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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 17, issue 2 | Copyright
Atmos. Chem. Phys., 17, 1297-1311, 2017
https://doi.org/10.5194/acp-17-1297-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 27 Jan 2017

Research article | 27 Jan 2017

Influence of enhanced Asian NOx emissions on ozone in the upper troposphere and lower stratosphere in chemistry–climate model simulations

Chaitri Roy1, Suvarna Fadnavis1, Rolf Müller2, D. C. Ayantika1, Felix Ploeger2, and Alexandru Rap3 Chaitri Roy et al.
  • 1Indian Institute of Tropical Meteorology, Pune, India
  • 2Forschungszentrum Jülich GmbH, IEK7, Jülich, Germany
  • 3School of Earth and Environment, University of Leeds, Leeds, UK

Abstract. The Asian summer monsoon (ASM) anticyclone is the most pronounced circulation pattern in the upper troposphere and lower stratosphere (UTLS) during northern hemispheric summer. ASM convection plays an important role in efficient vertical transport from the surface to the upper-level anticyclone. In this paper we investigate the potential impact of enhanced anthropogenic nitrogen oxide (NOx) emissions on the distribution of ozone in the UTLS using the fully coupled aerosol–chemistry–climate model, ECHAM5-HAMMOZ. Ozone in the UTLS is influenced both by the convective uplift of ozone precursors and by the uplift of enhanced-NOx-induced tropospheric ozone anomalies. We performed anthropogenic NOx emission sensitivity experiments over India and China. In these simulations, covering the years 2000–2010, anthropogenic NOx emissions have been increased by 38% over India and by 73% over China with respect to the emission base year 2000. These emission increases are comparable to the observed linear trends of 3.8% per year over India and 7.3% per year over China during the period 2000 to 2010. Enhanced NOx emissions over India by 38% and China by 73% increase the ozone radiative forcing in the ASM anticyclone (15–40°N, 60–120°E) by 16.3 and 78.5mWm−2 respectively. These elevated NOx emissions produce significant warming over the Tibetan Plateau and increase precipitation over India due to a strengthening of the monsoon Hadley circulation. However, increase in NOx emissions over India by 73% (similar to the observed increase over China) results in large ozone production over the Indo-Gangetic Plain and Tibetan Plateau. The higher ozone concentrations, in turn, induce a reversed monsoon Hadley circulation and negative precipitation anomalies over India. The associated subsidence suppresses vertical transport of NOx and ozone into the ASM anticyclone.

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Short summary
In the monsoon season, Asian NOx emissions are rapidly transported to the UTLS and can impact ozone in the UTLS. From chemistry–climate model simulations, we show that increasing Asian NOx emissions have enhanced ozone radiative forcing over Southeast Asia, which leads to significant warming over the Tibetan Plateau and increase precipitation over India. However, a further increase in NOx emissions elicited negative precipitation due to reversal of monsoon Hadley circulation.
In the monsoon season, Asian NOx emissions are rapidly transported to the UTLS and can impact...
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