atmosphere, while it is seldom observed at conventional radiation stations. Therefore, parameterization of DLR based on the near-surface meteorological variables provides a chance to estimate the DLR over most meteorological stations. This work established three parameterizations suited to estimating the DLR over China by using the measurements from the CBSRN with an accuracy of ~6.1 %.
Qiuyan Wang, Hua Zhang, Su Yang, Qi Chen, Xixun Zhou, Bing Xie, Yuying Wang, Guangyu Shi, and Martin Wild
Atmos. Chem. Phys., 22, 15867–15886, https://doi.org/10.5194/acp-22-15867-2022, https://doi.org/10.5194/acp-22-15867-2022, 2022
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The present-day land energy balance over East Asia is estimated for the first time. Results indicate that high aerosol loadings, clouds, and the Tibet Plateau (TP) over East Asia play vital roles in the shortwave budgets, while the TP is responsible for the longwave budgets during this regional energy budget assessment. This study provides a perspective to understand fully how the potential factors influence the diversifying regional energy budget assessments.
Kostas Eleftheratos, John Kapsomenakis, Ilias Fountoulakis, Christos S. Zerefos, Patrick Jöckel, Martin Dameris, Alkiviadis F. Bais, Germar Bernhard, Dimitra Kouklaki, Kleareti Tourpali, Scott Stierle, J. Ben Liley, Colette Brogniez, Frédérique Auriol, Henri Diémoz, Stana Simic, Irina Petropavlovskikh, Kaisa Lakkala, and Kostas Douvis
Atmos. Chem. Phys., 22, 12827–12855, https://doi.org/10.5194/acp-22-12827-2022, https://doi.org/10.5194/acp-22-12827-2022, 2022
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We present the future evolution of DNA-active ultraviolet (UV) radiation in view of increasing greenhouse gases (GHGs) and decreasing ozone depleting substances (ODSs). It is shown that DNA-active UV radiation might increase after 2050 between 50° N–50° S due to GHG-induced reductions in clouds and ozone, something that is likely not to happen at high latitudes, where DNA-active UV radiation will continue its downward trend mainly due to stratospheric ozone recovery from the reduction in ODSs.
Chenglong Zhou, Yuzhi Liu, Qingzhe Zhu, Qing He, Tianliang Zhao, Fan Yang, Wen Huo, Xinghua Yang, and Ali Mamtimin
Atmos. Chem. Phys., 22, 5195–5207, https://doi.org/10.5194/acp-22-5195-2022, https://doi.org/10.5194/acp-22-5195-2022, 2022
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Based on the radiosonde observations, an anomalously warm layer is measured at altitudes between 500 and 300 hPa over the Tarim Basin (TB) with an average intensity of 2.53 and 1.39 K in the spring and summer, respectively. The heat contributions of dust to this anomalously warm atmospheric layer in spring and summer were 13.77 and 10.25 %, respectively. Topographically, the TB is adjacent to the Tibetan Plateau; we propose the concept of the Tibetan heat source’s northward extension.
Akira Watanabe, Mizuo Kajino, Kazuhiko Ninomiya, Yoshitaka Nagahashi, and Atsushi Shinohara
Atmos. Chem. Phys., 22, 675–692, https://doi.org/10.5194/acp-22-675-2022, https://doi.org/10.5194/acp-22-675-2022, 2022
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This study summarizes continuous measurements of surface air concentrations and deposition of radiocesium in Fukushima city over 8 years after the Fukushima nuclear accident. The concentration in the city was high in winter and low in summer (inverse of the forest area). The decreasing trends were much faster in the earlier stage, probably because dissolved cesium discharged faster from the local environment. Biotite might play a key role in circulation of particulate cesium in Fukushima city.
Ilias Fountoulakis, Henri Diémoz, Anna Maria Siani, Alcide di Sarra, Daniela Meloni, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 21, 18689–18705, https://doi.org/10.5194/acp-21-18689-2021, https://doi.org/10.5194/acp-21-18689-2021, 2021
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The variability and trends of solar spectral UV irradiance have been studied for the periods 1996–2020 (for Rome) and 2006–2020 (for Lampedusa, Rome, and Aosta) with respect to the variability and trends of total ozone and geopotential height. Analyses revealed increasing UV in particular months at all sites, possibly due to decreasing lower-stratospheric ozone (at Rome in 1996–2020) and decreasing attenuation by aerosols and/or clouds (at all stations in 2006–2020).
