Ozonolysis of <i>α</i>-phellandrene – Part 1: Gas- and particle-phase characterisation

Mackenzie-Rae, Felix A.; Liu, Tengyu; Deng, Wei; Saunders, Sandra M.; Fang, Zheng; Zhang, Yanli; Wang, Xinming

doi:https://doi.org/10.5194/acp-17-6583-2017

Articles | Volume 17, issue 11

https://doi.org/10.5194/acp-17-6583-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

https://doi.org/10.5194/acp-17-6583-2017

© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Articles | Volume 17, issue 11

Research article

|

06 Jun 2017

Research article |

| 06 Jun 2017

Ozonolysis of α-phellandrene – Part 1: Gas- and particle-phase characterisation

Felix A. Mackenzie-Rae, Tengyu Liu, Wei Deng, Sandra M. Saunders, Zheng Fang, Yanli Zhang, and Xinming Wang

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Final revised paper (published on 06 Jun 2017)
Supplement to the final revised paper
Preprint (discussion started on 10 Jan 2017)
Supplement to the preprint

Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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RC1: 'Review of “Ozonolysis of a-phellandrene, Part 1: Gas- and particle-phase characterisation" by F. A. Mackenzie-Rae et al.', Anonymous Referee #1, 28 Feb 2017
RC2: 'Products of Reaction of a-Phellandrene with Ozone', Anonymous Referee #2, 31 Mar 2017
AC1: 'Response to Reviewers', Felix Mackenzie-Rae, 18 Apr 2017

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Anna Wenzel on behalf of the Authors (18 Apr 2017) Author's response

ED: Referee Nomination & Report Request started (18 Apr 2017) by Markus Petters

ED: Publish as is (01 May 2017) by Markus Petters

Short summary

The atmospheric decomposition of the biogenic α-phellandrene with ozone is characterised by conducting carefully controlled experiments in a smog chamber. Major gas-phase products are identified based on theoretical/mechanism insight, with yields quantified. Meanwhile, a significant amount of aerosol is formed and characterised, with Criegee intermediates found to be important for new particle formation. It is concluded that α-phellandrene contributes to aerosol formation/growth where emitted.