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Volume 17, issue 21 | Copyright

Special issue: Pan-Eurasian Experiment (PEEX)

Atmos. Chem. Phys., 17, 13361-13371, 2017
https://doi.org/10.5194/acp-17-13361-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 10 Nov 2017

Research article | 10 Nov 2017

Estimation of atmospheric particle formation rates through an analytical formula: validation and application in Hyytiälä and Puijo, Finland

Elham Baranizadeh1, Tuomo Nieminen1, Taina Yli-Juuti1, Markku Kulmala2, Tuukka Petäjä2, Ari Leskinen1,3, Mika Komppula3, Ari Laaksonen1,4, and Kari E. J. Lehtinen1,3 Elham Baranizadeh et al.
  • 1Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
  • 2Department of Physics, University of Helsinki, Helsinki, Finland
  • 3Finnish Meteorological Institute, Kuopio, Finland
  • 4Climate research Unit, Finnish Meteorological Institute, Helsinki, Finland

Abstract. The formation rates of 3nm particles were estimated at SMEAR IV, Puijo (Finland), where the continuous measurements extend only down to 7nm in diameter. We extrapolated the formation rates at 7nm (J7) down to 3nm (J3) based on an approximate solution to the aerosol general dynamic equation, assuming a constant condensational growth rate, a power-law size-dependent scavenging rate, and negligible self-coagulation rate for the nucleation mode particles. To evaluate our method, we first applied it to new particle formation (NPF) events in Hyytiälä (Finland), which extend down to 3nm, and, therefore, J3 and J7 can be determined directly from the measured size distribution evolution. The Hyytiälä results show that the estimated daily mean J3 values slightly overestimate the observed mean J3, but a promising 91% of the estimated J3 values are within a factor of 2 from the measured ones. However, when considering detailed daily time evolution, the agreement is not as good due to fluctuations in data as well as uncertainties in estimated growth rates, which are required in order to calculate the time lag between formation of 3 and 7nm particles. At Puijo, the mean J7 for clear NPF days during April 2007–December 2015 was 0.44cm−3s−1, while the extrapolated mean J3 was 0.61cm−3s−1.

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Extrapolation of the particle formation rates from one measured larger size (e.g., 7 nm) to smaller sizes (e.g., 3 nm) based on simplified growth-scavenging dynamics works fairly well to estimate mean daily formation rates, but it fails to predict the time evolution of the particle population. This points to the challenges in predicting atmospheric nucleation rates for locations where the particle growth and loss rates are size- and time-dependent.
Extrapolation of the particle formation rates from one measured larger size (e.g., 7 nm) to...
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