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Volume 17, issue 22 | Copyright
Atmos. Chem. Phys., 17, 13819-13831, 2017
https://doi.org/10.5194/acp-17-13819-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 20 Nov 2017

Research article | 20 Nov 2017

The role of highly oxygenated molecules (HOMs) in determining the composition of ambient ions in the boreal forest

Federico Bianchi et al.
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Cited articles
Arnold, F.: Atmospheric ions and aerosol formation, Space Sci. Rev., 137, 225–239, 2008.
Berndt, T., Richters, S., Jokinen, T., Hyttinen, N., Kurten, T., Otkjaer, R. V., Kjaergaard, H. G., Stratmann, F., Herrmann, H., Sipila, M., Kulmala, M., and Ehn, M.: Hydroxyl radical-induced formation of highly oxidized organic compounds, Nat. Commun., 7, 8, https://doi.org/10.1038/ncomms13677, 2016.
Bianchi, F., Dommen, J., Mathot, S., and Baltensperger, U.: On-line determination of ammonia at low pptv mixing ratios in the CLOUD chamber, Atmos. Meas. Tech., 5, 1719–1725, https://doi.org/10.5194/amt-5-1719-2012, 2012.
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Naturally charged highly oxidised molecules (HOMs) were characterized using advanced mass spectrometers. Two different classes of compounds, clustered with the nitrate and bisulfate ions, were identified: HOMs containing only carbon, hydrogen and oxygen and nitrogen-containing HOMs or organonitrates (ONs). They exhibit strong diurnal variations where HOMs peak during night and ONs during day. Finally, large clusters containing up to 40 carbon atoms (four oxidized α-pinene units) were observed.
Naturally charged highly oxidised molecules (HOMs) were characterized using advanced mass...
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