Articles | Volume 17, issue 12
https://doi.org/10.5194/acp-17-7459-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-7459-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Effects of the Wegener–Bergeron–Findeisen process on global black carbon distribution
Ling Qi
CORRESPONDING AUTHOR
Department of Atmospheric and Oceanic Sciences, University of
California, Los Angeles, CA, USA
Joint Institute for Regional Earth System Science and Engineering,
University of California, Los Angeles, CA, USA
Qinbin Li
Department of Atmospheric and Oceanic Sciences, University of
California, Los Angeles, CA, USA
Joint Institute for Regional Earth System Science and Engineering,
University of California, Los Angeles, CA, USA
Cenlin He
Department of Atmospheric and Oceanic Sciences, University of
California, Los Angeles, CA, USA
Joint Institute for Regional Earth System Science and Engineering,
University of California, Los Angeles, CA, USA
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou,
China
Jianping Huang
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou,
China
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Yue Zhou, Christopher P. West, Anusha P. S. Hettiyadura, Xiaoying Niu, Hui Wen, Jiecan Cui, Tenglong Shi, Wei Pu, Xin Wang, and Alexander Laskin
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Wei Pu, Tenglong Shi, Jiecan Cui, Yang Chen, Yue Zhou, and Xin Wang
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Tenglong Shi, Jiecan Cui, Yang Chen, Yue Zhou, Wei Pu, Xuanye Xu, Quanliang Chen, Xuelei Zhang, and Xin Wang
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Xiaoyu Hu, Jinming Ge, Jiajing Du, Qinghao Li, Jianping Huang, and Qiang Fu
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Jiecan Cui, Tenglong Shi, Yue Zhou, Dongyou Wu, Xin Wang, and Wei Pu
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Julián Gelman Constantin, Lucas Ruiz, Gustavo Villarosa, Valeria Outes, Facundo N. Bajano, Cenlin He, Hector Bajano, and Laura Dawidowski
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Wenfu Tang, Benjamin Gaubert, Louisa Emmons, Yonghoon Choi, Joshua P. DiGangi, Glenn S. Diskin, Xiaomei Xu, Cenlin He, Helen Worden, Simone Tilmes, Rebecca Buchholz, Hannah S. Halliday, and Avelino F. Arellano
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-864, https://doi.org/10.5194/acp-2020-864, 2020
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Zhiyuan Hu, Jianping Huang, Chun Zhao, Qinjian Jin, Yuanyuan Ma, and Ben Yang
Atmos. Chem. Phys., 20, 1507–1529, https://doi.org/10.5194/acp-20-1507-2020, https://doi.org/10.5194/acp-20-1507-2020, 2020
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Xin Wang, Xueying Zhang, and Wenjing Di
Atmos. Meas. Tech., 13, 39–52, https://doi.org/10.5194/amt-13-39-2020, https://doi.org/10.5194/amt-13-39-2020, 2020
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We developed an improved two-sphere integration (TSI) technique to quantify black carbon (BC) concentrations in the atmosphere and seasonal snow. The major advantage of this system is that it combines two distinct integrated spheres to reduce the scattering effect due to light-absorbing particles and thus provides accurate determinations of total light absorption from BC collected on Nuclepore filters.
Siqi Ma, Xuelei Zhang, Chao Gao, Daniel Q. Tong, Aijun Xiu, Guangjian Wu, Xinyuan Cao, Ling Huang, Hongmei Zhao, Shichun Zhang, Sergio Ibarra-Espinosa, Xin Wang, Xiaolan Li, and Mo Dan
Geosci. Model Dev., 12, 4603–4625, https://doi.org/10.5194/gmd-12-4603-2019, https://doi.org/10.5194/gmd-12-4603-2019, 2019
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Dust storms are thought to be a worldwide societal issue, and numerical modeling is an effective way to help us to predict dust events. Here we present the first comprehensive evaluation of dust emission modules in four commonly used air quality models for northeastern China. The results showed that most of these models were able to capture this dust event and indicated the dust source maps should be carefully selected or replaced with a new one that is constructed with local data.
Zhiyuan Hu, Jianping Huang, Chun Zhao, Yuanyuan Ma, Qinjian Jin, Yun Qian, L. Ruby Leung, Jianrong Bi, and Jianmin Ma
Atmos. Chem. Phys., 19, 12709–12730, https://doi.org/10.5194/acp-19-12709-2019, https://doi.org/10.5194/acp-19-12709-2019, 2019
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This study investigates aerosol chemical compositions and relative contributions to total aerosols in the western US. The results show that trans-Pacific aerosols have a maximum concentration in the boreal spring, with the greatest contribution from dust. Over western North America, the trans-Pacific aerosols dominate the column-integrated aerosol mass and number concentration. However, near the surface, aerosols mainly originated from local emissions.
Ling Qi and Shuxiao Wang
Atmos. Chem. Phys., 19, 11545–11557, https://doi.org/10.5194/acp-19-11545-2019, https://doi.org/10.5194/acp-19-11545-2019, 2019
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Black carbon (BC) contributes two-thirds of the climate impact of carbon dioxide, pushing methane into third place of the human contributors to global warming. This study shows that contributions from biomass burning (producing marginal lensing effect) have a strong spatial variation, from 20 % in Europe to 60 % in Africa. Thus, the inclusion of strong lensing-related absorption enhancement to all BC particles in previous estimates may lead to overestimating their positive radiative forcing.
Wei Pu, Jiecan Cui, Tenglong Shi, Xuelei Zhang, Cenlin He, and Xin Wang
Atmos. Chem. Phys., 19, 9949–9968, https://doi.org/10.5194/acp-19-9949-2019, https://doi.org/10.5194/acp-19-9949-2019, 2019
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LAPs (light-absorbing particles) deposited on snow can decrease snow albedo and increase the absorption of solar radiation. Radiative forcing by LAPs will affect the regional hydrological cycle and climate. We use MODIS observations to retrieve the radiative forcing by LAPs in snow across northeastern China (NEC). The results of radiative forcing present distinct spatial variability. We find that the biases are negatively correlated with LAP concentrations and range from
~ 5 % to ~ 350 %.
Xiaoyue Liu, Jianping Huang, Jiping Huang, Changyu Li, and Lei Ding
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Revised manuscript not accepted
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A large survey on measuring optical and chemical properties of insoluble light-absorbing impurities (ILAPs) from seven glaciers was conducted on the Tibetan Plateau (TP) during 2013–2015. The results indicated that the mixing ratios of black carbon (BC), organic carbon (OC), and iron (Fe) all showed a tendency to decrease from north to south, and the industrial pollution (33.1 %), biomass and biofuel burning (29.4 %), and soil dust (37.5 %) were the major sources of the ILAPs on the TP.
Yue Zhou, Hui Wen, Jun Liu, Wei Pu, Qingcai Chen, and Xin Wang
The Cryosphere, 13, 157–175, https://doi.org/10.5194/tc-13-157-2019, https://doi.org/10.5194/tc-13-157-2019, 2019
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We first investigated the optical characteristics and potential sources of chromophoric dissolved organic matter (CDOM) in seasonal snow over northwestern China. The abundance of CDOM showed regional variation. At some sites strongly influenced by local soil, the absorption of CDOM cannot be neglected compared to black carbon. We found two humic-like and one protein-like fluorophores in snow. The major sources of snow CDOM were soil, biomass burning, and anthropogenic pollution.
Zhiyuan Cong, Shaopeng Gao, Wancang Zhao, Xin Wang, Guangming Wu, Yulan Zhang, Shichang Kang, Yongqin Liu, and Junfeng Ji
The Cryosphere, 12, 3177–3186, https://doi.org/10.5194/tc-12-3177-2018, https://doi.org/10.5194/tc-12-3177-2018, 2018
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Cryoconites from glaciers on the Tibetan Plateau and surrounding area were studied for iron oxides. We found that goethite is the predominant iron oxide form. Using the abundance, speciation and optical properties of iron oxides, the total light absorption was quantitatively attributed to goethite, hematite, black carbon and organic matter. Such findings are essential to understand the relative significance of anthropogenic and natural impacts.
Cenlin He, Mark G. Flanner, Fei Chen, Michael Barlage, Kuo-Nan Liou, Shichang Kang, Jing Ming, and Yun Qian
Atmos. Chem. Phys., 18, 11507–11527, https://doi.org/10.5194/acp-18-11507-2018, https://doi.org/10.5194/acp-18-11507-2018, 2018
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Snow albedo plays a key role in the Earth and climate system. It can be affected by impurities and snow properties. This study implements new parameterizations into a widely used snow model to account for effects of snow shape and black carbon–snow mixing state on snow albedo reduction in the Tibetan Plateau. This study points toward an imperative need for extensive measurements and improved model characterization of snow grain shape and aerosol–snow mixing state in Tibet and elsewhere.
Kai Tang, Zhongwei Huang, Jianping Huang, Teruya Maki, Shuang Zhang, Atsushi Shimizu, Xiaojun Ma, Jinsen Shi, Jianrong Bi, Tian Zhou, Guoyin Wang, and Lei Zhang
Atmos. Chem. Phys., 18, 7131–7148, https://doi.org/10.5194/acp-18-7131-2018, https://doi.org/10.5194/acp-18-7131-2018, 2018
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To our knowledge, this is the first simultaneous field measurement of bioaerosols in dust events at four sites along the transport pathway of Asian dust. The samples were analyzed by means of fluorescence microscopy, scanning electron microscopy, and MiSeq sequencing analysis. The results indicate that dust clouds can carry many bacteria of various types into downwind regions, the alpha and beta diversity of which were investigated.
Xin Wang, Hui Wen, Jinsen Shi, Jianrong Bi, Zhongwei Huang, Beidou Zhang, Tian Zhou, Kaiqi Fu, Quanliang Chen, and Jinyuan Xin
Atmos. Chem. Phys., 18, 2119–2138, https://doi.org/10.5194/acp-18-2119-2018, https://doi.org/10.5194/acp-18-2119-2018, 2018
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A ground-based mobile laboratory was deployed near the dust source regions over northwestern China.
We not only captured natural dust but also characterized the properties of anthropogenic soil dust produced by agricultural cultivations.
The results indicate that large differences were found between the optical and microphysical properties of anthropogenic and natural dust.
Yingying Yan, Jintai Lin, and Cenlin He
Atmos. Chem. Phys., 18, 1185–1202, https://doi.org/10.5194/acp-18-1185-2018, https://doi.org/10.5194/acp-18-1185-2018, 2018
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Examining observed and simulated ozone at about 1000 sites during 1990–2014, we find a clear diurnal cycle both in the magnitude of ozone trends and in the relative importance of climate variability versus anthropogenic emissions to ozone changes, which has policy implications to mitigate ozone at night and other non-peak hours.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Jonathan H. Jiang, Qinbin Li, Rong Fu, Lei Huang, Xiaohong Liu, Xiangjun Shi, Hui Su, and Cenlin He
Atmos. Chem. Phys., 18, 1065–1078, https://doi.org/10.5194/acp-18-1065-2018, https://doi.org/10.5194/acp-18-1065-2018, 2018
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The interactions between aerosols and ice clouds represent one of the largest uncertainties among anthropogenic forcings on climate change. We find that the responses of ice crystal effective radius, a key parameter determining ice clouds' net radiative effect, to aerosol loadings are modulated by water vapor amount and vary from a significant negative correlation in moist conditions (consistent with the “Twomey effect” for liquid clouds) to a strong positive correlation in dry conditions.
