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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 18, issue 4 | Copyright
Atmos. Chem. Phys., 18, 2973-2983, 2018
https://doi.org/10.5194/acp-18-2973-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 01 Mar 2018

Research article | 01 Mar 2018

Water vapor increase in the lower stratosphere of the Northern Hemisphere due to the Asian monsoon anticyclone observed during the TACTS/ESMVal campaigns

Christian Rolf1, Bärbel Vogel1, Peter Hoor2, Armin Afchine1, Gebhard Günther1, Martina Krämer1, Rolf Müller1, Stefan Müller2,3, Nicole Spelten1, and Martin Riese1 Christian Rolf et al.
  • 1Institute for Energy and Climate Research (IEK-7), Forschungszentrum Jülich GmbH, Jülich, Germany
  • 2Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
  • 3now at: Enviscope GmbH, 60489 Frankfurt, Germany

Abstract. The impact of air masses originating in Asia and influenced by the Asian monsoon anticyclone on the Northern Hemisphere stratosphere is investigated based on in situ measurements. A statistically significant increase in water vapor (H2O) of about 0.5ppmv (11%) and methane (CH4) of up to 20ppbv (1.2%) in the extratropical stratosphere above a potential temperature of 380K was detected between August and September 2012 during the HALO aircraft missions Transport and Composition in the UT/LMS (TACTS) and Earth System Model Validation (ESMVal). We investigate the origin of the increased water vapor and methane using the three-dimensional Chemical Lagrangian Model of the Stratosphere (CLaMS). We assign the source of the moist air masses in the Asian region (northern and southern India, eastern China, southeast Asia, and the tropical Pacific) based on tracers of air mass origin used in CLaMS. The water vapor increase is correlated with an increase of the simulated Asian monsoon air mass contribution from about 10% in August to about 20% in September, which corresponds to a doubling of the influence from the Asian monsoon region. Additionally, back trajectories starting at the aircraft flight paths are used to differentiate transport from the Asian monsoon anticyclone and other source regions by calculating the Lagrangian cold point (LCP). The geographic location of the LCPs, which indicates the region where the set point of water vapor mixing ratio along these trajectories occurs, can be predominantly attributed to the Asian monsoon region.

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The Asian monsoon is a pronounced circulation system linked to rapid vertical transport of surface air from India and east Asia in the summer months. We found, based on aircraft measurements, higher concentration of water vapor in the lowermost stratosphere caused by the Asian monsoon. Enrichment of water vapor concentrations in the lowermost stratosphere impacts the radiation budget and thus climate. Understanding those variations in water vapor is important for climate projections.
The Asian monsoon is a pronounced circulation system linked to rapid vertical transport of...
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