The importance of mixed-phase and ice clouds for climate sensitivity in the global aerosol – climate model ECHAM 6-HAM 2

How clouds change in a warmer climate remains one of the largest uncertainties for the equilibrium climate sensitivity (ECS). While a large spread in the cloud feedback arises from low-level clouds, it was recently shown that mixed-phase clouds are also important for ECS. If mixedphase clouds in the current climate contain too few supercooled cloud droplets, too much ice will change to liquid water in a warmer climate. As shown by Tan et al. (2016), this overestimates the negative cloud-phase feedback and underestimates ECS in the CAM global climate model (GCM). Here we use the newest version of the ECHAM6-HAM2 GCM to investigate the importance of mixed-phase and ice clouds for ECS. Although we also considerably underestimate the fraction of supercooled liquid water globally in the reference version of the ECHAM6-HAM2 GCM, we do not obtain increases in ECS in simulations with more supercooled liquid water in the present-day climate, different from the findings by Tan et al. (2016). We hypothesize that it is not the global supercooled liquid water fraction that matters, but only how well lowand mid-level mixed-phase clouds with cloud-top temperatures in the mixed-phase temperature range between 0 and−35 C that are not shielded by higher-lying ice clouds are simulated. These occur most frequently in midlatitudes, in particular over the Southern Ocean where they determine the amount of absorbed shortwave radiation. In ECHAM6-HAM2 the amount of absorbed shortwave radiation over the Southern Ocean is only significantly overestimated if all clouds below 0 C consist exclusively of ice. Only in this simulation is ECS significantly smaller than in all other simulations and the cloud optical depth feedback is the dominant cloud feedback. In all other simulations, the cloud optical depth feedback is weak and changes in cloud feedbacks associated with cloud amount and cloud-top pressure dominate the overall cloud feedback. However, apart from the simulation with only ice below 0 C, differences in the overall cloud feedback are not translated into differences in ECS in our model. This insensitivity to the cloud feedback in our model is explained with compensating effects in the clear sky.


Introduction
Changes in clouds remain one of the largest uncertainties for the calculation of the response of the climate system to a given radiative forcing F (Dufresne and Bony, 2008).This response can be described with the following equation: (1) Here R represents the net radiative imbalance at the top of the atmosphere (TOA), H is the heat taken up by the ocean, T s is the net change in global annual mean surface temperature, and λ is the climate feedback parameter in W m −2 K −1 .R and T s change over time.In addition, some studies suggest that the heat uptake by the ocean is also time dependent and even λ is not a constant parameter (e.g., Knutti and Rugenstein, 2015).
Here we evaluate the increase in T s , which results from a doubling of carbon dioxide (CO 2 ) with respect to preindustrial concentrations, i.e., from a F 2×CO 2 on the order of 3.7 W m −2 (Solomon et al., 2007).There are two metrics that describe the temperature response to a doubling of CO 2 , the transient climate response (TCR) and the equilibrium climate sensitivity (ECS).TCR is estimated at the time of CO 2 doubling from atmosphere global climate model (GCM) simulations in which the CO 2 concentration increases by Published by Copernicus Publications on behalf of the European Geosciences Union.
1 % yr −1 and that are coupled to a dynamic ocean (e.g., Flato et al., 2013).ECS is obtained from coupled atmosphereocean simulations that are abruptly exposed to a CO 2 doubling relative to preindustrial concentrations and then run until a new equilibrium of the climate system has been established.This requires coupling of the atmosphere GCM to a fully coupled dynamic ocean model (e.g., Gregory et al., 2004;Flato et al., 2013).As such a coupled system takes a long time to reach a new equilibrium, sometimes ECS is approximated from coupled atmosphere-mixed-layer ocean (MLO) climate models (e.g., Meehl et al., 2007;Randall et al., 2007).
ECS can also be determined from the so-called Gregory method (Gregory et al., 2004), in which the TOA radiative flux is regressed against the annual global averaged surface air temperature change.While TCR is more relevant to present-day climate change because it is obtained from transient simulations that at the time of CO 2 doubling have not reached a new equilibrium climate, it is more expensive to calculate because it requires fully coupled atmosphere-ocean model simulations over the whole period.Therefore we focus on ECS from coupled atmosphere-MLO simulations in this paper.At the time of the new equilibrium in the, R and H vanish and Eq. ( 1) reduces to and T s equals the ECS.λ can be decomposed into different feedbacks (e.g., Soden et al., 2008;Shell et al., 2008).λ is the sum of the Planck feedback, the water vapor feedback, the lapse rate feedback, the surface albedo feedback, the cloud feedback λ c , that will be discussed further below, and a residual term (Shell et al., 2008).The residual term considers the interactions among the different components, nonlinear dependencies of ECS from the forcing (Vial et al., 2013) and errors in the radiative kernel method (Shell et al., 2008).This term needs to be small for the decomposition into individual feedbacks to explain the vast majority of the feedback.The average λ value from the GCMs that participated in the Coupled Model Intercomparison Project Phase 5 (CMIP5) is 1.1 W m −2 K −1 with a 90 % uncertainty range of ±0.5 W m −2 K −1 (Flato et al., 2013).The uncertainty in λ induces the uncertainty in ECS.Neither the average ECS of approximately 3 K (Collins et al., 2013) nor its uncertainty has changed much over time.
In a first model intercomparison paper by Cess et al. (1989), the estimates of ECS in GCMs varied between 1.4 and 4.1 K. Estimates from the GCMs used in CMIP5 are somewhat higher with 2.1 and 4.7 K (Forster et al., 2013;Flato et al., 2013), but the range in estimates remains similar.One of the prime contributors to this range in uncertainty are inter-model differences in the low-level shortwave cloud feedback (Yokohata et al., 2010).While the overall cloud feedback is positive with 0.3 W m −2 K −1 , the spread in λ c is larger than that of the overall climate feedback parameter and varies by ±0.7 W m −2 K −1 between the CMIP5 models (Flato et al., 2013).This means a negative λ c cannot be ruled out and the careful conclusion from the Fifth Assessment Report of the Intergovernmental Panel on Climate Change (IPCC AR5) was that λ c is likely (with a probability of 66 %) positive.Contributors to the positive net cloud feedback are a poleward shift of the midlatitude storms and decreases in the coverage of low-level clouds, both of which result in less scattering of solar radiation (Boucher et al., 2013).Another positive cloud feedback that operates mainly in the longwave radiation regime is the increase in the height of deep convective outflow.Because the troposphere warms but the cloud-top temperature remains at roughly the same temperature (fixed anvil temperature; Hartmann and Larson, 2002), the rate of longwave emission to space from these cloud tops does not keep pace with that of the underlying atmosphere, causing more longwave radiation to remain in the Earth-atmosphere system.
One of the more uncertain cloud feedbacks is the negative cloud optical depth (COD) feedback (e.g., Mitchell et al., 1989;Gordon and Klein, 2014;McCoy et al., 2015;Ceppi et al., 2016).The COD (τ ) is proportional to the cloud water path over the effective cloud particle size.Therefore changes in τ can occur due to changes in the cloud water path, which in turn originate from changes in the hydrological cycle, changes in the size of the cloud droplets and ice crystals and changes in cloud phase from ice to water or vice versa.The negative COD feedback is related to a shift from cloud ice in the present-day climate to cloud liquid water at the same altitude in the warmer climate.Because cloud droplets are generally smaller and more numerous than ice crystals and they have a different refractive index, the optical depth of liquid clouds is larger than that of ice clouds for a constant cloud water path.Precipitation formation is also less efficient for liquid clouds than for ice clouds (e.g., Lohmann, 1996;Hoose et al., 2008), further increasing cloud lifetime and τ of liquid clouds.If, in addition, the cloud water path increases in a warmer climate, τ will be further enlarged.All of these aspects result in a negative COD feedback.Tan et al. (2016) analyzed the ratio of supercooled liquid water to the sum of cloud liquid water and cloud ice (supercooled liquid fraction, SLF) between 0 and −35 • C in the CAM5 GCM.They found SLF to be systematically underestimated with respect to CALIOP observations, i.e., too much condensate to be in the form of ice at these temperatures.This led to a too negative cloud-phase feedback and in the CAM5 GCM to a too low ECS.When constraining the present-day SLF by satellite observations, their ECS increased by up to 1.3 • C. A similar increase in ECS of 1.5 • C was found by Frey and Kay (2017) when increasing the fraction of supercooled liquid clouds over the Southern Ocean.Terai et al. (2016) analyzed the low-COD feedback from eight CMIP5 models with that inferred from ISCCP, MODIS, and PAT-MOS satellite data.They also concluded that the low-COD feedback is likely too negative at mid and high latitudes in climate models.Motivated by these studies and to under-stand how universal the findings of the change in ECS using extreme assumptions about the liquid water/ice phase in mixed-phase clouds of Tan et al. (2016) are, here we use the ECHAM6-HAM2 GCM to calculate the impact of mixedphase and ice clouds on ECS.

