Articles | Volume 16, issue 4
https://doi.org/10.5194/acp-16-1877-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-1877-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
18 Feb 2016
Research article |
| 18 Feb 2016
Mid-21st century air quality at the urban scale under the influence of changed climate and emissions – case studies for Paris and Stockholm
Konstantinos Markakis
CORRESPONDING AUTHOR
Laboratoire de Meteorologie Dynamique, IPSL Laboratoire
CEA/CNRS/UVSQ, Ecole Polytechnique, 91128 Palaiseau CEDEX,
France
Myrto Valari
Laboratoire de Meteorologie Dynamique, IPSL Laboratoire
CEA/CNRS/UVSQ, Ecole Polytechnique, 91128 Palaiseau CEDEX,
France
Magnuz Engardt
Swedish Meteorological and Hydrological Institute,
60176 Norrköping, Sweden
Gwendoline Lacressonniere
Laboratoire des Sciences du Climat et de l'Environnement,
IPSL Laboratoire CEA/CNRS/UVSQ, Orme des Merisiers, 91191 Gif-sur-Yvette
CEDEX, France
Robert Vautard
Laboratoire des Sciences du Climat et de l'Environnement,
IPSL Laboratoire CEA/CNRS/UVSQ, Orme des Merisiers, 91191 Gif-sur-Yvette
CEDEX, France
Camilla Andersson
Swedish Meteorological and Hydrological Institute,
60176 Norrköping, Sweden
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Giancarlo Ciarelli, Mark R. Theobald, Marta G. Vivanco, Matthias Beekmann, Wenche Aas, Camilla Andersson, Robert Bergström, Astrid Manders-Groot, Florian Couvidat, Mihaela Mircea, Svetlana Tsyro, Hilde Fagerli, Kathleen Mar, Valentin Raffort, Yelva Roustan, Maria-Teresa Pay, Martijn Schaap, Richard Kranenburg, Mario Adani, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, Cornelis Cuvelier, Arineh Cholakian, Bertrand Bessagnet, Peter Wind, and Augustin Colette
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Mark R. Theobald, Marta G. Vivanco, Wenche Aas, Camilla Andersson, Giancarlo Ciarelli, Florian Couvidat, Kees Cuvelier, Astrid Manders, Mihaela Mircea, Maria-Teresa Pay, Svetlana Tsyro, Mario Adani, Robert Bergström, Bertrand Bessagnet, Gino Briganti, Andrea Cappelletti, Massimo D'Isidoro, Hilde Fagerli, Kathleen Mar, Noelia Otero, Valentin Raffort, Yelva Roustan, Martijn Schaap, Peter Wind, and Augustin Colette
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Atmos. Chem. Phys., 18, 10199–10218, https://doi.org/10.5194/acp-18-10199-2018, https://doi.org/10.5194/acp-18-10199-2018, 2018
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Erik Kjellström, Grigory Nikulin, Gustav Strandberg, Ole Bøssing Christensen, Daniela Jacob, Klaus Keuler, Geert Lenderink, Erik van Meijgaard, Christoph Schär, Samuel Somot, Silje Lund Sørland, Claas Teichmann, and Robert Vautard
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Didin Agustian Permadi, Nguyen Thi Kim Oanh, and Robert Vautard
Atmos. Chem. Phys., 18, 3321–3334, https://doi.org/10.5194/acp-18-3321-2018, https://doi.org/10.5194/acp-18-3321-2018, 2018
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This research quantified impacts resulted in the future (2030) from emission reduction measures for Southeast Asia (SEA) countries. Emission scenarios were developed based on current policies in Indonesia and Thailand. Impacts were quantified in terms of the avoided number of premature death and reduction in radiative forcing resulted from the emission reduction measures.
Didin Agustian Permadi, Nguyen Thi Kim Oanh, and Robert Vautard
Atmos. Chem. Phys., 18, 2725–2747, https://doi.org/10.5194/acp-18-2725-2018, https://doi.org/10.5194/acp-18-2725-2018, 2018
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Katja Frieler, Stefan Lange, Franziska Piontek, Christopher P. O. Reyer, Jacob Schewe, Lila Warszawski, Fang Zhao, Louise Chini, Sebastien Denvil, Kerry Emanuel, Tobias Geiger, Kate Halladay, George Hurtt, Matthias Mengel, Daisuke Murakami, Sebastian Ostberg, Alexander Popp, Riccardo Riva, Miodrag Stevanovic, Tatsuo Suzuki, Jan Volkholz, Eleanor Burke, Philippe Ciais, Kristie Ebi, Tyler D. Eddy, Joshua Elliott, Eric Galbraith, Simon N. Gosling, Fred Hattermann, Thomas Hickler, Jochen Hinkel, Christian Hof, Veronika Huber, Jonas Jägermeyr, Valentina Krysanova, Rafael Marcé, Hannes Müller Schmied, Ioanna Mouratiadou, Don Pierson, Derek P. Tittensor, Robert Vautard, Michelle van Vliet, Matthias F. Biber, Richard A. Betts, Benjamin Leon Bodirsky, Delphine Deryng, Steve Frolking, Chris D. Jones, Heike K. Lotze, Hermann Lotze-Campen, Ritvik Sahajpal, Kirsten Thonicke, Hanqin Tian, and Yoshiki Yamagata
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Camilla Andersson, Heléne Alpfjord, Lennart Robertson, Per Erik Karlsson, and Magnuz Engardt
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We show that high near-surface O3 concentrations in Sweden are decreasing and low O3 concentrations are increasing during 1990–2013. The cause for the change is a combination of change in hemispheric background, meteorology and anthropogenic emissions. We have identified systematic differences in the modelled trend that must be caused by incorrect trends in the utilized emissions or by too high sensitivity in the model. We based the analysis on fused measurements and modelling.
Augustin Colette, Camilla Andersson, Astrid Manders, Kathleen Mar, Mihaela Mircea, Maria-Teresa Pay, Valentin Raffort, Svetlana Tsyro, Cornelius Cuvelier, Mario Adani, Bertrand Bessagnet, Robert Bergström, Gino Briganti, Tim Butler, Andrea Cappelletti, Florian Couvidat, Massimo D'Isidoro, Thierno Doumbia, Hilde Fagerli, Claire Granier, Chris Heyes, Zig Klimont, Narendra Ojha, Noelia Otero, Martijn Schaap, Katarina Sindelarova, Annemiek I. Stegehuis, Yelva Roustan, Robert Vautard, Erik van Meijgaard, Marta Garcia Vivanco, and Peter Wind
Geosci. Model Dev., 10, 3255–3276, https://doi.org/10.5194/gmd-10-3255-2017, https://doi.org/10.5194/gmd-10-3255-2017, 2017
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The EURODELTA-Trends numerical experiment has been designed to assess the capability of chemistry-transport models to capture the evolution of surface air quality over the 1990–2010 period in Europe. It also includes sensitivity experiments in order to analyse the relative contribution of (i) emission changes, (ii) meteorological variability, and (iii) boundary conditions to air quality trends. The article is a detailed presentation of the experiment design and participating models.
Sylvain Mailler, Laurent Menut, Dmitry Khvorostyanov, Myrto Valari, Florian Couvidat, Guillaume Siour, Solène Turquety, Régis Briant, Paolo Tuccella, Bertrand Bessagnet, Augustin Colette, Laurent Létinois, Kostantinos Markakis, and Frédérik Meleux
Geosci. Model Dev., 10, 2397–2423, https://doi.org/10.5194/gmd-10-2397-2017, https://doi.org/10.5194/gmd-10-2397-2017, 2017
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CHIMERE is a chemistry-transport model initially designed for box-modelling of the regional atmospheric composition. In the recent years, CHIMERE has been extended to be able to model atmospheric composition at all scales from urban to hemispheric scale, which implied major changes on the coordinate systems as well as on physical processes. This study describes how and why these changes have been brought to the model, largely increasing the range of its possible use.
Pascal Yiou, Aglaé Jézéquel, Philippe Naveau, Frederike E. L. Otto, Robert Vautard, and Mathieu Vrac
Adv. Stat. Clim. Meteorol. Oceanogr., 3, 17–31, https://doi.org/10.5194/ascmo-3-17-2017, https://doi.org/10.5194/ascmo-3-17-2017, 2017
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The attribution of classes of extreme events, such as heavy precipitation or heatwaves, relies on the estimate of small probabilities (with and without climate change). Such events are connected to the large-scale atmospheric circulation. This paper links such probabilities with properties of the atmospheric circulation by using a Bayesian decomposition. We test this decomposition on a case of extreme precipitation in the UK, in January 2014.
