Articles | Volume 20, issue 7
https://doi.org/10.5194/acp-20-4313-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-4313-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
14 Apr 2020
Research article |
| 14 Apr 2020
| 14 Apr 2020
Simulation of organic aerosol formation during the CalNex study: updated mobile emissions and secondary organic aerosol parameterization for intermediate-volatility organic compounds
Quanyang Lu
CORRESPONDING AUTHOR
Center of Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, USA
Department of Mechanical Engineering, Carnegie Mellon University,
Pittsburgh, PA, USA
Oak Ridge Institute for Science and Education (ORISE) Research Participation Program at the Office of Research and Development, U.S. Environmental
Protection Agency, Research Triangle Park, NC, USA
Benjamin N. Murphy
Office of Research and Development, U.S. Environmental Protection
Agency, Research Triangle Park, NC, USA
Momei Qin
Oak Ridge Institute for Science and Education (ORISE) Research Participation Program at the Office of Research and Development, U.S. Environmental
Protection Agency, Research Triangle Park, NC, USA
now at: Nanjing University of Information Science and Technology, Nanjing, China
Peter J. Adams
Center of Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, USA
Yunliang Zhao
Center of Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, USA
Department of Mechanical Engineering, Carnegie Mellon University,
Pittsburgh, PA, USA
now at: California Air Resources Board, Sacramento, CA, USA
Havala O. T. Pye
Office of Research and Development, U.S. Environmental Protection
Agency, Research Triangle Park, NC, USA
Christos Efstathiou
General Dynamics Information Technology Research Triangle Park, North
Carolina, USA
Chris Allen
General Dynamics Information Technology Research Triangle Park, North
Carolina, USA
Allen L. Robinson
Center of Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA, USA
Department of Mechanical Engineering, Carnegie Mellon University,
Pittsburgh, PA, USA
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- A lumped species approach for the simulation of secondary organic aerosol production from intermediate-volatility organic compounds (IVOCs): application to road transport in PMCAMx-iv (v1.0) S. Manavi & S. Pandis 10.5194/gmd-15-7731-2022
- Modeling secondary organic aerosol formation from volatile chemical products E. Pennington et al. 10.5194/acp-21-18247-2021
- An updated comprehensive IVOC emission inventory for mobile sources in China J. Zhao et al. 10.1016/j.scitotenv.2022.158312
- Impacts of condensable particulate matter on atmospheric organic aerosols and fine particulate matter (PM2.5) in China M. Li et al. 10.5194/acp-22-11845-2022
- Measurement report: Emissions of intermediate-volatility organic compounds from vehicles under real-world driving conditions in an urban tunnel H. Fang et al. 10.5194/acp-21-10005-2021
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- Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels R. Miao et al. 10.5194/acp-21-16183-2021
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- Secondary organic aerosol formation from gasoline and diesel vehicle exhaust under light and dark conditions Y. Morino et al. 10.1039/D1EA00045D
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- Impacts of emission changes in China from 2010 to 2017 on domestic and intercontinental air quality and health effect Y. Zhang et al. 10.5194/acp-21-16051-2021
- A Scheme for Representing Aromatic Secondary Organic Aerosols in Chemical Transport Models: Application to Source Attribution of Organic Aerosols Over South Korea During the KORUS‐AQ Campaign J. Brewer et al. 10.1029/2022JD037257
- Contribution of intermediate-volatility organic compounds from on-road transport to secondary organic aerosol levels in Europe S. Manavi & S. Pandis 10.5194/acp-24-891-2024
- Comprehensive Assessment for the Impacts of S/IVOC Emissions from Mobile Sources on SOA Formation in China J. Zhao et al. 10.1021/acs.est.2c07265
- Advecting Superspecies: Efficiently Modeling Transport of Organic Aerosol With a Mass‐Conserving Dimensionality Reduction Method P. Sturm et al. 10.1029/2022MS003235
- Volatile Chemical Product Enhancements to Criteria Pollutants in the United States K. Seltzer et al. 10.1021/acs.est.1c04298
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- Full-volatility emission framework corrects missing and underestimated secondary organic aerosol sources X. Chang et al. 10.1016/j.oneear.2022.03.015
- Observations of Volatile Organic Compounds in the Los Angeles Basin during COVID-19 P. Van Rooy et al. 10.1021/acsearthspacechem.1c00248
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Discussed (final revised paper)
Latest update: 17 Apr 2024
Short summary
This research work investigates organic aerosol formation in California during the CalNex study. We update the chemical transport model with the most recent mobile-source emission data and introduce a simple parameterization for secondary organic aerosol formed from intermediate-volatility organic compounds. Our results highlight the important contribution of IVOCs to SOA production in the Los Angeles region but underscore that other uncertainties must be addressed to close the SOA mass balance.
This research work investigates organic aerosol formation in California during the CalNex study....
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