Marcia Akemi Yamasoe, Nilton Manuel Évora Rosário, Samantha Novaes Santos Martins Almeida, and Martin Wild
Atmos. Chem. Phys., 21, 6593–6603, https://doi.org/10.5194/acp-21-6593-2021, https://doi.org/10.5194/acp-21-6593-2021, 2021
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Spatio-temporal disparity to assess global dimming and brightening phenomena has been a critical topic. For instance, few studies addressed surface solar irradiation (SSR) long-term trend in South America. In this study, SSR, sunshine duration (SD) and the diurnal temperature range (DTR) are analysed for São Paulo, Brazil. We found a dimming phase, identified by SSR, SD and DTR, extending till 1983. Then, while SSR is still declining, consistent with cloud increasing, SD and DTR are increasing.
Guoyong Wen, Alexander Marshak, Si-Chee Tsay, Jay Herman, Ukkyo Jeong, Nader Abuhassan, Robert Swap, and Dong Wu
Atmos. Chem. Phys., 20, 10477–10491, https://doi.org/10.5194/acp-20-10477-2020, https://doi.org/10.5194/acp-20-10477-2020, 2020
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We combine the ground-based observations and radiative transfer model to quantify the impact of the 2017 solar eclipse on surface shortwave irradiation reduction. We find that the eclipse caused local reductions of time-averaged surface flux of about 379 W m-2 (50 %) and 329 W m-2 (46 %) during the ~ 3 h course of the eclipse at the Casper and Columbia sites, respectively. We estimate that the Moon’s shadow caused a reduction of approximately 7 %–8 % in global average surface broadband SW radiation.
Johannes Stapf, André Ehrlich, Evelyn Jäkel, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 20, 9895–9914, https://doi.org/10.5194/acp-20-9895-2020, https://doi.org/10.5194/acp-20-9895-2020, 2020
Nicholas D. Beres, Deep Sengupta, Vera Samburova, Andrey Y. Khlystov, and Hans Moosmüller
Atmos. Chem. Phys., 20, 6095–6114, https://doi.org/10.5194/acp-20-6095-2020, https://doi.org/10.5194/acp-20-6095-2020, 2020
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Brown carbon (BrC) aerosol can be produced by the smoldering combustion of peat, a wildland fuel common at high latitude, often adjacent to the cryosphere. However, little is known about how BrC deposition onto snow changes snow optical and radiative properties. Here, we artificially deposited BrC onto natural snow surfaces, monitored changes of the spectral surface albedo, characterized optical properties of deposited aerosol, and compared to modeled values of albedo and radiative forcing.
Mengqi Liu, Xiangdong Zheng, Jinqiang Zhang, and Xiangao Xia
Atmos. Chem. Phys., 20, 4415–4426, https://doi.org/10.5194/acp-20-4415-2020, https://doi.org/10.5194/acp-20-4415-2020, 2020
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This study uses 1 min radiation and lidar measurements at three stations over the Tibetan Plateau (TP) to parametrize downward longwave radiation (DLR) during summer months. Clear-sky DLR can be estimated from the best parametrization with a RMSE of 3.8 W m-2 and R2 > 0.98. Additionally cloud base height under overcast conditions is shown to play an important role in cloudy DLR parametrization, which is considered in the locally calibrated parametrization over the TP for the first time.
Stephan Nyeki, Stefan Wacker, Christine Aebi, Julian Gröbner, Giovanni Martucci, and Laurent Vuilleumier
Atmos. Chem. Phys., 19, 13227–13241, https://doi.org/10.5194/acp-19-13227-2019, https://doi.org/10.5194/acp-19-13227-2019, 2019
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The trends of meteorological parameters and surface downward shortwave radiation (DSR) and downward longwave radiation (DLR) were analysed at four stations (between 370 and 3580 m a. s. l.) in Switzerland for the 1996–2015 period. Trends in DSR and DLR were positive during cloudy as well as clear conditions. The trend due to the influence of clouds decreased in magnitude, which implies a reduction in cloud cover and/or a change towards a different cloud type over the four Swiss sites.
