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Volume 18, issue 21 | Copyright

Special issue: Regional transport and transformation of air pollution in...

Atmos. Chem. Phys., 18, 15921-15935, 2018
https://doi.org/10.5194/acp-18-15921-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 07 Nov 2018

Research article | 07 Nov 2018

Relationships between the planetary boundary layer height and surface pollutants derived from lidar observations over China: regional pattern and influencing factors

Tianning Su1, Zhanqing Li1,2, and Ralph Kahn3 Tianning Su et al.
  • 1Department of Atmospheric and Oceanic Sciences & ESSIC, University of Maryland, College Park, MD 20740, USA
  • 2State Key Laboratory of Earth Surface Processes and Resource Ecology and College of Global Change and Earth System Science, Beijing Normal University, 100875, Beijing, China
  • 3Climate and Radiation Laboratory, Earth Science Division, NASA Goddard Space Flight Center, Greenbelt, MD, USA

Abstract. The frequent occurrence of severe air pollution episodes in China has been a great concern and thus the focus of intensive studies. Planetary boundary layer height (PBLH) is a key factor in the vertical mixing and dilution of near-surface pollutants. However, the relationship between PBLH and surface pollutants, especially particulate matter (PM) concentration across China, is not yet well understood. We investigate this issue at  ∼ 1600 surface stations using PBLH derived from space-borne and ground-based lidar, and discuss the influence of topography and meteorological variables on the PBLH–PM relationship. Albeit the PBLH–PM correlations are roughly negative for most cases, their magnitude, significance, and even sign vary considerably with location, season, and meteorological conditions. Weak or even uncorrelated PBLH–PM relationships are found over clean regions (e.g., Pearl River Delta), whereas nonlinearly negative responses of PM to PBLH evolution are found over polluted regions (e.g., North China Plain). Relatively strong PBLH–PM interactions are found when the PBLH is shallow and PM concentration is high, which typically corresponds to wintertime cases. Correlations are much weaker over the highlands than the plains regions, which may be associated with lighter pollution loading at higher elevations and contributions from mountain breezes. The influence of horizontal transport on surface PM is considered as well, manifested as a negative correlation between surface PM and wind speed over the whole nation. Strong wind with clean upwind air plays a dominant role in removing pollutants, and leads to obscure PBLH–PM relationships. A ventilation rate is used to jointly consider horizontal and vertical dispersion, which has the largest impact on surface pollutant accumulation over the North China Plain. As such, this study contributes to improved understanding of aerosol–planetary boundary layer (PBL) interactions and thus our ability to forecast surface air pollution.

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Surface particulate concentration has often been estimated from column-integrated aerosol optical depth (AOD). Their relationship is affected by various factors, such as the planetary layer height, meteorology (atmospheric stability, wind, relative humidity, etc.), and topography, which are investigated thoroughly using a combination of ~1500 surface station datasets, two ground-based lidars, and CALIPSO space-based lidar measurements made across China. Improved estimation of PM2.5 is achieved.
Surface particulate concentration has often been estimated from column-integrated aerosol...
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