Zhijuan Zhang, Bin Chen, Jianping Huang, Jingjing Liu, Jianrong Bi, Tian Zhou, and Zhongwei Huang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-1000, https://doi.org/10.5194/acp-2017-1000, 2017
Revised manuscript not accepted
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Environmental problems caused by aerosols such as dust aerosols are influencing people's lives and work. Due to different radiative effects of different types of aerosols, detection of the aerosol type is vital for improving our air quality. In this study, the optical properties of pure dust and transported anthropogenic dust are compared by using ground-based Lidar data. Based on our conclusion, detection of different dust aerosols will be more accurate using satellite-based Lidar.
Siyu Chen, Jianping Huang, Nanxuan Jiang, Zhou Zang, Xiaodan Guan, Xiaojun Ma, Zhuo Jia, Xiaorui Zhang, Yanting Zhang, Kangning Huang, Xiaocong Xu, Guolong Zhang, Jiming Li, Ran Yang, and Shujie Liao
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-890, https://doi.org/10.5194/acp-2017-890, 2017
Revised manuscript not accepted
Ling Qi, Qinbin Li, Daven K. Henze, Hsien-Liang Tseng, and Cenlin He
Atmos. Chem. Phys., 17, 9697–9716, https://doi.org/10.5194/acp-17-9697-2017, https://doi.org/10.5194/acp-17-9697-2017, 2017
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We find that Asian anthropogenic sources are the largest contributors (~ 40 %) to surface BC in spring in the Arctic, inconsistent with previous studies which repeatedly identified sources of surface BC as anthropogenic emissions from Europe and Russia. It takes 12–17 days for Asian anthropogenic emissions to be transported to the Arctic surface. Additionally, a large fraction (40–65 %) of Asian contribution is in the form of chronic pollution on 1- to 2-month timescales.
Jinming Ge, Zeen Zhu, Chuang Zheng, Hailing Xie, Tian Zhou, Jianping Huang, and Qiang Fu
Atmos. Chem. Phys., 17, 9035–9047, https://doi.org/10.5194/acp-17-9035-2017, https://doi.org/10.5194/acp-17-9035-2017, 2017
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A modified method with a new noise reduction scheme that can reduce the noise distribution to a narrow range is proposed to distinguish clouds and other hydrometeors from noise and recognize more features with weak signal in cloud radar observations. It was found that our method has significant advantages in reducing the rates of both failed negative and false positive hydrometeor identifications in simulated clouds and recognizing clouds with weak signal from our cloud radar observations.
Jianrong Bi, Jianping Huang, Jinsen Shi, Zhiyuan Hu, Tian Zhou, Guolong Zhang, Zhongwei Huang, Xin Wang, and Hongchun Jin
Atmos. Chem. Phys., 17, 7775–7792, https://doi.org/10.5194/acp-17-7775-2017, https://doi.org/10.5194/acp-17-7775-2017, 2017
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We conducted a field campaign on exploring dust aerosol in Dunhuang farmland nearby Gobi deserts. The anthropogenic dust produced by agricultural cultivations exerted a significant superimposed effect on elevated dust loadings. Strong south wind in daytime scavenged the pollution and weak northeast wind at night favorably accumulated air pollutants near the surface. The local emissions remarkably modified the absorptive and optical characteristics of mineral dust in desert source region.
Wei Pu, Xin Wang, Hailun Wei, Yue Zhou, Jinsen Shi, Zhiyuan Hu, Hongchun Jin, and Quanliang Chen
The Cryosphere, 11, 1213–1233, https://doi.org/10.5194/tc-11-1213-2017, https://doi.org/10.5194/tc-11-1213-2017, 2017
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We conducted a large field campaign to collect snow samples in Xinjiang. We measured insoluble light-absorbing particles with estimated black carbon concentrations of 10–150 ngg-1. We found a probable shift in emission sources with the progression of winter and dominated contributions of BC and OC to light absorption. A PMF model indicated an optimal three-factor/source solution that included industrial pollution, biomass burning, and soil dust.
Siyu Chen, Jianping Huang, Litai Kang, Hao Wang, Xiaojun Ma, Yongli He, Tiangang Yuan, Ben Yang, Zhongwei Huang, and Guolong Zhang
Atmos. Chem. Phys., 17, 2401–2421, https://doi.org/10.5194/acp-17-2401-2017, https://doi.org/10.5194/acp-17-2401-2017, 2017
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Compared with the TD dust, the importance of the GD dust in eastern China, Japan, and Korea is always neglected. We focused primarily on the dynamic and thermodynamics mechanisms of dust emission and transport over TD and GD and further elucidate the influence of TD and GD dust on the entire East Asia based on a case study using WRF-Chem model in the study.
Xin Wang, Wei Pu, Yong Ren, Xuelei Zhang, Xueying Zhang, Jinsen Shi, Hongchun Jin, Mingkai Dai, and Quanliang Chen
Atmos. Chem. Phys., 17, 2279–2296, https://doi.org/10.5194/acp-17-2279-2017, https://doi.org/10.5194/acp-17-2279-2017, 2017
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A 2014 snow survey was performed across northeastern China to analyze light absorption of ILAPs in seasonal snow, and modeling studies were conducted to compare snow albedo reduction due to assumptions of internal–external mixing of BC in snow and different snow grain shapes. The results show that the simulated snow albedos from both SAMDS and SNICAR agree well with the observed values at low ILAP mixing ratios, but they tend to be higher than surface observations at high ILAP mixing ratios.
Ling Qi, Qinbin Li, Yinrui Li, and Cenlin He
Atmos. Chem. Phys., 17, 1037–1059, https://doi.org/10.5194/acp-17-1037-2017, https://doi.org/10.5194/acp-17-1037-2017, 2017
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The Arctic is the most vulnerable region for climate change. Black carbon (BC) in air and deposited on snow and ice warms the Arctic substantially, but simulations of BC climate effects are associated with large uncertainties. To reduce this uncertainty, it is imperative to improve the simulation of BC distribution in the Arctic. We evaluate the effects of controlling factors (emissions, dry and wet deposition) on BC distribution and call for more observations to constrain these processes.
Jianrong Bi, Jianping Huang, Brent Holben, and Guolong Zhang
Atmos. Chem. Phys., 16, 15501–15516, https://doi.org/10.5194/acp-16-15501-2016, https://doi.org/10.5194/acp-16-15501-2016, 2016
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Dating absorptive capacity of Asian dust is still an outstanding issue. In this study, we identify two types of Asian dust: Pure Dust (PDU) and Transported Anthropogenic Dust (TDU). Overall average SSA, ASY, Re, and Ri at 550 nm for PDU are 0.935, 0.742, 1.526, and 0.00226, respectively, with 0.921, 0.723, 1.521, and 0.00364 for TDU. Our results promise to update and improve accuracy of Asian dust characteristics in present-day remote sensing applications and regional climate models.
Xuelei Zhang, Daniel Q. Tong, Guangjian Wu, Xin Wang, Aijun Xiu, Yongxiang Han, Tianli Xu, Shichun Zhang, and Hongmei Zhao
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-681, https://doi.org/10.5194/acp-2016-681, 2016
Revised manuscript has not been submitted
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More detailed knowledge regarding recent variations in the characteristics of East Asian dust events and dust sources can effectively improve regional dust modeling and forecasts. Here we reassess the accuracy of previous predictions of trends in dust variations in East Asia, and establish a relatively detailed inventory of dust events based on satellite observations from 2000 to 2015.
Jin Ming Ge, Huayue Liu, Jianping Huang, and Qiang Fu
Atmos. Chem. Phys., 16, 7773–7783, https://doi.org/10.5194/acp-16-7773-2016, https://doi.org/10.5194/acp-16-7773-2016, 2016
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Nocturnal low-level jet (NLLJ), which refers to a narrow zone of strong winds, occurs frequently over the Taklimakan Desert. It is found that the NLLJ contains more momentum than without NLLJ, and the downward momentum transfer process is more intense and rapid in the warm season. The coincidence of the larger surface winds during NLLJ days with an enhancement of aerosol optical depth indicates that the NLLJ is an important mechanism for dust emission and transport over this region.
Xuezhe Xu, Weixiong Zhao, Qilei Zhang, Shuo Wang, Bo Fang, Weidong Chen, Dean S. Venables, Xinfeng Wang, Wei Pu, Xin Wang, Xiaoming Gao, and Weijun Zhang
Atmos. Chem. Phys., 16, 6421–6439, https://doi.org/10.5194/acp-16-6421-2016, https://doi.org/10.5194/acp-16-6421-2016, 2016
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We report on the field measurement of the optical properties and chemical composition of PM1.0 particles in a suburban environment in Beijing during the winter coal heating season. Organic mass was the largest contributor to the total extinction of PM1.0, while EC, owing to its high absorption efficiency, contributed appreciably to PM1.0 extinction and should be a key target to air quality controls. Non-BC absorption from secondary organic aerosol also contributes to particle absorption.
Bin Zhao, Kuo-Nan Liou, Yu Gu, Cenlin He, Wee-Liang Lee, Xing Chang, Qinbin Li, Shuxiao Wang, Hsien-Liang R. Tseng, Lai-Yung R. Leung, and Jiming Hao
Atmos. Chem. Phys., 16, 5841–5852, https://doi.org/10.5194/acp-16-5841-2016, https://doi.org/10.5194/acp-16-5841-2016, 2016
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We examine the impact of buildings on surface solar fluxes in Beijing by accounting for their 3-D structures. We find that inclusion of buildings changes surface solar fluxes by within ±1 W m−2, ±1–10 W m−2, and up to ±100 W m−2 at grid resolutions of 4 km, 800 m, and 90 m, respectively. We can resolve pairs of positive-negative flux deviations on different sides of buildings at ≤ 800 m resolutions. We should treat building-effect on solar fluxes differently in models with different resolutions.
Zhiyuan Hu, Chun Zhao, Jianping Huang, L. Ruby Leung, Yun Qian, Hongbin Yu, Lei Huang, and Olga V. Kalashnikova
Geosci. Model Dev., 9, 1725–1746, https://doi.org/10.5194/gmd-9-1725-2016, https://doi.org/10.5194/gmd-9-1725-2016, 2016
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This study conducts the simulation of WRF-Chem with the quasi-global configuration for 2010–2014, and evaluates the simulation with multiple observation datasets for the first time. This study demonstrates that the WRF-Chem quasi-global simulation can be used for investigating trans-Pacific transport of aerosols and providing reasonable inflow chemical boundaries for the western USA to further understand the impact of transported pollutants on the regional air quality and climate.
Xiaodan Guan, Jianping Huang, Yanting Zhang, Yongkun Xie, and Jingjing Liu
Atmos. Chem. Phys., 16, 5159–5169, https://doi.org/10.5194/acp-16-5159-2016, https://doi.org/10.5194/acp-16-5159-2016, 2016
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An obvious peak in the total anthropogenic dust column, with much higher magnitude than those of wet regions, was observed in semi-arid regions. The anthropogenic dust column burden of semi-arid takes a positively correlated with the population and population change, indicating the production of anthropogenic dust in semi-arid regions is partly induced by human activities.