Joana Soares, Mikhail Sofiev, Camilla Geels, Jens H. Christensen, Camilla Andersson, Svetlana Tsyro, and Joakim Langner
Atmos. Chem. Phys., 16, 13081–13104, https://doi.org/10.5194/acp-16-13081-2016, https://doi.org/10.5194/acp-16-13081-2016, 2016
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Multi-model comparison of four offline dispersion models driven by the global climate projection climate show that the major driver for the sea salt flux changes will be the seawater temperature, but there are substantial differences between the model predictions. The impact on regional radiative budget due to sea spray is considerable in the Mediterranean area, due to warmer temperatures and longer days during the winter.
Geert Jan van Oldenborgh, Sjoukje Philip, Emma Aalbers, Robert Vautard, Friederike Otto, Karsten Haustein, Florence Habets, Roop Singh, and Heidi Cullen
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2016-308, https://doi.org/10.5194/hess-2016-308, 2016
Manuscript not accepted for further review
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Extreme rain caused flooding in France and Germany at the end of May 2016. After such an event the question is always posed to what extent it can be attributed to anthropogenic climate change. Using observations and five model ensembles we give a first answer. For the 3-day precipitation extremes over the Seine and Loire basins that caused the flooding all methods agree that the probability has increased by a factor of about two. For 1-day precipitation extremes in Germany the methods disagree.
Li Liu, Fabien Solmon, Robert Vautard, Lynda Hamaoui-Laguel, Csaba Zsolt Torma, and Filippo Giorgi
Biogeosciences, 13, 2769–2786, https://doi.org/10.5194/bg-13-2769-2016, https://doi.org/10.5194/bg-13-2769-2016, 2016
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To study the distribution of airborne ragweed pollen in changing environments and associated health risks over Europe, we introduce an approach with explicit treatment of pollen ripening, release and dispersion due to environmental drivers in an online modelling framework where climate is integrated with dispersion and vegetation production. From a simulated pollen season and concentration pattern health risks are evaluated through calculation of exposure time above health-relevant threshold levels.
V. Marécal, V.-H. Peuch, C. Andersson, S. Andersson, J. Arteta, M. Beekmann, A. Benedictow, R. Bergström, B. Bessagnet, A. Cansado, F. Chéroux, A. Colette, A. Coman, R. L. Curier, H. A. C. Denier van der Gon, A. Drouin, H. Elbern, E. Emili, R. J. Engelen, H. J. Eskes, G. Foret, E. Friese, M. Gauss, C. Giannaros, J. Guth, M. Joly, E. Jaumouillé, B. Josse, N. Kadygrov, J. W. Kaiser, K. Krajsek, J. Kuenen, U. Kumar, N. Liora, E. Lopez, L. Malherbe, I. Martinez, D. Melas, F. Meleux, L. Menut, P. Moinat, T. Morales, J. Parmentier, A. Piacentini, M. Plu, A. Poupkou, S. Queguiner, L. Robertson, L. Rouïl, M. Schaap, A. Segers, M. Sofiev, L. Tarasson, M. Thomas, R. Timmermans, Á. Valdebenito, P. van Velthoven, R. van Versendaal, J. Vira, and A. Ung
Geosci. Model Dev., 8, 2777–2813, https://doi.org/10.5194/gmd-8-2777-2015, https://doi.org/10.5194/gmd-8-2777-2015, 2015
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This paper describes the air quality forecasting system over Europe put in place in the Monitoring Atmospheric Composition and Climate projects. It provides daily and 4-day forecasts and analyses for the previous day for major gas and particulate pollutants and their main precursors. These products are based on a multi-model approach using seven state-of-the-art models developed in Europe. An evaluation of the performance of the system is discussed in the paper.
A. I. Stegehuis, R. Vautard, P. Ciais, A. J. Teuling, D. G. Miralles, and M. Wild
Geosci. Model Dev., 8, 2285–2298, https://doi.org/10.5194/gmd-8-2285-2015, https://doi.org/10.5194/gmd-8-2285-2015, 2015
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Many climate models have difficulties in properly reproducing climate extremes such as heat wave conditions. We use a regional climate model with different atmospheric physics schemes to simulate the heat wave events of 2003 in western Europe and 2010 in Russia. The five best-performing and diverse physics scheme combinations may be used in the future to perform heat wave analysis and to investigate the impact of climate change in summer in Europe.
K. Markakis, M. Valari, O. Perrussel, O. Sanchez, and C. Honore
Atmos. Chem. Phys., 15, 7703–7723, https://doi.org/10.5194/acp-15-7703-2015, https://doi.org/10.5194/acp-15-7703-2015, 2015
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The efficacy of emission policies is explored by coarse resolution modeling applications. These were shown to be biased, overestimating that efficacy indicated in simulations with refined resolution. In order to improve our assessments, we need to quantify those biases. In this study we show that the ozone bias of the coarse run is reduced by 40% by adopting higher resolution emissions. For PM2.5, the coarse run cannot selectively incorporate local scale features in order to reduce model error.
M. A. Thomas, M. Kahnert, C. Andersson, H. Kokkola, U. Hansson, C. Jones, J. Langner, and A. Devasthale
Geosci. Model Dev., 8, 1885–1898, https://doi.org/10.5194/gmd-8-1885-2015, https://doi.org/10.5194/gmd-8-1885-2015, 2015
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We have showed that a coupled modelling system is beneficial in the sense that more complex processes can be included to better represent the aerosol processes starting from their formation, their interactions with clouds and provide better estimate of radiative forcing. Using this model set up, we estimated an annual mean 'indirect' radiative forcing of -0.64W/m2. This means that aerosols, solely by their capability of altering the microphysical properties of clouds can cool the Earth system.
E. Katragkou, M. García-Díez, R. Vautard, S. Sobolowski, P. Zanis, G. Alexandri, R. M. Cardoso, A. Colette, J. Fernandez, A. Gobiet, K. Goergen, T. Karacostas, S. Knist, S. Mayer, P. M. M. Soares, I. Pytharoulis, I. Tegoulias, A. Tsikerdekis, and D. Jacob
Geosci. Model Dev., 8, 603–618, https://doi.org/10.5194/gmd-8-603-2015, https://doi.org/10.5194/gmd-8-603-2015, 2015
C. Andersson, R. Bergström, C. Bennet, L. Robertson, M. Thomas, H. Korhonen, K. E. J. Lehtinen, and H. Kokkola
Geosci. Model Dev., 8, 171–189, https://doi.org/10.5194/gmd-8-171-2015, https://doi.org/10.5194/gmd-8-171-2015, 2015
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We have integrated the sectional aerosol dynamics model SALSA into the European scale chemistry-transport model MATCH. The combined model reproduces observed higher particle number concentration (PNCs) in central Europe and lower concentrations in remote regions; however, the total PNC is underestimated. The low nucleation rate coefficient used in this study is an important reason for the underestimation.
