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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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ACP | Articles | Volume 19, issue 7
Atmos. Chem. Phys., 19, 4991-5003, 2019
https://doi.org/10.5194/acp-19-4991-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 19, 4991-5003, 2019
https://doi.org/10.5194/acp-19-4991-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 12 Apr 2019

Research article | 12 Apr 2019

Turbulence-induced cloud voids: observation and interpretation

Turbulence-induced cloud voids
Katarzyna Karpińska1, Jonathan F. E. Bodenschatz2, Szymon P. Malinowski1, Jakub L. Nowak1, Steffen Risius2, Tina Schmeissner4, Raymond A. Shaw3, Holger Siebert4, Hengdong Xi2, Haitao Xu2, and Eberhard Bodenschatz2 Katarzyna Karpińska et al.
  • 1Institute of Geophysics, Faculty of Physics, University of Warsaw, Warsaw, Poland
  • 2Max Planck Institute for Dynamics and Self-Organization, Göttingen, Germany
  • 3Physics Department, Michigan Technological University, Houghton, MI, USA
  • 4Leibniz Institute for Tropospheric Research, Leipzig, Germany
Abstract
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The phenomenon of “cloud voids”, i.e., elongated volumes inside a cloud that are devoid of droplets, was observed with laser sheet photography in clouds at a mountain-top station. Two experimental cases, similar in turbulence conditions yet with diverse droplet size distributions and cloud void prevalence, are reported. A theoretical explanation is proposed based on the study of heavy inertial sedimenting particles inside a Burgers vortex. A general conclusion regarding void appearance is drawn from theoretical analysis. Numerical simulations of polydisperse droplet motion with realistic vortex parameters and Mie scattering visual effects accounted for can explain the presence of voids with sizes similar to that of the observed ones. Clustering and segregation effects in a vortex tube are discussed for reasonable cloud conditions.

1 Introduction
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The dynamics of heavy inertial particles in turbulent flow is a universal problem that appears in astrophysics, oceanography, engineering and atmospheric sciences. In particular, in cloud physics, deeper understanding of the interaction between atmospheric turbulence and cloud droplets is seen as a potential answer to many important questions (Bodenschatz et al.2010). Over the years, there has been considerable speculation about the possible role of coherent, long-lived vortex structures in cloud turbulence and microphysical processes, including both condensational growth and collision–coalescence growth (see Tennekes and Woods1973; Maxey and Corrsin1986; Shaw et al.1998; Shaw2000; Markowicz et al.2000; Hill2005). This paper describes the first in situ observation of a phenomenon we refer to as “cloud voids” – cylindrical volumes devoid of droplets recorded in real clouds – and is focused on determining whether inertially induced voids indeed may occur in clouds due to the presence of strong vortex structures.

Vortex tubes, sometimes called “worms”, are severely intermittent, coherent, elongated and long-lasting structures characteristic of high Reynolds number turbulent flows (e.g., Mouri et al.2000). Past theoretical and experimental studies lack general conclusions about their characteristic time and length scales, intensity and appearance in turbulence. In particular, most of the research was conducted under conditions different from multiscale atmospheric turbulence. Statistical analysis based on such research (see, e.g., Jiménez et al.1993; Belin et al.1999; Pirozzoli2012) showed that Burgers vortex core size δ (defined later in Eq. 2) scales roughly with the Kolmogorov length scale η:

(1)δ=mη,

and that m has a distribution ranging from a few units to a few tens with its mean around m=4. Moisy and Jimenez (2004) analyzing direct numerical simulation (DNS) instant velocity fields propose that vorticity structures' geometrical aspect ratios evolve towards long tubes (1:1:10) with increasing vorticity threshold. What is more, they show that these structures concentrate into clusters of the size in inertial range of scales. This implies the presence of large-scale organization of the small-scale intermittent structures. In the study by Biferale et al. (2000), statistics of vortex filament lifetime for a low Taylor microscale Reynolds number Reλ indicate that the maximum lifetime is on the order of the integral timescale, whereas its mean scales with the Kolmogorov timescale. Numerical experiments described in Tanahashi et al. (2008) suggest that there is a relation between root mean square velocity fluctuations and the circulation parameter Γ of a vortex tube modeled as a Burgers vortex.

Previous efforts to study dynamics of heavy inertial particles in vortices were made by simulating droplet trajectories in a prescribed velocity field for several simple single-vortex models. Such research for the simplest model of a line vortex with stretching was conducted by Markowicz et al. (2000) with limitation to horizontally oriented vortices. In order to better understand the problem of cloud droplet dynamics in atmospheric conditions, the same model but with arbitrary gravity alignment was studied by Karpinska and Malinowski (2014). Another model, free from the problem of unrealistic singularity on the vortex axis, is a Burgers vortex with stretching. It is commonly seen as a very good approximation of a real vortex tube (Neu1984; Jimenez and Wray1998). The specific features of droplet motion for monodisperse droplets in a Burgers vortex were examined by Hill (2005) for horizontal alignment and by Marcu et al. (1995) for arbitrary alignment with respect to gravity. Clustering and segregation effects are of importance when talking about interaction between particles and turbulent flow. We define clustering of particles of arbitrary sizes as an inhomogeneous distribution of particles in space. Segregation refers to the cases in which the spatial distributions of different-sized particles are anticorrelated. Different kinds of particle clustering in turbulent flow were reviewed by Gustavsson and Mehlig (2016); turbulence-induced segregation was, for example, treated by Calzavarini et al. (2008).

