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Volume 17, issue 2 | Copyright
Atmos. Chem. Phys., 17, 1453-1469, 2017
https://doi.org/10.5194/acp-17-1453-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 31 Jan 2017

Research article | 31 Jan 2017

Real-time detection of highly oxidized organosulfates and BSOA marker compounds during the F-BEACh 2014 field study

Martin Brüggemann et al.
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Baltensperger, U., Dommen, J., Alfarra, R.R., Duplissy, J., Gaeggeler, K., Metzger, A., Facchini, M. C.., Decesari, S., Finessi, E., Reinnig, C., Schott, M., Warnke, J., Hoffmann, T., Klatzer, B., Puxbaum, H., Geiser, M., Savi, M., Lang, D., Kalberer, M., and Geiser, T.: Combined Determination of the Chemical Composition and of Health Effects of Secondary Organic Aerosols: The POLYSOA Project, J. Aerosol Med. Pulm. Drug. Deliv., 21, 145–154, https://doi.org/10.1089/jamp.2007.0655, 2008.
Beck, M. and Hoffmann, T.: A detailed MSn study for the molecular identification of a dimer formed from oxidation of pinene, Atmos. Environ., 130, 120–126, https://doi.org/10.1016/j.atmosenv.2015.09.012, 2016.
Berndt, T., Jokinen, T., Sipilä, M., Mauldin, R. L., Herrmann, H., Stratmann, F., Junninen, H., and Kulmala, M.: H2SO4 formation from the gas-phase reaction of stabilized Criegee Intermediates with SO2: Influence of water vapour content and temperature, Atmos. Environ., 89, 603–612, https://doi.org/10.1016/j.atmosenv.2014.02.062, 2014.
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Using complementary mass spectrometric techniques during a field study in central Europe, characteristic contributors to the organic aerosol mass were identified. Besides common marker compounds for biogenic secondary organic aerosol, highly oxidized sulfur species were detected in the particle phase. High-time-resolution measurements revealed correlations between these organosulfates and particulate sulfate as well as gas-phase peroxyradicals, giving hints to underlying formation mechanisms.
Using complementary mass spectrometric techniques during a field study in central Europe,...
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