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Volume 16, issue 5
Atmos. Chem. Phys., 16, 3499–3523, 2016
https://doi.org/10.5194/acp-16-3499-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 3499–3523, 2016
https://doi.org/10.5194/acp-16-3499-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 17 Mar 2016

Research article | 17 Mar 2016

Exploring the uncertainty associated with satellite-based estimates of premature mortality due to exposure to fine particulate matter

Bonne Ford1 and Colette L. Heald2 Bonne Ford and Colette L. Heald
  • 1Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
  • 2Department of Civil and Environmental Engineering and Department of Earth, Atmospheric and Planetary Sciences, MIT, Cambridge, MA, USA

Abstract. The negative impacts of fine particulate matter (PM2.5) exposure on human health are a primary motivator for air quality research. However, estimates of the air pollution health burden vary considerably and strongly depend on the data sets and methodology. Satellite observations of aerosol optical depth (AOD) have been widely used to overcome limited coverage from surface monitoring and to assess the global population exposure to PM2.5 and the associated premature mortality. Here we quantify the uncertainty in determining the burden of disease using this approach, discuss different methods and data sets, and explain sources of discrepancies among values in the literature. For this purpose we primarily use the MODIS satellite observations in concert with the GEOS-Chem chemical transport model. We contrast results in the United States and China for the years 2004–2011. Using the Burnett et al. (2014) integrated exposure response function, we estimate that in the United States, exposure to PM2.5 accounts for approximately 2 % of total deaths compared to 14 % in China (using satellite-based exposure), which falls within the range of previous estimates. The difference in estimated mortality burden based solely on a global model vs. that derived from satellite is approximately 14 % for the US and 2 % for China on a nationwide basis, although regionally the differences can be much greater. This difference is overshadowed by the uncertainty in the methodology for deriving PM2.5 burden from satellite observations, which we quantify to be on the order of 20 % due to uncertainties in the AOD-to-surface-PM2.5 relationship, 10 % due to the satellite observational uncertainty, and 30 % or greater uncertainty associated with the application of concentration response functions to estimated exposure.

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As motivation for air quality research, many studies cite the fact that exposure to particulate matter is associated with premature mortality. Recently, more studies have also tried to quantify this burden; however, there are many data sets that can be used and many different methodological choices to be made. In this paper, we seek to explain the different sources of uncertainty in health impact assessments through the example of using model and satellite-based PM2.5 concentrations.
As motivation for air quality research, many studies cite the fact that exposure to particulate...
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