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Volume 17, issue 22 | Copyright

Special issue: Regional transport and transformation of air pollution in...

Atmos. Chem. Phys., 17, 13891-13901, 2017
https://doi.org/10.5194/acp-17-13891-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 22 Nov 2017

Research article | 22 Nov 2017

Insight into the in-cloud formation of oxalate based on in situ measurement by single particle mass spectrometry

Guohua Zhang et al.
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Cited articles
Bi, X. H., Zhang, G. H., Li, L., Wang, X. M., Li, M., Sheng, G. Y., Fu, J. M., and Zhou, Z.: Mixing state of biomass burning particles by single particle aerosol mass spectrometer in the urban area of PRD, China, Atmos. Environ., 45, 3447–3453, https://doi.org/10.1016/j.atmosenv.2011.03.034, 2011.
Bi, X. H., Lin, Q. H., Peng, L., Zhang, G. H., Wang, X. M., Brechtel, F. J., Chen, D. H., Li, M., Peng, P. A., Sheng, G. Y., and Zhou, Z.: In situ detection of the chemistry of individual fog droplet residues in the Pearl River Delta region, China, J. Geophys. Res.-Atmos., 121, 9105–9116, https://doi.org/10.1002/2016JD024886, 2016.
Carlton, A. G., Turpin, B. J., Lim, H. J., Altieri, K. E., and Seitzinger, S.: Link between isoprene and secondary organic aerosol (SOA): Pyruvic acid oxidation yields low volatility organic acids in clouds, Geophys. Res. Lett., 33, L06822, https://doi.org/10.1029/2005gl025374, 2006.
Carlton, A. G., Turpin, B. J., Altieri, K. E., Seitzinger, S., Reff, A., Lim, H. J., and Ervens, B.: Atmospheric oxalic acid and SOA production from glyoxal: Results of aqueous photooxidation experiments, Atmos. Environ., 41, 7588–7602, https://doi.org/10.1016/j.atmosenv.2007.05.035, 2007.
Cheng, C., Li, M., Chan, C. K., Tong, H., Chen, C., Chen, D., Wu, D., Li, L., Wu, C., Cheng, P., Gao, W., Huang, Z., Li, X., Zhang, Z., Fu, Z., Bi, Y., and Zhou, Z.: Mixing state of oxalic acid containing particles in the rural area of Pearl River Delta, China: implications for the formation mechanism of oxalic acid, Atmos. Chem. Phys., 17, 9519–9533, https://doi.org/10.5194/acp-17-9519-2017, 2017.
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We first reported the size-resolved mixing state of oxalate in the cloud droplet residual, the cloud interstitial, and cloud-free particles by single particle mass spectrometry. Individual particle analysis provides unique insight into the formation and evolution of oxalate during in-cloud processing. The data show that in-cloud aqueous reactions dramatically improved the formation of oxalate from organic acids that were strongly associated with the aged biomass burning particles.
We first reported the size-resolved mixing state of oxalate in the cloud droplet residual, the...
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