Articles | Volume 19, issue 9
https://doi.org/10.5194/acp-19-6497-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-6497-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 May 2019
Research article |
| 16 May 2019
| 16 May 2019
Effect of sea salt aerosol on tropospheric bromine chemistry
John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Daniel J. Jacob
John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
Sebastian D. Eastham
Laboratory for Aviation and the Environment, Massachusetts Institute of Technology, Cambridge, MA, USA
Melissa P. Sulprizio
John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Xuan Wang
John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA, USA
Tomás Sherwen
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, UK
National Centre for Atmospheric Science (NCAS), University of York, York, UK
Mat J. Evans
Wolfson Atmospheric Chemistry Laboratories, Department of Chemistry, University of York, York, UK
National Centre for Atmospheric Science (NCAS), University of York, York, UK
Qianjie Chen
Department of Atmospheric Sciences, University of Washington, Seattle, WA, USA
now at: Department of Chemistry, University of Michigan, Ann Arbor, MI, USA
Becky Alexander
Department of Atmospheric Sciences, University of Washington, Seattle, WA, USA
Theodore K. Koenig
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences (CIRES), Boulder, CO, USA
Rainer Volkamer
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences (CIRES), Boulder, CO, USA
L. Gregory Huey
School of Earth and Atmospheric Sciences, Georgia Tech, Atlanta, Georgia, USA
Michael Le Breton
The Centre for Atmospheric Science, School of Earth, Atmospheric and Environmental Sciences,
University of Manchester, Simon Building, Brunswick Street, Manchester M13 9PL, UK
Department of Chemistry and Molecular Biology, University of Gothenburg, Medicinaregatan 9 C, 40530 Gothenburg, Sweden
Thomas J. Bannan
The Centre for Atmospheric Science, School of Earth, Atmospheric and Environmental Sciences,
University of Manchester, Simon Building, Brunswick Street, Manchester M13 9PL, UK
Carl J. Percival
The Centre for Atmospheric Science, School of Earth, Atmospheric and Environmental Sciences,
University of Manchester, Simon Building, Brunswick Street, Manchester M13 9PL, UK
now at: Jet Propulsion Laboratory, California Institute of Technology, 4800 Oak Grove Drive, Pasadena, CA, USA
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36 citations as recorded by crossref.
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- Comparison of model and ground observations finds snowpack and blowing snow aerosols both contribute to Arctic tropospheric reactive bromine W. Swanson et al. 10.5194/acp-22-14467-2022
- An Expanded Definition of the Odd Oxygen Family for Tropospheric Ozone Budgets: Implications for Ozone Lifetime and Stratospheric Influence K. Bates & D. Jacob 10.1029/2019GL084486
- Causes of Enhanced Bromine Levels in Alpine Ice Cores During the 20th Century: Implications for Bromine in the Free European Troposphere M. Legrand et al. 10.1029/2020JD034246
- Typhoon- and pollution-driven enhancement of reactive bromine in the mid-latitude marine boundary layer S. Wang et al. 10.1093/nsr/nwae074
- The direct and indirect radiative effects of sea salt aerosols over the western Pacific using an online-coupled regional chemistry-climate model with a developed sea salt emission scheme J. Li et al. 10.1016/j.atmosres.2024.107325
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
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- Effect of bromine and iodine chemistry on tropospheric ozone over Asia-Pacific using the CMAQ model Y. Huang et al. 10.1016/j.chemosphere.2020.127595
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- Anthropogenic short-lived halogens increase human exposure to mercury contamination due to enhanced mercury oxidation over continents X. Fu et al. 10.1073/pnas.2315058121
- MAX-DOAS observation in the midlatitude marine boundary layer: Influences of typhoon forced air mass R. Zhang et al. 10.1016/j.jes.2021.12.010
- Anthropogenic Impacts on Tropospheric Reactive Chlorine Since the Preindustrial S. Zhai et al. 10.1029/2021GL093808
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34 citations as recorded by crossref.
