Constructing a data-driven receptor model for organic and inorganic aerosol – a synthesis analysis of eight mass spectrometric data sets from a boreal forest site

Äijälä, Mikko; Daellenbach, Kaspar R.; Canonaco, Francesco; Heikkinen, Liine; Junninen, Heikki; Petäjä, Tuukka; Kulmala, Markku; Prévôt, André S. H.; Ehn, Mikael

doi:https://doi.org/10.5194/acp-19-3645-2019

Articles | Volume 19, issue 6

https://doi.org/10.5194/acp-19-3645-2019

© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

https://doi.org/10.5194/acp-19-3645-2019

© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

Articles | Volume 19, issue 6

Research article

|

21 Mar 2019

Research article |

| 21 Mar 2019

Constructing a data-driven receptor model for organic and inorganic aerosol – a synthesis analysis of eight mass spectrometric data sets from a boreal forest site

Mikko Äijälä, Kaspar R. Daellenbach, Francesco Canonaco, Liine Heikkinen, Heikki Junninen, Tuukka Petäjä, Markku Kulmala, André S. H. Prévôt, and Mikael Ehn

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Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC1: 'Manuscript accepted subject to minor revisions.', Anonymous Referee #1, 17 Nov 2018
RC2: 'Referee comment', Anonymous Referee #2, 04 Dec 2018
AC1: 'Authors' response to Anonymous Referees #1 and #2', M. Äijälä, 21 Dec 2018

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by M. Äijälä on behalf of the Authors (18 Jan 2019) Author's response Manuscript

ED: Publish as is (15 Feb 2019) by Dominick Spracklen

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Short summary

Aerosol mass spectrometry produces large amounts of complex data, the analysis of which necessitates chemometrics – the application of advanced statistical and mathematical tools to chemical data. Here, we perform a data-driven analysis of multiple aerosol mass spectrometric data sets, to show that the traditional separation of organics and inorganics is not necessary. The resulting 7-component aerosol speciation explains 83 % to 96 % of observed variability at our boreal forest experiment site.