J. Klingberg, M. Engardt, P. E. Karlsson, J. Langner, and H. Pleijel
Biogeosciences, 11, 5269–5283, https://doi.org/10.5194/bg-11-5269-2014, https://doi.org/10.5194/bg-11-5269-2014, 2014
K. Markakis, M. Valari, A. Colette, O. Sanchez, O. Perrussel, C. Honore, R. Vautard, Z. Klimont, and S. Rao
Atmos. Chem. Phys., 14, 7323–7340, https://doi.org/10.5194/acp-14-7323-2014, https://doi.org/10.5194/acp-14-7323-2014, 2014
S. Kotlarski, K. Keuler, O. B. Christensen, A. Colette, M. Déqué, A. Gobiet, K. Goergen, D. Jacob, D. Lüthi, E. van Meijgaard, G. Nikulin, C. Schär, C. Teichmann, R. Vautard, K. Warrach-Sagi, and V. Wulfmeyer
Geosci. Model Dev., 7, 1297–1333, https://doi.org/10.5194/gmd-7-1297-2014, https://doi.org/10.5194/gmd-7-1297-2014, 2014
D. Simpson, C. Andersson, J.H. Christensen, M. Engardt, C. Geels, A. Nyiri, M. Posch, J. Soares, M. Sofiev, P. Wind, and J. Langner
Atmos. Chem. Phys., 14, 6995–7017, https://doi.org/10.5194/acp-14-6995-2014, https://doi.org/10.5194/acp-14-6995-2014, 2014
L. Menut, R. Vautard, A. Colette, D. Khvorostyanov, A. Potier, L. Hamaoui-Laguel, N. Viovy, and M. Thibaudon
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-10891-2014, https://doi.org/10.5194/acpd-14-10891-2014, 2014
Revised manuscript not accepted
P. Yiou, M. Boichu, R. Vautard, M. Vrac, S. Jourdain, E. Garnier, F. Fluteau, and L. Menut
Clim. Past, 10, 797–809, https://doi.org/10.5194/cp-10-797-2014, https://doi.org/10.5194/cp-10-797-2014, 2014
A. Colette, B. Bessagnet, R. Vautard, S. Szopa, S. Rao, S. Schucht, Z. Klimont, L. Menut, G. Clain, F. Meleux, G. Curci, and L. Rouïl
Atmos. Chem. Phys., 13, 7451–7471, https://doi.org/10.5194/acp-13-7451-2013, https://doi.org/10.5194/acp-13-7451-2013, 2013
L. Menut, B. Bessagnet, D. Khvorostyanov, M. Beekmann, N. Blond, A. Colette, I. Coll, G. Curci, G. Foret, A. Hodzic, S. Mailler, F. Meleux, J.-L. Monge, I. Pison, G. Siour, S. Turquety, M. Valari, R. Vautard, and M. G. Vivanco
Geosci. Model Dev., 6, 981–1028, https://doi.org/10.5194/gmd-6-981-2013, https://doi.org/10.5194/gmd-6-981-2013, 2013
E. Solazzo, R. Bianconi, G. Pirovano, M. D. Moran, R. Vautard, C. Hogrefe, K. W. Appel, V. Matthias, P. Grossi, B. Bessagnet, J. Brandt, C. Chemel, J. H. Christensen, R. Forkel, X. V. Francis, A. B. Hansen, S. McKeen, U. Nopmongcol, M. Prank, K. N. Sartelet, A. Segers, J. D. Silver, G. Yarwood, J. Werhahn, J. Zhang, S. T. Rao, and S. Galmarini
Geosci. Model Dev., 6, 791–818, https://doi.org/10.5194/gmd-6-791-2013, https://doi.org/10.5194/gmd-6-791-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Modeling the drivers of fine PM pollution over Central Europe: impacts and contributions of emissions from different sources
Reaction of SO3 with H2SO4 and its implications for aerosol particle formation in the gas phase and at the air–water interface
Weakened aerosol–radiation interaction exacerbating ozone pollution in eastern China since China's clean air actions
Uncertainties from biomass burning aerosols in air quality models obscure public health impacts in Southeast Asia
Oxidative potential apportionment of atmospheric PM1: a new approach combining high-sensitive online analysers for chemical composition and offline OP measurement technique
Aqueous-phase chemistry of glyoxal with multifunctional reduced nitrogen compounds: a potential missing route for secondary brown carbon
An updated modeling framework to simulate Los Angeles air quality – Part 1: Model development, evaluation, and source apportionment
Frequent haze events associated with transport and stagnation over the corridor between the North China Plain and Yangtze River Delta
Evaluation of WRF-Chem-simulated meteorology and aerosols over northern India during the severe pollution episode of 2016
How well are aerosol–cloud interactions represented in climate models? – Part 1: Understanding the sulfate aerosol production from the 2014–15 Holuhraun eruption
pH regulates the formation of organosulfates and inorganic sulfate from organic peroxide reaction with dissolved SO2 in aquatic media
Technical note: Accurate, reliable, and high-resolution air quality predictions by improving the Copernicus Atmosphere Monitoring Service using a novel statistical post-processing method
Contribution of intermediate-volatility organic compounds from on-road transport to secondary organic aerosol levels in Europe
Secondary Organic Aerosols Derived from Intermediate Volatility n-Alkanes Adopt Low Viscous Phase State
Development of an integrated model framework for multi-air-pollutant exposure assessments in high-density cities
Observation-Constrained Kinetic Modelling of Isoprene SOA Formation in the Atmosphere
CAMx–UNIPAR simulation of secondary organic aerosol mass formed from multiphase reactions of hydrocarbons under the Central Valley urban atmospheres of California
Impact of urbanization on fine particulate matter concentrations over central Europe
Measurement report: Assessing the impacts of emission uncertainty on aerosol optical properties and radiative forcing from biomass burning in peninsular Southeast Asia
Significant impact of urban-tree biogenic emissions on air quality estimated by a bottom-up inventory and chemistry-transport modeling
The Emissions Model Intercomparison Project (Emissions-MIP): quantifying model sensitivity to emission characteristics
Dynamics-based estimates of decline trend with fine temporal variations in China's PM2.5 emissions
Modeling atmospheric brown carbon in the GISS ModelE Earth system model
Dual roles of inorganic aqueous phase on SOA growth from benzene and phenol
Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US
Reactive organic carbon air emissions from mobile sources in the United States
Development and evaluation of processes affecting simulation of diel fine particulate matter variation in the GEOS-Chem model
Substantially positive contributions of new particle formation to cloud condensation nuclei under low supersaturation in China based on numerical model improvements
Evolution of atmospheric age of particles and its implications for the formation of a severe haze event in eastern China
A multimodel evaluation of the potential impact of shipping on particle species in the Mediterranean Sea
Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying pre-existing particles – Part 2: Modeling chemical drivers and 3-D NPF occurrence
How does tropospheric VOC chemistry affect climate? An investigation of preindustrial control simulations using the Community Earth System Model version 2
Anthropogenic amplification of biogenic secondary organic aerosol production
A dynamic parameterization of sulfuric acid–dimethylamine nucleation and its application in three-dimensional modeling
Modeling dust mineralogical composition: sensitivity to soil mineralogy atlases and their expected climate impacts
Assessment of the impacts of cloud chemistry on surface SO2 and sulfate levels in typical regions of China
Impact of Landes forest fires on air quality in France during the 2022 summer
Global nitrogen and sulfur deposition mapping using a measurement–model fusion approach
Comprehensive simulations of new particle formation events in Beijing with a cluster dynamics–multicomponent sectional model
Implications of differences between recent anthropogenic aerosol emission inventories for diagnosed AOD and radiative forcing from 1990 to 2019
Unbalanced emission reductions of different species and sectors in China during COVID-19 lockdown derived by multi-species surface observation assimilation
Simulating organic aerosol in Delhi with WRF-Chem using the volatility-basis-set approach: exploring model uncertainty with a Gaussian process emulator
Modelling wintertime sea-spray aerosols under Arctic haze conditions
Impact of solar geoengineering on wildfires in the 21st century in CESM2/WACCM6
Linking gas, particulate, and toxic endpoints to air emissions in the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMM)
Contribution of regional aerosol nucleation to low-level CCN in an Amazonian deep convective environment: results from a regionally nested global model
Coarse particulate matter air quality in East Asia: implications for fine particulate nitrate
Foreign emissions exacerbate PM2.5 pollution in China through nitrate chemistry
Analysis of new particle formation events and comparisons to simulations of particle number concentrations based on GEOS-Chem–advanced particle microphysics in Beijing, China
Simulation of organic aerosol, its precursors, and related oxidants in the Landes pine forest in southwestern France: accounting for domain-specific land use and physical conditions
Lukáš Bartík, Peter Huszár, Jan Karlický, Ondřej Vlček, and Kryštof Eben
Atmos. Chem. Phys., 24, 4347–4387, https://doi.org/10.5194/acp-24-4347-2024, https://doi.org/10.5194/acp-24-4347-2024, 2024
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The presented study deals with the attribution of fine particulate matter (PM2.5) concentrations to anthropogenic emissions over Central Europe using regional-scale models. It calculates the present-day contributions of different emissions sectors to concentrations of PM2.5 and its secondary components. Moreover, the study investigates the effect of chemical nonlinearities by using multiple source attribution methods and secondary organic aerosol calculation methods.