Description of the model and the sensitivity studies
In this paper we use the latest version of the aerosol-climate model ECHAM6.3-HAM2.3, which assembles the most recent versions of the atmospheric general circulation model ECHAM (namely ECHAM6, as described in Stevens et al. (2013) with the most recent changes described below) and the aerosol module HAM based on the HAM2 version as described in Zhang et al. (2012), Neubauer et al. (2014), andSchultz et al. (2018) and summarized below.As our simulations are conducted with monthly mean oxidant fields instead of with interactive chemistry as in HAMMOZ (Schultz et al., 2018), we refer to it as ECHAM6-HAM2.

ECHAM6
ECHAM6 is the latest generation of the atmospheric general circulation model developed by the Max Planck Institute for Meteorology (Stevens et al., 2013).Like its predecessors, ECHAM6 employs a spectral transform dynamical core and a flux-form semi-Lagrangian tracer transport algorithm from Lin and Rood (1996).Vertical mixing occurs through turbulent mixing, moist convection (including shallow, deep, and mid-level convection), and momentum transport by gravity waves arising from boundary effects or atmospheric disturbances.Sub-grid-scale cloudiness (stratiform clouds) is represented using the scheme of Sundqvist et al. (1989), which diagnostically calculates the grid cell cloud fraction as a function of the relative humidity in a given grid cell, once a threshold value is exceeded.Cloud liquid water and cloud ice mixing ratios are treated prognostically following Lohmann and Roeckner (1996).In ECHAM6-HAM2, additional prognostic equations for the number concentrations of cloud droplets and ice crystals are included (Lohmann et al., 2007).The two-moment cloud microphysics scheme and the aerosol scheme are described in Sect.2.2.Radiative transfer in ECHAM6 is represented using the radiation transfer broadband model PSrad (Pincus and Stevens, 2013), which considers 14 and 16 bands for the shortwave (820 to 50 000 cm −1 ) and longwave (10 to 3000 cm −1 ) parts of the spectrum, respectively (Iacono et al., 2008).
Radiative transfer is computed based on the amount of gases, aerosols, and clouds in the atmosphere and their related optical properties.Trace gas concentrations of longlived greenhouse gases are specified in the model.Optical properties of aerosol particles and clouds are precalculated for each band of the RRTMG scheme using Mie theory offline and they read from a look-up table based on the con-centration of cloud droplets and ice crystals as computed by the two-moment scheme.
ECHAM6 includes a new land-surface model JSBACH (Reick et al., 2013).JSBACH assumes that each grid box is composed of two fractions, one representing bare soil and the other being covered with vegetation, this one being further subdivided into tiles, one for each of the 11 plant functional types distinguished in JSBACH.Soil hydrology is represented with a single-layer bucket model.A new treatment of the surface albedo (Brovkin et al., 2013) is included, which accounts for the different sections of bare and vegetated areas.
In addition to the improved representation of solar radiative transfer by the RRTMG scheme and the improved surface albedo, smaller changes are included.The vertical discretization within the troposphere (in particular in the upper troposphere and lower stratosphere) is slightly different, the representation of convective triggering has been improved, and the tuning of various model parameters was adjusted.In contrast to ECHAM5, ECHAM6 is more commonly used in a middle-atmosphere configuration, i.e., with the two verticals grids L47 and L95 that resolve the atmosphere from the surface up to 0.01 hPa (roughly 80 km).
Changes from ECHAM6.1, as coupled to HAM2 in Neubauer et al. (2014), to ECHAM6.3 used here include small changes in convection, in the middle atmosphere, improvements in snow and sea ice coverage, an improved aerosol climatology (Kinne et al., 2013) combined with a simple plume implementation of anthropogenic aerosols (Stevens et al., 2017), and an improved submodel interface.ECHAM6.3uses the Monte Carlo independent column approximation radiation scheme with the option for spectral sampling in time (Pincus and Stevens, 2013).The land model JSBACH has been updated with an improved hydrology and soil model.Changes in the cloud cover scheme were made to improve cloud cover in stratocumulus regions.ECHAM6.1 suffered from artificial cloud blinking that occurred due to a bug in the cloud cover scheme, causing the (fractional) cloud cover to be either 0 or 1.This cloud blinking has been removed in ECHAM6.3.
As in previous versions of ECHAM-HAM, ECHAM drives the aerosol and chemistry modules through the generic sub-model interface by providing meteorological conditions such as wind, temperature, pressure, specific humidity, and conditions pertaining to the land surface (taken from JS-BACH) such as leaf area index.Aerosol particles and their precursors are transported in the same way as water vapor and cloud species.

