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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 17, 13049-13070, 2017
https://doi.org/10.5194/acp-17-13049-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
06 Nov 2017
In situ measurements of cloud microphysics and aerosol over coastal Antarctica during the MAC campaign
Sebastian J. O'Shea1, Thomas W. Choularton1, Michael Flynn1, Keith N. Bower1, Martin Gallagher1, Jonathan Crosier1,2, Paul Williams1,2, Ian Crawford1, Zoë L. Fleming3, Constantino Listowski4,a, Amélie Kirchgaessner4, Russell S. Ladkin4, and Thomas Lachlan-Cope4 1School of Earth and Environmental Sciences, University of Manchester, Oxford Road, Manchester, UK
2National Centre for Atmospheric Science, University of Manchester, Oxford Road, Manchester, UK
3National Centre for Atmospheric Science, Department of Chemistry, University of Leicester, Leicester, UK
4British Antarctic Survey, NERC, High Cross, Madingley Rd, Cambridge, UK
anow at: LATMOS/IPSL, UVSQ Université Paris-Saclay, UPMC Univ. Paris 06, CNRS, Guyancourt, France
Abstract. During austral summer 2015, the Microphysics of Antarctic Clouds (MAC) field campaign collected unique and detailed airborne and ground-based in situ measurements of cloud and aerosol properties over coastal Antarctica and the Weddell Sea. This paper presents the first results from the experiment and discusses the key processes important in this region, which is critical to predicting future climate change.

The sampling was predominantly of stratus clouds, at temperatures between −20 and 0 °C. These clouds were dominated by supercooled liquid water droplets, which had a median concentration of 113 cm−3 and an interquartile range of 86 cm−3. Both cloud liquid water content and effective radius increased closer to cloud top. The cloud droplet effective radius increased from 4 ± 2 µm near cloud base to 8 ± 3 µm near cloud top.

Cloud ice particle concentrations were highly variable with the ice tending to occur in small, isolated patches. Below approximately 1000 m, glaciated cloud regions were more common at higher temperatures; however, the clouds were still predominantly liquid throughout. When ice was present at temperatures higher than −10 °C, secondary ice production most likely through the Hallett–Mossop mechanism led to ice concentrations 1 to 3 orders of magnitude higher than the number predicted by commonly used primary ice nucleation parameterisations. The drivers of the ice crystal variability are investigated. No clear dependence on the droplet size distribution was found. The source of first ice in the clouds remains uncertain but may include contributions from biogenic particles, blowing snow or other surface ice production mechanisms.

The concentration of large aerosols (diameters 0.5 to 1.6 µm) decreased with altitude and were depleted in air masses that originated over the Antarctic continent compared to those more heavily influenced by the Southern Ocean and sea ice regions. The dominant aerosol in the region was hygroscopic in nature, with the hygroscopicity parameter κ having a median value for the campaign of 0.66 (interquartile range of 0.38). This is consistent with other remote marine locations that are dominated by sea salt/sulfate.


Citation: O'Shea, S. J., Choularton, T. W., Flynn, M., Bower, K. N., Gallagher, M., Crosier, J., Williams, P., Crawford, I., Fleming, Z. L., Listowski, C., Kirchgaessner, A., Ladkin, R. S., and Lachlan-Cope, T.: In situ measurements of cloud microphysics and aerosol over coastal Antarctica during the MAC campaign, Atmos. Chem. Phys., 17, 13049-13070, https://doi.org/10.5194/acp-17-13049-2017, 2017.
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Short summary
Few direct measurements have been made of Antarctic cloud and aerosol properties. As part of the 2015 Microphysics of Antarctic Clouds (MAC) field campaign, detailed airborne and ground-based measurements were made over the Weddell Sea and Antarctic coastal continent. This paper presents the first results from this campaign and discusses the cloud properties and processes important in this region.
Few direct measurements have been made of Antarctic cloud and aerosol properties. As part of the...
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