Articles | Volume 18, issue 1
https://doi.org/10.5194/acp-18-467-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-467-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
17 Jan 2018
Research article |
| 17 Jan 2018
| 17 Jan 2018
Secondary organic aerosol formation from ambient air in an oxidation flow reactor in central Amazonia
Brett B. Palm
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Suzane S. de Sá
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Weiwei Hu
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
Roger Seco
Dept. of Earth System Science, University of California, Irvine, CA, USA
Steven J. Sjostedt
Earth System Research Laboratory, National Oceanic and Atmospheric
Administration, Boulder, CO, USA
Jeong-Hoo Park
National Center for Atmospheric Research, Boulder, CO, USA
now at: Climate and Air Quality Research Department, National
Institute of Environmental Research (NIER), Incheon, 22689, Republic of
Korea
Alex B. Guenther
Dept. of Earth System Science, University of California, Irvine, CA, USA
Div. of Atmospheric Sciences & Global Change, Pacific Northwest
National Laboratory, Richland, WA, USA
Saewung Kim
Dept. of Earth System Science, University of California, Irvine, CA, USA
Joel Brito
Institute of Physics, University of São Paulo, São Paulo, Brazil
now at: Laboratory for Meteorological Physics (LaMP), Université
Clermont Auvergne, 63000 Clermont-Ferrand, France
Florian Wurm
Institute of Physics, University of São Paulo, São Paulo, Brazil
Paulo Artaxo
Institute of Physics, University of São Paulo, São Paulo, Brazil
Ryan Thalman
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
now at: Department of Chemistry, Snow College, Richfield, UT, USA
Jian Wang
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
Lindsay D. Yee
Department of Environmental Science, Policy, and Management,
University of California, Berkeley, CA, USA
Rebecca Wernis
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA, USA
Gabriel Isaacman-VanWertz
Department of Environmental Science, Policy, and Management,
University of California, Berkeley, CA, USA
now at: Department of Civil and Environmental Engineering, Virginia
Tech, Blacksburg, VA, USA
Allen H. Goldstein
Department of Environmental Science, Policy, and Management,
University of California, Berkeley, CA, USA
Department of Civil and Environmental Engineering, University of
California, Berkeley, CA, USA
Yingjun Liu
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA, USA
now at: Department of Environmental Science, Policy, and
Management, University of California, Berkeley, CA, USA
Stephen R. Springston
Environmental and Climate Sciences Department, Brookhaven National
Laboratory, Upton, NY, USA
Rodrigo Souza
University of the State of Amazonas, Manaus, Brazil
Matt K. Newburn
Environmental and Molecular Sciences Laboratory, Pacific Northwest
National Laboratory, Richland, WA, USA
M. Lizabeth Alexander
Environmental and Molecular Sciences Laboratory, Pacific Northwest
National Laboratory, Richland, WA, USA
Scot T. Martin
School of Engineering and Applied Sciences, Harvard University,
Cambridge, MA, USA
Department of Earth and Planetary Sciences, Harvard University,
Cambridge, MA, USA
Jose L. Jimenez
CORRESPONDING AUTHOR
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
Dept. of Chemistry, University of Colorado, Boulder, CO, USA
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- Rate constant and secondary organic aerosol formation from the gas-phase reaction of eugenol with hydroxyl radicals C. Liu et al. 10.5194/acp-19-2001-2019
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- No Particle Mass Enhancement from Induced Atmospheric Ageing at a Rural Site in Northern Europe E. Ahlberg et al. 10.3390/atmos10070408
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58 citations as recorded by crossref.
- Major Regional-Scale Production of O3 and Secondary Organic Aerosol in Remote Amazon Regions from the Dynamics and Photochemistry of Urban and Forest Emissions J. Nascimento et al. 10.1021/acs.est.2c01358
- Constraining nucleation, condensation, and chemistry in oxidation flow reactors using size-distribution measurements and aerosol microphysical modeling A. Hodshire et al. 10.5194/acp-18-12433-2018
- Quantification of the role of stabilized Criegee intermediates in the formation of aerosols in limonene ozonolysis Y. Gong & Z. Chen 10.5194/acp-21-813-2021
- Total OH Reactivity Changes Over the Amazon Rainforest During an El Niño Event E. Pfannerstill et al. 10.3389/ffgc.2018.00012
- Secondary Organic Aerosol Formation from Urban Roadside Air in Hong Kong T. Liu et al. 10.1021/acs.est.8b06587
- The Chamber Wall Index for Gas–Wall Interactions in Atmospheric Environmental Enclosures W. Brune 10.1021/acs.est.8b06260
- A computationally efficient model to represent the chemistry, thermodynamics, and microphysics of secondary organic aerosols (simpleSOM): model development and application to α-pinene SOA S. Jathar et al. 10.1039/D1EA00014D
- Urban Oxidation Flow Reactor Measurements Reveal Significant Secondary Organic Aerosol Contributions from Volatile Emissions of Emerging Importance R. Shah et al. 10.1021/acs.est.9b06531
- Experimental and model estimates of the contributions from biogenic monoterpenes and sesquiterpenes to secondary organic aerosol in the southeastern United States L. Xu et al. 10.5194/acp-18-12613-2018
- Towards a satellite formaldehyde – in situ hybrid estimate for organic aerosol abundance J. Liao et al. 10.5194/acp-19-2765-2019
- Observations of Manaus urban plume evolution and interaction with biogenic emissions in GoAmazon 2014/5 G. Cirino et al. 10.1016/j.atmosenv.2018.08.031