Aerosol and cloud microphysics scheme
The aerosol module HAM predicts the evolution of an aerosol ensemble considering five components: sulfate, black carbon, particulate organic matter, sea salt, and mineral dust.The aerosol spectrum is described by the superposition of www.atmos-chem-phys.net/18/8807/2018/Atmos.Chem.Phys., 18, 8807-8828, 2018 seven log-normal modes ranging from 0.005 to > 0.5 µm.Aerosol particles within a mode are assumed to be internally mixed, in the sense that each particle can consist of multiple components.Aerosols of different modes are externally mixed, meaning that they coexist in the atmosphere as independent particles.The seven modes of the aerosol number distribution are grouped into four geometrical size classes, including the nucleation, Aitken, accumulation, and coarse modes.Particles in four of the modes contain at least one soluble compound; thus they can take up water and are referred to as soluble.The particles in the other three modes consist of compounds with no or low water solubility and are referred to as insoluble.Through aging processes, insoluble particles can become soluble.Each mode of the aerosol size number distribution is described by the three moments, the aerosol number N, the number median radius r, and the standard deviation σ .The standard deviation is assumed to be constant and is set to 1.59 for the nucleation, Aitken, and accumulation modes and to 2 for the coarse modes.The median radius of each mode is calculated from the aerosol number and aerosol mass, which are transported as tracers.For more details, please refer to the description of HAM in Stier et al. (2005) and Zhang et al. (2012).
The two-moment cloud microphysics scheme that predicts the number concentrations and mass mixing ratios of cloud droplets and ice crystals in stratiform clouds as implemented in ECHAM5 is described in Lohmann et al. (2007) and Lohmann and Hoose (2009).The microphysics scheme includes all phase changes between the water components (condensation, evaporation, freezing, melting, deposition, and sublimation) and precipitation processes (autoconversion of cloud droplets, accretion of raindrops with cloud droplets and snow flakes with cloud droplets and ice crystals, aggregation of ice crystals).Moreover, evaporation of raindrops and melting and sublimation of snowflakes are considered, as well as sedimentation of cloud ice.The cloud microphysics scheme is coupled to the aerosol scheme HAM through the processes of cloud droplet activation and ice crystal nucleation (Lohmann et al., 2007) as well as through in-cloud and below-cloud scavenging (Croft et al., 2009;Croft et al., 2010).Convective clouds are not radiatively active and have much simpler conversion rates (Tiedtke, 1989).The detrained condensate from convective clouds is a source for the stratiform cloud scheme.
Heterogeneous freezing in mixed-phase clouds occurs by contact and immersion freezing as discussed below.In the standard configuration, cirrus clouds are assumed to form by homogeneous freezing of supercooled solution droplets (Lohmann and Kärcher, 2002).Homogeneous and heterogeneous nucleation strongly depends on the vertical velocity that results in supersaturation.The vertical velocity is a superposition of the grid-scale vertical velocity and a sub-gridscale component, which is linked to the turbulent kinetic energy (Lohmann and Kärcher, 2002).
Since the ECHAM-HAM model validation in Lohmann and Hoose (2009), the cloud microphysics scheme has undergone the following scientific improvements.
1.While in the previous ECHAM6-HAM version cloud droplet activation followed the empirical scheme by Lin and Leaitch (1997), it now uses a parameterization of cloud droplet activation based on Köhler theory by Abdul-Razzak and Ghan (2000) as discussed in Stier (2016).
2. Previously, the increase in cloud droplet number concentration (CDNC) from cloud droplets that were detrained from convective clouds, was applied everywhere in the grid box.We now weight the detrained CDNC by the detrained mass and add it to the mass-weighted CDNC of the stratiform part.In addition, the split of the detrained cloud water mass into liquid water and ice was made consistent between the number concentrations and mass mixing ratios of cloud droplets and ice crystals.
3. We now assume the shape of ice crystals to be hexagonal plates of crystal type P1a following Pruppacher and Klett (1997).Before we used the empirical mass-size relationships from their Table 2.4, which are only valid for crystals between 0.3 and 1.5 mm in size.We replaced that with their empirical relationship in Table 2.2, which is valid from 10 µm to 3 mm and thus covers the whole ice crystal size range.Also, while we assumed that all ice crystals are hexagonal plates in the cloud microphysics scheme, cirrus crystals were treated as spheres for the calculation of the effective ice crystal radius and ice cloud optical properties in Zhang et al. (2012).This inconsistency has been eliminated and ice crystals are now hexagonal plates everywhere in the module.
4. The heterogeneous nucleation scheme in the mixedphase cloud regime among temperatures between 273.15 and 238.15K considers contact nucleation by mineral dust and immersion nucleation by black carbon and mineral dust following Lohmann and Hoose (2009).However, because there is no evidence that Aitken mode particles contribute to freezing (Marcolli et al., 2007), we now limit the immersion freezing of black carbon to particles in the accumulation mode or larger.
5. The temperature dependence of sticking efficiency used for accretion of ice crystals by snow has been changed to the expression used in Seifert and Beheng (2006).
6.In previous versions, the minimum CDNC (CDNCmin) was set to 40 cm −3 .The justification for this choice was twofold: first, while observations of clouds with a lower CDNC exist (e.g, Terai et al., 2014;Wood et al., 2018), these smaller concentrations normally occur in clouds or pockets in clouds that are much smaller than our grid boxes.Second, so far we do not account for nitrate aerosols and our treatment of secondary organic aerosols is rather simplistic and likely underestimates the organic aerosol concentration (Zhang et al., 2012).Therefore we are likely to underestimate CDNC, which we partly buffer by using CDNCmin = 40 cm −3 .However, CDNCmin has a large impact on the aerosol radiative forcing (Hoose et al., 2009).Therefore we introduced the option to have two ECHAM6.3-HAM2.3versions, one that keeps the CDNCmin at 40 cm −3 and one in which we lower CDNCmin to 10 cm −3 .
In addition to the scientific improvements, we removed smaller inconsistencies, such that cloud droplets and ice crystals could both grow and evaporate/sublimate in one time step and that there is nonzero CDNC below 238.15 K, nonzero ice crystal number concentrations above 273.15K, and inconsistencies in the calculation of cloud cover, condensation, and the ice crystal number concentration in cirrus clouds.Moreover, the two-moment cloud microphysics scheme is now energy conserving and has been modularized.

