Articles | Volume 18, issue 23
https://doi.org/10.5194/acp-18-17705-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-17705-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Dec 2018
Research article |
| 13 Dec 2018
| 13 Dec 2018
Combined effects of boundary layer dynamics and atmospheric chemistry on aerosol composition during new particle formation periods
Liqing Hao
CORRESPONDING AUTHOR
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Olga Garmash
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Mikael Ehn
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Pasi Miettinen
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Paola Massoli
Aerodyne Research Inc., Billerica, MA 08121-3976, USA
Santtu Mikkonen
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Tuija Jokinen
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Pontus Roldin
Division of Nuclear Physics, Department of Physics, Lund University,
P.O. Box 118, 221 00, Lund, Sweden
Pasi Aalto
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Taina Yli-Juuti
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Jorma Joutsensaari
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Tuukka Petäjä
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Markku Kulmala
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Kari E. J. Lehtinen
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Finnish Meteorological Institute, Kuopio, Finland
Douglas R. Worsnop
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
Department of Physics, University of Helsinki, P.O. 64, Helsinki, Finland
Aerodyne Research Inc., Billerica, MA 08121-3976, USA
Annele Virtanen
CORRESPONDING AUTHOR
Department of Applied Physics, University of Eastern Finland, Kuopio,
Finland
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Cited
15 citations as recorded by crossref.
- The importance of sesquiterpene oxidation products for secondary organic aerosol formation in a springtime hemiboreal forest L. Barreira et al. 10.5194/acp-21-11781-2021
- Eight years of sub-micrometre organic aerosol composition data from the boreal forest characterized using a machine-learning approach L. Heikkinen et al. 10.5194/acp-21-10081-2021
- Measurement report: Increasing trend of atmospheric ion concentrations in the boreal forest J. Sulo et al. 10.5194/acp-22-15223-2022
- What caused severe air pollution episode of November 2016 in New Delhi? V. Kanawade et al. 10.1016/j.atmosenv.2019.117125
- Vertical transport of ultrafine particles and turbulence evolution impact on new particle formation at the surface & Canton Tower H. Wu et al. 10.1016/j.atmosres.2024.107290
- Statistical modelling of spatial and temporal variation in urban particle number size distribution at traffic and background sites L. Gerling et al. 10.1016/j.atmosenv.2020.117925
- Vertical Profiles of Particle Number Size Distribution and Variation Characteristics at the Eastern Slope of the Tibetan Plateau C. Shu et al. 10.3390/rs15225363
- Potential dual effect of anthropogenic emissions on the formation of biogenic secondary organic aerosol (BSOA) E. Kari et al. 10.5194/acp-19-15651-2019
- A phenomenology of new particle formation (NPF) at 13 European sites D. Bousiotis et al. 10.5194/acp-21-11905-2021
- Underestimated Contribution of Heavy Aromatics to Secondary Organic Aerosol Revealed by Comparative Assessments Using New and Traditional Methods L. Tian et al. 10.1021/acsearthspacechem.2c00252
- Regional characteristics of fine aerosol mass increase elucidated from long-term observations and KORUS-AQ campaign at a Northeast Asian background site S. Lim et al. 10.1525/elementa.2022.00020
- A novel lidar gradient cluster analysis method of nocturnal boundary layer detection during air pollution episodes Y. Zhang et al. 10.5194/amt-13-6675-2020
- Secondary Organic Aerosol Formation from Healthy and Aphid-Stressed Scots Pine Emissions C. Faiola et al. 10.1021/acsearthspacechem.9b00118
- The impact of the atmospheric turbulence-development tendency on new particle formation: a common finding on three continents H. Wu et al. 10.1093/nsr/nwaa157
- Characterization of the vertical evolution of urban nocturnal boundary layer by UAV measurements: Insights into relations to cloud radiative effect L. Shen et al. 10.1016/j.envres.2023.116323
15 citations as recorded by crossref.
- The importance of sesquiterpene oxidation products for secondary organic aerosol formation in a springtime hemiboreal forest L. Barreira et al. 10.5194/acp-21-11781-2021
- Eight years of sub-micrometre organic aerosol composition data from the boreal forest characterized using a machine-learning approach L. Heikkinen et al. 10.5194/acp-21-10081-2021
- Measurement report: Increasing trend of atmospheric ion concentrations in the boreal forest J. Sulo et al. 10.5194/acp-22-15223-2022
- What caused severe air pollution episode of November 2016 in New Delhi? V. Kanawade et al. 10.1016/j.atmosenv.2019.117125
- Vertical transport of ultrafine particles and turbulence evolution impact on new particle formation at the surface & Canton Tower H. Wu et al. 10.1016/j.atmosres.2024.107290
- Statistical modelling of spatial and temporal variation in urban particle number size distribution at traffic and background sites L. Gerling et al. 10.1016/j.atmosenv.2020.117925
- Vertical Profiles of Particle Number Size Distribution and Variation Characteristics at the Eastern Slope of the Tibetan Plateau C. Shu et al. 10.3390/rs15225363
- Potential dual effect of anthropogenic emissions on the formation of biogenic secondary organic aerosol (BSOA) E. Kari et al. 10.5194/acp-19-15651-2019
- A phenomenology of new particle formation (NPF) at 13 European sites D. Bousiotis et al. 10.5194/acp-21-11905-2021
- Underestimated Contribution of Heavy Aromatics to Secondary Organic Aerosol Revealed by Comparative Assessments Using New and Traditional Methods L. Tian et al. 10.1021/acsearthspacechem.2c00252
- Regional characteristics of fine aerosol mass increase elucidated from long-term observations and KORUS-AQ campaign at a Northeast Asian background site S. Lim et al. 10.1525/elementa.2022.00020
- A novel lidar gradient cluster analysis method of nocturnal boundary layer detection during air pollution episodes Y. Zhang et al. 10.5194/amt-13-6675-2020
- Secondary Organic Aerosol Formation from Healthy and Aphid-Stressed Scots Pine Emissions C. Faiola et al. 10.1021/acsearthspacechem.9b00118
- The impact of the atmospheric turbulence-development tendency on new particle formation: a common finding on three continents H. Wu et al. 10.1093/nsr/nwaa157
- Characterization of the vertical evolution of urban nocturnal boundary layer by UAV measurements: Insights into relations to cloud radiative effect L. Shen et al. 10.1016/j.envres.2023.116323
Discussed (final revised paper)
Latest update: 19 Apr 2024
Short summary
An aerosol mass spectrometer was used to characterize aerosol chemical composition during new particle formation periods. The time profiles of mass concentrations and chemical composition of observed aerosol particles are subjected to joint effects of boundary layer dilution, atmospheric chemistry and aerosol mixing in different boundary layers. During the nighttime, the increase in organic aerosol mass correlated well with the increase in condensed highly oxygenated organic molecules' mass.
An aerosol mass spectrometer was used to characterize aerosol chemical composition during new...
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