Articles | Volume 19, issue 5
https://doi.org/10.5194/acp-19-3137-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-3137-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Mar 2019
Research article |
| 12 Mar 2019
| 12 Mar 2019
The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings
Anna L. Hodshire
CORRESPONDING AUTHOR
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, USA
Pedro Campuzano-Jost
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
John K. Kodros
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, USA
Betty Croft
Dalhousie University, Department of Physics and Atmospheric Science,
Halifax, NS, B3H 4R2, Canada
Benjamin A. Nault
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Jason C. Schroder
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Jose L. Jimenez
Department of Chemistry, University of Colorado, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Jeffrey R. Pierce
Department of Atmospheric Science, Colorado State University, Fort
Collins, CO 80523, USA
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- Atmospheric Gas-Phase Formation of Methanesulfonic Acid J. Chen et al. 10.1021/acs.est.3c07120
- Oxygenated Aromatic Compounds are Important Precursors of Secondary Organic Aerosol in Biomass-Burning Emissions A. Akherati et al. 10.1021/acs.est.0c01345
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- Observed Relationships Between Cloud Droplet Effective Radius and Biogenic Gas Concentrations in Summertime Marine Stratocumulus Over the Eastern North Atlantic M. Miller et al. 10.1029/2021EA001929
- Implications for new particle formation in air of the use of monoethanolamine in carbon capture and storage V. Perraud et al. 10.1039/D4CP00316K
- Atmospherically Relevant Hydrogen-Bonded Interactions between Methanesulfonic Acid and H2SO4 Clusters: A Computational Study D. de Souza Gonçalves & P. Chaudhuri 10.1021/acs.jpca.0c09087
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- Impact of dry intrusion events on the composition and mixing state of particles during the winter Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) J. Tomlin et al. 10.5194/acp-21-18123-2021
- Methanesulfonic acid and sulfuric acid Aerosol Formed through oxidation of reduced sulfur compounds in a humid environment P. Van Rooy et al. 10.1016/j.atmosenv.2021.118504
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Discussed (final revised paper)
Latest update: 25 Apr 2024
Short summary
A global chemical-transport model is used to determine the impact of methanesulfonic acid (MSA) on the aerosol size distribution and associated radiative effects, testing varying assumptions of MSA’s effective volatility and nucleating ability. We find that MSA mass best matches the ATom airborne measurements when volatility varies as a function of temperature, relative humidity, and available gas-phase bases, and the MSA radiative forcing is on the order of -50 mW m-2 over the Southern Ocean.
A global chemical-transport model is used to determine the impact of methanesulfonic acid (MSA)...
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Final-revised paper
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