Model set-up and experiments
In this paper, we compare results from the release version of ECHAM6-HAM2 with CDNCmin = 40 cm −3 (simulation REF) and the sensitivity simulations discussed below with observations.To address the impact of SLF on ECS in ECHAM6-HAM2, we conducted one simulation with no supercooled liquid water below 0 • C (simulation ALL_ICE) and one simulation with no ice formation at temperatures > −35 • C (simulation ALL_LIQ), similar to what has been done in Tan et al. (2016) and Lohmann (2002).The simulation ALL_ICE is set up such that all cloud droplets that are advected to colder temperatures are forced to freeze instantaneously and all the detrained cloud condensate is in the form of ice at temperatures < 0 • C. The simulation ALL_LIQ is set up such that heterogeneous freezing is turned off in the temperature range between 0 and −35 • C and detrainment of ice crystals from convective clouds is restricted to temperatures below −35 • C. Ice crystals sedimenting from colder into warmer cloud layers melt at −35 • C. The number of cloud droplets which freeze at temperatures below −35 • C had to be reduced by a factor of 100 in order to keep the ice crystal number concentration realistic in simulation ALL_LIQ and to reduce tuning to a minimum.
In this paper we go beyond the study by Tan et al. (2016) and also test the impact of other aspects of clouds on ECS, such as the type of nucleation in cirrus.There are discussions if cirrus clouds are mainly formed by homogeneous nucleation as we assume in our reference simulation or are nucleated heterogeneously (Cziczo et al., 2013;Spichtinger and Krämer, 2012;Kärcher, 2017).We investigate the impact of homogeneous vs. heterogeneous freezing in cirrus clouds by performing one simulation in which all cirrus clouds form heterogeneously (simulation HET) instead of homogeneous nucleation in simulation REF.Heterogeneously nucleated cirrus clouds are optically thinner (Lohmann, 2008).Thus, with this simulation we aim to address the impact of cirrus on ECS that so far remains uncertain (Boucher et al., 2013).
Last but not least we investigate the impact of parameterized convection on ECS by performing a simulation in which we completely switched off convection (simulation NOCONV) as in Webb et al. (2015).This is normally performed only in simulations run at horizontal resolutions of less than 10 km, at which the vertical motions associated with deep convection start to be resolved.While our horizontal resolution is much coarser and thus a convective parameterization is needed, there are some inconsistencies in terms of microphysics between convective and stratiform clouds.Therefore we evaluate how the cloud fields, the climate in general, and ECS are simulated if only large-scale clouds are allowed to form.
All simulations were performed in T63 spectral resolution, which corresponds to 1.875 • × 1.875 • and 31 vertical layers with a top at 10 hPa.The present-day atmosphere-only simulations were run over 25 years, after a 3-month spin-up with fixed sea surface temperatures (SSTs) and sea-ice cover (averaged over the atmosphere model intercomparison project (AMIP) climatology for the years 2000-2015).To calculate ECS, ECHAM6-HAM2 has been coupled to a MLO of 50 m depth.The deep ocean heat flux is computed from the atmosphere-only simulations.Because the deep ocean heat flux adjusts to the different set-ups, we computed it individually for each of the five different set-ups used in this study.These simulations were spun up for 25 years after which the simulations were in equilibrium.We then ran them for another 25 years, over which the results were averaged.
The sensitivity studies conducted for our studies are summarized in Table 1.For the calculation of ECS, all simulations need to be in radiative equilibrium at the TOA.This might require retuning.To keep the different simulations as comparable as possible, we only adjusted two parameters inside the two-moment cloud microphysics scheme.γ r speeds up the autoconversion rate of cloud droplets to grow to raindrops by collision-coalescence and accounts for the missing sub-grid-scale variability in cloud water and CDNC (Wood, 2002).γ s is the corresponding process in the ice phase, which enhances the aggregation of ice crystals to form snow flakes (Lohmann and Ferrachat, 2010).The values of these two parameters are also included in Table 1.In addition to the changes in the tuning parameters, we needed to decrease the time step from 7.5 to 5 min in simulation NOCONV because of numerical stability.
All of the simulations listed in Table 1 were run in three different set-ups: (i) atmosphere-only simulations with prescribed SST and sea ice cover using the AMIP 2000-2015 climatology with present-day aerosol emissions and greenhouse gas concentrations for comparison with observations, (ii) atmosphere-MLO simulations at 1 × CO 2 concentrations from MODIS (Platnick et al., 2015(Platnick et al., , 2017)), 43.9 g m −2 from ATSR-2-AATSR (Stengel et al., 2017a;Poulsen et al., 2017), and 41 g m −2 from AVHRR-PM (Stengel et al., 2017b), illustrating the huge uncertainty of estimating LWP oc .All simulations except for ALL_LIQ fall within this range.In simulation ALL_LIQ, LWP oc amounts to 110 g m −2 because no ice is formed at temperatures > −35 • C. The annual zonal mean LWP and ice water path (IWP) from all simulations as well as from satellite observations of LWP from multiple satellite sensors (Elsaesser et al., 2018), the MODIS satellite (Platnick et al., 2015(Platnick et al., , 2017)), and the ATSR-2-AATSR satellites (Stengel et al., 2017a;Poulsen et al., 2017) and IWP from CALIPSO/CloudSat (Li et al., 2012) are shown in Fig. 1.Because the MAC-LWP observations are only available over oceans, we limit the comparison of LWP to ocean regions.Both retrievals from visiblenear-infrared sensors and microwave sensors have biases in retrieving LWP (Seethala and Horvath, 2010;Lebsock and Su, 2014).Lebsock and Su (2014) mentioned four biases in LWP retrievals for MODIS (visible-near-infrared sensor) and AMSR-E (microwave sensor): a bias at large solar zenith angles (MODIS), missing pixels of low-lying clouds that are not detected (MODIS), LWP retrievals in cloud-free scenes (AMSR-E), and the partitioning of the microwave signal between cloud and precipitation signals (AMSR-E).The LWP bias of microwave-sensor-based products in clearsky scenes has been recently corrected by Elsaesser et al. (2018).The LWP estimates of microwave retrieval products are most reliable in regions where LWP is much larger than the rainwater path (RWP).Thus, Elsaesser et al. (2018) recommend restricting the LWP satellite data to regions in which LWP/(LWP + RWP) > 0.8.This LWP oc,low_pr covers areas dominated by stratocumulus, trade wind cumulus regions in the subtropics, the Southern Ocean, high latitudes in the Northern Hemisphere, and parts of the north Atlantic and north Pacific.LWP oc,low_pr from MAC-LWP should thus have the smallest retrieval biases.Therefore we use it to evaluate the model LWP as shown in Fig. 1.
The new multi-satellite observations of LWP oc by Elsaesser et al. ( 2018), averaged over the years 1988-2016, show a maximum LWP in the tropics and, on average, their estimate is twice as high as the retrievals from MODIS and ATSR-2-AATSR both for the years 2003-2012.LWP oc from MODIS and ATSR-2-AATSR, conversely, increases towards the poles and only a weak secondary maximum is indicated near the Equator.All observations show high values of LWP oc in the storm tracks in both hemispheres, but the exact location varies among the different observations.The most noticeable difference between LWP oc and LWP oc,low_pr is the absence of data in the intertropical convergence zone (ITCZ).In fact, the agreement of simulations REF and HET in terms of the zonal mean structure of LWP oc,low_pr with observations is very good everywhere and better than with LWP oc .LWP oc,low_pr is too low at high latitudes in simulation ALL_ICE and the maxima in the extratropics are overestimated in simulation ALL_LIQ.LWP oc,low_pr is underestimated everywhere in simulation NOCONV because of the large speedup of the autoconversion rate required to reach radiative equilibrium at the TOA in this set-up.
The cloud-top CDNC for oceanic clouds (N l,oc,top ) with temperatures between 268 and 300 K has been obtained from satellite data (Bennartz and Rausch, 2017) for the years 2003-2015.From the model simulations, oceanic cloud-top CDNCs were used for temperatures > 273.2 K. N l,oc,top is less zonally symmetric than LWP as a result of the higher emissions in the Northern Hemisphere.N l,oc,top reaches values of > 100 cm −3 between 30 and 60 • N in the observations  Platnick et al. (2015Platnick et al. ( , 2017)), Stengel et al. (2017a), Poulsen et al. (2017), andElsaesser et al. (2018); of LWP oc,low_pr from Elsaesser et al. (2018); of IWP from the CloudSat/CALIPSO satellites (Li et al., 2012); of N l,oc,top from Bennartz and Rausch (2017) of total cloud cover from Stubenrauch et al. (2013) and Matus and L'Ecuyer (2017); of precipitation rate from the GPCP version 2.3 data set (Adler et al., 2003(Adler et al., , 2012)).The CRE satellite data are averaged over the period 2001-2011 from the Clouds and the Earth's Radiant Energy System Energy Balanced and Filled Ed2.6r data set (Boucher et al., 2013) and are described in Loeb et al. (2009Loeb et al. ( , 2018)).For the uncertainty range of the SW CRE data from CloudSat and CALIPSO are also considered (Matus and L'Ecuyer, 2017) and for LW CRE data from the TOVS satellite are also considered (Susskind et al., 1997).See legend of Fig. 1  (Fig. 1).All model simulations fail to produce such high values north of 40 • N, probably because of an insufficient transport of aerosol particles to the Arctic (Bourgeois and Bey, 2011), missing nitrate aerosols, and underestimation of particulate organic aerosols (Zhang et al., 2012), all of which contribute to underestimating the concentration of cloud condensation nuclei.N l,oc,top is well simulated south of 30 • N, especially in simulation ALL_LIQ.N l,oc,top is highest in simulation ALL_ICE (Table 2) and overestimated with respect to the observations.This is caused by the lower speedup of the autoconversion rate in simulation ALL_ICE (Table 1), which reduces the sink of cloud droplets in this simulation and causes higher CDNC at all altitudes compared to simulation REF (not shown).
