Articles | Volume 16, issue 11
https://doi.org/10.5194/acp-16-7067-2016
https://doi.org/10.5194/acp-16-7067-2016
Research article
 | 
10 Jun 2016
Research article |  | 10 Jun 2016

Using a combined power law and log-normal distribution model to simulate particle formation and growth in a mobile aerosol chamber

Miska Olin, Tatu Anttila, and Miikka Dal Maso

Abstract. We present the combined power law and log-normal distribution (PL+LN) model, a computationally efficient model to be used in simulations where the particle size distribution cannot be accurately represented by log-normal distributions, such as in simulations involving the initial steps of aerosol formation, where new particle formation and growth occur simultaneously, or in the case of inverse modeling. The model was evaluated against highly accurate sectional models using input parameter values that reflect conditions typical to particle formation occurring in the atmosphere and in vehicle exhaust. The model was tested in the simulation of a particle formation event performed in a mobile aerosol chamber at Mäkelänkatu street canyon measurement site in Helsinki, Finland. The number, surface area, and mass concentrations in the chamber simulation were conserved with the relative errors lower than 2 % using the PL+LN model, whereas a moment-based log-normal model and sectional models with the same computing time as with the PL+LN model caused relative errors up to 17 and 79 %, respectively.

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Short summary
We introduce a new representation of particle size distribution, in which a power law form is used in addition to the most commonly used log-normal representation. The new representation is beneficial in simulations involving the initial steps of aerosol formation, where power law behaviour is typically seen, instead of less accurate pure log-normal representation or computationally more expensive sectional representation.
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