Cenlin He, Qinbin Li, Kuo-Nan Liou, Ling Qi, Shu Tao, and Joshua P. Schwarz
Atmos. Chem. Phys., 16, 3077–3098, https://doi.org/10.5194/acp-16-3077-2016, https://doi.org/10.5194/acp-16-3077-2016, 2016
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Blarck carbon aging significantly affects its global distribution and thus climatic effects. This study develops a microphysics-based BC aging scheme in a global model, which substantially improves model simulations of BC over the remote Pacific. The microphysical scheme shows fast aging over source regions and much slower aging in remote regions. The microphysical aging significantly reduces global BC burden and lifetime, showing important implications for the estimate of BC radiative effects.
X. Guan, J. Huang, R. Guo, H. Yu, P. Lin, and Y. Zhang
Atmos. Chem. Phys., 15, 13777–13786, https://doi.org/10.5194/acp-15-13777-2015, https://doi.org/10.5194/acp-15-13777-2015, 2015
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Dynamical adjustment methodology has been applied to the raw surface air temperature and has successfully identified and separated the contribution of dynamically induced temperature (DIT) and radiatively forced temperature (RFT). It found that regional anthropogenic radiative forcing caused the enhanced warming in the semi-arid region, which may be closely associated with local human activities.
Y. Liu, Y. Sato, R. Jia, Y. Xie, J. Huang, and T. Nakajima
Atmos. Chem. Phys., 15, 12581–12594, https://doi.org/10.5194/acp-15-12581-2015, https://doi.org/10.5194/acp-15-12581-2015, 2015
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We firstly evaluated the Spectral Radiation-Transport Model for Aerosol Species combined with a non-hydrostatic regional model through comparing the simulation results and satellite observations, both in horizontal and vertical. The dust and anthropogenic aerosols in summer over the Tibetan Plateau are evaluated, and their distributions over the TP are presented. The transport of these aerosols over the Tibetan Plateau is also explored via combining the simulation results and reanalysis data.
C. He, K.-N. Liou, Y. Takano, R. Zhang, M. Levy Zamora, P. Yang, Q. Li, and L. R. Leung
Atmos. Chem. Phys., 15, 11967–11980, https://doi.org/10.5194/acp-15-11967-2015, https://doi.org/10.5194/acp-15-11967-2015, 2015
J. P. Huang, J. J. Liu, B. Chen, and S. L. Nasiri
Atmos. Chem. Phys., 15, 11653–11665, https://doi.org/10.5194/acp-15-11653-2015, https://doi.org/10.5194/acp-15-11653-2015, 2015
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To understand the contribution of anthropogenic dust to the total global dust load, a new technique for distinguishing anthropogenic dust from natural dust is proposed by using CALIPSO dust measurements and PBL height retrievals along with a land use data set. Results reveal that local anthropogenic dust aerosol accounts for about 25% of the global continental dust load.
Q. Jin, J. Wei, Z.-L. Yang, B. Pu, and J. Huang
Atmos. Chem. Phys., 15, 9897–9915, https://doi.org/10.5194/acp-15-9897-2015, https://doi.org/10.5194/acp-15-9897-2015, 2015
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Satellite data show that Indian summer monsoon (ISM) rainfall is closely associated with Middle East dust aerosols. Numerical modeling shows that the increased ISM rainfall is related to the enhanced southwesterly flow and moisture transport from the Arabian Sea to the Indian subcontinent, associated with the development of an anomalous low-pressure system over the Iranian Plateau and the Arabian Sea due to dust-induced atmospheric heating.
Y. H. Mao, Q. B. Li, D. K. Henze, Z. Jiang, D. B. A. Jones, M. Kopacz, C. He, L. Qi, M. Gao, W.-M. Hao, and K.-N. Liou
Atmos. Chem. Phys., 15, 7685–7702, https://doi.org/10.5194/acp-15-7685-2015, https://doi.org/10.5194/acp-15-7685-2015, 2015
R. Zhang, H. Wang, Y. Qian, P. J. Rasch, R. C. Easter, P.-L. Ma, B. Singh, J. Huang, and Q. Fu
Atmos. Chem. Phys., 15, 6205–6223, https://doi.org/10.5194/acp-15-6205-2015, https://doi.org/10.5194/acp-15-6205-2015, 2015
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We use the CAM5 model with a novel source-tagging technique to characterize the fate of BC particles emitted from various geographical regions and sectors and their transport pathways to the Himalayas and Tibetan Plateau (HTP). We show a comprehensive picture of the seasonal and regional dependence of BC source attributions, and find strong seasonal and spatial variations in BC-in-snow radiative forcing in the HTP that can be quantitatively attributed to the various regional/sectoral sources.
J. Li, J. Huang, K. Stamnes, T. Wang, Q. Lv, and H. Jin
Atmos. Chem. Phys., 15, 519–536, https://doi.org/10.5194/acp-15-519-2015, https://doi.org/10.5194/acp-15-519-2015, 2015
C. Zhao, Z. Hu, Y. Qian, L. Ruby Leung, J. Huang, M. Huang, J. Jin, M. G. Flanner, R. Zhang, H. Wang, H. Yan, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 14, 11475–11491, https://doi.org/10.5194/acp-14-11475-2014, https://doi.org/10.5194/acp-14-11475-2014, 2014
Y. H. Mao, Q. B. Li, D. Chen, L. Zhang, W.-M. Hao, and K.-N. Liou
Atmos. Chem. Phys., 14, 7195–7211, https://doi.org/10.5194/acp-14-7195-2014, https://doi.org/10.5194/acp-14-7195-2014, 2014
Hongru Yan, Zhanqing Li, Jianping Huang, Maureen Cribb, and Jianjun Liu
Atmos. Chem. Phys., 14, 7113–7124, https://doi.org/10.5194/acp-14-7113-2014, https://doi.org/10.5194/acp-14-7113-2014, 2014
C. He, Q. B. Li, K. N. Liou, J. Zhang, L. Qi, Y. Mao, M. Gao, Z. Lu, D. G. Streets, Q. Zhang, M. M. Sarin, and K. Ram
Atmos. Chem. Phys., 14, 7091–7112, https://doi.org/10.5194/acp-14-7091-2014, https://doi.org/10.5194/acp-14-7091-2014, 2014
A. Kumar, S. Wu, M. F. Weise, R. Honrath, R. C. Owen, D. Helmig, L. Kramer, M. Val Martin, and Q. Li
Atmos. Chem. Phys., 13, 12537–12547, https://doi.org/10.5194/acp-13-12537-2013, https://doi.org/10.5194/acp-13-12537-2013, 2013
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
L. Zhang, Q. B. Li, Y. Gu, K. N. Liou, and B. Meland
Atmos. Chem. Phys., 13, 7097–7114, https://doi.org/10.5194/acp-13-7097-2013, https://doi.org/10.5194/acp-13-7097-2013, 2013
D. N. Bernstein, J. D. Neelin, Q. B. Li, and D. Chen
Atmos. Chem. Phys., 13, 6373–6390, https://doi.org/10.5194/acp-13-6373-2013, https://doi.org/10.5194/acp-13-6373-2013, 2013
R. Zhang, D. A. Hegg, J. Huang, and Q. Fu
Atmos. Chem. Phys., 13, 6091–6099, https://doi.org/10.5194/acp-13-6091-2013, https://doi.org/10.5194/acp-13-6091-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
A new process-based and scale-aware desert dust emission scheme for global climate models – Part II: Evaluation in the Community Earth System Model version 2 (CESM2)
How well do Earth system models reproduce the observed aerosol response to rapid emission reductions? A COVID-19 case study
Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations
Impact of acidity and surface-modulated acid dissociation on cloud response to organic aerosol
The contribution of residential wood combustion to the PM2.5 concentrations in the Helsinki metropolitan area
Analysis of atmospheric particle growth based on vapor concentrations measured at the high-altitude GAW station Chacaltaya in the Bolivian Andes
Expanding the simulation of East Asian super dust storms: physical transport mechanisms impacting the western Pacific
Improving 3-day deterministic air pollution forecasts using machine learning algorithms
Opinion: The importance of historical and paleoclimate aerosol radiative effects
Assessing the assimilation of Himawari-8 observations on aerosol forecasts and radiative effects during pollution transport from South Asia to the Tibetan Plateau
Aerosol–meteorology feedback diminishes the transboundary transport of black carbon into the Tibetan Plateau
Associations of interannual variation in summer tropospheric ozone with the Western Pacific Subtropical High in China from 1999 to 2017
Climate intervention using marine cloud brightening (MCB) compared with stratospheric aerosol injection (SAI) in the UKESM1 climate model
Comparison of six approaches to predicting droplet activation of surface active aerosol – Part 2: Strong surfactants
Increased importance of aerosol–cloud interactions for surface PM2.5 pollution relative to aerosol–radiation interactions in China with the anthropogenic emission reductions
The role of temporal scales in extracting dominant meteorological drivers of major airborne pollutants
Biomass-burning smoke's properties and its interactions with marine stratocumulus clouds in WRF-CAM5 and southeastern Atlantic field campaigns
Air pollution trapping in the Dresden Basin from gray-zone scale urban modeling
The effect of atmospherically relevant aminium salts on water uptake
Droplet collection efficiencies estimated from satellite retrievals constrain effective radiative forcing of aerosol-cloud interactions
The impact of aerosols on stratiform clouds over southern West Africa: a large-eddy-simulation study
Numerical simulation and evaluation of global ultrafine particle concentrations at the Earth's surface
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
Molecular-level study on the role of methanesulfonic acid in iodine oxoacids nucleation
Global aviation contrail climate effects from 2019 to 2021
Global aerosol typing classification using a new hybrid algorithm utilizing Aerosol Robotic Network data
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis data sets
The underappreciated role of transboundary pollution in future air quality and health improvements in China
The export of African mineral dust across the Atlantic and its impact over the Amazon Basin
Assimilation of POLDER observations to estimate aerosol emissions
Effect of radiation interaction and aerosol processes on ventilation and aerosol concentrations in a real urban neighbourhood in Helsinki
Atlantic Multidecadal Oscillation modulates the relationship between El Niño–Southern Oscillation and fire weather in Australia
Sharp increase of Saharan dust intrusions over the Western Mediterranean and Euro-Atlantic region in winters 2020–2022 and associated atmospheric circulation
Phase state and viscosity of secondary organic aerosols over China simulated by WRF-Chem
Identifying climate model structural inconsistencies allows for tight constraint of aerosol radiative forcing
Sensitivity of global direct aerosol radiative forcing to uncertainties in aerosol optical properties
Impacts of reducing scattering and absorbing aerosols on the temporal extent and intensity of South Asian summer monsoon and East Asian summer monsoon
Superimposed effects of typical local circulations driven by mountainous topography and aerosol–radiation interaction on heavy haze in the Beijing–Tianjin–Hebei central and southern plains in winter
Multi-model ensemble projection of the global dust cycle by the end of 21st century using the Coupled Model Intercomparison Project version 6 data
A thermodynamic framework for bulk–surface partitioning in finite-volume mixed organic–inorganic aerosol particles and cloud droplets
Improved Simulations of Biomass Burning Aerosol Optical Properties and Lifetimes in the NASA GEOS Model during the ORACLES-I Campaign
Change from aerosol-driven to cloud-feedback-driven trend in short-wave radiative flux over the North Atlantic
A new process-based and scale-aware desert dust emission scheme for global climate models – Part I: Description and evaluation against inverse modeling emissions
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
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Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
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Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
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During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
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By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
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Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Danny M. Leung, Jasper F. Kok, Longlei Li, Natalie M. Mahowald, David M. Lawrence, Simone Tilmes, Erik Kluzek, Martina Klose, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 2287–2318, https://doi.org/10.5194/acp-24-2287-2024, https://doi.org/10.5194/acp-24-2287-2024, 2024
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This study uses a premier Earth system model to evaluate a new desert dust emission scheme proposed in our companion paper. We show that our scheme accounts for more dust emission physics, hence matching better against observations than other existing dust emission schemes do. Our scheme's dust emissions also couple tightly with meteorology, hence likely improving the modeled dust sensitivity to climate change. We believe this work is vital for improving dust representation in climate models.