The zonal distribution of N l,oc,top in simulation NOCONV differs from the other simulations.It peaks near the Equator because the clouds here cannot form by convection and instead the stratiform cloud scheme needs to take over.As the rain formation depends on CDNC only in the stratiform cloud microphysics scheme but not in the convective one, warm rain is less efficiently formed in the tropics in the stratiform scheme, causing a buildup of cloud droplets in simulation NOCONV as portrayed in Fig. 1.The CDNC peak in the tropics in simulation NOCONV deviates strongly from observations, as do the lower-than-observed values in the extratropics.
ECHAM6-HAM2 in general has problems simulating IWP values in the observed range.This deficiency can largely be attributed to an underestimation in the ice crystal size in simulation REF at least for clouds with a COD < 3 (Gasparini et al., 2018).The only simulation in which IWP in the global mean agrees with the observations is simulation HET (Table 2) because the heterogeneous nucleation is limited by the number concentration of dust aerosols.The dust number concentration is smaller than the number concentration of soluble aerosols that can freeze homogeneously and freezing commences at a lower relative humidity and a higher temperature in simulation HET.Because of the limited number concentration of dust aerosols and the faster depositional growth at higher temperatures, the heterogeneously nucleated ice crystals are larger than the ones nucleated homogeneously.Because of this, they sediment and aggregate more rapidly, causing simulation HET to be initially out of radiative balance.Here retuning was necessary to slow down the rate of aggregation and at the same time speed up the rate of autoconversion.This resulted in one of the lowest LWPs of all simulations and the highest IWPs with the highest ice crystal number concentration.
The IWP peak in the tropics in Fig. 1 is related to liquidorigin cirrus clouds (Wernli et al., 2016;Kraemer et al., 2016;Gasparini et al., 2018) forming the anvils from deep convection in the ITCZ as well as in the warm conveyor belt in the storm tracks.The peak in the ITCZ is not captured in any of the model simulations, suggesting that the model severely underestimates the detrained cloud ice in deep convective clouds.Cloud ice in the extratropics is underestimated in all simulations but simulations HET and ALL_ICE.IWP is largest in simulation HET due to retuning as discussed above.(Loeb et al., 2009(Loeb et al., , 2018)), the dashed ones from ERBE for the years 1985-1989, and the dotted ones for LW CRE from TOVS satellite data for the years 1985-1993 (Susskind et al., 1997).
Its zonal distribution shows that the underestimation of IWP in the tropics is compensated for by an overestimation in the extratropics.Simulation ALL_ICE best matches the magnitude of IWP in the extratropics but shifts the peaks slightly polewards of the observations.The total cloud cover in ECHAM6-HAM2 is that of largescale clouds because convective clouds are considered to be short lived and to decay within one model time step except for the detrained condensate in the anvils that is taken as a source for the stratiform cloud scheme.The global mean total cloud cover does not vary much among the different simulations and it falls within the observed range of 68 ±5 % (Stubenrauch et al., 2013) in all simulations.It is secondlargest in simulation ALL_LIQ because of its large LWP.It is highest in simulation NOCONV because here all clouds are large scale and contribute to the cloud cover.
The observed precipitation rate from GPCP of 2.7 mm d −1 (Adler et al., 2003) averaged over 1981-2010 is overestimated by 6-13 % in all simulations, a feature that ECHAM6-HAM2 shares with its host model ECHAM6 (Stevens et al., 2013).As discussed in Stevens et al. (2013), GPCP seems to underreport precipitation, and higher precipitation rates are more consistent with the best observational estimates of the surface energy budget (Stephens et al., 2012).
The cloud radiative effect (CRE) is the difference between the all-sky radiation at the TOA and the clear-sky radiation.The shortwave (SW) CRE amounts to −47.3 W m −2 with a range from −46 to −53.3 W m −2 in the satellite data (Loeb et al., 2009(Loeb et al., , 2018;;Zelinka et al., 2017).In all simulations, except ALL_LIQ, SW CRE amounts to about −50 W m −2 , which lies within the observed range.SW CRE is most negative and outside the observational range in simulation ALL_LIQ because of its high LWP and total cloud cover (see also Fig. 1).Conversely, it is least negative in simulation ALL_ICE, in which LWP is rather small and hence τ is smallest.Here SW CRE is severely underestimated south of 40 • S due to the lack of supercooled liquid water.While too much absorption of shortwave radiation over the South-ern Ocean has been a problem in the many GCMs because of insufficient supercooled liquid water (e.g., Williams et al., 2013;Bodas-Salcedo et al., 2014;Kay et al., 2016), in our model this problem only arises in the extreme simulation ALL_ICE.
LW CRE amounts to 26.2 W m −2 with a range from 22 to 30.5 W m −2 in the satellite data (Loeb et al., 2009(Loeb et al., , 2018;;Susskind et al., 1997;Zelinka et al., 2017).As for SW CRE, all simulations but ALL_LIQ calculate LW CRE to be about 24-25 W m −2 in good agreement with observations.Again LW CRE is smallest in simulation ALL_ICE and highest and outside the observational range in simulation ALL_LIQ (see also Fig. 1).Due to the severe underestimation of cloud ice in the tropics in all simulations, LW CRE is systematically underestimated in the tropics.The exception is simulation ALL_LIQ in which the underestimation in tropical cloud ice is compensated for by the thickest high level clouds (Fig. 2).
The global mean observed net CRE ranges between −17.1 and −22.8 W m −2 .Here all simulations are more negative than observed, i.e., they overestimate the net negative radiative effect of clouds.
The vertical distribution of the globally and annually averaged cloud liquid water and cloud ice is shown in Fig. 2. Cloud liquid water has its maximum at around 800 hPa associated with low clouds where it varies between 20 and 30 mg kg −1 in the different simulations.It is lowest in simulation NOCONV because of the drastically enhanced autoconversion rate (Table 1).Cloud liquid water decreases to zero at around 400 hPa except in simulation ALL_LIQ in which ice formation is limited to temperatures < −35 • C. Unfortunately no observational data of the vertical distribution of cloud liquid water are available.
The vertical distribution of cloud ice has been derived from CALIPSO/CloudSat (Li et al., 2012).It peaks at 400 hPa with 6 mg kg −1 and becomes negligible at altitudes above 100 hPa and below 900 hPa (Fig. 2).Here the differences among the sensitivity experiments are more pronounced.In simulations REF and NOCONV the shape of the distribution looks similar to the observed distribution, but the peak value is underestimated by 30-50 % and in simulation REF a secondary maximum is present at around 780 hPa.This peak is related to cloud ice over the Southern Ocean and Antarctica (not shown).In simulation ALL_LIQ, in which the global annual mean IWP is smallest due to suppressed ice formation in mixed-phase clouds, cloud ice peaks at 250 hPa and drops to zero at 600 hPa.This simulation differs most from the observations.It also has the lowest cloud cover in the lower troposphere and the highest cloud fraction between 200 and 400 hPa (Fig. 2).Conversely, simulation NOCONV has the highest coverage of low-level clouds and the smallest coverage of cirrus clouds.
In simulation ALL_ICE the comparison of cloud ice with observations is also less favorable compared to simulation REF because more cloud ice than observed is simulated in the lower atmosphere while the underestimation of cloud ice at higher altitudes has not noticeably improved.The overall best agreement with observations is seen in simulation HET.This is the only simulation in which the global annual mean IWP lies within the observational uncertainty (Table 2).However, the peak in cloud ice at 400 hPa is 25 % too large and too narrow.Although the freezing mechanism was only changed for cirrus clouds, the overall higher amount of cloud ice extends to lower altitudes, causing an overestimation in cloud ice between 600 and 900 hPa.This is mainly a result of the reduced speedup of the aggregation rate that also affects cloud ice in mixed-phase clouds.
SLF has been obtained from the CALIOP satellite and has been compared to an earlier version of ECHAM6-HAM2 (Komurcu et al., 2014).At that time ECHAM6-HAM2 seriously underestimated SLF.This can partly be explained by differences in the definition of SLF in the satellite data and in the model.In addition, some of the model improvements mentioned above were added after the study by Komurcu et al. (2014).As the lidar signal becomes attenuated at COD > 3, the CALIOP satellite data are only representative for all cloud tops not overlaid by clouds with COD > 3. SLF of the model data is diagnosed similarly to CALIOP starting from the highest cloud layers as long as the cumulative COD of these cloud layers is less than or equal to 3. As shown in Fig. 3, ECHAM6-HAM2 still underestimates SLF but on average simulates SLFs twice as high as presented in Komurcu et al. (2014).At −10 • C SLF amounts to 63 % in CALIOP but only 37 % in simulation REF.The difference between the observed and simulated SLF decreases at colder temperatures because of the general decrease in SLF with decreasing temperature.
SLF from all ECHAM simulations is significantly underestimated except for simulations ALL_LIQ and NOCONV.Simulation NOCONV actually matches the observed SLF rather well, mainly because supercooled liquid water exists at higher altitudes than in simulation REF (Fig. 2).This points to a potential deficiency as to how we handle detrainment from convective clouds or convection itself.In simulation REF we assume that if we are in the Wegener-Bergeron-Findeisen (WBF) regime, following the definition of Korolev (2007) as described in Lohmann and Hoose (2009), and cloud ice is already present, the detrained condensate will be in the form of ice.It is only detrained as supercooled liquid water if the vertical velocity is sufficiently high to exceed saturation with respect to liquid water.This assumption seems to cause a too efficient WBF process, thus depleting the supercooled liquid water too rapidly.We will rethink our approach in the future.
The control simulation in CESM from Tan et al. (2016) simulates a SLF of only 20 % at −10 • C. Based on their hypothesis that an underestimation in SLF translates into an underestimation in ECS, a smaller underestimation of SLF in simulation REF should lead to a smaller underestimation of ECS in ECHAM6-HAM2.Based on the simulated SLFs, we expect ECS to be lowest in simulation ALL_ICE and to suc-   1.