In this paper, we describe the serendipitous observation of numerous isolated voids in clouds, while conducting measurements at a mountain-top station. The voids were visually striking and generated great excitement from the scientific team. Here, we present direct, 2-D observations of the distinct types of patterns of clear air in clouds, along with accompanying turbulence and cloud microphysical measurements. We pose the question of whether the observed cloud voids are consistent with inertial droplet response to turbulence under atmospheric conditions. To answer this question, analysis of the particle dynamics in a Burgers vortex is further developed for the heavy sedimenting polydisperse case and the model is interpreted in the context of the observations.

The paper is structured as follows. Section 2 describes the measurement method and analysis of experimental data that show the phenomenon of cloud voids. Section 3 presents relevant features of single droplet trajectories in a vortex tube model. Section 4 extends the analysis to the motion of polydisperse droplets in a vortex to define the conditions of cloud void emergence. Section 5 outlines the influence of Mie scattering theory on droplet imaging and the implications for void observation. Section 6 presents void numerical simulation results. Section 7 incorporates the discussion and conclusions.

2 Experimental evidence
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Intriguing structures inside clouds, as presented in Fig. 1, were recorded by means of laser sheet photography during observations performed on 27 and 29 August 2011 at Umweltforschungsstation Schneefernerhaus (UFS) on the slopes of Zugspitze in the German Alps. Each time, the cloud event lasted for several hours. For a description of the observatory and characterization of the cloud and turbulence conditions on site, see Risius et al. (2015) and Siebert et al. (2015). Authors of these papers showed that turbulence and cloud microphysical properties at the measurement site are quite reasonable representations of measurements made in “free” clouds away from the surface.

https://www.atmos-chem-phys.net/19/4991/2019/acp-19-4991-2019-f01

Figure 1Examples of cloud voids observed at the UFS station with various camera–laser configurations. Images taken on 27 August (a) were chosen to estimate cloud void sizes. The ones recorded on 29 August in the evening (b) show the difference between inhomogeneities produced by cloud voids and those resulting from the mixing with clear air at the cloud edge. Other images from 29 August (c) suggest that the voids can be quite frequent in the sample volume. Bright spots and lines are due to presence of larger precipitation particles. The 10 cm long segment is shown to represent spatial scale assumed in the void size calculation. For more details, see the movies attached in Karpinska et al. (2018).

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Clouds were illuminated by a laser sheet created with a frequency-doubled high-power Nd:YAG laser (532 nm, 45 W). The sheet was set either vertical or oblique with respect to gravity. The angle between the laser sheet plane and camera recording plane in the oblique case was chosen to increase the scattering intensity on droplets and falls within the range of 30–40. The laser sheet in the observation region was around 50 cm wide and 1 cm thick. Images covering the approximately 2 m long section of the sheet at a distance approximately 10 m from the source were taken with a Nikon D3s 12 MP DSLR camera.

Laser sheet photography was accompanied by high-resolution measurements of small-scale turbulence and cloud microphysics, as described in Siebert et al. (2015). Flow turbulence was measured by 3-D ultrasonic anemometers operated at 10 Hz, from which the velocity structure functions were calculated using Taylor's frozen-flow hypothesis, and the mean energy dissipation rates were determined using inertial range scaling. Droplet size was measured by a phase Doppler interferometer (PDI) probe (Chuang et al.2008) mounted approximately 6 m down from the camera level. Figure 2 presents the measurement setup and recorded size spectra of droplets. Droplet and turbulence measurements are summarized in Table 1. The mean values refer to 30 min long record corresponding to the camera acquisition series.

https://www.atmos-chem-phys.net/19/4991/2019/acp-19-4991-2019-f02

Figure 2Droplet size distributions measured with a PDI probe (a) and the arrangement of instruments at the measurement site (b).

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Table 1Properties of turbulence and cloud droplets during observation periods.