- Global high-resolution emissions of soil NOx, sea salt aerosols, and biogenic volatile organic compounds H. Weng et al. 10.1038/s41597-020-0488-5
- Volatile compounds and odour characteristics during long-term storage of kombu seaweed (Laminaria ochroleuca) preserved by high pressure processing, freezing and salting O. López-Pérez et al. 10.1016/j.lwt.2019.108710
- Comparison of model and ground observations finds snowpack and blowing snow aerosols both contribute to Arctic tropospheric reactive bromine W. Swanson et al. 10.5194/acp-22-14467-2022
- An Expanded Definition of the Odd Oxygen Family for Tropospheric Ozone Budgets: Implications for Ozone Lifetime and Stratospheric Influence K. Bates & D. Jacob 10.1029/2019GL084486
- Causes of Enhanced Bromine Levels in Alpine Ice Cores During the 20th Century: Implications for Bromine in the Free European Troposphere M. Legrand et al. 10.1029/2020JD034246
- Typhoon- and pollution-driven enhancement of reactive bromine in the mid-latitude marine boundary layer S. Wang et al. 10.1093/nsr/nwae074
- The direct and indirect radiative effects of sea salt aerosols over the western Pacific using an online-coupled regional chemistry-climate model with a developed sea salt emission scheme J. Li et al. 10.1016/j.atmosres.2024.107325
- Global Observations of Tropospheric Bromine Monoxide (BrO) Columns From TROPOMI Y. Chen et al. 10.1029/2023JD039091
- Satellite‐based top‐down Lagrangian approach to quantify aerosol emissions over California S. Nizar & B. Dodamani 10.1002/qj.3756
- CAPRAM reduction towards an operational multiphase halogen and dimethyl sulfide chemistry treatment in the chemistry transport model COSMO-MUSCAT(5.04e) E. Hoffmann et al. 10.5194/gmd-13-2587-2020
- On the retrieval of aerosol optical depth over cryosphere using passive remote sensing L. Mei et al. 10.1016/j.rse.2020.111731
- Marine aerosol properties over the Southern Ocean in relation to the wintertime meteorological conditions M. Thomas et al. 10.5194/acp-22-119-2022
- Intercomparison Between Surrogate, Explicit, and Full Treatments of VSL Bromine Chemistry Within the CAM‐Chem Chemistry‐Climate Model R. Fernandez et al. 10.1029/2020GL091125
- Comparing the Effect of Anthropogenically Amplified Halogen Natural Emissions on Tropospheric Ozone Chemistry Between Pre‐Industrial and Present‐Day J. Barrera et al. 10.1029/2022JD038283
- The impacts of marine-emitted halogens on OH radicals in East Asia during summer S. Fan & Y. Li 10.5194/acp-22-7331-2022
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Global tropospheric halogen (Cl, Br, I) chemistry and its impact on oxidants X. Wang et al. 10.5194/acp-21-13973-2021
- Improved Mechanistic Model of the Atmospheric Redox Chemistry of Mercury V. Shah et al. 10.1021/acs.est.1c03160
- Origin of water-soluble organic aerosols at the Maïdo high-altitude observatory, Réunion Island, in the tropical Indian Ocean S. Simu et al. 10.5194/acp-21-17017-2021
- Role of Iodine Recycling on Sea‐Salt Aerosols in the Global Marine Boundary Layer Q. Li et al. 10.1029/2021GL097567
- Application of Satellite‐Based Detections of Arctic Bromine Explosion Events Within GEOS‐Chem P. Wales et al. 10.1029/2022MS003465
- Effect of bromine and iodine chemistry on tropospheric ozone over Asia-Pacific using the CMAQ model Y. Huang et al. 10.1016/j.chemosphere.2020.127595
- Contribution of expanded marine sulfur chemistry to the seasonal variability of dimethyl sulfide oxidation products and size-resolved sulfate aerosol L. Tashmim et al. 10.5194/acp-24-3379-2024
- A kinetic model for ozone uptake by solutions and aqueous particles containing I−and Br−, including seawater and sea-salt aerosol C. Moreno & M. Baeza-Romero 10.1039/C9CP03430G
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al. 10.5194/acp-21-13483-2021
- The Representation of Sea Salt Aerosols and Their Role in Polar Climate Within CMIP6 R. Lapere et al. 10.1029/2022JD038235
- Evaluating the impact of blowing-snow sea salt aerosol on springtime BrO and O<sub>3</sub> in the Arctic J. Huang et al. 10.5194/acp-20-7335-2020
- Sensitivity of tropospheric ozone to halogen chemistry in the chemistry–climate model LMDZ-INCA vNMHC C. Caram et al. 10.5194/gmd-16-4041-2023
- Trace elements and machine learning for Brazilian beef traceability E. De Nadai Fernandes et al. 10.1016/j.foodchem.2020.127462
- Exhaust and non-exhaust contributions from road transport to PM10 at a Southern European traffic site M. Scerri et al. 10.1016/j.envpol.2022.120569
- Latitudinal Distribution of Gaseous Elemental Mercury in Tropical Western Pacific: The Role of the Doldrums and the ITCZ F. Yue et al. 10.1021/acs.est.1c07229
- Anthropogenic short-lived halogens increase human exposure to mercury contamination due to enhanced mercury oxidation over continents X. Fu et al. 10.1073/pnas.2315058121
- MAX-DOAS observation in the midlatitude marine boundary layer: Influences of typhoon forced air mass R. Zhang et al. 10.1016/j.jes.2021.12.010
- Anthropogenic Impacts on Tropospheric Reactive Chlorine Since the Preindustrial S. Zhai et al. 10.1029/2021GL093808
Latest update: 24 Apr 2024
Short summary
We quantify the effect of sea salt aerosol on tropospheric bromine chemistry with a new mechanistic description of the halogen chemistry in a global atmospheric chemistry model. For the first time, we are able to reproduce the observed levels of bromide activation from the sea salt aerosol in a manner consistent with bromine oxide radical measured from various platforms. Sea salt aerosol plays a far more complex role in global tropospheric chemistry than previously recognized.
We quantify the effect of sea salt aerosol on tropospheric bromine chemistry with a new...
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