Equilibrium climate sensitivity
In a warmer climate, the saturation-specific humidity increases by 7 % • C −1 of temperature increase according to the Clausius-Clapeyron equation.Because the relative humidity has been found to remain rather constant (Soden et al., 2002), this causes an increase in the specific humidity and speeds up the hydrological cycle leading to higher liquid water contents in clouds and higher precipitation rates.
ECS from all our sensitivity simulations is shown in Table 3.It ranges between 1.8 and 2.6 K and with that lies on the lower side of the range of ECS estimated in the last IPCC re-port (Collins et al., 2013;Flato et al., 2013) and from CMIP5 models (Forster et al., 2013).Similar to Tan et al. (2016), ECS increases by ∼ 30 % when increasing SLF from almost zero to one (simulations ALL_ICE and ALL_LIQ in this paper vs. Low-SLF and High-SLF in Tan et al., 2016).Contrary to their large increase in ECS from their reference simulation to simulation High-SLF, ECS does not change among simulations REF, NOCONV, and ALL_LIQ but remains at ∼ 2.5-2.6K despite the increase in SLF at −10 • C from ∼ 30 % in HET and ∼ 40 % in REF to ∼ 70 % in NOCONV and 100 % in ALL_LIQ, i.e., only ECS in simulation ALL_ICE is noticeably different.This suggests that ECHAM6-HAM2 is more sensitive at low SLF.These results seem to support the hypothesis that an increase in ECS is only sensitive to SLF if too little shortwave radiation is reflected back to space from mixed-phase midlatitude clouds, i.e., when they are composed of ice instead of liquid water.This has also been suggested by Frey and Kay (2017), who modified CAM5 to detrain more liquid water at colder temperatures in shallow convective clouds, which occur in the cold sector of midlatitude cyclones, for example.It is important that these mixed-phase clouds are not shielded by ice clouds in order for a change in their cloud phase to affect ECS (Bodas-Salcedo, 2018).Since in ECHAM6-HAM2 this shortwave bias is most pronounced in simulation ALL_ICE, this is the only simulation with a distinctively lower ECS.In the reference version of CAM5, too much shortwave radiation is absorbed over the Southern Ocean in their present-day climate (Kay et al., 2016), which explains why ECS is also sensitive to an increase in SLF in this model (Tan et al., 2016).In addition, Tan et al. (2016) did not use a MLO, but a fully coupled dynamic ocean, which could impact the comparison with our results because different methods can lead to differing ECS estimates (Frey et al., 2017).
In order to prove our hypothesis for the different relationship between SLF and ECS in ECHAM6-HAM2, we evaluate the changes in cloud fraction as a function of cloud-top Table 3. Global annual mean changes of surface temperature ( T s ), liquid water path ( LWP), ice water path ( IWP), vertically integrated cloud droplet ( N l ) and ice crystal number concentration ( N i ), total cloud cover ( CC), SW CRE ( SW CRE), LW CRE ( LW CRE), and net CRE from the radiative kernel (RK) method and as normally diagnosed in equilibrium after a CO 2 doubling averaged over the years 26 to 50 of the coupled atmosphere -MLO model simulations as well as the net clear-sky feedback parameter λ cs diagnosed according to Block and Mauritsen (2013) pressure and COD between the 2 × CO 2 and 1 × CO 2 climates.Because mixed-phase clouds are more prevalent in midlatitudes and high latitudes than in the tropics and subtropics (Matus and L'Ecuyer, 2017), we expected the largest differences there.The histograms in Figs. 4 and 5 are taken polewards of 40 • latitude in both hemispheres.They are taken from a satellite perspective, by using the COSP-ISCCP simulator (Bodas-Salcedo et al., 2011).This means that the cloud-top pressure refers to the highest cloud in each single sub-column used by the simulator.Sub-columns are used in the simulator to account for sub-grid-scale variability in the cloud (top) distribution.From Fig. 4 we see that only in simulation ALL_ICE is there a large abundance of low-and mid-level optically thin extratropical clouds (with τ < 1.3) in the present climate.These clouds show a marked decrease accompanied with a marked increase in medium optical depth clouds (3.6 < τ < 60) between 560 and 800 hPa in the 2 × CO 2 climate (Fig. 5).These clouds and their changes are absent in all other simulations with a higher SLF (REF, HET, NOCONV, and ALL_LIQ).Only in simulation ALL_ICE are these optically thin ice clouds not shielded by higher clouds prevalent in the present-day climate (not shown) and are converted to low-and mid-level liquid water clouds of medium optical depth in the 2 × CO 2 climate.
To estimate the radiative effect of this increase in COD, we calculate the different components of the global cloud feedback parameter λ c using the radiative kernel decomposition method described in Zelinka et al. (2012a, b).This method decomposes λ c into feedbacks that are associated with changes in cloud amount λ amt , cloud-top pressure λ ctp , and COD λ τ as shown in Fig. 6 for all simulations.λ ctp is positive because of the shift of clouds to higher altitudes in the warmer climate (see also Fig. 7) that enhances their LW CRE.At the same time, the total cloud amount decreases in a warmer climate, most noticeable at lower altitudes (Fig. 7).This decrease in low/mid-level clouds reduces the negative net CRE and also constitutes a positive feedback.λ τ is negative in most simulations and smaller than other cloud feedbacks so that λ c is positive in most simulations.λ c is negative (−0.4 W m −2 K −1 ) only in simulation ALL_ICE because of its large negative λ τ .In all other simulations λ c ranges between 0.3 W m −2 K −1 and 0.6 W m −2 K −1 .The value of 0.6 W m −2 K −1 corresponds to the mean of the analyzed GCMs in AR5 (Boucher et al., 2013).The estimates from the other simulations (except ALL_ICE) fall within the 90 % range of the cloud feedback of −0.2 to 0.6 W m −2 K −1 as assessed in AR5 (Boucher et al., 2013).
The largest differences among the simulations are associated with changes in λ τ , which varies between −0.6 W m −2 K −1 in simulation ALL_ICE and 0.1 W m −2 K −1 in simulation NOCONV.In simulation ALL_ICE, the large negative value of λ τ can be explained with the largest increase in the LWP of 4.8 g m −2 (Table 3) due to the phase change from cloud ice to cloud liquid water mainly in low-and mid-level midlatitude clouds (Fig. 5).This causes a negative optical depth feedback in all regions, but most pronounced polewards of 40 • (Fig. 8).Note that simulation ALL_ICE is the only simulation in which the overall cloud feedback parameter is dominated by changes in COD.The results of simulation ALL_ICE agree qualitatively with the results from Bodas-Salcedo (2018) for regions with large-scale subsidence in which optically thin ice clouds in the present-day climate are not shielded by higher clouds and hence for which the COD feedback is most important.In all other simulations, the cloud feedback is dominated by changes in cloud amount and cloud-top pressure (Fig. 6).In the other simulations, shown in Fig. 5 for midlatitudes and high latitudes, a rather different picture emerges.Here τ of low clouds hardly changes or decreases as the majority of them are already composed of cloud droplets in the present climate and only a small phase change from ice to liquid occurs due to the doubling of CO 2 .In all simulations, except for simulation NOCONV, a negative cloud-phase feedback is also visible in the tropics.This negative feedback arises because some tropical clouds that glaciate at the tops, either due to the presence of ice-nucleating particles in the mixed-phase temperature regime or because their tops extend to altitudes with temperatures < −35 • C in the present climate, will remain supercooled in the warmer climate and hence become optically thicker (Figs. 8 and 9).
In the warmer climate, the static stability increases in areas with marine stratus, stratocumulus, and trade wind cumuli in all simulations.This is accompanied by a stronger moisture gradient, which promotes stronger drying by more entrainment (Gettelman and Sherwood, 2016), which in turn causes the marine subtropical clouds to become thinner and their optical depth to decrease.In most simulations this leads to a positive COD feedback in the subtropics as shown in Fig. 8.
The parameterization of convective clouds in ECHAM6-HAM2 assumes that they form and dissipate in one time step.During their lifetime, they can detrain cloud water and ice in the environment.Thus the negative COD feedback in the tropics and midlatitudes indicates that more cloud condensate is detrained in the form of liquid or supercooled liquid water rather than as cloud ice in the warmer climate.Thus, next to the rise of the melting level in the warmer climate, the rise of the homogeneous freezing level is also important for the negative cloud-phase feedback.This is best seen in simulation ALL_LIQ in which no ice exists at mixed-phase temperatures, yet the negative cloud-phase feedback still operates in the tropics (Figs. 8 and 9).In the global mean, this negative cloud-phase feedback is visible in all our simulations as a simultaneous increase in cloud liquid water and decrease in cloud ice in the warmer climate at a given pressure level (Fig. 7).In midlatitudes and the tropics it shows up as an increase in optically thicker clouds and decrease in optically thinner clouds for the same cloud-top pressure (Figs. 5  and 9).
The second most important contributor to the differences in the overall cloud feedback between simulations ALL_ICE and ALL_LIQ is the change in cloud-top pressure (λ ctp ).λ ctp varies between 0.1 W m −2 K −1 in simulation ALL_ICE and 0.4 W m −2 K −1 in simulation ALL_LIQ.The cloud-top pressure feedback is mainly related to cirrus clouds and has been estimated from satellite observations to amount to 0.2 W m −2 K −1 (Zhou et al., 2014).We obtain a cloud-top  pressure feedback of about this value in all other simulations.We also computed the cloud feedbacks separately for low and non-low clouds following the decomposition by Zelinka et al. (2016), which leads to a weaker cloud-top pressure feedback but in general qualitatively similar results for all simulations (not shown).
λ ctp is largest in simulation ALL_LIQ in which the global mean changes in cloud liquid water and cloud ice are distinctively different from all other simulations (Fig. 7).It is the only simulation in which cloud liquid water decreases throughout the lower and mid-troposphere because here the poleward shift of the storm tracks and the upward shift of convective clouds are least compensated for by changes from cloud ice to cloud liquid water.The changes in simulation ALL_LIQ are accompanied with the largest decrease in cloud cover between 750 and 370 hPa.Cloud liquid water increases between 250 and 400 hPa at the expense of cloud ice in simulation ALL_LIQ.In all other simulations, the concurrent increase in cloud liquid water and decrease in cloud ice occurs at altitudes below 400 hPa.The different vertical structure of cloud liquid water and cloud ice in simulation ALL_LIQ is a consequence of the design of this simulation.Because cloud ice only forms at temperatures below −35 • C, cloud droplets are carried upwards to this temperature, such that the optically thick clouds extend to higher altitudes in the 2 × CO 2 climate (see Figs. 5 and 9), causing the largest cloud-top pressure feedback as shown in Fig. 6.
The opposite effect can be seen in simulation ALL_ICE, in which all cloud water is converted to ice already at 0 • C. The increase in cloud liquid water in low and mid-level clouds in the warmer climate is largest in this simulation mainly because of the negative cloud-phase feedback (Fig. 7).This   1.
combined with only a modest increase in cloud ice and cloud cover between 250 and 100 hPa (Fig. 7) causes the cloud-top pressure feedback to be smallest in this simulation (Fig. 6).
Simulation NOCONV is the only simulation in which λ τ is slightly positive.λ τ is negative in all other simulations in the tropics (Fig. 8) because more cloud condensate is detrained in the form of liquid or supercooled liquid water in the warmer climate.The absence of a convection parameterization and hence detrainment in simulation NOCONV on average leads to a positive tropical λ τ , i.e., the tropical and subtropical clouds in simulation NOCONV become optically thinner.
To summarize, the negative COD feedback only dominates the overall cloud feedback if the low-and mid-level midlatitude clouds consist of ice in the present climate and change to liquid in the 2 × CO 2 climate as in simulation ALL_ICE.However, this does not imply that the overall cloud feedback remains more or less constant in the other simulations.In fact, λ c almost doubles from simulations REF and HET to simulations NOCONV and ALL_LIQ, caused by the large increase in cloud-top pressure feedback in simulation ALL_LIQ and a positive λ τ in simulation NOCONV as explained above.This marked increase in the overall cloud feedback from simulations HET and REF to simulations NO-CONV and ALL_LIQ is, however, not reflected in an increase in ECS because the net clear-sky feedback parameter, i.e., the sum of the clear-sky Planck, water vapor, lapse rate, and surface albedo feedbacks, is largest in simulation ALL_LIQ followed by simulation NOCONV (Table 3).We hypothesize that different processes contribute to the rather similar ECS in all simulations but ALL_ICE: in simulation ALL_LIQ, this seems to be caused by the optically thick clouds that tend to cluster in the tropics and become optically thicker there.This is apparent from Fig. 9, in which the upward shift in cirrus clouds with an increase in cirrus optical depth between 180 and 310 hPa is much more pronounced in simulation ALL_LIQ than in simulation REF.In addition, the negative cloud-phase feedback is restricted to ice clouds that formed at altitudes with temperatures < −35 • C in the 1 × CO 2 climate that are now liquid clouds (Fig. 7).
This increase in optical depth of high clouds causes their SW CRE to be more negative and completely offsets the reduction in LW CRE from the decrease in cloud cover in the tropics in simulation ALL_LIQ (Fig. 10).Such a clustering of convective clouds was found by Lohmann and Roeckner (1995) using the ECHAM4 model when the emissivity of cirrus clouds was set to 1 (black cirrus), i.e., when the infrared optical depth was increased.No convective clustering was seen in the reference simulation in which the cirrus emissivity was calculated as a function of ice water path and in a simulation with transparent cirrus in the infrared.In a warmer climate, convective clouds have been found to cluster further (Bony et al., 2016).The clustering of convective clouds in the warmer climate arises because cloud tops remain at nearly the same temperature in a warmer climate (e.g., Hartmann and Larson, 2002) but are in a more stable environment, which decreases anvil outflow in the upper troposphere and decreases the anvil cloud fraction (Bony et al., 2016).In ECHAM this decrease is most pronounced at altitudes below 250 hPa (Fig. 7) from which more longwave radiation is emitted to space.This leads to an overall negative feedback (e.g., Hartmann and Larson, 2002;Mauritsen and Stevens, 2015) because of the much larger clear-sky area and offsets the positive cloud feedback.In the present-day climate of simulation ALL_LIQ, the least amount of outgoing longwave radiation is emitted to space because the clouds are optically thickest in this simulation.In a warmer climate, these clouds cluster further in the intertropical convergence zone as can be seen from the largest increase in LW CRE as diagnosed from the radiative kernel (RK) method (Fig. 10).Because these clouds are optically thick, this large increase in LW CRE (RK) is overcompensated for by a decrease in SW CRE (RK), causing the net CRE (RK) in the intertropical convergence zone to be as negative in simulation ALL_LIQ as in simulation REF.
The cloud-top pressure feedback in the extratropics that is significantly positive in all simulations but ALL_ICE where it is close to zero (not shown) is overcompensated for by decreases in cloud cover.As shown in Fig. 10 10. Changes in the annual zonal SW and LW net clear-sky radiation in watts per square meter at the top-of-the-atmosphere and surface temperature (K) (a); changes in SW, LW, and net cloud radiative effects between the 2 × CO 2 and 1 × CO 2 climates calculated based on the radiative kernel method (b) and normally diagnosed (c) for the simulations described in Table 1.Negative values for the change in clear-sky outgoing longwave radiation denote higher values in the 2 × CO 2 climate.Please note the different vertical axes.smaller positive and larger negative changes in net CRE than in net CRE (RK) are caused by compensating changes in non-cloud climate components as described in detail in Shell et al. (2008).In high latitudes, the decrease in surface albedo due to melting of Arctic sea ice causes especially large negative SW CRE and net CRE values polewards of 70 • N. In the clear-sky, water vapor and CO 2 absorb more longwave radiation in the warmer climate than in the present day.This decreases the difference between all-sky and clear-sky fluxes and causes the LW CRE to be less positive.Differences in surface temperature operate in opposite ways.While more longwave radiation is emitted to space in the warmer climate (negative Planck feedback), more longwave radiation is also absorbed by clouds and re-emitted to the surface (positive cloud feedback).This clear-sky compensation in the longwave is most pronounced in simulation ALL_LIQ, which is the only simulation in which the global mean LW CRE (RK) is positive (Table 3).
The changes between simulation REF and ALL_LIQ are qualitatively comparable to the ones from Lohmann and Roeckner (1995), for which the difference in climate sensitivity was also rather small between the reference simulation and the black cirrus simulation, both of which also had a positive cloud feedback and an increase in net CRE.There was a noticeable difference between the transparent cirrus and the reference simulation because only the transparent cirrus sim-ulation produced a negative cloud feedback and a decrease in net CRE.While in our simulation CRE is always negative or close to zero, it is most negative in simulation ALL_ICE, which corresponds to the transparent cirrus simulation.
ECS in simulation HET is also similar to simulation REF, but differences in LW CRE (RK) exist.As in simulation ALL_LIQ, in simulation HET the increase in LW CRE (RK) in the tropics is also larger than in simulation REF (Fig. 10) because of the upward shift of ice clouds (Fig. 7) and their increase in optical depth (Fig. 9).Because these ice clouds are of medium optical depth, the large LW CRE (RK) is overcompensated for by a decrease in SW CRE (RK), causing net CRE (RK) and net CRE to be similar to in simulation REF (Table 3).
In simulation NOCONV the outgoing longwave clear-sky radiation is increased the most.While it is also slightly decreased in the tropics, the decrease is smallest in this simulation because of the absence of convection (Fig. 10).The associated absence of detrainment slows down the Wegener-Bergeron-Findeisen process on the one hand, but required the largest speedup of the autoconversion rate on the other hand (Table 1).The latter causes the present-day cloud liquid water and its increase in the warmer climate to be smallest (Tables 2 and 3).This explains the overall positive λ τ and the second largest λ c .The most negative clear-sky LW radiation changes in NOCONV explain why ECS does not increase compared to in simulation REF.The absence of convection also seems to limit the increase in cirrus clouds (increase in cloud cover at altitudes above 250 hPa; Fig. 7).

