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ACP | Articles | Volume 18, issue 13
Atmos. Chem. Phys., 18, 9617–9629, 2018
https://doi.org/10.5194/acp-18-9617-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Chem. Phys., 18, 9617–9629, 2018
https://doi.org/10.5194/acp-18-9617-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 09 Jul 2018

Research article | 09 Jul 2018

An apportionment method for the oxidative potential of atmospheric particulate matter sources: application to a one-year study in Chamonix, France

Samuël Weber et al.

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Abrams, J. Y., Weber, R. J., Klein, M., Samat, S. E., Chang, H. H., Strickland, M. J., Verma, V., Fang, T., Bates, J. T., Mulholland, J. A., Russell, A. G., and Tolbert, P. E.: Associations between Ambient Fine Particulate Oxidative Potential and Cardiorespiratory Emergency Department Visits, Environ. Health Persp., 125, https://doi.org/10.1289/EHP1545, 2017. a
ANSES ExPOSURE: Etude multi-sites des variations du Potentiel Oxydant des PM atmosphériques en France, en liaison avec leur chimie et leurs sources, Tech. rep., ANSES, http://www.ige-grenoble.fr/recherche/equipes/chimie-atmospherique-chianti/projets/article/exposure?lang=en, 2017. a
Aymoz, G., Jaffrezo, J.-L., Jacob, V., Colomb, A., and George, Ch.: Evolution of organic and inorganic components of aerosol during a Saharan dust episode observed in the French Alps, Atmos. Chem. Phys., 4, 2499–2512, https://doi.org/10.5194/acp-4-2499-2004, 2004. a, b
Ayres, J. G., Borm, P., Cassee, F. R., Castranova, V., Donaldson, K., Ghio, A., Harrison, R. M., Hider, R., Kelly, F., Kooter, I. M., Marano, F., Maynard, R. L., Mudway, I., Nel, A., Sioutas, C., Smith, S., Baeza-Squiban, A., Cho, A., Duggan, S., and Froines, J.: Evaluating the Toxicity of Airborne Particulate Matter and Nanoparticles by Measuring Oxidative Stress Potential – A Workshop Report and Consensus Statement, Inhalation Toxicology, 20, 75–99, https://doi.org/10.1080/08958370701665517, 2008. a, b
Bates, J. T., Weber, R. J., Abrams, J., Verma, V., Fang, T., Klein, M., Strickland, M. J., Sarnat, S. E., Chang, H. H., Mulholland, J. A., Tolbert, P. E., and Russell, A. G.: Reactive oxygen species generation linked to sources of atmospheric particulate matter and cardiorespiratory effects, Environ. Sci. Technol., 49, 13605–13612, https://doi.org/10.1021/acs.est.5b02967, 2015. a, b, c, d
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The oxidative potential (OP) of the PM appears to be a relevant proxy of health outcomes from PM exposure. We developed a new statistical model using a coupled approach with positive matrix factorization (PMF) and multiple linear regressions to attribute a redox activity per PM sources. Our results highlight the importance of biomass burning and vehicular sources to explain the observed OP of PM. A different contribution of the sources is observed when considering OP or the mass of the PM10.
The oxidative potential (OP) of the PM appears to be a relevant proxy of health outcomes from PM...
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