Ruth A. R. Digby, Nathan P. Gillett, Adam H. Monahan, Knut von Salzen, Antonis Gkikas, Qianqian Song, and Zhibo Zhang
Atmos. Chem. Phys., 24, 2077–2097, https://doi.org/10.5194/acp-24-2077-2024, https://doi.org/10.5194/acp-24-2077-2024, 2024
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The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected regional aerosol optical depth (AOD) and compare the observed changes to predictions from Earth system models. Only India has an observed AOD reduction outside of typical variability. Models overestimate the response in some regions, but when key biases have been addressed, the agreement is improved. Our results suggest that current models can realistically predict the effects of future emission changes.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
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This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
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The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Leena Kangas, Jaakko Kukkonen, Mari Kauhaniemi, Kari Riikonen, Mikhail Sofiev, Anu Kousa, Jarkko V. Niemi, and Ari Karppinen
Atmos. Chem. Phys., 24, 1489–1507, https://doi.org/10.5194/acp-24-1489-2024, https://doi.org/10.5194/acp-24-1489-2024, 2024
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Residential wood combustion is a major source of fine particulate matter. This study has evaluated the contribution of residential wood combustion to fine particle concentrations and its year-to-year and seasonal variation in te Helsinki metropolitan area. The average concentrations attributed to wood combustion in winter were up to 10- or 15-fold compared to summer. Wood combustion caused 12 % to 14 % of annual fine particle concentrations. In winter, the contribution ranged from 16 % to 21 %.
Arto Heitto, Cheng Wu, Diego Aliaga, Luis Blacutt, Xuemeng Chen, Yvette Gramlich, Liine Heikkinen, Wei Huang, Radovan Krejci, Paolo Laj, Isabel Moreno, Karine Sellegri, Fernando Velarde, Kay Weinhold, Alfred Wiedensohler, Qiaozhi Zha, Federico Bianchi, Marcos Andrade, Kari E. J. Lehtinen, Claudia Mohr, and Taina Yli-Juuti
Atmos. Chem. Phys., 24, 1315–1328, https://doi.org/10.5194/acp-24-1315-2024, https://doi.org/10.5194/acp-24-1315-2024, 2024
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Particle growth at the Chacaltaya station in Bolivia was simulated based on measured vapor concentrations and ambient conditions. Major contributors to the simulated growth were low-volatility organic compounds (LVOCs). Also, sulfuric acid had major role when volcanic activity was occurring in the area. This study provides insight on nanoparticle growth at this high-altitude Southern Hemispheric site and hence contributes to building knowledge of early growth of atmospheric particles.
Steven Soon-Kai Kong, Saginela Ravindra Babu, Sheng-Hsiang Wang, Stephen M. Griffith, Jackson Hian-Wui Chang, Ming-Tung Chuang, Guey-Rong Sheu, and Neng-Huei Lin
Atmos. Chem. Phys., 24, 1041–1058, https://doi.org/10.5194/acp-24-1041-2024, https://doi.org/10.5194/acp-24-1041-2024, 2024
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In this study, we combined ground observations from 7-SEAS Dongsha Experiment, MERRA-2 reanalysis, and MODIS satellite images for evaluation and improvement of the CMAQ dust model for cases of East Asian Dust reaching the Taiwan region, including Dongsha in the western Pacific. We proposed a better CMAQ dust treatment over East Asia and for the first time revealed the impact of typhoons on dust transport.
Zhiguo Zhang, Christer Johansson, Magnuz Engardt, Massimo Stafoggia, and Xiaoliang Ma
Atmos. Chem. Phys., 24, 807–851, https://doi.org/10.5194/acp-24-807-2024, https://doi.org/10.5194/acp-24-807-2024, 2024
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Up-to-date information on present and near-future air quality help people avoid exposure to high levels of air pollution. We apply different machine learning models to significantly improve traditional forecasts of PM10, NOx, and O3 in Stockholm, Sweden. It is shown that forecasts of all air pollutants are improved by the input of lagged measurements and taking calendar information into account. The final modelled errors are substantially smaller than uncertainties in the measurements.
Natalie M. Mahowald, Longlei Li, Samuel Albani, Douglas S. Hamilton, and Jasper F. Kok
Atmos. Chem. Phys., 24, 533–551, https://doi.org/10.5194/acp-24-533-2024, https://doi.org/10.5194/acp-24-533-2024, 2024
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Estimating past aerosol radiative effects and their uncertainties is an important topic in climate science. Aerosol radiative effects propagate into large uncertainties in estimates of how present and future climate evolves with changing greenhouse gas emissions. A deeper understanding of how aerosols interacted with the atmospheric energy budget under past climates is hindered in part by a lack of relevant paleo-observations and in part because less attention has been paid to the problem.
Min Zhao, Tie Dai, Daisuke Goto, Hao Wang, and Guangyu Shi
Atmos. Chem. Phys., 24, 235–258, https://doi.org/10.5194/acp-24-235-2024, https://doi.org/10.5194/acp-24-235-2024, 2024
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During a springtime pollution input from South Asia to the Tibetan Plateau, we combined atmospheric chemistry modeling and data assimilation methods to assimilate and forecast aerosols from South Asia and the Tibetan Plateau. Assimilation of observations over a whole time window leads to a more reasonable distribution of daily variations in the aerosol forecast field. We also find that aerosol assimilation can improve the surface solar energy forecast in the Tibetan Plateau region.
Yuling Hu, Haipeng Yu, Shichang Kang, Junhua Yang, Mukesh Rai, Xiufeng Yin, Xintong Chen, and Pengfei Chen
Atmos. Chem. Phys., 24, 85–107, https://doi.org/10.5194/acp-24-85-2024, https://doi.org/10.5194/acp-24-85-2024, 2024
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The Tibetan Plateau (TP) saw a record-breaking aerosol pollution event from April 20 to May 10, 2016. We studied the impact of aerosol–meteorology feedback on the transboundary transport flux of black carbon (BC) during this severe pollution event. It was found that the aerosol–meteorology feedback decreases the transboundary transport flux of BC from the central and western Himalayas towards the TP. This study is of great significance for the protection of the ecological environment of the TP.
Xiaodong Zhang, Ruiyu Zhugu, Xiaohu Jian, Xinrui Liu, Kaijie Chen, Shu Tao, Junfeng Liu, Hong Gao, Tao Huang, and Jianmin Ma
Atmos. Chem. Phys., 23, 15629–15642, https://doi.org/10.5194/acp-23-15629-2023, https://doi.org/10.5194/acp-23-15629-2023, 2023
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WRF-Chem modeling was conducted to assess impacts of Western Pacific Subtropical High Pressure (WPSH) on interannual fluctuations of O3 pollution in China. We find that, while precursor emissions dominated the long-term trend and magnitude of O3 from 1999 to 2017, WPSH determined interannual variation of summer O3. The response of O3 pollution to WPSH in major urban clusters depended on the proximity of these urban areas to WPSH. The results could help long-term O3 pollution mitigation planning.
Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
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The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Sampo Vepsäläinen, Silvia M. Calderón, and Nønne L. Prisle
Atmos. Chem. Phys., 23, 15149–15164, https://doi.org/10.5194/acp-23-15149-2023, https://doi.org/10.5194/acp-23-15149-2023, 2023
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Atmospheric aerosols act as seeds for cloud formation. Many aerosols contain surface active material that accumulates at the surface of growing droplets. This can affect cloud droplet activation, but the broad significance of the effect and the best way to model it are still debated. We compare predictions of six models to surface activity of strongly surface active aerosol and find significant differences between the models, especially with large fractions of surfactant in the dry particles.
Da Gao, Bin Zhao, Shuxiao Wang, Yuan Wang, Brian Gaudet, Yun Zhu, Xiaochun Wang, Jiewen Shen, Shengyue Li, Yicong He, Dejia Yin, and Zhaoxin Dong
Atmos. Chem. Phys., 23, 14359–14373, https://doi.org/10.5194/acp-23-14359-2023, https://doi.org/10.5194/acp-23-14359-2023, 2023
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Surface PM2.5 concentrations can be enhanced by aerosol–radiation interactions (ARIs) and aerosol–cloud interactions (ACIs). In this study, we found PM2.5 enhancement induced by ACIs shows a significantly smaller decrease ratio than that induced by ARIs in China with anthropogenic emission reduction from 2013 to 2021, making ACIs more important for enhancing PM2.5 concentrations. ACI-induced PM2.5 enhancement needs to be emphatically considered to meet the national PM2.5 air quality standard.
Miaoqing Xu, Jing Yang, Manchun Li, Xiao Chen, Qiancheng Lv, Qi Yao, Bingbo Gao, and Ziyue Chen
Atmos. Chem. Phys., 23, 14065–14076, https://doi.org/10.5194/acp-23-14065-2023, https://doi.org/10.5194/acp-23-14065-2023, 2023
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Although the temporal-scale effects on PM2.5–meteorology associations have been discussed, no quantitative evidence has proved this before. Based on rare 3 h meteorology data, we revealed that the dominant meteorological factor for PM2.5 concentrations across China extracted at the 3 h and 24 h scales presented large variations. This research suggests that data sources of different temporal scales should be comprehensively considered for better attribution and prevention of airborne pollution.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Michael Weger and Bernd Heinold
Atmos. Chem. Phys., 23, 13769–13790, https://doi.org/10.5194/acp-23-13769-2023, https://doi.org/10.5194/acp-23-13769-2023, 2023
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This study investigates the effects of complex terrain on air pollution trapping using a numerical model which simulates the dispersion of emissions under real meteorological conditions. The additionally simulated aerosol age allows us to distinguish areas that accumulate aerosol over time from areas that are more influenced by fresh emissions. The Dresden Basin, a widened section of the Elbe Valley in eastern Germany, is selected as the target area in a case study to demonstrate the concept.
