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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 17, issue 14 | Copyright
Atmos. Chem. Phys., 17, 9145-9162, 2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 31 Jul 2017

Research article | 31 Jul 2017

Cloud albedo changes in response to anthropogenic sulfate and non-sulfate aerosol forcings in CMIP5 models

Lena Frey, Frida A.-M. Bender, and Gunilla Svensson Lena Frey et al.
  • Department of Meteorology and Bolin Centre for Climate Research, Stockholm University, Stockholm, Sweden

Abstract. The effects of different aerosol types on cloud albedo are analysed using the linear relation between total albedo and cloud fraction found on a monthly mean scale in regions of subtropical marine stratocumulus clouds and the influence of simulated aerosol variations on this relation. Model experiments from the Coupled Model Intercomparison Project phase 5 (CMIP5) are used to separately study the responses to increases in sulfate, non-sulfate and all anthropogenic aerosols. A cloud brightening on the month-to-month scale due to variability in the background aerosol is found to dominate even in the cases where anthropogenic aerosols are added. The aerosol composition is of importance for this cloud brightening, that is thereby region dependent. There is indication that absorbing aerosols to some extent counteract the cloud brightening but scene darkening with increasing aerosol burden is generally not supported, even in regions where absorbing aerosols dominate. Month-to-month cloud albedo variability also confirms the importance of liquid water content for cloud albedo. Regional, monthly mean cloud albedo is found to increase with the addition of anthropogenic aerosols and more so with sulfate than non-sulfate. Changes in cloud albedo between experiments are related to changes in cloud water content as well as droplet size distribution changes, so that models with large increases in liquid water path and/or cloud droplet number show large cloud albedo increases with increasing aerosol. However, no clear relation between model sensitivities to aerosol variations on the month-to-month scale and changes in cloud albedo due to changed aerosol burden is found.

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In this study, the cloud albedo effect in climate models is investigated, separating the influence of anthropogenic sulfate and non-sulfate aerosols. Cloud albedo changes induced by added anthropogenic aerosols are found to be determined by changes in the cloud water content rather than model sensitivity to monthly aerosol variations. The results also indicate that the background aerosol is the main driver for a cloud brightening effect on the month-to-month scale.
In this study, the cloud albedo effect in climate models is investigated, separating the...