Christophe Bellisario, Helen E. Brindley, Simon F. B. Tett, Rolando Rizzi, Gianluca Di Natale, Luca Palchetti, and Giovanni Bianchini
Atmos. Chem. Phys., 19, 7927–7937, https://doi.org/10.5194/acp-19-7927-2019, https://doi.org/10.5194/acp-19-7927-2019, 2019
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We explore the possibility of inferring far-infrared downwelling radiances from mid-infrared observations to better constrain radiation schemes in climate models. Our results imply that while it is feasible to use this type of approach, the quality of the extension will be strongly dependent on the noise characteristics of the observations and on the accurate characterisation of the atmospheric state.
Germar Bernhard and Boyan Petkov
Atmos. Chem. Phys., 19, 4703–4719, https://doi.org/10.5194/acp-19-4703-2019, https://doi.org/10.5194/acp-19-4703-2019, 2019
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Solar radiation at ultraviolet, visible, and infrared wavelengths was measured during the total solar eclipse of 21 August 2017. Data were used to study the wavelength-dependent changes of solar radiation at Earth’s surface and to validate parameterizations of solar limb darkening (LD), which describes the change in the Sun’s brightness between its center and its edge. The study highlights the importance of the LD effect when calculating total ozone and aerosol optical depth during an eclipse.
Kaisa Lakkala, Alberto Redondas, Outi Meinander, Laura Thölix, Britta Hamari, Antonio Fernando Almansa, Virgilio Carreno, Rosa Delia García, Carlos Torres, Guillermo Deferrari, Hector Ochoa, Germar Bernhard, Ricardo Sanchez, and Gerrit de Leeuw
Atmos. Chem. Phys., 18, 16019–16031, https://doi.org/10.5194/acp-18-16019-2018, https://doi.org/10.5194/acp-18-16019-2018, 2018
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Solar UV irradiances were measured at Ushuaia (54° S) and Marambio (64° S) during 2000–2013. The measurements were part of the Antarctic NILU-UV network, which was maintained as a cooperation between Spain, Argentina and Finland. The time series of the network were analysed for the first time in this study. At both stations maximum UV indices and daily doses were measured when spring-time ozone loss episodes occurred. The maximum UV index was 13 and 12 in Ushuaia and Marambio, respectively.
Chunlüe Zhou, Yanyi He, and Kaicun Wang
Atmos. Chem. Phys., 18, 8113–8136, https://doi.org/10.5194/acp-18-8113-2018, https://doi.org/10.5194/acp-18-8113-2018, 2018
Pamela Trisolino, Alcide di Sarra, Fabrizio Anello, Carlo Bommarito, Tatiana Di Iorio, Daniela Meloni, Francesco Monteleone, Giandomenico Pace, Salvatore Piacentino, and Damiano Sferlazzo
Atmos. Chem. Phys., 18, 7985–8000, https://doi.org/10.5194/acp-18-7985-2018, https://doi.org/10.5194/acp-18-7985-2018, 2018
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The long-term (2002–2016) variability of global and diffuse PAR over the central Mediterranean is investigated based on measurements from Lampedusa. PAR modulates biological processes and this study provides useful insight into its variability. Seasonal and interannual variability of global and diffuse PAR is characterized and the effects of clouds are quantified. The analysis suggests that 77 % of the global PAR interannual variability may be ascribed to clouds.
Stelios Kazadzis, Dimitra Founda, Basil E. Psiloglou, Harry Kambezidis, Nickolaos Mihalopoulos, Arturo Sanchez-Lorenzo, Charikleia Meleti, Panagiotis I. Raptis, Fragiskos Pierros, and Pierre Nabat
Atmos. Chem. Phys., 18, 2395–2411, https://doi.org/10.5194/acp-18-2395-2018, https://doi.org/10.5194/acp-18-2395-2018, 2018
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The National Observatory of Athens has been collecting solar radiation, sunshine duration, and cloud and visibility data/observations since the beginning of the 20th century. In this work we present surface solar radiation data since 1953 and reconstructed data since 1900. We have attempted to show and discuss the long-term changes in solar surface radiation over Athens, Greece, using these unique datasets.