Conclusions
In this study we used the newly developed ECHAM6.3-HAM2.3coupled global aerosol-climate model to assess the influence of different cloud processes for ECS.This work was motivated by the findings of Tan et al. (2016) using CAM5, who showed a large influence of correcting the underestimated SLF in present-day mixed-phase clouds on ECS.An underestimate of SLF has also been found in other models (Komurcu et al., 2014;Barrett et al., 2017a, b) and in a different version of CAM5 (Kay et al., 2016).The SLF was found to be most sensitive to the glaciation rate, which in turn is influenced by cloud ice microphysics and the model's vertical resolution (Barrett et al., 2017a, b).In ECHAM6-HAM2, SLF could be improved when switching off the convective parameterization entirely.The absence of convection and hence detrained cloud ice slows down the glaciation rate in ECHAM6-HAM2, which corroborates the findings by Barrett et al. (2017a) on the importance of the glaciation rate for SLF.
In ECHAM6-HAM2, ECS is much smaller than in the CAM5 GCM used by Tan et al. (2016).It varies between 1.8 and 2.5 K in ECHAM6-HAM2 versus between 3.9 and 5.7 K in CAM5 (Tan et al., 2016).Thus, while ECS is on the low side of the ECS range between 2.1 and 4.7 K in IPCC AR5 (Forster et al., 2013;Flato et al., 2013) in ECHAM6-HAM2, it is on the high side in CAM5.Note that the percentage increase in ECS of 30 % between the extreme scenarios (ALL_ICE to ALL_LIQ in ECHAM6-HAM2 vs. Low-SLF to High-SLF in CAM5) is similar, indicating that the relative contribution of the negative cloud-phase feedback to the overall ECS is comparable in both GCMs.
However, important differences between the two GCM studies are apparent: increasing SLF in ECHAM6-HAM2 from its calculated values in the reference simulation to one as in simulation ALL_LIQ does not increase ECS in contrast to the findings by Tan et al. (2016).Part of this difference could be caused by the overestimation of shortwave absorption over the Southern Ocean due to too efficient freezing in low-and mid-level shallow convective clouds in CAM5 (Kay et al., 2016).We hypothesize that it is the SLF of these optically thin low-and mid-level midlatitude clouds not shielded by overlying clouds that matters for ECS because the cloudtop temperature of these clouds is in the mixed-phase temperature range.Hence, the cloud phase at the cloud top of these clouds plays an important role in the TOA radiation budget.If the absorption of shortwave radiation over the Southern Ocean is correctly simulated, then SLF in other clouds does not matter for ECS.At least this is what the ECHAM6-HAM2 results show because only in simulation ALL_ICE is significantly less shortwave radiation reflected back to space from Southern Ocean clouds and this is the only simulation in which ECS is significantly smaller than in all other simulations.In all other simulations sufficient or even too much shortwave radiation is reflected back to space from Southern Ocean clouds and all of them have similar values of ECS.
The reason why an underestimation of SLF in cloud types other than thin midlatitude clouds with cloud-top temperatures between 0 and −35 • C does not seem to matter is because radiative changes in clouds in the warm sector of extratropical cyclones are masked by ice clouds above them (Bodas-Salcedo et al., 2016).In addition, the tops of tropical deep convective and deep frontal clouds consist of ice and that will not change in a warmer climate.Low-level clouds in the tropics and subtropics already consist of liquid water and therefore their cloud phase will also not change in the future climate.
In our model, it is not only the cloud-phase feedback and the overall cloud feedback that matters for ECS.If this were the case, ECS should be largest in simulation ALL_LIQ, in which the cloud feedback parameter is highest.It seems that in simulation ALL_LIQ tropical deep convective clouds tend to aggregate, which causes a negative feedback by increasing the clear-sky area and with that the longwave emission from clear-sky regions to space (e.g., Hartmann and Larson, 2002;Mauritsen and Stevens, 2015).This negative feedback reduces the positive cloud feedback and causes the changes in the net cloud radiative effect and ECS to be the same in simulations REF and ALL_LIQ.Also in simulation NOCONV, in which we switched off the convection parameterization, SLF is higher than in simulation REF because of a reduced Wegener-Bergeron-Findeisen process.Again, ECS remains the same because of the smallest increase in cirrus cloud cover in this simulation that allows more clear-sky longwave radiation emission to space than in the reference simulation.
As discussed by Frey et al. (2017), while cloud-phase improvements in the extratropics affect ECS in their model, they do not seem to matter for the warming during the 21st century in the Community Earth System Model (CESM) because of compensating responses in ocean circulation.Whether this is also the case in other Earth system models, will be subject to future investigations.