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Two kinds of events in which droplet spatial distribution is visibly inhomogeneous were distinguished in the collected images. The first kind was characterized by an irregular interface separating clear-air and cloudy-air volumes and/or cloudy volumes of visibly different properties over a wide range of spatial scales (Fig. 1b). Inhomogeneities of the second kind, present within the cloudy volumes, were called cloud voids in “Swiss cheese” clouds. Cloud voids were small (a few centimeters' scale), the interface was usually blurry (see Fig. 1a, c), and the shapes of clear-air regions were often close to round or elliptic (see magnified voids in Fig. 3). It is important to point out that the more intuitive expression “cloud holes” with regards to these inhomogeneities is avoided on purpose because it is commonly used referring to the cloud-free regions occurring in stratocumulus decks, as described, for example, in Gerber et al. (2005). Inhomogeneities of the first kind are argued to be created in the process of cloud–clear-air mixing (e.g., Warhaft2000). In contrast, in some series of images and movies, the shape of the recorded tracks of cloud droplets suggests the following cloud void origin hypothesis: they result from interactions between inertial, heavy cloud droplets and small-scale vortices present in a turbulent cloud. Comparison of the two described cases becomes straightforward when conducted on the basis of the movies in the database (Karpinska et al.2018). In the movie “ms01”, between 13 and 22 s, there are two cloud void appearances. Motion of the void in the homogeneous cloud field resembles motion of a worm. Movie “ms02” presents cloudy- and clear-air mixing at the cloud edges.

https://www.atmos-chem-phys.net/19/4991/2019/acp-19-4991-2019-f03

Figure 3Example close-ups of variously shaped cloud voids observed at the UFS station with different camera–laser configurations. The 5 cm long segment is shown to represent spatial scale assumed in the void size calculation.

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There were a few series of cloud void images collected with various camera–laser settings on the two experimental days. The best quality series, made on the morning of the 27th, was chosen for void size analysis. For the series of 17 photos selected for analysis, there were four in which voids were not clear enough to be accounted for. In the remaining 13 photos, 27 voids were identified. Each one's size was manually determined. In the case of a round void, the diameter was taken as the size; in the case of flattened or ellipsoidal void, the maximal chord was taken. The typical void diameter was estimated to be 3.5±1 cm; the maximal, 12±4 cm; the minimal, 1±0.5 cm. Images from the analyzed series from the morning of 27 August showing examples of objects identified as voids are presented in Fig. 1a. Voids captured on 29 August were not analyzed due to the large uncertainty resulting from the unknown geometry of the camera–laser setup. The general experimental observation was that the voids were smaller than those on 27 August. Definitive experimental verification of the cloud void origin is not possible on the basis of collected data only; however, in next sections, we argue that void creation due to inertia of droplets present inside vortex tubes is highly probable.

3 Motion of heavy inertial particles in the vortex tube model
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To address theoretically the issue of cloud void origin, the concept of the polydisperse inertial droplet population response to a coherent vortex pattern is followed. Here, the first step on this track is taken by presenting relevant features of single droplet trajectory in the chosen vortex tube model. A population of particles is assumed to form a dilute collection of material points, heavy and inertial, displaced by gravity force and viscous force (Stokes drag) only. Burgers vortex (Burgers1948) is used as a model of a steady vortex tube. The z axis in the cylindrical coordinate system (r,φ,z) is aligned with the vortex axis. The 3-D velocity field v is determined by two parameters: circulation Γ and stretching strength γ:

(2)v=-γ2re^r+Γ2πr1-e-r22δ2e^φ+γze^z,

where δ=2ν/γ is the vortex core size and ν denotes the kinematic viscosity. A particle's equation of motion is as follows:

(3)r¨=1τpv-r˙+g,

where τp is the particle relaxation time and g=-gsinθey^+cosθez^ is gravitational acceleration inclined by the angle θ[0,90] with respect to the vortex axis.

The analysis of single droplet motion in projection on a plane (r,φ) perpendicular to the vortex axis (henceforth called 2-D space) was conducted by Marcu et al. (1995). Here, it is summarized and completed with in-depth evaluation.

The behavior of a droplet inside the vortex depends on a set of six parameters {Γ,γ,θ,τp,g,ν}. The non-dimensionalization of the equations leads to Eq. (4) and gives a set of dimensionless parameters {St,Sv,θ,A}:

(4)r¨-rφ˙2=-St-1Ar+r˙+Svsinφ2r˙φ˙+rφ¨=St-112πr(1-e-r22)-rφ˙-Svcosφz¨=St-1Az-z˙-Svcotθ.

Henceforth, dimensionless variables are denoted by . Stokes number St here is calculated with the use of the characteristic timescale of the Burgers vortex flow, which is the vortex core rotation time τf=δ2Γ-1, so St=τpτf-1=τpΓδ-2. The sedimentation parameter Sv is a ratio of τf to the timescale of sedimentation through the vortex: Sv=τfτg-1=δgτpsinθΓ-1. It characterizes motion in a plane perpendicular to the vortex axis. The last quantity A=νΓ-1=1/Rev is the non-dimensional strain parameter, the inverse of vortex Reynolds number Rev. It is worth mentioning that the ratio of Stokes number to the sedimentation parameter, called Froude number Fr=StSv-1, is a measure of the influence of gravitational force on the droplet motion. In the limit of a large Froude number, gravity is considered negligible.

As one can see in Eq. (4), the equation describing particle motion along the vortex axis is independent from the equations describing motion in 2-D space. Thus, these components can be analyzed separately.