Rui Wang, Yang Cheng, Shasha Chen, Rongrong Li, Yue Hu, Xiaokai Guo, Tianlei Zhang, Fengmin Song, and Hao Li
Atmos. Chem. Phys., 24, 4029–4046, https://doi.org/10.5194/acp-24-4029-2024, https://doi.org/10.5194/acp-24-4029-2024, 2024
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We used quantum chemical calculations, Born–Oppenheimer molecular dynamics simulations, and the ACDC kinetic model to characterize SO3–H2SO4 interaction in the gas phase and at the air–water interface and to study the effect of H2S2O7 on H2SO4–NH3-based clusters. The work expands our understanding of new pathways for the loss of SO3 in acidic polluted areas and helps reveal some missing sources of NPF in metropolitan industrial regions and understand the atmospheric organic–sulfur cycle better.
Hao Yang, Lei Chen, Hong Liao, Jia Zhu, Wenjie Wang, and Xin Li
Atmos. Chem. Phys., 24, 4001–4015, https://doi.org/10.5194/acp-24-4001-2024, https://doi.org/10.5194/acp-24-4001-2024, 2024
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The present study quantifies the response of aerosol–radiation interaction (ARI) to anthropogenic emission reduction from 2013 to 2017, with the main focus on the contribution to changed O3 concentrations over eastern China both in summer and winter using the WRF-Chem model. The weakened ARI due to decreased anthropogenic emission aggravates the summer (winter) O3 pollution by +0.81 ppb (+0.63 ppb), averaged over eastern China.
Margaret R. Marvin, Paul I. Palmer, Fei Yao, Mohd Talib Latif, and Md Firoz Khan
Atmos. Chem. Phys., 24, 3699–3715, https://doi.org/10.5194/acp-24-3699-2024, https://doi.org/10.5194/acp-24-3699-2024, 2024
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We use an atmospheric chemistry model to investigate aerosols emitted from fire activity across Southeast Asia. We find that the limited nature of measurements in this region leads to large uncertainties that significantly hinder the model representation of these aerosols and their impacts on air quality. As a result, the number of monthly attributable deaths is underestimated by as many as 4500, particularly in March at the peak of the mainland burning season.
Julie Camman, Benjamin Chazeau, Nicolas Marchand, Amandine Durand, Grégory Gille, Ludovic Lanzi, Jean-Luc Jaffrezo, Henri Wortham, and Gaëlle Uzu
Atmos. Chem. Phys., 24, 3257–3278, https://doi.org/10.5194/acp-24-3257-2024, https://doi.org/10.5194/acp-24-3257-2024, 2024
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Fine particle (PM1) pollution is a major health issue in the city of Marseille, which is subject to numerous pollution sources. Sampling carried out during the summer enabled a fine characterization of the PM1 sources and their oxidative potential, a promising new metric as a proxy for health impact. PM1 came mainly from combustion sources, secondary ammonium sulfate, and organic nitrate, while the oxidative potential of PM1 came from these sources and from resuspended dust in the atmosphere.
Yuemeng Ji, Zhang Shi, Wenjian Li, Jiaxin Wang, Qiuju Shi, Yixin Li, Lei Gao, Ruize Ma, Weijun Lu, Lulu Xu, Yanpeng Gao, Guiying Li, and Taicheng An
Atmos. Chem. Phys., 24, 3079–3091, https://doi.org/10.5194/acp-24-3079-2024, https://doi.org/10.5194/acp-24-3079-2024, 2024
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The formation mechanisms for secondary brown carbon (SBrC) contributed by multifunctional reduced nitrogen compounds (RNCs) remain unclear. Hence, from combined laboratory experiments and quantum chemical calculations, we investigated the heterogeneous reactions of glyoxal (GL) with multifunctional RNCs, which are driven by four-step indirect nucleophilic addition reactions. Our results show a possible missing source for SBrC formation on urban, regional, and global scales.
Elyse A. Pennington, Yuan Wang, Benjamin C. Schulze, Karl M. Seltzer, Jiani Yang, Bin Zhao, Zhe Jiang, Hongru Shi, Melissa Venecek, Daniel Chau, Benjamin N. Murphy, Christopher M. Kenseth, Ryan X. Ward, Havala O. T. Pye, and John H. Seinfeld
Atmos. Chem. Phys., 24, 2345–2363, https://doi.org/10.5194/acp-24-2345-2024, https://doi.org/10.5194/acp-24-2345-2024, 2024
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To assess the air quality in Los Angeles (LA), we improved the CMAQ model by using dynamic traffic emissions and new secondary organic aerosol schemes to represent volatile chemical products. Source apportionment demonstrates that the urban areas of the LA Basin and vicinity are NOx-saturated, with the largest sensitivity of O3 to changes in volatile organic compounds in the urban core. The improvement and remaining issues shed light on the future direction of the model development.
Feifan Yan, Hang Su, Yafang Cheng, Rujin Huang, Hong Liao, Ting Yang, Yuanyuan Zhu, Shaoqing Zhang, Lifang Sheng, Wenbin Kou, Xinran Zeng, Shengnan Xiang, Xiaohong Yao, Huiwang Gao, and Yang Gao
Atmos. Chem. Phys., 24, 2365–2376, https://doi.org/10.5194/acp-24-2365-2024, https://doi.org/10.5194/acp-24-2365-2024, 2024
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PM2.5 pollution is a major air quality issue deteriorating human health, and previous studies mostly focus on regions like the North China Plain and Yangtze River Delta. However, the characteristics of PM2.5 concentrations between these two regions are studied less often. Focusing on the transport corridor region, we identify an interesting seesaw transport phenomenon with stagnant weather conditions, conducive to PM2.5 accumulation over this region, resulting in large health effects.
Prerita Agarwal, David S. Stevenson, and Mathew R. Heal
Atmos. Chem. Phys., 24, 2239–2266, https://doi.org/10.5194/acp-24-2239-2024, https://doi.org/10.5194/acp-24-2239-2024, 2024
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Air pollution levels across northern India are amongst some of the worst in the world, with episodic and hazardous haze events. Here, the ability of the WRF-Chem model to predict air quality over northern India is assessed against several datasets. Whilst surface wind speed and particle pollution peaks are over- and underestimated, respectively, meteorology and aerosol trends are adequately captured, and we conclude it is suitable for investigating severe particle pollution events.
George Jordan, Florent Malavelle, Ying Chen, Amy Peace, Eliza Duncan, Daniel G. Partridge, Paul Kim, Duncan Watson-Parris, Toshihiko Takemura, David Neubauer, Gunnar Myhre, Ragnhild Skeie, Anton Laakso, and James Haywood
Atmos. Chem. Phys., 24, 1939–1960, https://doi.org/10.5194/acp-24-1939-2024, https://doi.org/10.5194/acp-24-1939-2024, 2024
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The 2014–15 Holuhraun eruption caused a huge aerosol plume in an otherwise unpolluted region, providing a chance to study how aerosol alters cloud properties. This two-part study uses observations and models to quantify this relationship’s impact on the Earth’s energy budget. Part 1 suggests the models capture the observed spatial and chemical evolution of the plume, yet no model plume is exact. Understanding these differences is key for Part 2, where changes to cloud properties are explored.
Lin Du, Xiaofan Lv, Makroni Lily, Kun Li, and Narcisse Tsona Tchinda
Atmos. Chem. Phys., 24, 1841–1853, https://doi.org/10.5194/acp-24-1841-2024, https://doi.org/10.5194/acp-24-1841-2024, 2024
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This study explores the pH effect on the reaction of dissolved SO2 with selected organic peroxides. Results show that the formation of organic and/or inorganic sulfate from these peroxides strongly depends on their electronic structures, and these processes are likely to alter the chemical composition of dissolved organic matter in different ways. The rate constants of these reactions exhibit positive pH and temperature dependencies within pH 1–10 and 240–340 K ranges.
Angelo Riccio and Elena Chianese
Atmos. Chem. Phys., 24, 1673–1689, https://doi.org/10.5194/acp-24-1673-2024, https://doi.org/10.5194/acp-24-1673-2024, 2024
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Starting from the Copernicus Atmosphere Monitoring Service (CAMS), we provided a novel ensemble statistical post-processing approach to improve their air quality predictions. Our approach is able to provide reliable short-term forecasts of pollutant concentrations, which is a key challenge in supporting national authorities in their tasks related to EU Air Quality Directives, such as planning and reporting the state of air quality to the citizens.