- Study of secondary organic aerosol formation and aging using ambient air in an oxidation flow reactor during high pollution events over Delhi V. Goel et al. 10.1016/j.envres.2024.118542
- Changes in biogenic volatile organic compound emissions in response to the El Niño–Southern Oscillation R. Vella et al. 10.5194/bg-20-4391-2023
- Assessing the degree of plug flow in oxidation flow reactors (OFRs): a study on a potential aerosol mass (PAM) reactor D. Mitroo et al. 10.5194/amt-11-1741-2018
- Single-particle characterization of aerosols collected at a remote site in the Amazonian rainforest and an urban site in Manaus, Brazil L. Wu et al. 10.5194/acp-19-1221-2019
- Unexpected Biomass Burning Aerosol Absorption Enhancement Explained by Black Carbon Mixing State C. Denjean et al. 10.1029/2020GL089055
- In-situ measurement of secondary aerosol formation potential using a flow reactor: Livestock agricultural area F. Ashraf et al. 10.1016/j.atmosenv.2023.119695
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- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
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- Tropical and Boreal Forest – Atmosphere Interactions: A Review P. Artaxo et al. 10.16993/tellusb.34
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- Oxidation Flow Reactor Results in a Chinese Megacity Emphasize the Important Contribution of S/IVOCs to Ambient SOA Formation W. Hu et al. 10.1021/acs.est.1c03155
- How weather events modify aerosol particle size distributions in the Amazon boundary layer L. Machado et al. 10.5194/acp-21-18065-2021
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- Urban pollution greatly enhances formation of natural aerosols over the Amazon rainforest M. Shrivastava et al. 10.1038/s41467-019-08909-4
- Urban influence on the concentration and composition of submicron particulate matter in central Amazonia S. de Sá et al. 10.5194/acp-18-12185-2018
- Effects of gas–wall interactions on measurements of semivolatile compounds and small polar molecules X. Liu et al. 10.5194/amt-12-3137-2019
- Long-range transported North American wildfire aerosols observed in marine boundary layer of eastern North Atlantic G. Zheng et al. 10.1016/j.envint.2020.105680
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- The Chemical Characteristics and Formation of Potential Secondary Aerosol (PSA) using an Oxidation Flow Reactor (OFR) in the Summer: Focus on the Residential Area, Suwon G. Park et al. 10.5572/KOSAE.2019.35.6.786
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- Estimation of Secondary Organic Aerosol Formation During a Photochemical Smog Episode in Shanghai, China H. Wang et al. 10.1029/2019JD032033
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- Measurement of Formation Rates of Secondary Aerosol in the Ambient Urban Atmosphere Using a Dual Smog Chamber System S. Jorga et al. 10.1021/acs.est.9b03479
- Secondary organic aerosol formation and aging from ambient air in an oxidation flow reactor during wintertime in Beijing, China W. Xu et al. 10.1016/j.envres.2022.112751
- Contributions of biomass-burning, urban, and biogenic emissions to the concentrations and light-absorbing properties of particulate matter in central Amazonia during the dry season S. de Sá et al. 10.5194/acp-19-7973-2019
- Secondary organic aerosol production from local emissions dominates the organic aerosol budget over Seoul, South Korea, during KORUS-AQ B. Nault et al. 10.5194/acp-18-17769-2018
- Rate constant and secondary organic aerosol formation from the gas-phase reaction of eugenol with hydroxyl radicals C. Liu et al. 10.5194/acp-19-2001-2019
- Characterization of Aerosol Aging Potentials at Suburban Sites in Northern and Southern China Utilizing a Potential Aerosol Mass (Go:PAM) Reactor and an Aerosol Mass Spectrometer J. Li et al. 10.1029/2018JD029904
- Interactive relations between plants, the phyllosphere microbial community, and particulate matter pollution M. Mandal et al. 10.1016/j.scitotenv.2023.164352
- No Particle Mass Enhancement from Induced Atmospheric Ageing at a Rural Site in Northern Europe E. Ahlberg et al. 10.3390/atmos10070408
- Total OH reactivity over the Amazon rainforest: variability with temperature, wind, rain, altitude, time of day, season, and an overall budget closure E. Pfannerstill et al. 10.5194/acp-21-6231-2021
- Key challenges for tropospheric chemistry in the Southern Hemisphere C. Paton-Walsh et al. 10.1525/elementa.2021.00050
- Aerosols from anthropogenic and biogenic sources and their interactions – modeling aerosol formation, optical properties, and impacts over the central Amazon basin J. Nascimento et al. 10.5194/acp-21-6755-2021
- Role of space station instruments for improving tropical carbon flux estimates using atmospheric data P. Palmer et al. 10.1038/s41526-022-00231-6
- Understanding the Evolution of Smoke Mass Extinction Efficiency Using Field Campaign Measurements P. Saide et al. 10.1029/2022GL099175
Latest update: 18 Apr 2024
Short summary
Ambient air was oxidized by OH or O3 in an oxidation flow reactor during both wet and dry seasons in the GoAmazon2014/5 campaign to study secondary organic aerosol (SOA) formation. We investigated how much biogenic, urban, and biomass burning sources contributed to the ambient concentrations of SOA precursor gases and how their contributions changed diurnally and seasonally. SOA yields and hygroscopicity of organic aerosol in the oxidation flow reactor were also studied.
Ambient air was oxidized by OH or O3 in an oxidation flow reactor during both wet and dry...
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