Motion along the vortex axis is determined by stretching outflow drag and gravity force. As a consequence, the particle z position shows an exponential dependence on time. What is more, every droplet has one unstable equilibrium point at z0=SvA-1cotθ=ν-1gδτpcosθ. The analytical solution was presented in Karpinska and Malinowski (2014). The solutions of Eq. (4) in 2-D space have several different attractors. It is helpful to distinguish two cases: with gravity and without gravity (valid as well when gravity is parallel to the vortex axis).

For the case of a vertical vortex or no gravity, for every particle of a given radius, a stable, circular periodic orbit exists if St<Stcr=16π2A. For StStcr, there exists a stable equilibrium point positioned on the vortex axis. A radius of the periodic orbit satisfies the equation

(5)r2A/St-1-exp-r2/2/2π=0.

Motion in 2-D space with gravity included is much more complicated. Nonparallel alignment of the gravity vector and vortex axis (θ≠0) destroys the axial symmetry of the system and introduces the presence of other attractors, such as limit cycles and equilibrium points outside the axis. The rest of this section is devoted to thorough analysis of these attractors.

For a nonzero θ, every particle always has equilibrium points in 2-D space. Positions of these points are determined by Sv and A. They can be obtained by solving the equation for the radial component r:

(6)rA1+1-exp-r222πAr22=Sv.

Now, let fA(r) be the left-hand side of Eq. (6). A plot of this function for a given A is called an equilibrium curve (see Fig. 2 in Marcu et al.1995). Detailed analysis of equilibrium curve dependence on parameters is performed in the next paragraph and leads to the conclusions summarized in Table 2.

Table 2Existence of equilibrium points with respect to A and Sv parameters. Acr, rs, rmin, Svmin and Svmax are defined in the text body.

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It is easy to find that fA(0)=0 and limrfA(r)=. Moreover, there exists a critical value Acr for which bifurcation from one unique solution (for AAcr) to maximally three solutions (for A<Acr) occurs. Acr corresponds to the equilibrium curve that has a horizontal slope at the inflection point. Acr value was estimated numerically (see Table 3).

For AAcr, the equilibrium curve is a monotonically increasing function of r so there exists exactly one solution for every Sv value. For A<Acr, the equilibrium curve always has one maximum at rmax and one minimum at rmin. The inflection point at A=Acr on the equilibrium curve lies at ri (see Table 3). It restricts values of rmax from above and values of rmin from below. Consequently, for Sv<fA(rmin) and for Sv>fA(rmax), there is only one solution. For Svmin=fA(rmin) and for Svmax=fA(rmax), there are two solutions. For fA(rmin)<Sv<fA(rmax), there are three solutions.

Table 3Burgers vortex non-dimensional numbers.

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Not only is the existence of the solutions important but their stability as well. Let r0 denote an arbitrary solution of Eq. (6). The exact form of the stability condition of the solution r0 is governed by the function ϕ(r0) (as defined in Marcu et al.1995). The condition can take two different forms depending on the sign of this function

ϕ(r0)=1(2π)21-exp(-r02/2)r02(7)1-exp(-r02/2)r02-exp(-r02/2).

The function has only one zero at rs (see Table 3). For small radii (r0<rs), the equilibrium is stable if

(8)StA1|ϕ(r0)|.

For greater radii (r0>rs), the condition for stability depends explicitly only on A:

(9)Aϕ(r0).

The equilibrium point satisfying the first type of the condition was shown to be a focus, the second type to be a node. Analysis of the equilibrium point stability conditions by Marcu et al. (1995) is expanded in the next paragraph with emphasis on the dependence on strain parameter A. The results are summarized in Table 4.

Table 4Stability conditions of particle equilibrium points present in the Burgers vortex with respect to vortex strain parameter A and dimensionless distance from the vortex axis r. At, φ(r), rs, rmin and rmax are defined in the text body.

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Generally, stability conditions are different for A ranges separated by At=maxr0φ(r0) (approximate value obtained numerically in Table 3). A>At always satisfies then the condition expressed by Eq. (9). The term “partly unstable” in the table refers to the following. In the range of rmaxr0<rmin, for a given A, only a small fraction of the total range (near points rmax and rmin) is stable. This range grows with increasing A. Numerical experiments show, however, that their domain of attraction in the presence of other stable points (at least one exists always) is relatively small.

The combination of multiple existence conditions with stability conditions creates a variety of single particle motion scenarios. Some of them are shown in Fig. 4 in Marcu et al. (1995). These scenarios are used in Sect. 4 to carry out a search for vortex model parameter values that produce a void. Figure 4 here illustrates one of these scenarios in which there are three equilibrium points: I – unstable point near the axis; II – unstable middle distance point; III – stable point far from the axis. A particle, depending on initial position and velocity, rotates around point I or is weakly attracted by unstable point II or is strongly attracted by stable point III.

https://www.atmos-chem-phys.net/19/4991/2019/acp-19-4991-2019-f04

Figure 4Example illustration of monodisperse droplets' trajectories in 2-D space (projection on a plane perpendicular to the vortex axis) with zero initial velocity. Particle trajectories (color lines) show the presence of three equilibrium points marked with black dots: I – unstable near vortex axis; II – unstable middle distance point; III – stable point far from the axis. Some droplets rotate around the vortex core on various orbits; some of these orbits may correspond to limit cycles. Different attraction regions can be noticed.

