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Volume 17, issue 11
Atmos. Chem. Phys., 17, 6631–6650, 2017
https://doi.org/10.5194/acp-17-6631-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 6631–6650, 2017
https://doi.org/10.5194/acp-17-6631-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 06 Jun 2017

Research article | 06 Jun 2017

Investigation of the β-pinene photooxidation by OH in the atmosphere simulation chamber SAPHIR

Martin Kaminski et al.

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Cited articles

Arey, J., Atkinson, R., and Aschmann, S. M.: Product study of the gas-phase reactions of monoterpenes with the OH radical in the presence of NOx, J. Geophys. Res.-Atmos., 95, 18539–18546, https://doi.org/10.1029/JD095iD11p18539, 1990.
Atkinson, R.: Atmospheric chemistry of VOCs and NOx, Atmos. Environ., 34, 2063–2101, https://doi.org/10.1016/s1352-2310(99)00460-4, 2000.
Atkinson, R. and Arey, J.: Gas-phase tropospheric chemistry of biogenic volatile organic compounds: a review, Atmos. Environ., 37, Supplement 2, 197–219, https://doi.org/10.1016/s1352-2310(03)00391-1, 2003.
Bates, K. H., Crounse, J. D., St Clair, J. M., Bennett, N. B., Nguyen, T. B., Seinfeld, J. H., Stoltz, B. M., and Wennberg, P. O.: Gas Phase Production and Loss of Isoprene Epoxydiols, J. Phys. Chem. A, 118, 1237–1246, https://doi.org/10.1021/jp4107958, 2014.
Bohn, B. and Zilken, H.: Model-aided radiometric determination of photolysis frequencies in a sunlit atmosphere simulation chamber, Atmos. Chem. Phys., 5, 191–206, https://doi.org/10.5194/acp-5-191-2005, 2005.
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Short summary
Monoterpenes emitted by trees are among the volatile organic compounds with the highest global emission rates. The atmospheric degradation of the monoterpene β-pinene was investigated in the atmosphere simulation chamber SAPHIR in Jülich under low NOx and atmospheric β-pinene concentrations. While the budget of OH was balanced, both OH and HO2 concentrations were underestimated in the simulation results. These observations suggest the existence of unaccounted sources of HO2.
Monoterpenes emitted by trees are among the volatile organic compounds with the highest global...
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