Articles | Volume 16, issue 14
https://doi.org/10.5194/acp-16-9321-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-9321-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
28 Jul 2016
Research article |
| 28 Jul 2016
Multiple new-particle growth pathways observed at the US DOE Southern Great Plains field site
Anna L. Hodshire
CORRESPONDING AUTHOR
Department of Atmospheric Science, Colorado State University, Fort
Collins, 80523, USA
Michael J. Lawler
Atmospheric Chemistry Observations & Modeling, National Center for
Atmospheric Research, Boulder, 80305, USA
now at: Department of Chemistry, University of California, Irvine,
92697-2025, USA
Department of Mechanical Engineering, University of Minnesota-Twin
Cities, Minneapolis, 55455, USA
now at: School of Atmospheric Sciences, Sun Yat-sen University,
Guangzhou, 510275, China
John Ortega
Atmospheric Chemistry Observations & Modeling, National Center for
Atmospheric Research, Boulder, 80305, USA
Department of Mechanical Engineering, University of Minnesota-Twin
Cities, Minneapolis, 55455, USA
now at: Environmental Science, Policy, and Management, University of
California, Berkeley, 94720-3114, USA
Taina Yli-Juuti
Department of Applied Physics, University of Eastern Finland, Kupio,
70211, Finland
Jared F. Brewer
Department of Atmospheric Science, Colorado State University, Fort
Collins, 80523, USA
Jack K. Kodros
Department of Atmospheric Science, Colorado State University, Fort
Collins, 80523, USA
Kelley C. Barsanti
Department of Civil and Environmental Engineering, Portland State
University, Portland, 97201, USA
now at: Chemical and Environmental Engineering, University of
California, Riverside, 92521, USA
Dave R. Hanson
Department of Chemistry, Augsburg College, Minneapolis, 55454, USA
Peter H. McMurry
Department of Mechanical Engineering, University of Minnesota-Twin
Cities, Minneapolis, 55455, USA
James N. Smith
Department of Chemistry, University of California, Irvine, 92697-2025,
USA
Jeffery R. Pierce
Department of Atmospheric Science, Colorado State University, Fort
Collins, 80523, USA
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Cited
31 citations as recorded by crossref.
- Kinetics and Products of the Aqueous Phase Oxidation of Triethylamine by OH Y. Tao et al. 10.1021/acsearthspacechem.1c00162
- Long- and short-term temporal variability in cloud condensation nuclei spectra over a wide supersaturation range in the Southern Great Plains site R. Perkins et al. 10.5194/acp-22-6197-2022
- The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings A. Hodshire et al. 10.5194/acp-19-3137-2019
- Atmospheric fungal nanoparticle bursts M. Lawler et al. 10.1126/sciadv.aax9051
- Ambient Particulate Matter Size Distributions Drive Regional and Global Variability in Particle Deposition in the Respiratory Tract J. Kodros et al. 10.1029/2018GH000145
- Chemical identification of new particle formation and growth precursors through positive matrix factorization of ambient ion measurements D. Katz et al. 10.5194/acp-23-5567-2023
- New Particle Formation in the Atmosphere: From Molecular Clusters to Global Climate S. Lee et al. 10.1029/2018JD029356
- Organic Condensation and Particle Growth to CCN Sizes in the Summertime Marine Arctic Is Driven by Materials More Semivolatile Than at Continental Sites J. Burkart et al. 10.1002/2017GL075671
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Atmospheric new particle formation and growth: review of field observations V. Kerminen et al. 10.1088/1748-9326/aadf3c
- Revisiting matrix-based inversion of scanning mobility particle sizer (SMPS) and humidified tandem differential mobility analyzer (HTDMA) data M. Petters 10.5194/amt-14-7909-2021
- Limited Role of Malonic Acid in Sulfuric Acid–Dimethylamine New Particle Formation S. Fomete et al. 10.1021/acsomega.3c01643
- Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles C. Peng et al. 10.1016/j.jes.2022.03.006
- Perspective on the Recent Measurements of Reduced Nitrogen Compounds in the Atmosphere S. Lee 10.3389/fenvs.2022.868534