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4 Cloud void creation conditions
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Using conclusions concerning the motion of a single particle, the following hypothesis on polydisperse particle collective behavior can be formulated: a void can be created if a majority of the droplets have an unstable equilibrium point close to the axis r0<rs, leading to a limit cycle or periodic orbit attraction. The radius of curvature should be large enough for a void to be noticeable. If multiple equilibrium points exist, attraction by a stable equilibrium point far from the axis r0>rmin should not considerably influence droplet trajectories close to the void considerably. The first and the last condition are inspected in Sect. 4.1; the second condition is in Sect. 4.2.

4.1 Polydisperse particles

Obtaining a mathematically strict condition for creation of an arbitrary-sized void in arbitrary polydisperse collection of droplets would be too detailed and too complicated to be profitable for the interpretation of crude experimental results. Thorough analysis of single droplet motion in addition to what was presented in the paper (Marcu et al.1995) was performed and used to draw approximate conclusions about polydisperse droplet motion.

The most obvious conclusion is that when circulation of the vortex is too small, AAcr, the motion of particles is determined mostly by the gravitational force and resembles sedimentation through the vortex with curved trajectories. Circulation must then be large enough: at least AAcr for the void to be created.

The other condition is that equilibrium points near the vortex center for the majority of the particles are unstable, allowing circulation around the vortex axis. Inequality Eq. (8) is exploited here to find the qualitative dependence between vortex and particle parameters that fulfills this condition.

First, distance from the vortex axis of the equilibrium point should be in the range rrs. It allows approximation of relation described by Eq. (6) in the vicinity of r=0. The approximation is made with the assumption that in this vicinity the dependence on A is weak (see Fig. 2 in Marcu et al.1995).

SvA2=r21+1-exp-r2/22πAr22=r2+(1-exp-r2/2)2(2πAr)2r2(10)+14π2A2r24=r21+(4πA)-2,

So, in the end,

(11)r04πSv1+(4πA)2-12.

Secondly, the function ϕ(r0) (see Fig. 3 in Marcu et al.1995) is approximated in the chosen r range by linear dependence on r: ϕ(r0)-1-r0/rs16π2-1. At r=0, it has the same form as obtained for the case without gravity in Marcu et al. (1995). The above approximations are used simplifying the stability condition determined by Eq. (8). In the end, the condition for unstable points near the axis are algebraically transformed and expressed by splitting it in two parts. The first part concerns only the vortex parameters and the second part the particle sizes.

The first part requires that strain parameter A is small enough:

(12)A<AmaxB1/3,

and consequently circulation Γ large enough:

(13)Γ>ΓminB-1/3.

The second part demands that particle Stokes number falls within the range (St1,St1+ΔSt) and it is related to the vortex parameters (results shown to the leading term order in A):

(14)St1AΔStBA-2.

B is a new dimensionless parameter depending on vortex core size δ and gravity influence gsin θ:

(15)B=rs28π3constν2gsinθδ3.

The maximal strain parameter Amax (minimal circulation Γmin) increases (decreases) weakly with B. So the larger the vortex core size δ and gravity influence gsin θ, the larger the minimal circulation needed.

The following conclusions can be drawn from the above approximate relations:

  • There is a threshold (minimal) value of circulation needed for void creation. It increases with inclination angle (sin θ) and vortex size δ.

  • The greater the circulation, the smaller the particles that have their unstable points near the axis.

  • The range of particles having unstable points near the axis increases with increasing circulation and decreases with increasing gravity influence and vortex size δ.

Building up on these results, it may be concluded that it is harder to observe voids created by horizontally aligned vortices than vertically aligned ones and also more difficult to observe voids the larger particle size range is.

4.2 Particle orbit in a void – the radius of curvature

In order to obtain a void, a majority of the droplets must circle around the axis and the curvature of their trajectories should be large enough for a void to be noticeable. In order to estimate the curvature radius, we perform the following reasoning. For simplicity, particle and vortex constants and parameters are now chosen to match those of water droplets in the cloudy air, and henceforward particles are called droplets. Firstly, a basic vortex spatial scale is established for the measurement conditions. Premises found in the literature discussed in the introduction were used for making the assumption that the proportionality constant in Eq. (1) is in the range m[3.5,24]. It means δ[0.18,1.20] cm for 27 August measurements. Secondly, the droplet trajectory curvature radius is approximated by the periodic orbit radius which is a solution of Eq. (5). For this reason, solutions of Eq. (5) are presented in Fig. 5 for various representative vortex parameters. Every color represents one of droplet sizes: R=3,13,23µm chosen to be within the experimental range for 27 August (see Table 1). Overlapping colored surfaces match regions in which solutions can exist (what corresponds to the condition St<Stcr). Dashed lines are contour plots of solutions of chosen (close to experimental) void sizes: 0.5, 1.5 and 3 cm. Using the information presented in this plot, the analyzed strain parameter was further limited, from A<Acr down to A[10-4,8×10-3].