Noora Hyttinen
Atmos. Chem. Phys., 23, 13809–13817, https://doi.org/10.5194/acp-23-13809-2023, https://doi.org/10.5194/acp-23-13809-2023, 2023
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Water activity in aerosol particles describes how particles respond to variations in relative humidity. Here, water activities were calculated for a set of 80 salts that may be present in aerosol particles using a state-of-the-art quantum-chemistry-based method. The effect of the dissociated salt on water activity varies with both the cation and anion. Most of the studied salts increase water uptake compared to pure water-soluble organic particles.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
EGUsphere, https://doi.org/10.5194/egusphere-2023-2161, https://doi.org/10.5194/egusphere-2023-2161, 2023
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Single-layer warm liquid clouds cover nearly one-third of the earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth Systems Model estimates of the radiative forcing due to the interactions of aerosols with clouds due to warm rain processes.
Lambert Delbeke, Chien Wang, Pierre Tulet, Cyrielle Denjean, Maurin Zouzoua, Nicolas Maury, and Adrien Deroubaix
Atmos. Chem. Phys., 23, 13329–13354, https://doi.org/10.5194/acp-23-13329-2023, https://doi.org/10.5194/acp-23-13329-2023, 2023
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Low-level stratiform clouds (LLSCs) appear frequently over southern West Africa during the West African monsoon. Local and remote aerosol sources (biomass burning aerosols from central Africa) play a significant role in the LLSC life cycle. Based on measurements by the DACCIWA campaign, large-eddy simulation (LES) was conducted using different aerosol scenarios. The results show that both indirect and semi-direct effects can act individually or jointly to influence the life cycles of LLSCs.
Matthias Kohl, Jos Lelieveld, Sourangsu Chowdhury, Sebastian Ehrhart, Disha Sharma, Yafang Cheng, Sachchida Nand Tripathi, Mathew Sebastian, Govindan Pandithurai, Hongli Wang, and Andrea Pozzer
Atmos. Chem. Phys., 23, 13191–13215, https://doi.org/10.5194/acp-23-13191-2023, https://doi.org/10.5194/acp-23-13191-2023, 2023
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Knowledge on atmospheric ultrafine particles (UFPs) with a diameter smaller than 100 nm is crucial for public health and the hydrological cycle. We present a new global dataset of UFP concentrations at the Earth's surface derived with a comprehensive chemistry–climate model and evaluated with ground-based observations. The evaluation results are combined with high-resolution primary emissions to downscale UFP concentrations to an unprecedented horizontal resolution of 0.1° × 0.1°.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
EGUsphere, https://doi.org/10.5194/egusphere-2023-2070, https://doi.org/10.5194/egusphere-2023-2070, 2023
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the Southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass-burning plumes.
Jing Li, Nan Wu, An Ning, and Xiuhui Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2023-2084, https://doi.org/10.5194/egusphere-2023-2084, 2023
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Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas, however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3-HIO2-based nucleation is unclear. Our study provides molecular-level evidence that MSA can efficiently promote the formation of HIO3-HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help to deeply understand marine NPF events with burst of iodine particles.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc Stettler
EGUsphere, https://doi.org/10.5194/egusphere-2023-1859, https://doi.org/10.5194/egusphere-2023-1859, 2023
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The radiative forcing attributable to aviation contrails is estimated for 2019–21. We estimate a global contrail net RF that is approximately half the best estimate of a previous study. Contrail climate impacts have not scaled proportionally with air traffic growth due to higher growth in regions where contrails are less likely to form. There are significant opportunities to mitigate contrail impacts as only 2 % of all flights globally account for 80 % of the annual contrail energy forcing.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
EGUsphere, https://doi.org/10.5194/egusphere-2023-1754, https://doi.org/10.5194/egusphere-2023-1754, 2023
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A new aerosol-type classification algorithm was proposed. It includes an optical database building by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated using the new algorithm to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Yahui Che, Bofu Yu, and Katherine Bracco
EGUsphere, https://doi.org/10.5194/egusphere-2023-1710, https://doi.org/10.5194/egusphere-2023-1710, 2023
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Dust events over Australia concentrated in the north and southeast in spring, and can occur anywhere to the east in summer, with the dust season finishing in autumn using a combined DAOD. Near-surface dust concentrations were the highest over the cente, and weakened radially away the center, decreasing along two main pathways. Total dust emission was about 40 Mt (mega-tonnes) per year from1980–2020, of which nearly 50 % was deposited on land; the rest as net export from the Australian continent.
Jun-Wei Xu, Jintai Lin, Dan Tong, and Lulu Chen
Atmos. Chem. Phys., 23, 10075–10089, https://doi.org/10.5194/acp-23-10075-2023, https://doi.org/10.5194/acp-23-10075-2023, 2023
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This study highlights the necessity of a low-carbon pathway in foreign countries for China to achieve air quality goals and to protect public health. We find that adopting the low-carbon instead of the fossil-fuel-intensive pathway in foreign countries would prevent 63 000–270 000 transboundary PM2.5-associated mortalities in China in 2060. Our study provides direct evidence of the necessity of inter-regional cooperation for air quality improvement.
Xurong Wang, Qiaoqiao Wang, Maria Prass, Christopher Pöhlker, Daniel Moran-Zuloaga, Paulo Artaxo, Jianwei Gu, Ning Yang, Xiajie Yang, Jiangchuan Tao, Juan Hong, Nan Ma, Yafang Cheng, Hang Su, and Meinrat O. Andreae
Atmos. Chem. Phys., 23, 9993–10014, https://doi.org/10.5194/acp-23-9993-2023, https://doi.org/10.5194/acp-23-9993-2023, 2023
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In this work, with an optimized particle mass size distribution, we captured observed aerosol optical depth (AOD) and coarse aerosol concentrations over source and/or receptor regions well, demonstrating good performance in simulating export of African dust toward the Amazon Basin. In addition to factors controlling the transatlantic transport of African dust, the study investigated the impact of African dust over the Amazon Basin, including the nutrient inputs associated with dust deposition.
Athanasios Tsikerdekis, Otto P. Hasekamp, Nick A. J. Schutgens, and Qirui Zhong
Atmos. Chem. Phys., 23, 9495–9524, https://doi.org/10.5194/acp-23-9495-2023, https://doi.org/10.5194/acp-23-9495-2023, 2023
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Aerosols are tiny particles of different substances (species) that can be emitted into the atmosphere by natural processes or by anthropogenic activities. However, the actual aerosol emission amount per species is highly uncertain. Thus in this work we correct the aerosol emissions used to drive a global aerosol–climate model using satellite observations through a process called data assimilation. These more accurate aerosol emissions can lead to a more accurate weather and climate prediction.
Jani Strömberg, Xiaoyu Li, Mona Kurppa, Heino Kuuluvainen, Liisa Pirjola, and Leena Järvi
Atmos. Chem. Phys., 23, 9347–9364, https://doi.org/10.5194/acp-23-9347-2023, https://doi.org/10.5194/acp-23-9347-2023, 2023
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We conclude that with low wind speeds, solar radiation has a larger decreasing effect (53 %) on pollutant concentrations than aerosol processes (18 %). Additionally, our results showed that with solar radiation included, pollutant concentrations were closer to observations (−13 %) than with only aerosol processes (+98 %). This has implications when planning simulations under calm conditions such as in our case and when deciding whether or not simulations need to include these processes.
Guanyu Liu, Jing Li, and Tong Ying
Atmos. Chem. Phys., 23, 9217–9228, https://doi.org/10.5194/acp-23-9217-2023, https://doi.org/10.5194/acp-23-9217-2023, 2023
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Fires in Australia are positively correlated with the El Niño–Southern Oscillation (ENSO). However, the correlation between ENSO and the Australian Fire Weather Index (FWI) increases from 0.17 to 0.70 when the Atlantic Multidecadal Oscillation (AMO) shifts from a negative to positive phase. This is explained by the teleconnection effect through which the warmer AMO generates Rossby wave trains and results in high pressures and a weather condition conducive to wildfires.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
EGUsphere, https://doi.org/10.5194/egusphere-2023-1749, https://doi.org/10.5194/egusphere-2023-1749, 2023
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In 2020–2022, several international agencies and media reported severe winter dust intrusions in Europe. Although winter dust intrusions are more common in the eastern Mediterranean, these events largely affected the western Mediterranean and Canary Islands. The present work provides a catalogue of dust events over the western Mediterranean region and describes their characteristics during the climatological (2003–2019) and recent anomalous (2020–2022) periods.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
EGUsphere, https://doi.org/10.5194/egusphere-2023-1444, https://doi.org/10.5194/egusphere-2023-1444, 2023
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Secondary organic aerosols (SOA) can exist in liquid, semi-solid or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in the northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David M. H. Sexton, Christopher Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John W. Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 8749–8768, https://doi.org/10.5194/acp-23-8749-2023, https://doi.org/10.5194/acp-23-8749-2023, 2023
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Aerosol forcing of Earth’s energy balance has persisted as a major cause of uncertainty in climate simulations over generations of climate model development. We show that structural deficiencies in a climate model are exposed by comprehensively exploring parametric uncertainty and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. This provides a future pathway towards building models with greater physical realism and lower uncertainty.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
EGUsphere, https://doi.org/10.5194/egusphere-2023-1096, https://doi.org/10.5194/egusphere-2023-1096, 2023
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Aerosols influence the Earth’s Energy balance. The uncertainty in this radiative forcing is large, depending partly on uncertainty in measurements of aerosol optical properties. We develop a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty but that non-aerosol uncertainties must also be considered.
Chenwei Fang, Jim M. Haywood, Ju Liang, Ben T. Johnson, Ying Chen, and Bin Zhu
Atmos. Chem. Phys., 23, 8341–8368, https://doi.org/10.5194/acp-23-8341-2023, https://doi.org/10.5194/acp-23-8341-2023, 2023
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The responses of Asian summer monsoon duration and intensity to air pollution mitigation are identified given the net-zero future. We show that reducing scattering aerosols makes the rainy season longer and stronger across South Asia and East Asia but that absorbing aerosol reduction has the opposite effect. Our results hint at distinct monsoon responses to emission controls that target different aerosols.
Yue Peng, Hong Wang, Xiaoye Zhang, Zhaodong Liu, Wenjie Zhang, Siting Li, Chen Han, and Huizheng Che
Atmos. Chem. Phys., 23, 8325–8339, https://doi.org/10.5194/acp-23-8325-2023, https://doi.org/10.5194/acp-23-8325-2023, 2023
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This study demonstrates a strong link between local circulation, aerosol–radiation interaction (ARI), and haze pollution. Under the weak weather-scale systems, the typical local circulation driven by mountainous topography is the main cause of pollutant distribution in the Beijing–Tianjin–Hebei region, and the ARI mechanism amplifies this influence of local circulation on pollutants, making haze pollution aggravated by the superposition of both.
Yuan Zhao, Xu Yue, Yang Cao, Jun Zhu, Chenguang Tian, Hao Zhou, Yuwen Chen, Yihan Hu, Weijie Fu, and Xu Zhao
Atmos. Chem. Phys., 23, 7823–7838, https://doi.org/10.5194/acp-23-7823-2023, https://doi.org/10.5194/acp-23-7823-2023, 2023
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We project the future changes of dust emissions and loading using an ensemble of model outputs from the Coupled Model Intercomparison Project version 6 under four scenarios. We find increased dust emissions and loading in North Africa, due to increased drought and strengthened surface wind, and decreased dust loading over Asia, following enhanced precipitation. Such a spatial pattern remains similar, though the regional intensity varies among different scenarios.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 23, 7741–7765, https://doi.org/10.5194/acp-23-7741-2023, https://doi.org/10.5194/acp-23-7741-2023, 2023
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Aerosol particles below 100 nm in diameter have high surface-area-to-volume ratios. The enrichment of compounds in the surface of an aerosol particle may lead to depletion of that species in the interior bulk of the particle. We present a framework for modeling the equilibrium bulk–surface partitioning of mixed organic–inorganic particles, including cases of co-condensation of semivolatile organic compounds and species with extremely limited solubility in the bulk or surface of a particle.
