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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 18, issue 2 | Copyright
Atmos. Chem. Phys., 18, 1185-1202, 2018
https://doi.org/10.5194/acp-18-1185-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 30 Jan 2018

Research article | 30 Jan 2018

Ozone trends over the United States at different times of day

Yingying Yan1, Jintai Lin1, and Cenlin He2 Yingying Yan et al.
  • 1Laboratory for Climate and Ocean-Atmosphere Studies, Department of Atmospheric and Oceanic Sciences, School of Physics, Peking University, Beijing 100871, China
  • 2Joint Institute for Regional Earth System Science and Engineering, Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, Los Angeles, California, USA

Abstract. In the United States, the decline of summertime daytime peak ozone in the last 20 years has been clearly connected to reductions in anthropogenic emissions. However, questions remain about how and through what mechanisms ozone at other times of day have changed over recent decades. Here we analyze the interannual variability and trends of ozone at different hours of day, using observations from about 1000 US sites during 1990–2014. We find a clear diurnal cycle both in the magnitude of ozone trends and in the relative importance of climate variability versus anthropogenic emissions to ozone changes. Interannual climate variability has mainly been associated with the detrended fluctuation in the US annual daytime ozone over 1990–2014, with a much smaller effect on the nighttime ozone. Reductions in anthropogenic emissions of nitrogen oxides have led to substantial growth in the US annual average nighttime ozone due to reduced ozone titration, while the summertime daytime ozone has declined. Environmental policymaking might consider further improvements to reduce ozone levels at night and other non-peak hours.

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Examining observed and simulated ozone at about 1000 sites during 1990–2014, we find a clear diurnal cycle both in the magnitude of ozone trends and in the relative importance of climate variability versus anthropogenic emissions to ozone changes, which has policy implications to mitigate ozone at night and other non-peak hours.
Examining observed and simulated ozone at about 1000 sites during 1990–2014, we find a clear...
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