https://www.atmos-chem-phys.net/19/4991/2019/acp-19-4991-2019-f05

Figure 5Contour plot of stable periodic 2-D orbit radius for droplets of radii R=3,13,23µm covering the experimental range on 27 August. Selected ranges of vortex parameters: vortex core size δ and strain A are in the x and y axes, respectively. Overlapping (blue on top, then pink and green) colored surfaces match subspaces in which stable periodic 2-D orbit exist for droplet radius given by its color. Dashed lines are contour plots of solutions of chosen void sizes: 0.5, 1.5 and 3 cm. Black points represent parameters set for simulations as described in Sect. 5.

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5 Mie scattering influence on particle imaging
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Cloud voids were measured by recording light scattered by droplets within an illuminated laser-light sheet. The ability to visualize a void therefore depends not only on the positions and number density of cloud particles but on the scattering properties of the particles. In this section, we consider this optical perspective of the measurement problem.

The Mie scattering theory is a rigorous mathematical theory describing the problem of elastic scattering of light by a dielectric sphere of arbitrary size and homogeneous refractive index in the case in which a sphere size is similar to or larger than the wavelength of the incident light. It shows a complex angular and particle size dependency of the scattered light intensity (van de Hulst1957). Thus, brightness of images of laser light scattered by polydisperse set of droplets is not expected to be monotonic with the droplet size. The reasons are described in next paragraphs.

Firstly, the camera sensor pixel responds with a signal registration only if it receives an amount of energy exceeding a certain threshold. Light scattered by a particle passes through the optics and undergoes some transformations. What is more, the particle image on the sensor is characterized by the internal intensity distribution (diffraction pattern). Image size depends on particle size, optics' magnification, position with respect to the focus and other factors (see Olsen and Adrian2000).

Secondly, the scattered light intensity at an arbitrary angle depends nonlinearly on particle size. A larger particle can give a lower scattered intensity than a smaller one, or there may be several orders of magnitude difference in intensity between particles differing by 1 order of magnitude in size.

For the purpose of our simplified analysis, the following assumptions are made:

  • one particle image is recorded by one pixel,

  • the signal received by a pixel changes linearly with incident light intensity only,

  • each particle is in focus and its image size and depends linearly on the particle size, and

  • the experiment in clouds was set up to allow best visualization of maximal number of particles possible.

In order to compare results of the simulations with the measurements, a procedure of droplet size and color scaling is proposed. Calculation of the Mie scattering intensity is performed with the help of an algorithm that was described in Bohren and Huffman (1998). The scattering angle corresponds to 40. In the size range of cloud particles, the light intensity has a general growing tendency, but it is still strongly nonlinear. There are 3 orders of magnitude difference between particles of 1 and 30 µm radius. Relative intensity is calculated on this basis. Next, the brightness scaling is made. It assumes that experiment was set up to enable visualization of 95 % of particle size spectrum. The particle size at which the cumulant of the particle size distribution reaches 95 % was calculated. Particles larger than this size have brightness equal to 1 in the plots. Brightness for the other particles scales linearly with relative scattered light intensity. To mimic camera sensitivity, there is a threshold below which particles get brightness 0. In the plot with white background, the relation is opposite, so the brightest particles are black, and the least bright are white. This color scaling was used in Sect. 6 for numerical simulation plots.

6 Numerical simulation results
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The hypothesis of cloud void appearance was verified by numerical simulations. To imitate processes occurring in real vortex tubes in clouds and examine the effect exerted on a droplet field by the presence of a vortex, a cylinder-shaped domain was chosen. At t=0, the domain was filled uniformly with a given number concentration n of droplets. Droplets leaving the simulation domain were removed, and no interaction between droplets was imposed. Initial positions of the new droplets at t>0 were randomized on the cylinder surface to obtain conditions “outside the cylinder” of homogeneous spatial distribution with the same n. The initial velocity of these droplets was adjusted to the radial inflow velocity. The simulation domain size was chosen to be capable of showing phenomena at scales larger than standard experimental cloud void size, such that Z=20 cm long and D=5 cm in radius. Sensitivity to different values of D was examined, and no significant dependence on void creation was noticed. Droplet trajectories were calculated by solving numerically Eq. (3) in the Burgers vortex velocity field. Droplet number concentration within the domain is almost constant and the pattern does not change. The droplet radius distribution matches the experimental distribution from 27 August (see Table 1 and Fig. 2 for comparison). Since droplets do not interact with each other and results do not depend on droplet concentration, n=10 cm−3 was chosen as a compromise between computational costs and visibility purposes. After a few seconds, each simulation becomes steady. A 40 scattering angle was chosen for calculation of Mie effect in the post-processing of simulation results.

