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ACP | Articles | Volume 18, issue 8
Atmos. Chem. Phys., 18, 5861–5877, 2018
https://doi.org/10.5194/acp-18-5861-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Special issue: Surface Ocean Aerosol Production (SOAP) (ACP/OS inter-journal...

Atmos. Chem. Phys., 18, 5861–5877, 2018
https://doi.org/10.5194/acp-18-5861-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 26 Apr 2018

Research article | 26 Apr 2018

Gradient flux measurements of sea–air DMS transfer during the Surface Ocean Aerosol Production (SOAP) experiment

Murray J. Smith et al.

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Cited articles

Andreae, M. O. and Crutzen, P. J.: Atmospheric aerosols: Biogeochemical sources and role in atmospheric chemistry, Science, 276, 1052–1058, https://doi.org/10.1126/science.276.5315.1052, 1997. 
Bell, T. G.: DMS Data Selection, available at: http://saga.pmel.noaa.gov/dms/select.php, last access: 11 April 2018. 
Bell, T. G., De Bruyn, W., Miller, S. D., Ward, B., Christensen, K. H., and Saltzman, E. S.: Air–sea dimethylsulfide (DMS) gas transfer in the North Atlantic: evidence for limited interfacial gas exchange at high wind speed, Atmos. Chem. Phys., 13, 11073–11087, https://doi.org/10.5194/acp-13-11073-2013, 2013. 
Bell, T. G., De Bruyn, W., Marandino, C. A., Miller, S. D., Law, C. S., Smith, M. J., and Saltzman, E. S.: Dimethylsulfide gas transfer coefficients from algal blooms in the Southern Ocean, Atmos. Chem. Phys., 15, 1783–1794, https://doi.org/10.5194/acp-15-1783-2015, 2015. 
Bell, T. G., Landwehr, S., Miller, S. D., de Bruyn, W. J., Callaghan, A. H., Scanlon, B., Ward, B., Yang, M., and Saltzman, E. S.: Estimation of bubble-mediated air–sea gas exchange from concurrent DMS and CO2 transfer velocities at intermediate–high wind speeds, Atmos. Chem. Phys., 17, 9019–9033, https://doi.org/10.5194/acp-17-9019-2017, 2017. 
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The transfer of gases across the air–sea interface has a significant influence on climate. During a research voyage in the South Pacific we measured the transfer rate of the biogenic gas dimethyl sulfide (DMS) from the ocean using two independent methods. The agreement between the techniques provides confidence in their use in compilations of global gas transfer. We also identified physical conditions under which the observations are not well predicted by a standard gas transfer model.
The transfer of gases across the air–sea interface has a significant influence on climate....
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