Stella E. I. Manavi and Spyros N. Pandis
Atmos. Chem. Phys., 24, 891–909, https://doi.org/10.5194/acp-24-891-2024, https://doi.org/10.5194/acp-24-891-2024, 2024
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Organic vapors of intermediate volatility have often been neglected as sources of atmospheric organic aerosol. In this work we use a new approach for their simulation and quantify the contribution of these compounds emitted by transportation sources (gasoline and diesel vehicles) to particulate matter over Europe. The estimated secondary organic aerosol levels are on average 60 % higher than predicted by previous approaches. However, these estimates are probably lower limits.
Tommaso Galeazzo, Bernard Aumont, Marie Camredon, Richard Valorso, Yong B. Lim, Paul J. Ziemann, and Manabu Shiraiwa
EGUsphere, https://doi.org/10.5194/egusphere-2024-51, https://doi.org/10.5194/egusphere-2024-51, 2024
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SOA derived from n-alkanes is a major component of anthropogenic particulate matter. We provide a comprehensive analysis of n-alkane SOA by explicit chemistry modeling, machine learning, and laboratory experiments, showing that n-alkane SOA adopt low viscous semisolid or liquid states. Our results indicate little kinetic limitations of mass accommodation in SOA formation, supporting the application of equilibrium partitioning for simulating n-alkane SOA in large-scale atmospheric models.
Zhiyuan Li, Kin-Fai Ho, Harry Fung Lee, and Steve Hung Lam Yim
Atmos. Chem. Phys., 24, 649–661, https://doi.org/10.5194/acp-24-649-2024, https://doi.org/10.5194/acp-24-649-2024, 2024
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This study developed an integrated model framework for accurate multi-air-pollutant exposure assessments in high-density and high-rise cities. Following the proposed integrated model framework, we established multi-air-pollutant exposure models for four major PM10 chemical species as well as four criteria air pollutants with R2 values ranging from 0.73 to 0.93. The proposed framework serves as an important tool for combined exposure assessment in epidemiological studies.
Chuanyang Shen, Xiaoyan Yang, Joel Thornton, John Shilling, Chenyang Bi, Gabriel Isaacman-VanWertz, and Haofei Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-97, https://doi.org/10.5194/egusphere-2024-97, 2024
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In this work, a multiphase condensed isoprene oxidation mechanism was developed to simulate isoprene SOA formation from chamber and field studies. Our results show that the measured isoprene SOA mass can be reasonably reproduced using the new mechanism. The simulation results indicate that multifunctional low-volatility products contribute significantly to total isoprene SOA. Our findings emphasize that the pathways to produce these low-volatility species should be considered in models.
Yujin Jo, Myoseon Jang, Sanghee Han, Azad Madhu, Bonyoung Koo, Yiqin Jia, Zechen Yu, Soontae Kim, and Jinsoo Park
Atmos. Chem. Phys., 24, 487–508, https://doi.org/10.5194/acp-24-487-2024, https://doi.org/10.5194/acp-24-487-2024, 2024
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The CAMx–UNIPAR model simulated the SOA budget formed via multiphase reactions of hydrocarbons and the impact of emissions and climate on SOA characteristics under California’s urban environments during winter 2018. SOA growth was dominated by daytime oxidation of long-chain alkanes and nighttime terpene oxidation with O3 and NO−3 radicals. The spatial distributions of anthropogenic SOA were affected by the northwesterly wind, whereas those of biogenic SOA were insensitive to wind directions.
Peter Huszar, Alvaro Patricio Prieto Perez, Lukáš Bartík, Jan Karlický, and Anahi Villalba-Pradas
Atmos. Chem. Phys., 24, 397–425, https://doi.org/10.5194/acp-24-397-2024, https://doi.org/10.5194/acp-24-397-2024, 2024
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Urbanization transforms rural land into artificial land, while due to human activities, it also introduces a great quantity of emissions. We quantify the impact of urbanization on the final particulate matter pollutant levels by looking not only at these emissions, but also at the way urban land cover influences meteorological conditions, how the removal of pollutants changes due to urban land cover, and how biogenic emissions from vegetation change due to less vegetation in urban areas.
Yinbao Jin, Yiming Liu, Xiao Lu, Xiaoyang Chen, Ao Shen, Haofan Wang, Yinping Cui, Yifei Xu, Siting Li, Jian Liu, Ming Zhang, Yingying Ma, and Qi Fan
Atmos. Chem. Phys., 24, 367–395, https://doi.org/10.5194/acp-24-367-2024, https://doi.org/10.5194/acp-24-367-2024, 2024
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This study aims to address these issues by evaluating eight independent biomass burning (BB) emission inventories (GFED, FINN1.5, FINN2.5 MOS, FINN2.5 MOSVIS, GFAS, FEER, QFED, and IS4FIRES) using the WRF-Chem model and analyzing their impact on aerosol optical properties (AOPs) and direct radiative forcing (DRF) during wildfire events in peninsular Southeast Asia (PSEA) that occurred in March 2019.
Alice Maison, Lya Lugon, Soo-Jin Park, Alexia Baudic, Christopher Cantrell, Florian Couvidat, Barbara D'Anna, Claudia Di Biagio, Aline Gratien, Valérie Gros, Carmen Kalalian, Julien Kammer, Vincent Michoud, Jean-Eudes Petit, Marwa Shahin, Leila Simon, Myrto Valari, Jérémy Vigneron, Andrée Tuzet, and Karine Sartelet
EGUsphere, https://doi.org/10.5194/egusphere-2023-2786, https://doi.org/10.5194/egusphere-2023-2786, 2023
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This study presents the development of a bottom-up inventory of urban-tree biogenic emissions. Emissions are computed for each tree based on their location and characteristics and are integrated in the regional air-quality model WRF-CHIMERE. The impact of these biogenic emissions on air quality is quantified for June–July 2022. Over Paris city, urban trees increase the concentrations of particulate organic matter by 4.6 %, of PM2.5 by 0.6 % and of ozone by 1.0 % on average over the two months.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Zhen Peng, Lili Lei, Zhe-Min Tan, Meigen Zhang, Aijun Ding, and Xingxia Kou
Atmos. Chem. Phys., 23, 14505–14520, https://doi.org/10.5194/acp-23-14505-2023, https://doi.org/10.5194/acp-23-14505-2023, 2023
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Annual PM2.5 emissions in China consistently decreased by about 3% to 5% from 2017 to 2020 with spatial variations and seasonal dependencies. High-temporal-resolution and dynamics-based PM2.5 emission estimates provide quantitative diurnal variations for each season. Significant reductions in PM2.5 emissions in the North China Plain and northeast of China in 2020 were caused by COVID-19.
Maegan A. DeLessio, Kostas Tsigaridis, Susanne E. Bauer, Jacek Chowdhary, and Gregory L. Schuster
EGUsphere, https://doi.org/10.5194/egusphere-2023-2472, https://doi.org/10.5194/egusphere-2023-2472, 2023
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This study presents the first explicit representation of brown carbon aerosols in the GISS ModelE Earth system model (ESM). Model sensitivity to a range of brown carbon parameters, as well as model performance compared to AERONET and MODIS retrievals of total aerosol properties, was assessed. General recommendations for incorporating brown carbon into ESMs are also included.
Jiwon Choi, Myoseon Jang, and Spencer Blau
EGUsphere, https://doi.org/10.5194/egusphere-2023-2461, https://doi.org/10.5194/egusphere-2023-2461, 2023
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A persistent phenoxy radical (PPR) effectively forms via a heterogeneous reaction of phenol and phenol-related products in the presence of wet-inorganic aerosol. These PPR can catalytically consume ozone during a NOx cycle and negatively influence SOA formation. SOA formation from phenol or benzene is simulated using the UNIPAR model which predicted SOA formation via multiphase reactions of hydrocarbons and compared with chamber data obtained under varying NOx levels, humidity, and seed types.
Stylianos Kakavas, Spyros N. Pandis, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13555–13564, https://doi.org/10.5194/acp-23-13555-2023, https://doi.org/10.5194/acp-23-13555-2023, 2023
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Water uptake from organic species in aerosol can affect the partitioning of semi-volatile inorganic compounds but are not considered in global and chemical transport models. We address this with a version of the PM-CAMx model that considers such organic water effects and use it to carry out 1-year aerosol simulations over the continental US. We show that such organic water impacts can increase dry PM1 levels by up to 2 μg m-3 when RH levels and PM1 concentrations are high.
