Articles | Volume 18, issue 2
https://doi.org/10.5194/acp-18-979-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-979-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 Jan 2018
Research article |
| 25 Jan 2018
| 25 Jan 2018
Atmospheric histories and emissions of chlorofluorocarbons CFC-13 (CClF3), ΣCFC-114 (C2Cl2F4), and CFC-115 (C2ClF5)
Laboratory for Air Pollution and Environmental Technology, Empa, Swiss Federal Laboratories for Materials Science and Technology,
Überlandstrasse 129, 8600 Dübendorf, Switzerland
Dickon Young
Atmospheric Chemistry Research Group, School of Chemistry, University of Bristol, Bristol, UK
Cathy M. Trudinger
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Jens Mühle
Scripps Institution of Oceanography, University of California at San Diego, La Jolla, California, USA
Stephan Henne
Laboratory for Air Pollution and Environmental Technology, Empa, Swiss Federal Laboratories for Materials Science and Technology,
Überlandstrasse 129, 8600 Dübendorf, Switzerland
Matthew Rigby
Atmospheric Chemistry Research Group, School of Chemistry, University of Bristol, Bristol, UK
Sunyoung Park
Kyungpook Institute of Oceanography, Kyungpook National University, South Korea
Shanlan Li
Kyungpook Institute of Oceanography, Kyungpook National University, South Korea
Myriam Guillevic
METAS, Federal Institute of Metrology, Lindenweg 50, Bern-Wabern, Switzerland
Blagoj Mitrevski
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Christina M. Harth
Scripps Institution of Oceanography, University of California at San Diego, La Jolla, California, USA
Benjamin R. Miller
Earth System Research Laboratory, NOAA, Boulder, Colorado, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, Colorado, USA
Stefan Reimann
Laboratory for Air Pollution and Environmental Technology, Empa, Swiss Federal Laboratories for Materials Science and Technology,
Überlandstrasse 129, 8600 Dübendorf, Switzerland
Bo Yao
Meteorological Observation Centre (MOC), China Meteorological Administration (CMA), Beijing, China
L. Paul Steele
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Simon A. Wyss
Laboratory for Air Pollution and Environmental Technology, Empa, Swiss Federal Laboratories for Materials Science and Technology,
Überlandstrasse 129, 8600 Dübendorf, Switzerland
Chris R. Lunder
Norwegian Institute for Air Research, Kjeller, Norway
Jgor Arduini
Department of Pure and Applied Sciences, University of Urbino, Urbino, Italy
Institute of Atmospheric Sciences and Climate, Italian National Research Council, Bologna, Italy
Archie McCulloch
Atmospheric Chemistry Research Group, School of Chemistry, University of Bristol, Bristol, UK
Songhao Wu
Kyungpook Institute of Oceanography, Kyungpook National University, South Korea
Tae Siek Rhee
Korea Polar Research Institute, KIOST, Incheon, South Korea
Ray H. J. Wang
School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, Georgia, USA
Peter K. Salameh
Scripps Institution of Oceanography, University of California at San Diego, La Jolla, California, USA
Ove Hermansen
Norwegian Institute for Air Research, Kjeller, Norway
Matthias Hill
Laboratory for Air Pollution and Environmental Technology, Empa, Swiss Federal Laboratories for Materials Science and Technology,
Überlandstrasse 129, 8600 Dübendorf, Switzerland
Ray L. Langenfelds
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Diane Ivy
Center for Global Change Science, Massachusetts Institute of Technology, Cambridge, Massachusetts, USA
Simon O'Doherty
Atmospheric Chemistry Research Group, School of Chemistry, University of Bristol, Bristol, UK
Paul B. Krummel
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Michela Maione
Department of Pure and Applied Sciences, University of Urbino, Urbino, Italy
Institute of Atmospheric Sciences and Climate, Italian National Research Council, Bologna, Italy
David M. Etheridge
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Lingxi Zhou
Chinese Academy of Meteorological Sciences (CAMS), China Meteorological Administration (CMA), Beijing, China
Paul J. Fraser
Climate Science Centre, CSIRO Oceans and Atmosphere, Aspendale, Victoria, Australia
Ronald G. Prinn
Center for Global Change Science, Massachusetts Institute of Technology, Cambridge, Massachusetts, USA
Ray F. Weiss
Scripps Institution of Oceanography, University of California at San Diego, La Jolla, California, USA
Peter G. Simmonds
Atmospheric Chemistry Research Group, School of Chemistry, University of Bristol, Bristol, UK
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- Australian chlorofluorocarbon (CFC) emissions: 1960–2017 P. Fraser et al. 10.1071/EN19322
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- Renewed and emerging concerns over the production and emission of ozone-depleting substances M. Chipperfield et al. 10.1038/s43017-020-0048-8
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- Automated fragment formula annotation for electron ionisation, high resolution mass spectrometry: application to atmospheric measurements of halocarbons M. Guillevic et al. 10.1186/s13321-021-00544-w
- Global increase of ozone-depleting chlorofluorocarbons from 2010 to 2020 L. Western et al. 10.1038/s41561-023-01147-w
32 citations as recorded by crossref.
