Estimating the atmospheric concentration of Criegee intermediates and their possible interference in a FAGE-LIF instrument

Novelli, Anna; Hens, Korbinian; Tatum Ernest, Cheryl; Martinez, Monica; Nölscher, Anke C.; Sinha, Vinayak; Paasonen, Pauli; Petäjä, Tuukka; Sipilä, Mikko; Elste, Thomas; Plass-Dülmer, Christian; Phillips, Gavin J.; Kubistin, Dagmar; Williams, Jonathan; Vereecken, Luc; Lelieveld, Jos; Harder, Hartwig

doi:https://doi.org/10.5194/acp-17-7807-2017

Articles | Volume 17, issue 12

https://doi.org/10.5194/acp-17-7807-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

https://doi.org/10.5194/acp-17-7807-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 17, issue 12

Research article

|

29 Jun 2017

Research article |

| 29 Jun 2017

Estimating the atmospheric concentration of Criegee intermediates and their possible interference in a FAGE-LIF instrument

Anna Novelli, Korbinian Hens, Cheryl Tatum Ernest, Monica Martinez, Anke C. Nölscher, Vinayak Sinha, Pauli Paasonen, Tuukka Petäjä, Mikko Sipilä, Thomas Elste, Christian Plass-Dülmer, Gavin J. Phillips, Dagmar Kubistin, Jonathan Williams, Luc Vereecken, Jos Lelieveld, and Hartwig Harder

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Final revised paper (published on 29 Jun 2017)
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Preprint (discussion started on 24 Oct 2016)
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Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC1: 'Review of "Identification of Criegee Intermediates as Potential Oxidants in the Troposphere" by Novelli et al', Anonymous Referee #1, 01 Dec 2016
RC2: 'Review of Novelli et al.', Anonymous Referee #2, 14 Dec 2016
AC1: 'Authors responses to the referees', Anna Novelli, 07 Mar 2017

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Anna Novelli on behalf of the Authors (12 Mar 2017) Author's response Manuscript

ED: Reconsider after minor revisions (Editor review) (22 Apr 2017) by Kyung-Eun Min

AR by Anna Novelli on behalf of the Authors (02 May 2017) Author's response Manuscript

ED: Publish as is (19 May 2017) by Kyung-Eun Min

AR by Anna Novelli on behalf of the Authors (26 May 2017)

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Short summary

The ambient concentration of stabilised Criegee intermediates (SCIs) was estimated for two environments using field data. The low concentrations predicted indicate that SCIs are unlikely to have a large impact on atmospheric chemistry. Concurrent measurements of an OH background signal using the Mainz IPI-LIF-FAGE instrument were found to be consistent with the chemistry of SCIs during the measurement campaigns.