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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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ACP | Articles | Volume 19, issue 3
ACP | Articles | Volume 19, issue 3
Atmos. Chem. Phys., 19, 1753–1766, 2019
https://doi.org/10.5194/acp-19-1753-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 19, 1753–1766, 2019
https://doi.org/10.5194/acp-19-1753-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
ACP | Articles | Volume 19, issue 3

Research article 08 Feb 2019

Research article | 08 Feb 2019

Kinetic mass-transfer calculation of water isotope fractionation due to cloud microphysics in a regional meteorological model

I-Chun Tsai et al.
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In conventional models, isotope exchange between liquid and gas phases is usually assumed to be in equilibrium, and the highly kinetic phase transformation processes inferred in clouds are yet to be fully investigated. We show that different factors controlling isotopic composition, including water vapor sources, atmospheric transport, phase transition pathways of water in clouds, and kinetic-versus-equilibrium mass transfer, contributed significantly to the variations in isotope composition.
In conventional models, isotope exchange between liquid and gas phases is usually assumed to be...
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