Sampa Das, Peter Colarco, Huisheng Bian, and Santiago Gasso
EGUsphere, https://doi.org/10.5194/egusphere-2023-1311, https://doi.org/10.5194/egusphere-2023-1311, 2023
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The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 23, 6743–6773, https://doi.org/10.5194/acp-23-6743-2023, https://doi.org/10.5194/acp-23-6743-2023, 2023
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We determine what causes long-term trends in short-wave (SW) radiative fluxes in two climate models. A positive trend occurs between 1850 and 1970 (increasing SW reflection) and a negative trend between 1970 and 2014; the pre-1970 positive trend is mainly driven by an increase in cloud droplet number concentrations due to increases in aerosol, and the 1970–2014 trend is driven by a decrease in cloud fraction, which we attribute to changes in clouds caused by greenhouse gas-induced warming.
Danny M. Leung, Jasper F. Kok, Longlei Li, Gregory S. Okin, Catherine Prigent, Martina Klose, Carlos Pérez García-Pando, Laurent Menut, Natalie M. Mahowald, David M. Lawrence, and Marcelo Chamecki
Atmos. Chem. Phys., 23, 6487–6523, https://doi.org/10.5194/acp-23-6487-2023, https://doi.org/10.5194/acp-23-6487-2023, 2023
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Desert dust modeling is important for understanding climate change, as dust regulates the atmosphere's greenhouse effect and radiation. This study formulates and proposes a more physical and realistic desert dust emission scheme for global and regional climate models. By considering more aeolian processes in our emission scheme, our simulations match better against dust observations than existing schemes. We believe this work is vital in improving dust representation in climate models.
Cited articles
Andreae, M. O. and Rosenfeld, D.: Aerosol–cloud–precipitation interactions. Part 1. The nature and sources of cloud-active aerosols, Earth-Sci. Rev., 89, 13–41, 2008.
Barahona, D., Molod, A., Bacmeister, J., Nenes, A., Gettelman, A., Morrison, H., Phillips, V., and Eichmann, A.: Development of two-moment cloud microphysics for liquid and ice within the NASA Goddard Earth Observing System Model (GEOS-5), Geosci. Model Dev., 7, 1733–1766, https://doi.org/10.5194/gmd-7-1733-2014, 2014.
Bergeron, T.: On the physics of clouds and precipitation. Proces Verbaux de l'Association de Météorologie, International Union of Geodesy and Geophysics, Imprimerie Paul Dupont, Paris, France, 156–178, 1935.
Bond, T. C., Bhardwaj, E., Dong, R., Jogani, R., Jung, S., Roden, C., Streets, D. G., and Trautmann, N. M.: Historical emissions of black and organic carbon aerosol from energy-related combustion, 1850–2000, Global Biogeochem. Cy., 21, GB2018, https://doi.org/10.1029/2006gb002840, 2007.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, https://doi.org/10.1002/jgrd.50171, 2013.
Bourgeois, Q. and Bey, I.: Pollution transport efficiency toward the Arctic: Sensitivity to aerosol scavenging and source regions, J. Geophys. Res., 116, D08213, https://doi.org/10.1029/2010jd015096, 2011.
Browse, J., Carslaw, K. S., Arnold, S. R., Pringle, K., and Boucher, O.: The scavenging processes controlling the seasonal cycle in Arctic sulphate and black carbon aerosol, Atmos. Chem. Phys., 12, 6775–6798, https://doi.org/10.5194/acp-12-6775-2012, 2012.
Castro, L. M., Pio, C. A., Harrison, R. M., and Smith, D. J. T.: Carbonaceous aerosol in urban and rural European atmospheres: Estimation of secondary organic carbon concentrations, Atmos. Environ., 33, 2771–2781, 1999.
Cerqueira, M., Pio, C., Legrand, M., Puxbaum, H., Kasper-Giebl, A., Afonso, J., Preunkert, S., Gelencsér, A., and Fialho, P.: Particulate carbon in precipitation at European background sites, J. Aerosol Sci., 41, 51–61, https://doi.org/10.1016/j.jaerosci.2009.08.002, 2010.
Chow, J. C., Watson, J. G., Pritchett, L. C., Pierson, W. R., Frazier, C. A., and Purcell, R. G.: The Dri Thermal Optical Reflectance Carbon Analysis System – Description, Evaluation and Applications in United-States Air-Quality Studies, Atmos. Environ. A-Gen., 27, 1185–1201, https://doi.org/10.1016/0960-1686(93)90245-T, 1993.
Chow, J. C., Watson, J. G., Chen, L. W. A., Arnott, W. P., Moosmuller, H., and Fung, K.: Equivalence of elemental carbon by thermal/optical reflectance and transmittance with different temperature protocols, Environ. Sci. Technol., 38, 4414–4422, https://doi.org/10.1021/Es034936u, 2004.
Cooke, W. F., Liousse, C., Cachier, H., and Feichter, J.: Construction of a 1° × 1° fossil fuel emission data set for carbonaceous aerosol and implementation and radiative impact in the ECHAM4 model, J. Geophys. Res., 104, 22137–22162, https://doi.org/10.1029/1999jd900187, 1999.
Cozic, J., Verheggen, B., Mertes, S., Connolly, P., Bower, K., Petzold, A., Baltensperger, U., and Weingartner, E.: Scavenging of black carbon in mixed phase clouds at the high alpine site Jungfraujoch, Atmos. Chem. Phys., 7, 1797–1807, https://doi.org/10.5194/acp-7-1797-2007, 2007.
Cozic, J., Mertes, S., Verheggen, B., Cziczo, D. J., Gallavardin, S., Walter, S., Baltensperger, U., and Weingartner, E.: Black carbon enrichment in atmospheric ice particle residuals observed in lower tropospheric mixed phase clouds, J. Geophys. Res., 113, D15209, https://doi.org/10.1029/2007JD009266, 2008.
Doherty, S. J., Warren, S. G., Grenfell, T. C., Clarke, A. D., and Brandt, R. E.: Light-absorbing impurities in Arctic snow, Atmos. Chem. Phys., 10, 11647–11680, https://doi.org/10.5194/acp-10-11647-2010, 2010.
Doherty, S. J., Dang, C., Hegg, D. A., Zhang, R. D., and Warren, S. G.: Black carbon and other light-absorbing particles in snow of central North America, J. Geophys. Res.-Atmos., 119, 12807–12831, https://doi.org/10.1002/2014jd022350, 2014.
EUROPA: Directive 2008/50/EC of the European Parliament and of the Council, Official Journal of the European Union, 152 pp., 2008
EMEP/MSC-W, EMEP/CCC, EMEP/CEIP, IDAEA-CSIC, CCE/RIVM, and FMI: Transboundary particulate matter, photo-oxidants, acidifying and eutrophying components, Meteorologisk Institutt (Norwegian Meteorological Institute), EMEP Report 1/2014, 216 pp., 2014.
Findeisen, W.: Kolloid-meteorologische Vorgänge bei Neiderschlags-bildung, Meteorol. Z., 55, 121–133, 1938.
Flanner, M. G., Zender, C. S., Randerson, J. T., and Rasch, P. J.: Present-day climate forcing and response from black carbon in snow, J. Geophys. Res., 112, D11202, https://doi.org/10.1029/2006JD008003, 2007.
Fukuta, N. and Takahashi, T.: The Growth of Atmospheric Ice Crystals: A Summary of Findings in Vertical Supercooled Cloud Tunnel Studies, J. Atmos. Sci., 56, 1963–1979, https://doi.org/10.1175/1520-0469(1999)056<1963:TGOAIC>2.0.CO;2, 1999.
Gayet, J., Treffeisen, R., Helbig, A., Bareiss, J., Matsuki, A., Herber, A., and Schwarzenboeck, A.: On the onset of the ice phase in boundary layer Arctic clouds, J. Geophys. Res., 114, D19201, https://doi.org/10.1029/2008JD011348, 2009.
Ghan, S. J., Abdul-Razzak, H., Nenes, A., Ming, Y., Liu, X., Ovchinnikov, M., Shipway, B., Meskhidze, N., Xu, J., and Shi, X.: Droplet nucleation: Physically-based parameterizations and comparative evaluation, Journal of Advances in Modeling Earth Systems, 3, M10001, https://doi.org/10.1029/2011ms000074, 2011.
Gieray, R., Wieser, P., Engelhardt, T., Swietlicki, E., Hansson, H. C., Mentes, B., Orsini, D., Martinsson, B., Svenningsson, B., Noone, K. J., and Heintzenberg, J.: Phase partitioning of aerosol constituents in cloud based on single-particle and bulk analysis, Atmos. Environ., 31, 2491–2502, https://doi.org/10.1016/S1352-2310(96)00298-1, 1997.
Gilardoni, S., Massoli, P., Giulianelli, L., Rinaldi, M., Paglione, M., Pollini, F., Lanconelli, C., Poluzzi, V., Carbone, S., Hillamo, R., Russell, L. M., Facchini, M. C., and Fuzzi, S.: Fog scavenging of organic and inorganic aerosol in the Po Valley, Atmos. Chem. Phys., 14, 6967–6981, https://doi.org/10.5194/acp-14-6967-2014, 2014.
Giorgi, F. and Chameides, W. L.: Rainout lifetimes of highly soluble aerosols and gases as inferred from simulations with a general circulation model, J. Geophys. Res., 91, 14367–14376, https://doi.org/10.1029/JD091iD13p14367, 1986.
Gorbunov, B., Baklanov, A., Kakutkina, N., Windsor, H., and Toumi, R.: Ice nucleation on soot particles, J. Aerosol Sci., 32, 199–215, 2001.
Hadley, O. L., Corrigan, C. E., and Kirchstetter, T. W.: Modified Thermal-Optical Analysis Using Spectral Absorption Selectivity To Distinguish Black Carbon from Pyrolized Organic Carbon, Environ. Sci. Technol., 42, 8459–8464, https://doi.org/10.1021/Es800448n, 2008.
Hadley, O. L., Corrigan, C. E., Kirchstetter, T. W., Cliff, S. S., and Ramanathan, V.: Measured black carbon deposition on the Sierra Nevada snow pack and implication for snow pack retreat, Atmos. Chem. Phys., 10, 7505–7513, https://doi.org/10.5194/acp-10-7505-2010, 2010.
Hallberg, A., Ogren, J. A., Noone, K. J., Heintzenberg, J., Berner, A., Solly, I., Kruisz, C., Reischl, G., Fuzzi, S., Facchini, M. C., Hansson, H. C., Wiedensohler, A., and Svenningsson, I. B.: Phase Partitioning for Different Aerosol Species in Fog, Tellus B, 44, 545–555, https://doi.org/10.1034/j.1600-0889.1992.t01-2-00008.x, 1992.