- Indicators of Global Climate Change 2022: annual update of large-scale indicators of the state of the climate system and human influence P. Forster et al. 10.5194/essd-15-2295-2023
- Rapid increase in ozone-depleting chloroform emissions from China X. Fang et al. 10.1038/s41561-018-0278-2
- A review of ozone-depleting substances and fluorinated greenhouse gases in China Y. ZHANG et al. 10.3724/j.issn.1007-2802.20240042
- Seasonal cycles in baseline mixing ratios of a large number of trace gases at the Mace Head, Ireland atmospheric research station R. Derwent et al. 10.1016/j.atmosenv.2020.117531
- Eco‐friendly blowing agent, HCFO‐1233zd, for the synthesis of polyurethane foam as cryogenic insulation J. Park et al. 10.1002/app.51492
- The shared socio-economic pathway (SSP) greenhouse gas concentrations and their extensions to 2500 M. Meinshausen et al. 10.5194/gmd-13-3571-2020
- Despite Effective Ban, Ozone-destroying Chemicals Still Up in the Air C. Palmer 10.1016/j.eng.2023.07.004
- Airborne Observations of CFCs Over Hebei Province, China in Spring 2016 S. Benish et al. 10.1029/2021JD035152
- Abundances, emissions, and loss processes of the long-lived and potent greenhouse gas octafluorooxolane (octafluorotetrahydrofuran, <i>c</i>-C<sub>4</sub>F<sub>8</sub>O) in the atmosphere M. Vollmer et al. 10.5194/acp-19-3481-2019
- Inhalation exposure to volatile organic compounds in the printing industry A. Alabdulhadi et al. 10.1080/10962247.2019.1629355
- Very Strong Atmospheric Methane Growth in the 4 Years 2014–2017: Implications for the Paris Agreement E. Nisbet et al. 10.1029/2018GB006009
- Perfluorocyclobutane (PFC-318, <i>c</i>-C<sub>4</sub>F<sub>8</sub>) in the global atmosphere J. Mühle et al. 10.5194/acp-19-10335-2019
- History of chemically and radiatively important atmospheric gases from the Advanced Global Atmospheric Gases Experiment (AGAGE) R. Prinn et al. 10.5194/essd-10-985-2018
- Swiss halocarbon emissions for 2019 to 2020 assessed from regional atmospheric observations D. Rust et al. 10.5194/acp-22-2447-2022
- Identifying imprints of externally derived dust and halogens in the sedimentary record of an Iberian alpine lake for the past ∼13,500 years – Lake Peixão, Serra da Estrela (Central Portugal) J. Moreno et al. 10.1016/j.scitotenv.2023.166179
- Recent increases in the atmospheric growth rate and emissions of HFC-23 (CHF<sub>3</sub>) and the link to HCFC-22 (CHClF<sub>2</sub>) production P. Simmonds et al. 10.5194/acp-18-4153-2018
- Estimating Source Region Influences on Black Carbon Abundance, Microphysics, and Radiative Effect Observed Over South Korea K. Lamb et al. 10.1029/2018JD029257
- Dynamic–gravimetric preparation of metrologically traceable primary calibration standards for halogenated greenhouse gases M. Guillevic et al. 10.5194/amt-11-3351-2018
- Trends in N<sub>2</sub>O and SF<sub>6</sub> mole fractions in archived air samples from Cape Meares, Oregon (USA), 1978–1996 T. Rolfe & A. Rice 10.5194/acp-19-8967-2019
- CFCs measurements at high altitudes in northern China during 2017–2018: Concentrations and potential emission source regions M. Yang et al. 10.1016/j.scitotenv.2020.142290
- Bayesian assessment of chlorofluorocarbon (CFC), hydrochlorofluorocarbon (HCFC) and halon banks suggest large reservoirs still present in old equipment M. Lickley et al. 10.5194/acp-22-11125-2022
- Progress in the development and use of refrigerants and unintended environmental consequences A. Vuppaladadiyam et al. 10.1016/j.scitotenv.2022.153670
- Observing the atmospheric evolution of ozone-depleting substances S. Reimann et al. 10.1016/j.crte.2018.08.008
- Long-term temporal variations and source changes of halocarbons in the Greater Pearl River Delta region, China L. Zeng et al. 10.1016/j.atmosenv.2020.117550
- Australian chlorofluorocarbon (CFC) emissions: 1960–2017 P. Fraser et al. 10.1071/EN19322
- Unexpected nascent atmospheric emissions of three ozone-depleting hydrochlorofluorocarbons M. Vollmer et al. 10.1073/pnas.2010914118
- Unfinished business after five decades of ozone-layer science and policy S. Solomon et al. 10.1038/s41467-020-18052-0
- Renewed and emerging concerns over the production and emission of ozone-depleting substances M. Chipperfield et al. 10.1038/s43017-020-0048-8
- Challenges for the recovery of the ozone layer X. Fang et al. 10.1038/s41561-019-0422-7
- Temperature dependence of source profiles for volatile organic compounds from typical volatile emission sources Z. Niu et al. 10.1016/j.scitotenv.2020.141741
- Automated fragment formula annotation for electron ionisation, high resolution mass spectrometry: application to atmospheric measurements of halocarbons M. Guillevic et al. 10.1186/s13321-021-00544-w
- Global increase of ozone-depleting chlorofluorocarbons from 2010 to 2020 L. Western et al. 10.1038/s41561-023-01147-w
Discussed (preprint)
Latest update: 26 Apr 2024
Short summary
We measured the three chlorofluorocarbons (CFCs) CFC-13, CFC-114, and CFC-115 in the atmosphere because they are important in stratospheric ozone depletion. These compounds should have decreased in the atmosphere because they are banned by the Montreal Protocol but we find the opposite. Emissions over the last decade have not declined on a global scale. We use inverse modeling and our observations to find that a large part of the emissions originate in the Asian region.
We measured the three chlorofluorocarbons (CFCs) CFC-13, CFC-114, and CFC-115 in the atmosphere...
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