Articles | Volume 18, issue 20
https://doi.org/10.5194/acp-18-15017-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-15017-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Oct 2018
Research article |
| 19 Oct 2018
| 19 Oct 2018
Adjoint inversion of Chinese non-methane volatile organic compound emissions using space-based observations of formaldehyde and glyoxal
Hansen Cao
Department of Atmospheric and Oceanic Sciences and Laboratory for
Climate and Ocean-Atmosphere Studies, School of Physics, Peking University,
Beijing, 100871, China
Tzung-May Fu
CORRESPONDING AUTHOR
Department of Atmospheric and Oceanic Sciences and Laboratory for
Climate and Ocean-Atmosphere Studies, School of Physics, Peking University,
Beijing, 100871, China
Lin Zhang
Department of Atmospheric and Oceanic Sciences and Laboratory for
Climate and Ocean-Atmosphere Studies, School of Physics, Peking University,
Beijing, 100871, China
Daven K. Henze
Department of Mechanical Engineering, University of Colorado, Boulder,
USA
Christopher Chan Miller
Atomic and Molecular Physics Division, Harvard-Smithsonian Center for
Astrophysics, Cambridge, Massachusetts, USA
Christophe Lerot
Belgian Institute for Space Aeronomy, Brussels, Belgium
Gonzalo González Abad
Atomic and Molecular Physics Division, Harvard-Smithsonian Center for
Astrophysics, Cambridge, Massachusetts, USA
Isabelle De Smedt
Belgian Institute for Space Aeronomy, Brussels, Belgium
Qiang Zhang
Center for Earth System Science, Tsinghua University, Beijing, China
Michel van Roozendael
Belgian Institute for Space Aeronomy, Brussels, Belgium
François Hendrick
Belgian Institute for Space Aeronomy, Brussels, Belgium
Kelly Chance
Atomic and Molecular Physics Division, Harvard-Smithsonian Center for
Astrophysics, Cambridge, Massachusetts, USA
Jie Li
Institute of Atmospheric Physics, Chinese Academy of Sciences,
Beijing, China
Junyu Zheng
College of Environmental Science and Engineering, South China
University of Technology, Guangzhou, China
Yuanhong Zhao
Department of Atmospheric and Oceanic Sciences and Laboratory for
Climate and Ocean-Atmosphere Studies, School of Physics, Peking University,
Beijing, 100871, China
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Latest update: 19 Apr 2024
Short summary
Our top-down estimates for annual total Chinese NMVOC emissions was 30.7 to 49.5 Tg y−1, including 16.4 to 23.6 Tg y−1 from anthropogenic sources, 12.2 to 22.8 Tg y−1 from biogenic sources, and 2.08 to 3.13 Tg y−1 from biomass burning. Our four inversions consistently showed that the emissions of Chinese anthropogenic NMVOC precursors of glyoxal were larger than the a priori estimates. The glyoxal and formaldehyde constraints helped distinguish the NMVOC species from different sources.
Our top-down estimates for annual total Chinese NMVOC emissions was 30.7 to 49.5 Tg y−1,...
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