Hallberg, A., Noone, K. J., Ogren, J. A., Svenningsson, I. B., Flossmann, A., Wiedensohler, A., Hansson, H. C., Heintzenberg, J., Anderson, T. L., Arends, B. G., and Maser, R.: Phase Partitioning of Aerosol Particles in Clouds at Kleiner Feldberg, in: The Kleiner Feldberg Cloud Experiment 1990: EUROTRAC Subproject Ground-Based Cloud Experiment (GCE), edited by: Fuzzi, S., Springer Netherlands, Dordrecht, 107–127, 1994.
He, C., Li, Q. B., Liou, K. N., Zhang, J., Qi, L., Mao, Y., Gao, M., Lu, Z., Streets, D. G., Zhang, Q., Sarin, M. M., and Ram, K.: A global 3-D CTM evaluation of black carbon in the Tibetan Plateau, Atmos. Chem. Phys., 14, 7091–7112, https://doi.org/10.5194/acp-14-7091-2014, 2014a.
He, C., Li, Q. B., Liou, K. N., Takano, Y., Gu, Y., Qi, L., Mao, Y. H., and Leung, L. R.: Black carbon radiative forcing over the Tibetan Plateau, Geophys. Res. Lett., 41, 7806–7813, https://doi.org/10.1002/2014gl062191, 2014b.
He, C., Li, Q., Liou, K.-N., Qi, L., Tao, S., and Schwarz, J. P.: Microphysics-based black carbon aging in a global CTM: constraints from HIPPO observations and implications for global black carbon budget, Atmos. Chem. Phys., 16, 3077–3098, https://doi.org/10.5194/acp-16-3077-2016, 2016.
Hegg, D. A., Clarke, A. D., Doherty, S. J., and Ström, J.: Measurements of black carbon aerosol washout ratio on Svalbard, Tellus B, 63, 891–900, https://doi.org/10.1111/j.1600-0889.2011.00577.x, 2011.
Heintzenberg, J. and Leck, C.: Seasonal-Variation of the Atmospheric Aerosol near the Top of the Marine Boundary-Layer over Spitsbergen Related to the Arctic Sulfur Cycle, Tellus B, 46, 52–67, https://doi.org/10.1034/j.1600-0889.1994.00005.x, 1994.
Henning, S., Bojinski, S., Diehl, K., Ghan, S., Nyeki, S., Weingartner, E., Wurzler, S., and Baltensperger, U.: Aerosol partitioning in natural mixed-phase clouds, Geophys. Res. Lett., 31, L06101, https://doi.org/10.1029/2003GL019025, 2004.
Hitzenberger, R., Berner, A., Kromp, R., Kasper-Giebl, A., Limbeck, A., Tscherwenka, W., and Puxbaum, H.: Black carbon and other species at a high-elevation European site (Mount Sonnblick, 3106 m, Austria): Concentrations and scavenging efficiencies, J. Geophys. Res., 105, 24637, https://doi.org/10.1029/2000jd900349, 2000.
Hitzenberger, R., Berner, A., Giebl, H., Drobesch, K., Kasper-Giebl, A., Loeflund, M., Urban, H., and Puxbaum, H.: Black carbon (BC) in alpine aerosols and cloud water – concentrations and scavenging efficiencies, Atmos. Environ., 35, 5135–5141, 2001.
Huang, J. P., Fu, Q. A., Zhang, W., Wang, X., Zhang, R. D., Ye, H., and Warren, S. G.: Dust and Black Carbon in Seasonal Snow across Northern China, B. Am. Meteorol. Soc., 92, 175–181, https://doi.org/10.1175/2010bams3064.1, 2011.
IPCC: Climate Change 2014: Synthesis Report. Contribution of Working Groups I, II and III to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Core Writing Team, Pachauri, R. K., and Meyer, L. A., IPCC, Geneva, Switzerland, 151 pp., 2014.
Kamphus, M., Ettner-Mahl, M., Klimach, T., Drewnick, F., Keller, L., Cziczo, D. J., Mertes, S., Borrmann, S., and Curtius, J.: Chemical composition of ambient aerosol, ice residues and cloud droplet residues in mixed-phase clouds: single particle analysis during the Cloud and Aerosol Characterization Experiment (CLACE 6), Atmos. Chem. Phys., 10, 8077–8095, https://doi.org/10.5194/acp-10-8077-2010, 2010.
Koch, D., Menon, S., Del Genio, A., Ruedy, R., Alienov, I., and Schmidt, G. A.: Distinguishing Aerosol Impacts on Climate over the Past Century, J. Climate, 22, 2659–2677, https://doi.org/10.1175/2008jcli2573.1, 2009.
Kondo, Y., Sahu, L., Moteki, N., Khan, F., Takegawa, N., Liu, X., Koike, M., and Miyakawa, T.: Consistency and traceability of black carbon measurements made by laser-induced incandescence, thermal-optical transmittance, and filter-based photo-absorption techniques, Aerosol Sci. Tech., 45, 295–312, https://doi.org/10.1080/02786826.2010.533215, 2011.
Li, J. L. F., Waliser, D. E., Chen, W. T., Guan, B., Kubar, T., Stephens, G., Ma, H. Y., Deng, M., Donner, L., Seman, C., and Horowitz, L.: An observationally based evaluation of cloud ice water in CMIP3 and CMIP5 GCMs and contemporary reanalyses using contemporary satellite data, J. Geophys. Res., 117, D16105, https://doi.org/10.1029/2012JD017640, 2012.
Liou, K. N., Takano, Y., He, C., Yang, P., Leung, L. R., Gu, Y., and Lee, W. L.: Stochastic parameterization for light absorption by internally mixed BC/dust in snow grains for application to climate models, J. Geophys. Res.-Atmos., 119, 7616–7632, https://doi.org/10.1002/2014jd021665, 2014.
Liu, H., Jacob, D. J., Bey, I., and Yantosca, R. M.: Constraints from 210Pb and 7Be on wet deposition and transport in a global three-dimensional chemical tracer model driven by assimilated meteorological fields, J. Geophys. Res., 106, 12109–12128, https://doi.org/10.1029/2000JD900839, 2001.
Liu, J., Fan, S., Horowitz, L. W., and Levy, H.: Evaluation of factors controlling long-range transport of black carbon to the Arctic, J. Geophys. Res., 116, D04307, https://doi.org/10.1029/2010JD015145, 2011.
Malm, W. C., Sisler, J. F., Huffman, D., Eldred, R. A., and Cahill, T. A.: Spatial and Seasonal Trends in Particle Concentration and Optical Extinction in the United-States, J. Geophys. Res., 99, 1347–1370, https://doi.org/10.1029/93jd02916, 1994.
Mao, Y. H., Li, Q. B., Zhang, L., Chen, Y., Randerson, J. T., Chen, D., and Liou, K. N.: Biomass burning contribution to black carbon in the Western United States Mountain Ranges, Atmos. Chem. Phys., 11, 11253–11266, https://doi.org/10.5194/acp-11-11253-2011, 2011.
Mao, Y. H., Li, Q. B., Chen, D., Zhang, L., Hao, W.-M., and Liou, K.-N.: Top-down estimates of biomass burning emissions of black carbon in the Western United States, Atmos. Chem. Phys., 14, 7195–7211, https://doi.org/10.5194/acp-14-7195-2014, 2014.
Mori, T., Kondo, Y., Ohata, S., Moteki, N., Matsui, H., Oshima, N., and Iwasaki, A.: Wet deposition of black carbon at a remote site in the East China Sea, J. Geophys. Res.-Atmos., 119, 10485–10498, https://doi.org/10.1002/2014jd022103, 2014.
Morrison, H., de Boer, G., Feingold, G., Harrington, J., Shupe, M. D., and Sulia, K.: Resilience of persistent Arctic mixed-phase clouds, Nat. Geosci., 5, 11–17, https://doi.org/10.1038/ngeo1332, 2012.
Moteki, N., Kondo, Y., Oshima, N., Takegawa, N., Koike, M., Kita, K., Matsui, H., and Kajino, M.: Size dependence of wet removal of black carbon aerosols during transport from the boundary layer to the free troposphere, Geophys. Res. Lett., 39, L13802, https://doi.org/10.1029/2012GL052034, 2012.
Murray, B. J., O'Sullivan, D., Atkinson, J. D., and Webb, M. E.: Ice nucleation by particles immersed in supercooled cloud droplets, Chem. Soc. Rev., 41, 6519–6554, https://doi.org/10.1039/C2CS35200A, 2012.
Myhre, G., Samset, B. H., Schulz, M., Balkanski, Y., Bauer, S., Berntsen, T. K., Bian, H., Bellouin, N., Chin, M., Diehl, T., Easter, R. C., Feichter, J., Ghan, S. J., Hauglustaine, D., Iversen, T., Kinne, S., Kirkevåg, A., Lamarque, J.-F., Lin, G., Liu, X., Lund, M. T., Luo, G., Ma, X., van Noije, T., Penner, J. E., Rasch, P. J., Ruiz, A., Seland, Ø., Skeie, R. B., Stier, P., Takemura, T., Tsigaridis, K., Wang, P., Wang, Z., Xu, L., Yu, H., Yu, F., Yoon, J.-H., Zhang, K., Zhang, H., and Zhou, C.: Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations, Atmos. Chem. Phys., 13, 1853–1877, https://doi.org/10.5194/acp-13-1853-2013, 2013.
Niu, J., Carey, L. D., Yang, P., and Vonder Haar, T. H.: Optical properties of a vertically inhomogeneous mid-latitude mid-level mixed-phase altocumulus in the infrared region, Atmos. Res., 88, 234–242, https://doi.org/10.1016/j.atmosres.2007.11.020, 2008.
Noone, K. J. and Clarke, A. D.: Soot Scavenging Measurements in Arctic Snowfall, Atmos. Environ., 22, 2773–2778, https://doi.org/10.1016/0004-6981(88)90444-1, 1988.
Ogren, J. A., Heintzenberg, J., and Charlson, R. J.: In-situ sampling of clouds with a droplet to aerosol converter, Geophys. Res. Lett., 12, 121–124, https://doi.org/10.1029/GL012i003p00121, 1985.
Park, R. J., Jacob, D. J., Chin, M., and Martin, R. V.: Sources of carbonaceous aerosols over the United States and implications for natural visibility, J. Geophys. Res., 108, 4355, https://doi.org/10.1029/2002JD003190, 2003.
Park, R. J., Jacob, D. J., Palmer, P. I., Clarke, A. D., Weber, R. J., Zondlo, M. A., Eisele, F. L., Bandy, A. R., Thornton, D. C., Sachse, G. W., and Bond, T. C.: Export efficiency of black carbon aerosol in continental outflow: Global implications, J. Geophys. Res., 110, D11205, https://doi.org/10.1029/2004JD005432, 2005.
Pinto, J. O.: Autumnal Mixed-Phase Cloudy Boundary Layers in the Arctic, J. Atmos. Sci., 55, 2016–2038, https://doi.org/10.1175/1520-0469, 1998.