The parameter sets for three representative simulations are presented in Table 5. Two of them, (1) and (2), may result in the presence of a round or close to round void around the vortex axis. Simulation (3) does not show anything close to void creation or any other persistent pattern formation.

Table 5Sets of vortex and particle parameters chosen for numerical simulation. St, Sv and Fr are mean values. Only sets (1) and (2) give the visual effects of the cloud void.

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Figure 6 presents a 3-D views (Fig. 6a, b) with a 2-D cross-sections (Fig. 6c, d) at the last, quasi-stationary stage of simulations (1) and (2). In the database (Karpinska et al.2018), one may find 2-D and 3-D animations from the simulations. Animations “ms03” and “ms04” correspond to set (1), “ms05” and “ms06” to set (2), “ms07” and “ms08” to set (3).

https://www.atmos-chem-phys.net/19/4991/2019/acp-19-4991-2019-f06

Figure 6Positions of droplets in simulations (1) (a, c) and (2) (b, d) as described in Table 5 in perspective view (a, b) and in 4 cm thick central slice projected on a plane perpendicular to the vortex axis (c, d). The blue arrow shows the direction of gravity. In panels (a)(d), droplet size and color are scaled, respectively, to the rules described in Sect. 5. The red tracks behind the particles in panels (a) and (b) reflect the last Δt=0.0055 s of the droplet trajectory (for clarity, every 10th droplet is drawn). The dashed circles in panels (c) and (d) reflect the approximate shape and size of the visible void in the droplet field. Panels (e) and (f) present the number concentration of droplets n with different blue shading colors representing the contribution from different size groups – left axis, droplet mean real radius (solid red line) and mean visible radius (dashed red line) – right axis, all with respect to the distance from the vortex axis r.

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The droplet spatial distribution in and around presented voids show signs of clustering and segregation. Standard quantitative indicators of these phenomena (radial distribution function, fractal dimension, Voronoi diagram, segregation length) designed for homogeneous isotropic turbulence in our case would be difficult to interpret, so another approach is proposed.

The droplet size distribution was divided into five bins in such a way that the bins are equal in droplet number. Number concentration n with respect to the distance from the vortex axis r was plotted in Fig. 6e, f. The plotted n values represent the mean over 50 successive time instants. Different shading colors represent contributions from different size groups, so the darkest plot represents smallest droplets – first size group, the brighter represents the first and the second size group together, etc. If the distribution of droplets in the domain was homogeneous, it would be plotted as horizontal, parallel, equally spaced lines. Red line plots in the same panel present droplet mean radius R and droplet mean visible radius S versus distance from the vortex axis. The visible radius reflects droplet relative sizes in the camera image estimated by including Mie scattering and the camera threshold sensitivity influence as defined in Sect. 5. In the absence of sorting, both plots would approach one horizontal line.

Figure 6e, f show that droplets around the void are non-homogeneously distributed and segregated by size in space. The most inner part of the figure in Fig. 6e is almost devoid of droplets. The larger distance from the axis, the bigger the particles circling around the void. Animations of motion clearly show that this is caused by limit cycle attraction, where the radius of a limit cycle grows with droplet size. This is pronounced in Fig. 6c as well. The visible void radius is around 2.5 cm, whereas the “real” (no droplets) void radius is estimated to be 1 cm. Figure 6f shows the more complex situation: the inner part of the vortex is not empty, but the droplets are smaller (less visible) than those further away from the axis. For increasing visibility threshold, the visible void size increases in both cases.

Values of St, Sv (mean of polydisperse particle set) in simulated vortices differ essentially from values in Table 1. Estimations of St and Sv in 3-D real turbulence flow are based on a global value of the Kolmogorov timescale. The calculation in the simulation uses vortex model characteristic times. Local parameter values of single vortex in intermittent turbulent flow can be completely different than global flow characteristics.

In summary, there are two possible factors together creating the visible effect of the void. The first one is collective droplet dynamics: the majority of the droplets move on helical trajectories, being attracted in 2-D space by the limit cycle or by a stable point near the axis. Large droplets may be slowly attracted by their equilibrium point far from the vortex axis in 2-D space, but in the course of attraction they circle around the axis. At the same time, a significant ratio of the characteristic timescale of motion in the plane perpendicular to vortex axis with respect to motion along the vortex axis is needed. Secondly, segregation of particles with respect to the distance from the vortex axis can influence visible void size due to Mie scattering effects. Even if the circulation is not strong enough to displace the smallest particles far from the vortex axis, it is possible that their images are not recorded by the camera. Therefore, visible void size can depend vitally on imaging capability.