- Earth System Model Aerosol–Cloud Diagnostics (ESMAC Diags) package, version 1: assessing E3SM aerosol predictions using aircraft, ship, and surface measurements S. Tang et al. 10.5194/gmd-15-4055-2022
- Turbulent Flux Measurements of the Near‐Surface and Residual‐Layer Small Particle Events M. Islam et al. 10.1029/2021JD036289
- Quantitation of 11 alkylamines in atmospheric samples: separating structural isomers by ion chromatography B. Place et al. 10.5194/amt-10-1061-2017
- Look Up: Probing the Vertical Profile of New Particle Formation and Growth in the Planetary Boundary Layer With Models and Observations S. O’Donnell et al. 10.1029/2022JD037525
- Estimation of Possible Primary Biological Particle Emissions and Rupture Events at the Southern Great Plains ARM Site T. Subba et al. 10.1029/2021JD034679
- Examining the vertical heterogeneity of aerosols over the Southern Great Plains Y. Wang et al. 10.5194/acp-23-15671-2023
- Vertically resolved concentration and liquid water content of atmospheric nanoparticles at the US DOE Southern Great Plains site H. Chen et al. 10.5194/acp-18-311-2018
- Quantifying aerosol size distributions and their temporal variability in the Southern Great Plains, USA P. Marinescu et al. 10.5194/acp-19-11985-2019
- The importance of ammonia for springtime atmospheric new particle formation and aerosol number abundance over the United States A. Nair et al. 10.1016/j.scitotenv.2022.160756
- What chemical species are responsible for new particle formation and growth in the Netherlands? A hybrid positive matrix factorization (PMF) analysis using aerosol composition (ACSM) and size (SMPS) F. Nursanto et al. 10.5194/acp-23-10015-2023
- Changes in the new particle formation and shrinkage events of the atmospheric ions during the COVID-19 lockdown A. Kamra et al. 10.1016/j.uclim.2022.101214
- Errors in nanoparticle growth rates inferred from measurements in chemically reacting aerosol systems C. Li & P. McMurry 10.5194/acp-18-8979-2018
- Comprehensive simulations of new particle formation events in Beijing with a cluster dynamics–multicomponent sectional model C. Li et al. 10.5194/acp-23-6879-2023
- Study of new particle formation events in southern Italy A. Dinoi et al. 10.1016/j.atmosenv.2020.117920
- Temperature-Dependent Diffusion of H2SO4 in Air at Atmospherically Relevant Conditions: Laboratory Measurements Using Laminar Flow Technique D. Brus et al. 10.3390/atmos8070132
- Overview of the HI-SCALE Field Campaign: A New Perspective on Shallow Convective Clouds J. Fast et al. 10.1175/BAMS-D-18-0030.1
- The acidity of atmospheric particles and clouds H. Pye et al. 10.5194/acp-20-4809-2020
31 citations as recorded by crossref.
- Kinetics and Products of the Aqueous Phase Oxidation of Triethylamine by OH Y. Tao et al. 10.1021/acsearthspacechem.1c00162
- Long- and short-term temporal variability in cloud condensation nuclei spectra over a wide supersaturation range in the Southern Great Plains site R. Perkins et al. 10.5194/acp-22-6197-2022
- The potential role of methanesulfonic acid (MSA) in aerosol formation and growth and the associated radiative forcings A. Hodshire et al. 10.5194/acp-19-3137-2019
- Atmospheric fungal nanoparticle bursts M. Lawler et al. 10.1126/sciadv.aax9051
- Ambient Particulate Matter Size Distributions Drive Regional and Global Variability in Particle Deposition in the Respiratory Tract J. Kodros et al. 10.1029/2018GH000145
- Chemical identification of new particle formation and growth precursors through positive matrix factorization of ambient ion measurements D. Katz et al. 10.5194/acp-23-5567-2023
- New Particle Formation in the Atmosphere: From Molecular Clusters to Global Climate S. Lee et al. 10.1029/2018JD029356
- Organic Condensation and Particle Growth to CCN Sizes in the Summertime Marine Arctic Is Driven by Materials More Semivolatile Than at Continental Sites J. Burkart et al. 10.1002/2017GL075671
