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Volume 16, issue 2
Atmos. Chem. Phys., 16, 585–596, 2016
https://doi.org/10.5194/acp-16-585-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 585–596, 2016
https://doi.org/10.5194/acp-16-585-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 19 Jan 2016

Research article | 19 Jan 2016

A sub-decadal trend in diacids in atmospheric aerosols in eastern Asia

S. Kundu et al.

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Boreddy, S. K. R. and Kawamura, K.: A 12-year observation of water-soluble ions in TSP aerosols collected at a remote marine location in the western North Pacific: an outflow region of Asian dust, Atmos. Chem. Phys., 15, 6437–6453, https://doi.org/10.5194/acp-15-6437-2015, 2015.
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster, P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S. K., Sherwood, S., Stevens, B., and Zhang, X. Y.: Clouds and Aerosols, in: Climate Change 2013: The Physical Science Basis. Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 595–599, 2013.
Charbouillot, T., Gorini, S., Voyard, G., Parazols, M., Brigante, M., Deguillaume, L., Delort, A.-M., and Mailhot, G.: Mechanism of carboxylic acid photooxidation in atmospheric aqueous phase: Formation, fate and reactivity, Atmos. Environ., 56, 1–8, https://doi.org/10.1016/j.atmosenv.2012.03.079, 2012.
Decesari, S., Fuzzi, S., Facchini, M. C., Mircea, M., Emblico, L., Cavalli, F., Maenhaut, W., Chi, X., Schkolnik, G., Falkovich, A., Rudich, Y., Claeys, M., Pashynska, V., Vas, G., Kourtchev, I., Vermeylen, R., Hoffer, A., Andreae, M. O., Tagliavini, E., Moretti, F., and Artaxo, P.: Characterization of the organic composition of aerosols from Rondônia, Brazil, during the LBA-SMOCC 2002 experiment and its representation through model compounds, Atmos. Chem. Phys., 6, 375–402, https://doi.org/10.5194/acp-6-375-2006, 2006.
Ding, X., Wang, X.-M., Gao, B., Fu, X.-X., He, Q.-F., Zhao, X.-Y., Yu, J.-Z., and Zheng, M.: Tracer-based estimation of secondary organic carbon in the Pearl River Delta, south China, J. Geophys. Res.-Atmos., 117, D05313, https://doi.org/10.1029/2011JD016596, 2012.
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Chemistry-transport models have predicted a change in secondary organic aerosols (SOA) in the future atmosphere with a large uncertainty. This study measures diacids, major water-soluble surrogates of SOA, on a sub-decadal scale in atmospheric aerosols in eastern Asia. Diacids are observed to increase by 3.9–47.4 % per year. The increases in the water-soluble organic acid fraction could modify the aerosol organic composition and its sensitivity to climate-relevant physical properties.
Chemistry-transport models have predicted a change in secondary organic aerosols (SOA) in the...
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