Klára Čížková, Kamil Láska, Ladislav Metelka, and Martin Staněk
Atmos. Chem. Phys., 18, 1805–1818, https://doi.org/10.5194/acp-18-1805-2018, https://doi.org/10.5194/acp-18-1805-2018, 2018
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In order to broaden the knowledge of long-term UV radiation variability, we have reconstructed and analyzed a 50-year-long UV radiation time series from Hradec Králové, Czech Republic. The UV radiation intensities increased greatly following the decline of ozone amounts in the 1980s and 1990s. High UV radiation doses were observed in days with low ozone amounts, clear or partly cloudy skies, or snow cover.
Janusz W. Krzyścin and Piotr S. Sobolewski
Atmos. Chem. Phys., 18, 1–11, https://doi.org/10.5194/acp-18-1-2018, https://doi.org/10.5194/acp-18-1-2018, 2018
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Maintaining homogeneity of long-term UV time series taken from various instruments and thus trend estimation are challenging tasks, especially for remote Arctic sites.
Highlights: method of the UV data homogenization is proposed to be used at any remote site. Past UV data built from satellite total O3 and ground-based sunshine duration. Yearly UV doses trendless in the southern Svalbard for 34-year period since 1983. Long-term cloud effects on UV more important than the ozone effects there.
Werner Eugster, Carmen Emmel, Sebastian Wolf, Nina Buchmann, Joseph P. McFadden, and Charles David Whiteman
Atmos. Chem. Phys., 17, 14887–14904, https://doi.org/10.5194/acp-17-14887-2017, https://doi.org/10.5194/acp-17-14887-2017, 2017
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The effects of penumbral shading of the solar eclipse of 20 March 2015 on near-surface meteorology across Switzerland (occultation 65.8–70.1 %) was investigated. Temperature effects at 184 weather stations are compared with temperature drops reported in the literature since 1834. A special focus is, however, put on wind direction effects observed at six flux sites (with 20 Hz data) and 165 meteorological stations (with 10 min resolution data). Results show the importance of local topography.
Axel Kreuter, Mario Blumthaler, Martin Tiefengraber, Richard Kift, and Ann R. Webb
Atmos. Chem. Phys., 17, 14353–14364, https://doi.org/10.5194/acp-17-14353-2017, https://doi.org/10.5194/acp-17-14353-2017, 2017
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We have done measurements of the sky's brightness at the Italian coast and show the influence of the underlying surface: looking towards the land, the sky can be up to 50 % brighter than opposite viewing directions towards the ocean as a result of higher land reflectivity. At low solar elevations, the specular reflection from the ocean, or sun glint, increases the zenith brightness. Understanding these effects requires a 3-D model and is important when retrieving, e.g., aerosol properties.
Reinout Boers, Theo Brandsma, and A. Pier Siebesma
Atmos. Chem. Phys., 17, 8081–8100, https://doi.org/10.5194/acp-17-8081-2017, https://doi.org/10.5194/acp-17-8081-2017, 2017
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In the Netherlands 9 W m−2 more solar radiation falls on the surface today than 50 years ago. Often this increase, which has also been detected in surrounding western Europe, has been attributed to decreasing air pollution due to improved regulatory practices. However, over the Netherlands clouds play an important but ambiguous role. Cloud cover has increased but have become optically thinner as well. Here, the impact of clouds on radiation is in fact more important than that of air pollution.
Jizeng Du, Kaicun Wang, Jiankai Wang, and Qian Ma
Atmos. Chem. Phys., 17, 4931–4944, https://doi.org/10.5194/acp-17-4931-2017, https://doi.org/10.5194/acp-17-4931-2017, 2017
Bomidi Lakshmi Madhavan, Hartwig Deneke, Jonas Witthuhn, and Andreas Macke
Atmos. Chem. Phys., 17, 3317–3338, https://doi.org/10.5194/acp-17-3317-2017, https://doi.org/10.5194/acp-17-3317-2017, 2017
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A method has been introduced to assess the representativeness of the time series of a point measurement compared to results for a larger area centered around the measurement location. This method allows one to determine the optimal accuracy that can be achieved for the validation of satellite products for a given pixel footprint, or the evaluation of an atmospheric model with a given grid-cell resolution.