Pio, C. A., Legrand, M., Oliveira, T., Afonso, J., Santos, C., Caseiro, A., Fialho, P., Barata, F., Puxbaum, H., Sanchez-Ochoa, A., Kasper-Giebl, A., Gelencsér, A., Preunkert, S., and Schock, M.: Climatology of aerosol composition (organic versus inorganic) at nonurban sites on a west-east transect across Europe, J. Geophys. Res., 112, D23S02, https://doi.org/10.1029/2006JD008038, 2007.
Pruppacher, H. R. and Klett, J. D.: Microphysics of clouds and precipitation, in: Atmospheric and Oceanographic Sciences Library, Springer Netherlands, 18, 954 pp., https://doi.org/10.1007/978-0-306-48100-0, 2010.
Qi, L., Li, Q., Li, Y., and He, C.: Factors controlling black carbon distribution in the Arctic, Atmos. Chem. Phys., 17, 1037–1059, https://doi.org/10.5194/acp-17-1037-2017, 2017.
Ramanathan, V. and Carmichael, G.: Global and regional climate changes due to black carbon, Nat. Geosci., 1, 221–227, 2008.
Randerson, J. T., Chen, Y., van der Werf, G. R., Rogers, B. M., and Morton, D. C.: Global burned area and biomass burning emissions from small fires, J. Geophys. Res., 117, G04012, https://doi.org/10.1029/2012JG002128, 2012.
Samset, B. H. and Myhre, G.: Vertical dependence of black carbon, sulphate and biomass burning aerosol radiative forcing, Geophys. Res. Lett., 38, L24802, https://doi.org/10.1029/2011GL049697, 2011.
Schulz, M., Textor, C., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Dentener, F., Guibert, S., Isaksen, I. S. A., Iversen, T., Koch, D., Kirkevåg, A., Liu, X., Montanaro, V., Myhre, G., Penner, J. E., Pitari, G., Reddy, S., Seland, Ø., Stier, P., and Takemura, T.: Radiative forcing by aerosols as derived from the AeroCom present-day and pre-industrial simulations, Atmos. Chem. Phys., 6, 5225–5246, https://doi.org/10.5194/acp-6-5225-2006, 2006.
Schwarz, J. P., Gao, R. S., Spackman, J. R., Watts, L. A., Thomson, D. S., Fahey, D. W., Ryerson, T. B., Peischl, J., Holloway, J. S., Trainer, M., Frost, G. J., Baynard, T., Lack, D. A., de Gouw, J. A., Warneke, C., and Del Negro, L. A.: Measurement of the mixing state, mass, and optical size of individual black carbon particles in urban and biomass burning emissions, Geophys. Res. Lett., 35, L13810, https://doi.org/10.1029/2008GL033968, 2008.
Schwarz, J. P., Spackman, J. R., Gao, R. S., Watts, L. A., Stier, P., Schulz, M., Davis, S. M., Wofsy, S. C., and Fahey, D. W.: Global-scale black carbon profiles observed in the remote atmosphere and compared to models, Geophys. Res. Lett., 37, L18812, https://doi.org/10.1029/2010GL044372, 2010.
Sellegri, K., Laj, P., Dupuy, R., Legrand, M., Preunkert, S., and Putaud, J. P.: Size-dependent scavenging efficiencies of multicomponent atmospheric aerosols in clouds, J. Geophys. Res., 108, 4334, https://doi.org/10.1029/2002JD002749, 2003.
Shupe, M. D., Matrosov, S. Y., and Uttal, T.: Arctic Mixed-Phase Cloud Properties Derived from Surface-Based Sensors at SHEBA, J. Atmos. Sci., 63, 697–711, https://doi.org/10.1175/JAS3659.1, 2006.
Smith, A. J., Larson, V. E., Niu, J., Kankiewicz, J. A., and Carey, L. D.: Processes that generate and deplete liquid water and snow in thin midlevel mixed-phase clouds, J. Geophys. Res., 114, D12203, https://doi.org/10.1029/2008JD011531, 2009.
Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125–1156, https://doi.org/10.5194/acp-5-1125-2005, 2005.
Stohl, A., Klimont, Z., Eckhardt, S., Kupiainen, K., Shevchenko, V. P., Kopeikin, V. M., and Novigatsky, A. N.: Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions, Atmos. Chem. Phys., 13, 8833–8855, https://doi.org/10.5194/acp-13-8833-2013, 2013.
Tan, I., Storelvmo, T., and Zelinka, M. D.: Observational constraints on mixed-phase clouds imply higher climate sensitivity, Science, 352, 224–227, https://doi.org/10.1126/science.aad5300, 2016.
Taylor, J. W., Allan, J. D., Allen, G., Coe, H., Williams, P. I., Flynn, M. J., Le Breton, M., Muller, J. B. A., Percival, C. J., Oram, D., Forster, G., Lee, J. D., Rickard, A. R., Parrington, M., and Palmer, P. I.: Size-dependent wet removal of black carbon in Canadian biomass burning plumes, Atmos. Chem. Phys., 14, 13755–13771, https://doi.org/10.5194/acp-14-13755-2014, 2014.
Textor, C., Schulz, M., Guibert, S., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Feichter, H., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Horowitz, L., Huang, P., Isaksen, I., Iversen, I., Kloster, S., Koch, D., Kirkevåg, A., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Liu, X., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, Ø., Stier, P., Takemura, T., and Tie, X.: Analysis and quantification of the diversities of aerosol life cycles within AeroCom, Atmos. Chem. Phys., 6, 1777–1813, https://doi.org/10.5194/acp-6-1777-2006, 2006.
Wang, Q., Jacob, D. J., Fisher, J. A., Mao, J., Leibensperger, E. M., Carouge, C. C., Le Sager, P., Kondo, Y., Jimenez, J. L., Cubison, M. J., and Doherty, S. J.: Sources of carbonaceous aerosols and deposited black carbon in the Arctic in winter-spring: implications for radiative forcing, Atmos. Chem. Phys., 11, 12453–12473, https://doi.org/10.5194/acp-11-12453-2011, 2011.
Wang, Q., Jacob, D. J., Spackman, J. R., Perring, A. E., Schwarz, J. P., Moteki, N., Marais, E. A., Ge, C., Wang, J., and Barrett, S. R. H.: Global budget and radiative forcing of black carbon aerosol: Constraints from pole-to-pole (HIPPO) observations across the Pacific, J. Geophys. Res.-Atmos., 119, 195–206, https://doi.org/10.1002/2013JD020824, 2014
Wang, X., Heald, C. L., Ridley, D. A., Schwarz, J. P., Spackman, J. R., Perring, A. E., Coe, H., Liu, D., and Clarke, A. D.: Exploiting simultaneous observational constraints on mass and absorption to estimate the global direct radiative forcing of black carbon and brown carbon, Atmos. Chem. Phys., 14, 10989–11010, https://doi.org/10.5194/acp-14-10989-2014, 2014.
Wang, X., Doherty, S. J., and Huang, J. P.: Black carbon and other light-absorbing impurities in snow across Northern China, J. Geophys. Res.-Atmos., 118, 1471–1492, https://doi.org/10.1029/2012jd018291, 2013.
Wang, X., Xu, B. Q., and Ming, J.: An Overview of the Studies on Black Carbon and Mineral Dust Deposition in Snow and Ice Cores in East Asia, Journal of Meteorological Research, 28, 354–370, https://doi.org/10.1007/S13351-014-4005-7, 2014.
Wang, Z. W., Gallet, J. C., Pedersen, C. A., Zhang, X. S., Ström, J., and Ci, Z. J.: Elemental carbon in snow at Changbai Mountain, northeastern China: concentrations, scavenging ratios, and dry deposition velocities, Atmos. Chem. Phys., 14, 629–640, https://doi.org/10.5194/acp-14-629-2014, 2014.
Wegener, A.: Thermodynamik der Atmosphäre, J. A. Barth, Leipzig, 331 pp., 1911.
Weingartner, E., Burtscher, H., and Baltensperger, U.: Hygroscopic properties of carbon and diesel soot particles, Atmos. Environ., 31, 2311–2327, https://doi.org/10.1016/S1352-2310(97)00023-X, 1997.
Wesely, M. L.: Parameterization of Surface Resistances to Gaseous Dry Deposition in Regional-Scale Numerical-Models, Atmos. Environ., 23, 1293–1304, https://doi.org/10.1016/0004-6981(89)90153-4, 1989.
Wyslouzil, B. E., Carleton, K. L., Sonnenfroh, D. M., Rawlins, W. T., and Arnold, S.: Observation of hydration of single, modified carbon aerosols, Geophys. Res. Lett., 21, 2107–2110, https://doi.org/10.1029/94GL01588, 1994.
Ye, H., Zhang, R. D., Shi, J. S., Huang, J. P., Warren, S. G., and Fu, Q.: Black carbon in seasonal snow across northern Xinjiang in northwestern China, Environ. Res. Lett., 7, 044002, https://doi.org/10.1088/1748-9326/7/4/044002, 2012.
Zhang, D., Wang, Z., and Liu, D.: A global view of midlevel liquid-layer topped stratiform cloud distribution and phase partition from CALIPSO and CloudSat measurements, J. Geophys. Res., 115, D00H13, https://doi.org/10.1029/2009jd012143, 2010.
Zhang, L. M., Gong, S. L., Padro, J., and Barrie, L.: A size-segregated particle dry deposition scheme for an atmospheric aerosol module, Atmos. Environ., 35, 549–560, https://doi.org/10.1016/S1352-2310(00)00326-5, 2001.
Zhang, Q., Streets, D. G., Carmichael, G. R., He, K. B., Huo, H., Kannari, A., Klimont, Z., Park, I. S., Reddy, S., Fu, J. S., Chen, D., Duan, L., Lei, Y., Wang, L. T., and Yao, Z. L.: Asian emissions in 2006 for the NASA INTEX-B mission, Atmos. Chem. Phys., 9, 5131–5153, https://doi.org/10.5194/acp-9-5131-2009, 2009.
Zhang, R., Khalizov, A. F., Pagels, J., Zhang, D., Xue, H., and McMurry, P. H.: Variability in morphology, hygroscopicity, and optical properties of soot aerosols during atmospheric processing, P. Natl. Acad. Sci. USA, 105, 10291–10296, https://doi.org/10.1073/pnas.0804860105, 2008.
Zhang, R., Hegg, D. A., Huang, J., and Fu, Q.: Source attribution of insoluble light-absorbing particles in seasonal snow across northern China, Atmos. Chem. Phys., 13, 6091–6099, https://doi.org/10.5194/acp-13-6091-2013, 2013.
Zhang, X. Y., Wang, Y. Q., Zhang, X. C., Guo, W., and Gong, S. L.: Carbonaceous aerosol composition over various regions of China during 2006, J. Geophys. Res.-Atmos., 113, D14111, https://doi.org/10.1029/2007jd009525, 2008.
Short summary
Black carbon (BC) is the second only to CO2 in heating the planet, but the simulation of BC is associated with large uncertainties. BC burden is largely underestimated over land and overestimated over ocean. Our study finds that a missing process in current Wegener–Bergeron–Findeisen models largely explains the discrepancy in BC simulation over land. We call for more observations of BC in mixed-phase clouds to understand this process and improve the simulation of global BC.
Black carbon (BC) is the second only to CO2 in heating the planet, but the simulation of BC is...
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