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Volume 17, issue 23
Atmos. Chem. Phys., 17, 14645–14660, 2017
https://doi.org/10.5194/acp-17-14645-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: CHemistry and AeRosols Mediterranean EXperiments (ChArMEx)...

Atmos. Chem. Phys., 17, 14645–14660, 2017
https://doi.org/10.5194/acp-17-14645-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 08 Dec 2017

Research article | 08 Dec 2017

Primary marine aerosol physical flux and chemical composition during a nutrient enrichment experiment in mesocosms in the Mediterranean Sea

Allison N. Schwier et al.

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Albert, M. F. M. A., Schaap, M., Manders, A. M. M., Scannell, C., O'Dowd, C. D., and de Leeuw, G.: Uncertainties in the determination of global sub-micron marine organic matter emissions, Atmos. Environ., 57, 289–300, 2012.
Asmi, E., Freney, E., Hervo, M., Picard, D., Rose, C., Colomb, A., and Sellegri, K.: Aerosol cloud activation in summer and winter at puy-de-Dôme high altitude site in France, Atmos. Chem. Phys., 12, 11589–11607, https://doi.org/10.5194/acp-12-11589-2012, 2012.
Aymoz, G., Jaffrezo, J. L., Chapuis, D., Cozic, J., and Maenhaut, W.: Seasonal variation of PM10 main constituents in two valleys of the French Alps. I: EC/OC fractions, Atmos. Chem. Phys., 7, 661–675, https://doi.org/10.5194/acp-7-661-2007, 2007.
Bardouki, H., Liakakou, H., , Economou, C., Sciare, J., Smolikık, J., Zdımal, V., Eleftheriadis, K., Lazaridis, M., Dye, C., and Mihalopoulos, N.: Chemical composition of size-resolved atmospheric aerosols in the eastern Mediterranean during summer and winter, Atmos. Environ., 37, 195–208, https://doi.org/10.1016/S1352-2310(02)00859-2, 2003.
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In the present paper, we quantify sea-to-air emission fluxes of aerosol to the atmosphere and characterize their physical and chemical properties as a function of the seawater biochemical and physical properties. Fluxes are evaluated with an original approach, a "lab in the field" experiment that preserves the seawater and atmospheric complexity while isolating air-to-sea exchanges from their surroundings. We show different features of the aerosol emission fluxes compared to previous findings.
In the present paper, we quantify sea-to-air emission fluxes of aerosol to the atmosphere and...
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