Benjamin N. Murphy, Darrell Sonntag, Karl M. Seltzer, Havala O. T. Pye, Christine Allen, Evan Murray, Claudia Toro, Drew R. Gentner, Cheng Huang, Shantanu Jathar, Li Li, Andrew A. May, and Allen L. Robinson
Atmos. Chem. Phys., 23, 13469–13483, https://doi.org/10.5194/acp-23-13469-2023, https://doi.org/10.5194/acp-23-13469-2023, 2023
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We update methods for calculating organic particle and vapor emissions from mobile sources in the USA. Conventionally, particulate matter (PM) and volatile organic carbon (VOC) are speciated without consideration of primary semivolatile emissions. Our methods integrate state-of-the-science speciation profiles and correct for common artifacts when sampling emissions in a laboratory. We quantify impacts of the emission updates on ambient pollution with the Community Multiscale Air Quality model.
Yanshun Li, Randall V. Martin, Chi Li, Brian L. Boys, Aaron van Donkelaar, Jun Meng, and Jeffrey R. Pierce
Atmos. Chem. Phys., 23, 12525–12543, https://doi.org/10.5194/acp-23-12525-2023, https://doi.org/10.5194/acp-23-12525-2023, 2023
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We developed and evaluated processes affecting within-day (diel) variability in PM2.5 concentrations in a chemical transport model over the contiguous US. Diel variability in PM2.5 for the contiguous US is driven by early-morning accumulation into a shallow mixed layer, decreases from mid-morning through afternoon with mixed-layer growth, increases from mid-afternoon through evening as the mixed-layer collapses, and decreases overnight as emissions decrease.
Chupeng Zhang, Shangfei Hai, Yang Gao, Yuhang Wang, Shaoqing Zhang, Lifang Sheng, Bin Zhao, Shuxiao Wang, Jingkun Jiang, Xin Huang, Xiaojing Shen, Junying Sun, Aura Lupascu, Manish Shrivastava, Jerome D. Fast, Wenxuan Cheng, Xiuwen Guo, Ming Chu, Nan Ma, Juan Hong, Qiaoqiao Wang, Xiaohong Yao, and Huiwang Gao
Atmos. Chem. Phys., 23, 10713–10730, https://doi.org/10.5194/acp-23-10713-2023, https://doi.org/10.5194/acp-23-10713-2023, 2023
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New particle formation is an important source of atmospheric particles, exerting critical influences on global climate. Numerical models are vital tools to understanding atmospheric particle evolution, which, however, suffer from large biases in simulating particle numbers. Here we improve the model chemical processes governing particle sizes and compositions. The improved model reveals substantial contributions of newly formed particles to climate through effects on cloud condensation nuclei.
Xiaodong Xie, Jianlin Hu, Momei Qin, Song Guo, Min Hu, Dongsheng Ji, Hongli Wang, Shengrong Lou, Cheng Huang, Chong Liu, Hongliang Zhang, Qi Ying, Hong Liao, and Yuanhang Zhang
Atmos. Chem. Phys., 23, 10563–10578, https://doi.org/10.5194/acp-23-10563-2023, https://doi.org/10.5194/acp-23-10563-2023, 2023
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The atmospheric age of particles reflects how long particles have been formed and suspended in the atmosphere, which is closely associated with the evolution processes of particles. An analysis of the atmospheric age of PM2.5 provides a unique perspective on the evolution processes of different PM2.5 components. The results also shed lights on how to design effective emission control actions under unfavorable meteorological conditions.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Sara Jutterström, Jana Moldanova, Elisa Majamäki, and Jukka-Pekka Jalkanen
Atmos. Chem. Phys., 23, 10163–10189, https://doi.org/10.5194/acp-23-10163-2023, https://doi.org/10.5194/acp-23-10163-2023, 2023
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The Mediterranean Sea is a heavily trafficked shipping area, and air quality monitoring stations in numerous cities along the Mediterranean coast have detected high levels of air pollutants originating from shipping emissions. The current study investigates how existing restrictions on shipping-related emissions to the atmosphere ensure compliance with legislation. Focus was laid on fine particles and particle species, which were simulated with five different chemical transport models.
Ming Chu, Xing Wei, Shangfei Hai, Yang Gao, Huiwang Gao, Yujiao Zhu, Biwu Chu, Nan Ma, Juan Hong, Yele Sun, and Xiaohong Yao
EGUsphere, https://doi.org/10.5194/egusphere-2023-540, https://doi.org/10.5194/egusphere-2023-540, 2023
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We used a 20-bin WRF-Chem model to simulate NPF events in the NCP during a three-week observational period in the summer of 2019. The model was able to reproduce the observations during June 29–July 6, which was characterized by a high frequency of NPF occurrence.
Noah A. Stanton and Neil F. Tandon
Atmos. Chem. Phys., 23, 9191–9216, https://doi.org/10.5194/acp-23-9191-2023, https://doi.org/10.5194/acp-23-9191-2023, 2023
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Chemistry in Earth’s atmosphere has a potentially strong but very uncertain impact on climate. Past attempts to fully model chemistry in Earth’s troposphere (the lowest layer of the atmosphere) typically simplified the representation of Earth’s surface, which in turn limited the ability to simulate changes in climate. The cutting-edge model that we use in this study does not require such simplification, and we use it to examine the climate effects of chemical interactions in the troposphere.
Yiqi Zheng, Larry W. Horowitz, Raymond Menzel, David J. Paynter, Vaishali Naik, Jingyi Li, and Jingqiu Mao
Atmos. Chem. Phys., 23, 8993–9007, https://doi.org/10.5194/acp-23-8993-2023, https://doi.org/10.5194/acp-23-8993-2023, 2023
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Biogenic secondary organic aerosols (SOAs) account for a large fraction of fine aerosol at the global scale. Using long-term measurements and a climate model, we investigate anthropogenic impacts on biogenic SOA at both decadal and centennial timescales. Results show that despite reductions in biogenic precursor emissions, SOA has been strongly amplified by anthropogenic emissions since the preindustrial era and exerts a cooling radiative forcing.
Yuyang Li, Jiewen Shen, Bin Zhao, Runlong Cai, Shuxiao Wang, Yang Gao, Manish Shrivastava, Da Gao, Jun Zheng, Markku Kulmala, and Jingkun Jiang
Atmos. Chem. Phys., 23, 8789–8804, https://doi.org/10.5194/acp-23-8789-2023, https://doi.org/10.5194/acp-23-8789-2023, 2023
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We set up a new parameterization for 1.4 nm particle formation rates from sulfuric acid–dimethylamine (SA–DMA) nucleation, fully including the effects of coagulation scavenging and cluster stability. Incorporating the new parameterization into 3-D chemical transport models, we achieved better consistencies between simulation results and observation data. This new parameterization provides new insights into atmospheric nucleation simulations and its effects on atmospheric pollution or health.
María Gonçalves Ageitos, Vincenzo Obiso, Ron L. Miller, Oriol Jorba, Martina Klose, Matt Dawson, Yves Balkanski, Jan Perlwitz, Sara Basart, Enza Di Tomaso, Jerónimo Escribano, Francesca Macchia, Gilbert Montané, Natalie M. Mahowald, Robert O. Green, David R. Thompson, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 8623–8657, https://doi.org/10.5194/acp-23-8623-2023, https://doi.org/10.5194/acp-23-8623-2023, 2023
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Dust aerosols affect our climate differently depending on their mineral composition. We include dust mineralogy in an atmospheric model considering two existing soil maps, which still have large associated uncertainties. The soil data and the distribution of the minerals in different aerosol sizes are key to our model performance. We find significant regional variations in climate-relevant variables, which supports including mineralogy in our current models and the need for improved soil maps.
Jianyan Lu, Sunling Gong, Jian Zhang, Jianmin Chen, Lei Zhang, and Chunhong Zhou
Atmos. Chem. Phys., 23, 8021–8037, https://doi.org/10.5194/acp-23-8021-2023, https://doi.org/10.5194/acp-23-8021-2023, 2023
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WRF/CUACE was used to assess the cloud chemistry contribution in China. Firstly, the CUACE cloud chemistry scheme was found to reproduce well the cloud processing and consumption of H2O2, O3, and SO2, as well as the increase of sulfate. Secondly, during cloud availability in December under a heavy pollution episode, sulfate production increased 60–95 % and SO2 was reduced by over 80 %. This study provides a way to analyze the phenomenon of overestimation of SO2 in many chemical transport models.