Colette Brogniez, Frédérique Auriol, Christine Deroo, Antti Arola, Jukka Kujanpää, Béatrice Sauvage, Niilo Kalakoski, Mikko Riku Aleksi Pitkänen, Maxime Catalfamo, Jean-Marc Metzger, Guy Tournois, and Pierre Da Conceicao
Atmos. Chem. Phys., 16, 15049–15074, https://doi.org/10.5194/acp-16-15049-2016, https://doi.org/10.5194/acp-16-15049-2016, 2016
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The atmospheric ozone layer is changing, thus the UV radiation at the surface is changing. Due to both beneficial and adverse effects of UV on the biosphere, monitoring of UV is essential. Satellite sensors provide estimates of UV at the surface with a global coverage. Validation of satellite-sensor UV is therefore needed and this can be done by comparison with ground-based measurements. The present validation in three sites (midlatitude, tropical) shows that OMI and GOME-2 provide reliable UV.
Katsumasa Tanaka, Atsumu Ohmura, Doris Folini, Martin Wild, and Nozomu Ohkawara
Atmos. Chem. Phys., 16, 13969–14001, https://doi.org/10.5194/acp-16-13969-2016, https://doi.org/10.5194/acp-16-13969-2016, 2016
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Surface solar radiation observed in Japan generally shows a strong decline until the end of the 1980s and then a recovery up until around 2000. A substantial number of measurement stations are located close to populated areas and are speculated to have been influenced by air pollution. However, data obtained at 14 meteorological observatories suggest that the large decadal variations in surface solar radiation occur on a large scale and not limited to urban areas.
Jianping Guo, Yucong Miao, Yong Zhang, Huan Liu, Zhanqing Li, Wanchun Zhang, Jing He, Mengyun Lou, Yan Yan, Lingen Bian, and Panmao Zhai
Atmos. Chem. Phys., 16, 13309–13319, https://doi.org/10.5194/acp-16-13309-2016, https://doi.org/10.5194/acp-16-13309-2016, 2016
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The large-scale PBL climatology from sounding observations is still lacking in China. This work investigated the BLH characterization at diurnal, monthly and seasonal timescales throughout China, showing large geographic and meteorological dependences. BLH is, on average, negatively (positively) associated with the surface pressure and lower tropospheric stability (wind speed and temperature). Cloud tends to suppress the development of the PBL, which has implications for air quality forecasts.
Veronica Manara, Michele Brunetti, Angela Celozzi, Maurizio Maugeri, Arturo Sanchez-Lorenzo, and Martin Wild
Atmos. Chem. Phys., 16, 11145–11161, https://doi.org/10.5194/acp-16-11145-2016, https://doi.org/10.5194/acp-16-11145-2016, 2016
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This paper presents the temporal evolution of solar radiation over Italy for the 1959–2013 period and discusses possible reasons for differences between all-sky and clear-sky conditions in order to understand which part of the solar radiation variability depends on aerosols or clouds. The results give evidence of a relevant influence of both anthropogenic and natural aerosols on solar radiation long-term variability.
Weidong Guo, Xueqian Wang, Jianning Sun, Aijun Ding, and Jun Zou
Atmos. Chem. Phys., 16, 9875–9890, https://doi.org/10.5194/acp-16-9875-2016, https://doi.org/10.5194/acp-16-9875-2016, 2016
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Basic characteristics of land–atmosphere interactions at four neighboring sites with different underlying surfaces in southern China, a typical monsoon region, are analyzed systematically. Despite the same climate background, the differences in land surface characteristics like albedo and aerodynamic roughness length due to land use/cover change exert distinct influences on the surface radiative budget and energy allocation and result in differences of near-surface micrometeorological elements.
Fanny Finger, Frank Werner, Marcus Klingebiel, André Ehrlich, Evelyn Jäkel, Matthias Voigt, Stephan Borrmann, Peter Spichtinger, and Manfred Wendisch
Atmos. Chem. Phys., 16, 7681–7693, https://doi.org/10.5194/acp-16-7681-2016, https://doi.org/10.5194/acp-16-7681-2016, 2016
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Solar spectra of optical layer properties of cirrus have been derived from the first truly collocated airborne radiation measurements using an aircraft and a towed sensor platform. The measured layer properties differ slightly due to horizontal cirrus inhomogeneities and the influence of low-level water clouds. Applying a 1-D radiative transfer model sensitivity studies were performed. It was found that if a low-level cloud is not considered, the solar cooling of the cirrus is strongly overestimated.
