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Volume 17, issue 15 | Copyright

Special issue: CHemistry and AeRosols Mediterranean EXperiments (ChArMEx)...

Atmos. Chem. Phys., 17, 9567-9583, 2017
https://doi.org/10.5194/acp-17-9567-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 09 Aug 2017

Research article | 09 Aug 2017

Spatial extent of new particle formation events over the Mediterranean Basin from multiple ground-based and airborne measurements

Kevin Berland1, Clémence Rose1, Jorge Pey2, Anais Culot1, Evelyn Freney1, Nikolaos Kalivitis3, Giorgios Kouvarakis3, José Carlos Cerro4, Marc Mallet7, Karine Sartelet5, Matthias Beckmann6, Thierry Bourriane7, Greg Roberts7, Nicolas Marchand2, Nikolaos Mihalopoulos3,8, and Karine Sellegri1 Kevin Berland et al.
  • 1Laboratoire de Météorologie Physique, CNRS UMR 6016, Université Blaise Pascal, Aubière, France
  • 2Aix-Marseille Université, CNRS, LCE, UMR 7376, 13331, Marseille, France
  • 3Environmental Chemical Processes Laboratory, University of Crete, Heraklion, Crete, 71003, Greece
  • 4Laboratory of Environmental Analytical Chemistry, Illes Balears University, Palma, 07122, Spain
  • 5CEREA, joint laboratory Ecole des Ponts ParisTech – EDF R&D, Université Paris-Est, 77455 Champs sur Marne, France
  • 6Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR-CNRS 7583, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
  • 7Centre National de Recherches Météorologiques, Météo-France, Toulouse, URA1357, France
  • 8IERSD, National Observatory of Athens, P. Penteli, 15236, Athens, Greece

Abstract. Over the last two decades, new particle formation (NPF), i.e., the formation of new particle clusters from gas-phase compounds followed by their growth to the 10–50nm size range, has been extensively observed in the atmosphere at a given location, but their spatial extent has rarely been assessed. In this work, we use aerosol size distribution measurements performed simultaneously at Ersa (Corsica) and Finokalia (Crete) over a 1-year period to analyze the occurrence of NPF events in the Mediterranean area. The geographical location of these two sites, as well as the extended sampling period, allows us to assess the spatial and temporal variability in atmospheric nucleation at a regional scale. Finokalia and Ersa show similar seasonalities in the monthly average nucleation frequencies, growth rates, and nucleation rates, although the two stations are located more than 1000km away from each other. Within this extended period, aerosol size distribution measurements were performed during an intensive campaign (3 July to 12 August 2013) from a ground-based station on the island of Mallorca, as well as onboard the ATR-42 research aircraft. This unique combination of stationary and mobile measurements provides us with detailed insights into the horizontal and vertical development of the NPF process on a daily scale. During the intensive campaign, nucleation events occurred simultaneously both at Ersa and Mallorca over delimited time slots of several days, but different features were observed at Finokalia. The results show that the spatial extent of the NPF events over the Mediterranean Sea might be as large as several hundreds of kilometers, mainly determined by synoptic conditions. Airborne measurements gave additional information regarding the origin of the clusters detected above the sea. The selected cases depicted contrasting situations, with clusters formed in the marine boundary layer or initially nucleated above the continent or in the free troposphere (FT) and further transported above the sea.

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New particle formation (NPF) from gas-phase precursors is a process that is expected to drive the total number concentration of particles in the atmosphere. Here we use measurements performed simultaneously in Corsica, Crete and Mallorca to show that the spatial extent of the NPF events are several hundreds of kilometers large. Airborne measurements additionally show that nanoparticles in the marine atmosphere can either be of marine origin or from higher altitudes above the continent.
New particle formation (NPF) from gas-phase precursors is a process that is expected to drive...
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