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Atmospheric new particle formation and growth: review of field observations V. Kerminen et al. 10.1088/1748-9326/aadf3c
- Revisiting matrix-based inversion of scanning mobility particle sizer (SMPS) and humidified tandem differential mobility analyzer (HTDMA) data M. Petters 10.5194/amt-14-7909-2021
- Limited Role of Malonic Acid in Sulfuric Acid–Dimethylamine New Particle Formation S. Fomete et al. 10.1021/acsomega.3c01643
- Measurement of atmospheric nanoparticles: Bridging the gap between gas-phase molecules and larger particles C. Peng et al. 10.1016/j.jes.2022.03.006
- Perspective on the Recent Measurements of Reduced Nitrogen Compounds in the Atmosphere S. Lee 10.3389/fenvs.2022.868534
- Earth System Model Aerosol–Cloud Diagnostics (ESMAC Diags) package, version 1: assessing E3SM aerosol predictions using aircraft, ship, and surface measurements S. Tang et al. 10.5194/gmd-15-4055-2022
- Turbulent Flux Measurements of the Near‐Surface and Residual‐Layer Small Particle Events M. Islam et al. 10.1029/2021JD036289
- Quantitation of 11 alkylamines in atmospheric samples: separating structural isomers by ion chromatography B. Place et al. 10.5194/amt-10-1061-2017
- Look Up: Probing the Vertical Profile of New Particle Formation and Growth in the Planetary Boundary Layer With Models and Observations S. O’Donnell et al. 10.1029/2022JD037525
- Estimation of Possible Primary Biological Particle Emissions and Rupture Events at the Southern Great Plains ARM Site T. Subba et al. 10.1029/2021JD034679
- Examining the vertical heterogeneity of aerosols over the Southern Great Plains Y. Wang et al. 10.5194/acp-23-15671-2023
- Vertically resolved concentration and liquid water content of atmospheric nanoparticles at the US DOE Southern Great Plains site H. Chen et al. 10.5194/acp-18-311-2018
- Quantifying aerosol size distributions and their temporal variability in the Southern Great Plains, USA P. Marinescu et al. 10.5194/acp-19-11985-2019
- The importance of ammonia for springtime atmospheric new particle formation and aerosol number abundance over the United States A. Nair et al. 10.1016/j.scitotenv.2022.160756
- What chemical species are responsible for new particle formation and growth in the Netherlands? A hybrid positive matrix factorization (PMF) analysis using aerosol composition (ACSM) and size (SMPS) F. Nursanto et al. 10.5194/acp-23-10015-2023
- Changes in the new particle formation and shrinkage events of the atmospheric ions during the COVID-19 lockdown A. Kamra et al. 10.1016/j.uclim.2022.101214
- Errors in nanoparticle growth rates inferred from measurements in chemically reacting aerosol systems C. Li & P. McMurry 10.5194/acp-18-8979-2018
- Comprehensive simulations of new particle formation events in Beijing with a cluster dynamics–multicomponent sectional model C. Li et al. 10.5194/acp-23-6879-2023
- Study of new particle formation events in southern Italy A. Dinoi et al. 10.1016/j.atmosenv.2020.117920
- Temperature-Dependent Diffusion of H2SO4 in Air at Atmospherically Relevant Conditions: Laboratory Measurements Using Laminar Flow Technique D. Brus et al. 10.3390/atmos8070132
- Overview of the HI-SCALE Field Campaign: A New Perspective on Shallow Convective Clouds J. Fast et al. 10.1175/BAMS-D-18-0030.1
- The acidity of atmospheric particles and clouds H. Pye et al. 10.5194/acp-20-4809-2020
Saved (preprint)
Discussed (final revised paper)
Latest update: 18 Apr 2024
Short summary
Processes that control the growth of newly formed particles are not well understood and limit predictions of aerosol climate impacts. We combine state-of-the-art measurements at a central-US site with a particle-growth model to investigate the species and processes contributing to growth. Observed growth was dominated by organics, sulfate salts, or a mixture of these two. The model qualitatively captures the variability between different days.
Processes that control the growth of newly formed particles are not well understood and limit...
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