Laurent Menut, Arineh Cholakian, Guillaume Siour, Rémy Lapere, Romain Pennel, Sylvain Mailler, and Bertrand Bessagnet
Atmos. Chem. Phys., 23, 7281–7296, https://doi.org/10.5194/acp-23-7281-2023, https://doi.org/10.5194/acp-23-7281-2023, 2023
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This study is about the wildfires occurring in France during the summer 2022. We study the forest fires that took place in the Landes during the summer of 2022. We show the direct impact of these fires on the air quality, especially downstream of the smoke plume towards the Paris region. We quantify the impact of these fires on the pollutants peak concentrations and the possible exceedance of thresholds.
Hannah J. Rubin, Joshua S. Fu, Frank Dentener, Rui Li, Kan Huang, and Hongbo Fu
Atmos. Chem. Phys., 23, 7091–7102, https://doi.org/10.5194/acp-23-7091-2023, https://doi.org/10.5194/acp-23-7091-2023, 2023
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We update the 2010 global deposition budget for nitrogen (N) and sulfur (S) with new regional wet deposition measurements, improving the ensemble results of 11 global chemistry transport models from HTAP II. Our study demonstrates that a global measurement–model fusion approach can substantially improve N and S deposition model estimates at a regional scale and represents a step forward toward the WMO goal of global fusion products for accurately mapping harmful air pollution.
Chenxi Li, Yuyang Li, Xiaoxiao Li, Runlong Cai, Yaxin Fan, Xiaohui Qiao, Rujing Yin, Chao Yan, Yishuo Guo, Yongchun Liu, Jun Zheng, Veli-Matti Kerminen, Markku Kulmala, Huayun Xiao, and Jingkun Jiang
Atmos. Chem. Phys., 23, 6879–6896, https://doi.org/10.5194/acp-23-6879-2023, https://doi.org/10.5194/acp-23-6879-2023, 2023
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New particle formation and growth in polluted environments are not fully understood despite intensive research. We applied a cluster dynamics–multicomponent sectional model to simulate the new particle formation events observed in Beijing, China. The simulation approximately captures how the events evolve. Further diagnosis shows that the oxygenated organic molecules may have been under-detected, and modulating their abundance leads to significantly improved simulation–observation agreement.
Marianne Tronstad Lund, Gunnar Myhre, Ragnhild Bieltvedt Skeie, Bjørn Hallvard Samset, and Zbigniew Klimont
Atmos. Chem. Phys., 23, 6647–6662, https://doi.org/10.5194/acp-23-6647-2023, https://doi.org/10.5194/acp-23-6647-2023, 2023
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Here we show that differences, in magnitude and trend, between recent global anthropogenic emission inventories have a notable influence on simulated regional abundances of anthropogenic aerosol over the 1990–2019 period. This, in turn, affects estimates of radiative forcing. Our findings form a basis for comparing existing and upcoming studies on anthropogenic aerosols using different emission inventories.
Lei Kong, Xiao Tang, Jiang Zhu, Zifa Wang, Yele Sun, Pingqing Fu, Meng Gao, Huangjian Wu, Miaomiao Lu, Qian Wu, Shuyuan Huang, Wenxuan Sui, Jie Li, Xiaole Pan, Lin Wu, Hajime Akimoto, and Gregory R. Carmichael
Atmos. Chem. Phys., 23, 6217–6240, https://doi.org/10.5194/acp-23-6217-2023, https://doi.org/10.5194/acp-23-6217-2023, 2023
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A multi-air-pollutant inversion system has been developed in this study to estimate emission changes in China during COVID-19 lockdown. The results demonstrate that the lockdown is largely a nationwide road traffic control measure with NOx emissions decreasing by ~40 %. Emissions of other species only decreased by ~10 % due to smaller effects of lockdown on other sectors. Assessment results further indicate that the lockdown only had limited effects on the control of PM2.5 and O3 in China.
Ernesto Reyes-Villegas, Douglas Lowe, Jill S. Johnson, Kenneth S. Carslaw, Eoghan Darbyshire, Michael Flynn, James D. Allan, Hugh Coe, Ying Chen, Oliver Wild, Scott Archer-Nicholls, Alex Archibald, Siddhartha Singh, Manish Shrivastava, Rahul A. Zaveri, Vikas Singh, Gufran Beig, Ranjeet Sokhi, and Gordon McFiggans
Atmos. Chem. Phys., 23, 5763–5782, https://doi.org/10.5194/acp-23-5763-2023, https://doi.org/10.5194/acp-23-5763-2023, 2023
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Organic aerosols (OAs), their sources and their processes remain poorly understood. The volatility basis set (VBS) approach, implemented in air quality models such as WRF-Chem, can be a useful tool to describe primary OA (POA) production and aging. However, the main disadvantage is its complexity. We used a Gaussian process simulator to reproduce model results and to estimate the sources of model uncertainty. We do this by comparing the outputs with OA observations made at Delhi, India, in 2018.
Eleftherios Ioannidis, Kathy S. Law, Jean-Christophe Raut, Louis Marelle, Tatsuo Onishi, Rachel M. Kirpes, Lucia M. Upchurch, Thomas Tuch, Alfred Wiedensohler, Andreas Massling, Henrik Skov, Patricia K. Quinn, and Kerri A. Pratt
Atmos. Chem. Phys., 23, 5641–5678, https://doi.org/10.5194/acp-23-5641-2023, https://doi.org/10.5194/acp-23-5641-2023, 2023
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Remote and local anthropogenic emissions contribute to wintertime Arctic haze, with enhanced aerosol concentrations, but natural sources, which also contribute, are less well studied. Here, modelled wintertime sea-spray aerosols are improved in WRF-Chem over the wider Arctic by including updated wind speed and temperature-dependent treatments. As a result, anthropogenic nitrate aerosols are also improved. Open leads are confirmed to be the main source of sea-spray aerosols over northern Alaska.
Wenfu Tang, Simone Tilmes, David M. Lawrence, Fang Li, Cenlin He, Louisa K. Emmons, Rebecca R. Buchholz, and Lili Xia
Atmos. Chem. Phys., 23, 5467–5486, https://doi.org/10.5194/acp-23-5467-2023, https://doi.org/10.5194/acp-23-5467-2023, 2023
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Globally, total wildfire burned area is projected to increase over the 21st century under scenarios without geoengineering and decrease under the two geoengineering scenarios. Geoengineering reduces fire by decreasing surface temperature and wind speed and increasing relative humidity and soil water. However, geoengineering also yields reductions in precipitation, which offset some of the fire reduction.
Havala O. T. Pye, Bryan K. Place, Benjamin N. Murphy, Karl M. Seltzer, Emma L. D'Ambro, Christine Allen, Ivan R. Piletic, Sara Farrell, Rebecca H. Schwantes, Matthew M. Coggon, Emily Saunders, Lu Xu, Golam Sarwar, William T. Hutzell, Kristen M. Foley, George Pouliot, Jesse Bash, and William R. Stockwell
Atmos. Chem. Phys., 23, 5043–5099, https://doi.org/10.5194/acp-23-5043-2023, https://doi.org/10.5194/acp-23-5043-2023, 2023
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Chemical mechanisms describe how emissions from vehicles, vegetation, and other sources are chemically transformed in the atmosphere to secondary products including criteria and hazardous air pollutants. The Community Regional Atmospheric Chemistry Multiphase Mechanism integrates gas-phase radical chemistry with pathways to fine-particle mass. New species were implemented, resulting in a bottom-up representation of organic aerosol, which is required for accurate source attribution of pollutants.
Xuemei Wang, Hamish Gordon, Daniel P. Grosvenor, Meinrat O. Andreae, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 4431–4461, https://doi.org/10.5194/acp-23-4431-2023, https://doi.org/10.5194/acp-23-4431-2023, 2023
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New particle formation in the upper troposphere is important for the global boundary layer aerosol population, and they can be transported downward in Amazonia. We use a global and a regional model to quantify the number of aerosols that are formed at high altitude and transported downward in a 1000 km region. We find that the majority of the aerosols are from outside the region. This suggests that the 1000 km region is unlikely to be a
closed loopfor aerosol formation, transport and growth.
