Articles | Volume 19, issue 19
https://doi.org/10.5194/acp-19-12797-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-12797-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
14 Oct 2019
Research article |
| 14 Oct 2019
| 14 Oct 2019
Secondary organic aerosol formation from the laboratory oxidation of biomass burning emissions
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
now at: Department of Chemistry, University of Toronto, Toronto, ON,
Canada
David H. Hagan
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
Matthew M. Coggon
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Abigail R. Koss
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
now at: TOFWERK USA, Boulder, CO, USA
Kanako Sekimoto
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Graduate School of Nanobioscience, Yokohama City University, Yokohama,
Japan
Joost de Gouw
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Carsten Warneke
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory, Chemical Sciences Division,
Boulder, CO, USA
Christopher D. Cappa
Department of Civil and Environmental Engineering, University of
California, Davis, CA, USA
Department of Civil and Environmental Engineering, Massachusetts
Institute of Technology, Cambridge, MA, USA
Publisher's note: the Supplement was exchanged on 28 April 2023.
In the original version of the Supplement, the authors had mistakenly published primary organic aerosol (POA) values that were not corrected for AMS collection efficiency. The error is limited to Table S1 and Figure S9b in the Supplement and does not impact any other figures or conclusions in the paper. In the attached version of the Supplement, the authors have edited Table S1 and Figure S9b to use the properly corrected POA values.
In the original version of the Supplement, the authors had mistakenly published primary organic aerosol (POA) values that were not corrected for AMS collection efficiency. The error is limited to Table S1 and Figure S9b in the Supplement and does not impact any other figures or conclusions in the paper. In the attached version of the Supplement, the authors have edited Table S1 and Figure S9b to use the properly corrected POA values.
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- Fire Influence on Regional to Global Environments and Air Quality (FIREX‐AQ) C. Warneke et al. 10.1029/2022JD037758
- Production of oxygenated volatile organic compounds from the ozonolysis of coastal seawater D. Kilgour et al. 10.5194/acp-24-3729-2024
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
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- Laboratory Investigation of Renoxification from the Photolysis of Inorganic Particulate Nitrate Q. Shi et al. 10.1021/acs.est.0c06049
- Secondary organic aerosol formation in China from urban-lifestyle sources: Vehicle exhaust and cooking emission Z. Zhang et al. 10.1016/j.scitotenv.2022.159340
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- Rate coefficients for the gas‐phase OH + furan (C4H4O) reaction between 273 and 353 K M. Angelaki et al. 10.1002/kin.21697
- Modeling Novel Aqueous Particle and Cloud Chemistry Processes of Biomass Burning Phenols and Their Potential to Form Secondary Organic Aerosols J. Zhang et al. 10.1021/acs.est.3c07762
- Hygroscopicity of amino acids and their effect on the water uptake of ammonium sulfate in the mixed aerosol particles Q. Luo et al. 10.1016/j.scitotenv.2020.139318
- Influence of biomass burning vapor wall loss correction on modeling organic aerosols in Europe by CAMx v6.50 J. Jiang et al. 10.5194/gmd-14-1681-2021
- Can Delhi's Pollution be Affected by Crop Fires in the Punjab Region? M. Takigawa et al. 10.2151/sola.2020-015
- An experimental and kinetic modeling study of the pyrolysis of isoprene, a significant biogenic hydrocarbon in naturally occurring vegetation fires E. Grajales-González et al. 10.1016/j.combustflame.2022.112206
- Impact of Fire Emissions on U.S. Air Quality from 1997 to 2016–A Modeling Study in the Satellite Era Z. Tao et al. 10.3390/rs12060913
- Dilution impacts on smoke aging: evidence in Biomass Burning Observation Project (BBOP) data A. Hodshire et al. 10.5194/acp-21-6839-2021
- Atmospheric aging enhances the ice nucleation ability of biomass-burning aerosol L. Jahl et al. 10.1126/sciadv.abd3440
- Estimating the air quality and health impacts of biomass burning in northern South America using a chemical transport model K. Ballesteros-González et al. 10.1016/j.scitotenv.2020.139755
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Short summary
Wildfires are a large source of gases and particles to the atmosphere, both of which impact human health and climate. The amount and composition of particles from wildfires can change with time in the atmosphere; however, the impact of aging is not well understood. In a series of controlled laboratory experiments, we show that the particles are oxidized and a significant fraction of the gas-phase carbon (24 %–56 %) is converted to particle mass over the course of several days in the atmosphere.
Wildfires are a large source of gases and particles to the atmosphere, both of which impact...
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