Gerald M. Lohmann, Adam H. Monahan, and Detlev Heinemann
Atmos. Chem. Phys., 16, 6365–6379, https://doi.org/10.5194/acp-16-6365-2016, https://doi.org/10.5194/acp-16-6365-2016, 2016
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Increasing numbers of photovoltaic (PV) power systems call for the characterization of irradiance variability with very high spatiotemporal resolution. We use 1 Hz irradiance data recorded by as many as 99 pyranometers and show mixed sky conditions to differ substantially from clear and overcast skies. For example, the probabilities of strong fluctuations and their respective spatial autocorrelation structures are appreciably distinct under mixed conditions.
John H. Marsham, Douglas J. Parker, Martin C. Todd, Jamie R. Banks, Helen E. Brindley, Luis Garcia-Carreras, Alexander J. Roberts, and Claire L. Ryder
Atmos. Chem. Phys., 16, 3563–3575, https://doi.org/10.5194/acp-16-3563-2016, https://doi.org/10.5194/acp-16-3563-2016, 2016
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The roles of water, clouds and airborne dust in controlling the heating of the Sahara are uncertain, which has major implications for the West African monsoon. Observations from the Fennec project, with satellite data, show that total atmospheric water content provides a far stronger control on total radiative heating than dust does, but dust provides the stronger control on surface heating. Therefore major heating errors in global models are likely due to known errors in water transport.
Adel Imamovic, Katsumasa Tanaka, Doris Folini, and Martin Wild
Atmos. Chem. Phys., 16, 2719–2725, https://doi.org/10.5194/acp-16-2719-2016, https://doi.org/10.5194/acp-16-2719-2016, 2016
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Systematic measurements of surface solar radiation revealed a worldwide decrease from the 1960s to the mid-1980s. The role of urbanization for this so called global dimming is still under debate. We developed a set of population-data based urbanization indicators and found no correlation between urbanization and global dimming for Europe and Japan, while an urbanization impact can't be precluded for Asia. It is thus called into question whether the global dimming was mainly a local phenomenon.
Ilias Fountoulakis, Alkiviadis F. Bais, Konstantinos Fragkos, Charickleia Meleti, Kleareti Tourpali, and Melina Maria Zempila
Atmos. Chem. Phys., 16, 2493–2505, https://doi.org/10.5194/acp-16-2493-2016, https://doi.org/10.5194/acp-16-2493-2016, 2016
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Short- and long-term variability of spectral UV irradiance at Thessaloniki, Greece, is discussed in association with changes in total ozone column, aerosols and cloudiness. The UV data set from two Brewer spectrophotometers is used for the analysis. For the entire period 1994–2014, positive, statistically significant increases of UV irradiance were found, mainly attributable to changes in aerosols. UV irradiance is mainly increased from 1994 to 2006 and remains relatively stable thereafter.
Costas A. Varotsos, Chris G. Tzanis, and Nicholas V. Sarlis
Atmos. Chem. Phys., 16, 2007–2011, https://doi.org/10.5194/acp-16-2007-2016, https://doi.org/10.5194/acp-16-2007-2016, 2016
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It has been recently reported that the current 2015–2016 El Niño could become "one of the strongest on record". To further explore this claim, we performed a new analysis that allows the detection of precursory signals of the strong El Niño events by using a recently developed non-linear dynamics tool. The analysis of the SOI time series shows that the 2015–2016 El Niño would be rather a "moderate to strong" or even a "strong” event and not "one of the strongest on record", as that of 1997–1998.
X. Guan, J. Huang, R. Guo, H. Yu, P. Lin, and Y. Zhang
Atmos. Chem. Phys., 15, 13777–13786, https://doi.org/10.5194/acp-15-13777-2015, https://doi.org/10.5194/acp-15-13777-2015, 2015
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Dynamical adjustment methodology has been applied to the raw surface air temperature and has successfully identified and separated the contribution of dynamically induced temperature (DIT) and radiatively forced temperature (RFT). It found that regional anthropogenic radiative forcing caused the enhanced warming in the semi-arid region, which may be closely associated with local human activities.
