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Volume 16, issue 9 | Copyright

Special issue: EARLINET aerosol profiling: contributions to atmospheric and...

Special issue: BACCHUS – Impact of Biogenic versus Anthropogenic emissions...

Atmos. Chem. Phys., 16, 5905-5931, 2016
https://doi.org/10.5194/acp-16-5905-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 17 May 2016

Research article | 17 May 2016

Potential of polarization lidar to provide profiles of CCN- and INP-relevant aerosol parameters

Rodanthi-Elisavet Mamouri1,2 and Albert Ansmann3 Rodanthi-Elisavet Mamouri and Albert Ansmann
  • 1Cyprus University of Technology, Dep. of Civil Engineering and Geomatics, Limassol, Cyprus
  • 2National Observatory of Athens, Athens, Greece
  • 3Leibniz Institute for Tropospheric Research, Leipzig, Germany

Abstract. We investigate the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nucleus (CCN) and ice nucleating particle (INP) number concentrations can be estimated. We show that height profiles of particle number concentrations n50, dry considering dry aerosol particles with radius  > 50nm (reservoir of CCN in the case of marine and continental non-desert aerosols), n100, dry (particles with dry radius  > 100nm, reservoir of desert dust CCN), and of n250, dry (particles with dry radius  > 250nm, reservoir of favorable INP), as well as profiles of the particle surface area concentration sdry (used in INP parameterizations) can be retrieved from lidar-derived aerosol extinction coefficients σ with relative uncertainties of a factor of 1.5–2 in the case of n50, dry and n100, dry and of about 25–50% in the case of n250, dry and sdry. Of key importance is the potential of polarization lidar to distinguish and separate the optical properties of desert aerosols from non-desert aerosol such as continental and marine particles. We investigate the relationship between σ, measured at ambient atmospheric conditions, and n50, dry for marine and continental aerosols, n100, dry for desert dust particles, and n250, dry and sdry for three aerosol types (desert, non-desert continental, marine) and for the main lidar wavelengths of 355, 532, and 1064nm. Our study is based on multiyear Aerosol Robotic Network (AERONET) photometer observations of aerosol optical thickness and column-integrated particle size distribution at Leipzig, Germany, and Limassol, Cyprus, which cover all realistic aerosol mixtures. We further include AERONET data from field campaigns in Morocco, Cabo Verde, and Barbados, which provide pure dust and pure marine aerosol scenarios. By means of a simple CCN parameterization (with n50, dry or n100, dry as input) and available INP parameterization schemes (with n250, dry and sdry as input) we finally compute profiles of the CCN-relevant particle number concentration nCCN and the INP number concentration nINP. We apply the method to a lidar observation of a heavy dust outbreak crossing Cyprus and a case dominated by continental aerosol pollution.

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