Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 17, 12827-12843, 2017
https://doi.org/10.5194/acp-17-12827-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
27 Oct 2017
Adverse effects of increasing drought on air quality via natural processes
Yuxuan Wang1,2,*, Yuanyu Xie1,*, Wenhao Dong1, Yi Ming3, Jun Wang4, and Lu Shen5 1Department of Earth System Sciences, Tsinghua University, Beijing, China
2Department of Earth and Atmospheric Sciences, University of Houston, Houston, TX, USA
3NOAA/Geophysical Fluid Dynamics Laboratory, Princeton, NJ, USA
4Center for Global and Regional Environmental Research & Dept. of Chemical and Biochemical Engineering & Interdisciplinary Graduate Program in GeoInformatics, University of Iowa, Iowa City, IA, USA
5School of Engineering and Applied Science, Harvard University, Cambridge, MA, USA
*These authors contributed equally to this work.
Abstract. Drought is a recurring extreme of the climate system with well-documented impacts on agriculture and water resources. The strong perturbation of drought to the land biosphere and atmospheric water cycle will affect atmospheric composition, the nature and extent of which are not well understood. Here we present observational evidence that US air quality is significantly correlated with drought severity. Severe droughts during the period of 1990–2014 were found associated with growth-season (March–October) mean enhancements in surface ozone and PM2.5 of 3.5 ppbv (8 %) and 1.6 µg m−3 (17 %), respectively. The pollutant enhancements associated with droughts do not appear to be affected by the decreasing trend of US anthropogenic emissions, indicating natural processes as the primary cause. Elevated ozone and PM2.5 are attributed to the combined effects of drought on deposition, natural emissions (wildfires, biogenic volatile organic compounds (BVOCs), and dust), and chemistry. Most climate–chemistry models are not able to reproduce the observed correlations of ozone and PM2.5 to drought severity. The model deficiencies are partly attributed to the lack of drought-induced changes in land–atmosphere exchanges of reactive gases and particles and misrepresentation of cloud changes under drought conditions. By applying the observed relationships between drought and air pollutants to climate model projected drought occurrences, we estimate an increase of 1–6 % for ground-level O3 and 1–16 % for PM2.5 in the US by 2100 compared to the 2000s due to increasing drought alone. Drought thus poses an important aspect of climate change penalty on air quality, and a better prediction of such effects would require improvements in model processes.

Citation: Wang, Y., Xie, Y., Dong, W., Ming, Y., Wang, J., and Shen, L.: Adverse effects of increasing drought on air quality via natural processes, Atmos. Chem. Phys., 17, 12827-12843, https://doi.org/10.5194/acp-17-12827-2017, 2017.
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Short summary
Besides the well-known large impact on agriculture and water resources, drought is associated with significant adverse effects on air quality. Drought-induced degradation of air quality is largely due to natural processes, offsetting the effort of anthropogenic emission reduction during the past decades. Such adverse impacts should be included in modeling processes under current and future climate for mitigation policy.
Besides the well-known large impact on agriculture and water resources, drought is associated...
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