C.-M. Gan, J. Pleim, R. Mathur, C. Hogrefe, C. N. Long, J. Xing, D. Wong, R. Gilliam, and C. Wei
Atmos. Chem. Phys., 15, 12193–12209, https://doi.org/10.5194/acp-15-12193-2015, https://doi.org/10.5194/acp-15-12193-2015, 2015
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This study attempts to determine the consequences of the changes in tropospheric aerosol burden arising from substantial reductions in emissions of SO2 and NOx associated with control measures under the Clean Air Act especially on trends in solar radiation. Comparisons of model results with observations of aerosol optical depth, aerosol concentration, and radiation demonstrate that the coupled WRF-CMAQ model is capable of replicating the trends well even though it tends to underestimate the AOD.
G. Bernhard, A. Arola, A. Dahlback, V. Fioletov, A. Heikkilä, B. Johnsen, T. Koskela, K. Lakkala, T. Svendby, and J. Tamminen
Atmos. Chem. Phys., 15, 7391–7412, https://doi.org/10.5194/acp-15-7391-2015, https://doi.org/10.5194/acp-15-7391-2015, 2015
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Surface erythemal UV data from the Ozone Monitoring Instrument (OMI) are validated for high northern latitudes (Arctic and Scandinavia) using ground-based measurements. The bias in OMI data caused by incorrect assumptions of the surface albedo are quantified and the mechanism that causes this bias is discussed. Methods to improve the accuracy of OMI data products are presented.
S. R. Wilson
Atmos. Chem. Phys., 15, 7337–7349, https://doi.org/10.5194/acp-15-7337-2015, https://doi.org/10.5194/acp-15-7337-2015, 2015
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Measurements of the photolysis rates which drive production of OH from ozone are reported for Cape Grim, a "clean-air" site in the southern midlatitudes. This remote maritime site sits in the Southern Ocean, a region of the globe which is little studied. From the 6 years of data the dependence of this photolysis on solar zenith angle and stratospheric ozone is determined. Included with the reported values is an estimate of the uncertainties in these measurements.
C. A. Varotsos, S. Lovejoy, N. V. Sarlis, C. G. Tzanis, and M. N. Efstathiou
Atmos. Chem. Phys., 15, 7301–7306, https://doi.org/10.5194/acp-15-7301-2015, https://doi.org/10.5194/acp-15-7301-2015, 2015
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Varotsos et al. (Theor. Appl. Climatol., 114, 725–727, 2013) found that the solar ultraviolet (UV) wavelengths exhibit 1/f-type power-law correlations. In this study, we show that the residues of the spectral solar incident flux with respect to the Planck law over a wider range of wavelengths (i.e. UV-visible) have a scaling regime too.
P. Wang, M. Allaart, W. H. Knap, and P. Stammes
Atmos. Chem. Phys., 15, 4131–4144, https://doi.org/10.5194/acp-15-4131-2015, https://doi.org/10.5194/acp-15-4131-2015, 2015
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A green light sensor has been developed at KNMI to measure actinic flux profiles together with an ozonesonde. The impact of clouds on the actinic flux is clearly detected. Good agreement is found between the DAK-simulated actinic flux profiles and the observations for single-layer clouds in fully overcast scenes. The instrument is suitable for operational balloon measurements because of its simplicity and low cost.
V. De Bock, H. De Backer, R. Van Malderen, A. Mangold, and A. Delcloo
Atmos. Chem. Phys., 14, 12251–12270, https://doi.org/10.5194/acp-14-12251-2014, https://doi.org/10.5194/acp-14-12251-2014, 2014
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WMO/UNEP, available at: https://wedocs.unep.org/bitstream/handle/20.500.11822/26858/SAOD-2018.pdf?sequence=1&isAllowed=y (last access: 19 May 2020), 2018.
Short summary
In 2017, new measurements of UV radiation started in Marambio, Antarctica, by the Finnish Meteorological Institute in collaboration with the Argentinian Servicio Meteorológico Nacional. The paper presents the results of UV irradiance measurements from March 2017 to March 2019, and it
compares them with those from 2000–2008 and also with UV measurements at other Antarctic stations. In 2017/2018, below average UV radiation levels were recorded due to favourable ozone and cloud conditions.
In 2017, new measurements of UV radiation started in Marambio, Antarctica, by the Finnish...
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