Figure 2 .
Figure 2. Annual global mean cloud liquid water content (a), ice water content (b) in milligrams per kilogram, and cloud cover (c) in percent as a function of pressure in hectopascals from the various sensitivity atmosphere-only present-day simulations for the years 2003-2012 described in Table 1 and observations of the ice water content from CALIPSO-CloudSat for the years 2006-2010 by Li et al. (2012).

Figure 3 .
Figure 3. Frequency of occurrence of SLF in percent for clouds with COD < 3 in different temperature bins from CALIOP observations for the years 2006-2010 and the various sensitivity simulations from the atmosphere-only present-day simulations for the years 2003-2012 described in Table1.

Figure 4 .
Figure 4. Distribution of cloud fraction in the extratropics (> 40 • S and N) as a function of cloud optical depth and cloud-top pressure between the 2 × CO 2 and the 1 × CO 2 climate in simulations ALL_ICE, HET, REF, NOCONV, and ALL_LIQ from the last 25 years of the MLO simulations described in Table1.

Figure 5 .
Figure 5. Changes in the distribution of cloud fraction in the extratropics (> 40 • S and N) as a function of cloud optical depth and cloud-top pressure between the 2 × CO 2 and the 1 × CO 2 climates in simulations ALL_ICE, HET, REF, NOCONV, and ALL_LIQ from the last 25 years of the MLO simulations described in Table1.

Figure 6 .
Figure6.Components of the globally averaged cloud feedback parameter λ c in W m −2 K −1 for the simulations described in Table1.λ τ accounts for changes in cloud optical depth, λ amt accounts for changes in cloud amount, and λ ctp accounts for changes in cloudtop pressure.

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Figure 7. Change in the annual global mean cloud liquid water content (LWC, a) and ice water content (IWC, b) in milligrams per kilogram as a function of pressure in hectopascals between the 2 × CO 2 and 1 × CO 2 climates for the simulations described in Table1.

Figure 8 .
Figure 8. Tropical, subtropical, extratropical, and global cloud optical depth feedback parameter λ τ in W m −2 K −1 for the sensitivity simulations described in Table1.

Table 1 .
Set-up of the simulations together with the two tuning parameters that differ among the simulations.

Table 2 .
Global annual mean of oceanic LWP oc ; LWP oc,low_pr ; IWP; vertically integrated global cloud droplet (N l ); CDNC at cloud top over oceans (N l,oc,top ); ice crystal number concentration (N i ); total cloud cover (CC); precipitation rate (P ); shortwave (SW), longwave (LW), and net cloud radiative effect (CRE) from observations; and 20-year atmosphere-only present-day model simulations with prescribed SST as described in Table1for 2003-2012.The satellite observations of LWP oc are taken from for details of the observations.
. The individual simulations are described in Table 1.Different from Table 2, here the changes in LWP are global and not limited to ocean regions.
, SW CRE and SW CRE (RK) become less negative in the extratropics and dominate over the decrease in LW CRE and LW CRE (RK), causing a positive net CRE at midlatitudes.The generally U. Lohmann and D. Neubauer: Ice containing clouds and climate sensitivity