7 Discussion and conclusions
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Visualizations of cloud droplets by means of laser sheet photography performed at the Schneefernerhaus observatory revealed the presence of voids – holes in the form of curved elongated cylinders with a radius of a few centimeters. The possibility of such cloud voids or “Swiss cheese” cuts in clouds was suggested by former studies of the Stokes motion of particles in idealized vortices. The original work of Marcu et al. (1995) elaborating on single particle motion in a Burgers vortex was adopted to explain the behavior for a specific scenario: polydisperse cloud droplets inside a vortex, with cloud particle and vortex properties scaled to the ranges consistent with our cloud microphysical and turbulence observations.

Using information on cloud droplet size distributions and turbulence parameters collected in the course of observations, as well as literature discussions on vortex tubes in turbulent flows, we have shown that the cloud voids observed under the experimental conditions were likely a result of the presence of relatively thin yet long vortex tubes. Approximate theoretical conditions of void creation were proposed and vortex circulation was shown to be the parameter of the greatest importance in the conditions' formulation. The calculations are consistent with the observation that voids are present under some conditions and not under others. Comparison of the modeled and experimental voids led to the conclusion that properties of the Mie scattering are crucial for reproducing the proper size and shape of cloud voids observed by laser imaging.

Our analysis shows that existence of Burgers-like vortices in the measurement conditions is likely and they may explain the observed phenomenon. This finding, if confirmed in clouds far from the atmospheric surface layer, might help to better understand the effect of high Reynolds number turbulence on clustering, size segregation and probably collisions of cloud droplets. In the literature, several perspectives on the clustering mechanism were presented, to name just a few: Maxey (1987), Coleman and Vassilicos (2009), Falkovich and Pumir (2007) and Gustavsson and Mehlig (2011). The paper of Gustavsson and Mehlig (2016) presents a thorough review of research on clustering. It is recognized that consideration of droplet motion within a single vortex, as a representative of coherent dissipative structures expected to exist in turbulent flows, is a strong simplification in comparison to the cited works. The use of simplified models can be accepted at a semi-quantitative level to understand what factors influence void formation but cannot replace statistical analysis of the droplet spatial distribution in fully three-dimensional turbulent flow. There are very few numerical simulations of particle-laden 3-D turbulence that capture the range of scales relevant to this problem, however, i.e., from the large scales that feed the intermittent formation of intense vortices to the dissipation scales relevant to actual droplet clustering. Thus, it is reasonable to explore the essential physics of the problem using vortex models; for example, the research conducted for non-sedimenting particles in a simple vortex by Ravichandran and Govindarajan (2015) and Deepu et al. (2017) suggests that fixed point attraction and caustics formed by limit cycle attraction strongly increase the clustering and collision probability of particles near single and multiple vortices. This fact should become very distinct motivation for investing in both experimental and theoretical research aiming at thorough quantitative characterization of cloud void events.

Code and data availability
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Code and data availability. 

Numerical simulation code is available on demand. The data repository containing experimental movies and animations of simulations is retrieved from https://doi.org/10.13140/RG.2.2.21345.35689 (Karpinska et al.2018).

Author contributions
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Author contributions. 

RAS, HS and EB designed the experiment. SPM formulated the aim for theoretical and numerical analysis. SR, TS, RAS, HS, HeX, HaX, JFEB and EB provided resources and carried out the experiment. TS, SR, HaX and EB maintained and synthesized experimental data. SPM and EB acquired financial support. KK and SPM developed the numerical model. KK analyzed the experimental data, conducted theoretical analysis, designed and implemented the code for numerical analysis, conducted validation and verification of numerical results and wrote the original draft of the paper. KK and SR provided visualization of the results. SPM was responsible for supervision. KK, SPM, JLN, SR, RAS and HS edited the original draft to prepare it for submission.

Competing interests
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Competing interests. 

The authors declare that they have no conflict of interest.

Acknowledgements
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Acknowledgements. 

We are grateful to Markus Neumann and the staff at UFS for their technical help at UFS and the Bavarian Umweltministerium for the financial support of the station. Financial support from Max Planck Society, Deutsche Forschungsgemeinschaft (DFG) through the SPP 1276 Metström, the EU COST Action MP0806 Particles in Turbulence and through the US National Science Foundation (NSF grants AGS-1026123 and AGS-1754244) is gratefully acknowledged. Theoretical analysis and simulations were possible due to the support from the Polish National Science Centre (grant 2013/08/A/ST10/00291). We thank Marta Wacławczyk and Liang Ping Wang for the comments on the manuscript.

Review statement
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Review statement. 

This paper was edited by Barbara Ervens and reviewed by Toshiyuki Gotoh and three anonymous referees.

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Observations of clouds at a mountain-top laboratory revealed for the first time the presence of “voids”, i.e., elongated volumes inside a cloud that are devoid of droplets. Theoretical and numerical analyses suggest that these voids are a result of strong and long-lasting vortex presence in turbulent air. If this is confirmed in further investigation, the effect may become an important part of models describing cloud evolution and rain formation.
Observations of clouds at a mountain-top laboratory revealed for the first time the presence of...
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