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ACP | Articles | Volume 19, issue 4
Atmos. Chem. Phys., 19, 2327–2341, 2019
https://doi.org/10.5194/acp-19-2327-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 19, 2327–2341, 2019
https://doi.org/10.5194/acp-19-2327-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 22 Feb 2019

Research article | 22 Feb 2019

Quantifying primary and secondary humic-like substances in urban aerosol based on emission source characterization and a source-oriented air quality model

Xinghua Li et al.

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Appel, K. W., Pouliot, G. A., Simon, H., Sarwar, G., Pye, H. O. T., Napelenok, S. L., Akhtar, F., and Roselle, S. J.: Evaluation of dust and trace metal estimates from the Community Multiscale Air Quality (CMAQ) model version 5.0, Geosci. Model Dev., 6, 883–899, https://doi.org/10.5194/gmd-6-883-2013, 2013. 
Baduel, C., Voisin, D., and Jaffrezo, J.-L.: Seasonal variations of concentrations and optical properties of water soluble HULIS collected in urban environments, Atmos. Chem. Phys., 10, 4085–4095, https://doi.org/10.5194/acp-10-4085-2010, 2010. 
Beine, H., Anastasio, C., Esposito, G., Patten, K., Wilkening, E., Domine, F., Voisin, D., Barret, M., Houdier, S., and Hall, S.: Soluble, light absorbing species in snow at Barrow, Alaska, J. Geophys. Res., 116, D00R05, https://doi.org/10.1029/2011JD016181, 2011. 
Cheng, Y., Engling, G., He, K.-B., Duan, F.-K., Ma, Y.-L., Du, Z.-Y., Liu, J.-M., Zheng, M., and Weber, R. J.: Biomass burning contribution to Beijing aerosol, Atmos. Chem. Phys., 13, 7765–7781, https://doi.org/10.5194/acp-13-7765-2013, 2013. 
Chow, J. C., Watson, J. G., Chen, L. W. A., Chang, M. C. O., Robinson, N. F., Trimble D., and Kohl, S.: The IMPROVE-A temperature protocol for thermal/optical carbon analysis: maintaining consistency with a long-term database, J. Air Waste Manage., 57, 1014–1023, 2007. 
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Short summary
HULIS are widely distributed in atmospheric aerosol. Their sources are rarely studied quantitatively. Biomass burning is generally accepted as a major primary source with additional secondary material formed in the atmosphere. The present study provides direct evidence that residential coal burning is also a significant source of ambient HULIS in northern China based on source measurements, ambient sampling and analysis, and apportionment with source-oriented CMAQ modeling.
HULIS are widely distributed in atmospheric aerosol. Their sources are rarely studied...
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