Shixian Zhai, Daniel J. Jacob, Drew C. Pendergrass, Nadia K. Colombi, Viral Shah, Laura Hyesung Yang, Qiang Zhang, Shuxiao Wang, Hwajin Kim, Yele Sun, Jin-Soo Choi, Jin-Soo Park, Gan Luo, Fangqun Yu, Jung-Hun Woo, Younha Kim, Jack E. Dibb, Taehyoung Lee, Jin-Seok Han, Bruce E. Anderson, Ke Li, and Hong Liao
Atmos. Chem. Phys., 23, 4271–4281, https://doi.org/10.5194/acp-23-4271-2023, https://doi.org/10.5194/acp-23-4271-2023, 2023
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Anthropogenic fugitive dust in East Asia not only causes severe coarse particulate matter air pollution problems, but also affects fine particulate nitrate. Due to emission control efforts, coarse PM decreased steadily. We find that the decrease of coarse PM is a major driver for a lack of decrease of fine particulate nitrate, as it allows more nitric acid to form fine particulate nitrate. The continuing decrease of coarse PM requires more stringent ammonia and nitrogen oxides emission controls.
Jun-Wei Xu, Jintai Lin, Gan Luo, Jamiu Adeniran, and Hao Kong
Atmos. Chem. Phys., 23, 4149–4163, https://doi.org/10.5194/acp-23-4149-2023, https://doi.org/10.5194/acp-23-4149-2023, 2023
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Research on the sources of Chinese PM2.5 pollution has focused on the contributions of China’s domestic emissions. However, the impact of foreign anthropogenic emissions has typically been simplified or neglected. Here we find that foreign anthropogenic emissions play an important role in Chinese PM2.5 pollution through chemical interactions between foreign-transported pollutants and China’s local emissions. Thus, foreign emission reductions are essential for improving Chinese air quality.
Kun Wang, Xiaoyan Ma, Rong Tian, and Fangqun Yu
Atmos. Chem. Phys., 23, 4091–4104, https://doi.org/10.5194/acp-23-4091-2023, https://doi.org/10.5194/acp-23-4091-2023, 2023
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From 12 March to 6 April 2016 in Beijing, there were 11 typical new particle formation days, 13 non-event days, and 2 undefined days. We first analyzed the favorable background of new particle formation in Beijing and then conducted the simulations using four nucleation schemes based on a global chemistry transport model (GEOS-Chem) to understand the nucleation mechanism.
Arineh Cholakian, Matthias Beekmann, Guillaume Siour, Isabelle Coll, Manuela Cirtog, Elena Ormeño, Pierre-Marie Flaud, Emilie Perraudin, and Eric Villenave
Atmos. Chem. Phys., 23, 3679–3706, https://doi.org/10.5194/acp-23-3679-2023, https://doi.org/10.5194/acp-23-3679-2023, 2023
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This article revolves around the simulation of biogenic secondary organic aerosols in the Landes forest (southwestern France). Several sensitivity cases involving biogenic emission factors, land cover data, anthropogenic emissions, and physical or meteorological parameters were performed and each compared to measurements both in the forest canopy and around the forest. The chemistry behind the formation of these aerosols and their production and transport in the forest canopy is discussed.
Cited articles
AIRPARIF: Evaluation Prospective des emissions et des concentrations des
pollutants atmospheriques a l'horizon 2020 en Ile-De-France – Gain sur les
emissions en 2015, available at: http://www.airparif.asso.fr/_pdf/publications/ppa-rapport-121119.pdf (last access: 30 September 2015),
2012.
Allen, G., Sioutas, C., Koutrakis, P., Reiss, R., Lurmann, F. W., and Roberts,
P. T.: Evaluation of the TEOM method for measurement of ambient particulate
mass in urban areas, J. Air Waste Manage., 47, 682–689, 1997.
Andersson, C. and Engardt, M.: European ozone in a future climate: Importance
of changes in dry deposition and isoprene emissions, J. Geophys. Res., 115,
D02303, https://doi.org/10.1029/2008JD011690, 2010.
Andersson, C., Langner, J., and Bergström, R.: Interannual variation and
trends in air pollution over Europe due to climate variability during
1958–2001 simulated with a regional CTM coupled to the ERA40 reanalysis,
Tellus B, 59, 77–98, https://doi.org/10.1111/j.1600-0889.2006.00196.x, 2007.
Andersson, C., Bergström, R., Bennet, C., Robertson, L., Thomas, M.,
Korhonen, H., Lehtinen, K. E. J., and Kokkola, H.: MATCH-SALSA – Multi-scale
Atmospheric Transport and CHemistry model coupled to the SALSA aerosol
microphysics model – Part 1: Model description and evaluation, Geosci. Model
Dev., 8, 171–189, https://doi.org/10.5194/gmd-8-171-2015, 2015.
Aw, J. and Kleeman, M. J.: Evaluating the first-order effect of intra-annual
temperature variability on urban air pollution, J. Geophys. Res., 108, 4365,
https://doi.org/10.1029/2002JD002688, 2003.
Beekmann, M. and Vautard, R.: A modelling study of photochemical regimes over
Europe: robustness and variability, Atmos. Chem. Phys., 10, 10067–10084,
https://doi.org/10.5194/acp-10-10067-2010, 2010.
Bergström, R., Denier van der Gon, H. A. C., Prévôt, A. S. H.,
Yttri, K. E., and Simpson, D.: Modelling of organic aerosols over Europe
(2002–2007) using a volatility basis set (VBS) framework: application of
different assumptions regarding the formation of secondary organic aerosol,
Atmos. Chem. Phys., 12, 8499–8527, https://doi.org/10.5194/acp-12-8499-2012, 2012.
Bergström, R., Hallquist, M., Simpson, D., Wildt, J., and Mentel, T. F.:
Biotic stress: a significant contributor to organic aerosol in Europe?,
Atmos. Chem. Phys., 14, 13643–13660, https://doi.org/10.5194/acp-14-13643-2014, 2014.
Bessagnet, B., Menut, L., Curci, G., Hodzic, A., Guillaume, B., Liousse, C.,
Moukhtar, S., Pun, B., Seigneur, C., and Schulz, M.: Regional modeling of
carbonaceous aerosols over Europe – Focus on Secondary Organic Aerosols, J.
Atmos. Chem., 61, 175–202, 2009.
Butler, T. M., Stock, Z. S., Russo, M. R., Denier van der Gon, H. A. C., and
Lawrence, M. G.: Megacity ozone air quality under four alternative future
scenarios, Atmos. Chem. Phys., 12, 4413–4428,
https://doi.org/10.5194/acp-12-4413-2012, 2012.
Coleman, L., Martin, D., Varghese, S., Jennings, S. G., and O' Dowd, C. D.:
Assessment of changing meteorology and emissions on air quality using a
regional climate model: Impact on ozone, Atmos. Environ., 69, 198–210, 2014.
Colette, A., Granier, C., Hodnebrog, Ø., Jakobs, H., Maurizi, A., Nyiri,
A., Rao, S., Amann, M., Bessagnet, B., D'Angiola, A., Gauss, M., Heyes, C.,
Klimont, Z., Meleux, F., Memmesheimer, M., Mieville, A., Rouïl, L.,
Russo, F., Schucht, S., Simpson, D., Stordal, F., Tampieri, F., and Vrac, M.:
Future air quality in Europe: a multi-model assessment of projected exposure
to ozone, Atmos. Chem. Phys., 12, 10613–10630,
https://doi.org/10.5194/acp-12-10613-2012, 2012.
Colette, A., Bessagnet, B., Vautard, R., Szopa, S., Rao, S., Schucht, S.,
Klimont, Z., Menut, L., Clain, G., Meleux, F., Curci, G., and Rouïl, L.:
European atmosphere in 2050, a regional air quality and climate perspective
under CMIP5 scenarios, Atmos. Chem. Phys., 13, 7451–7471,
https://doi.org/10.5194/acp-13-7451-2013, 2013.
Clarke, L., Edmonds, J., Jacoby, H., Pitcher, H., Reilly, J., and Richels,
R.: Scenarios of Greenhouse Gas Emissions and Atmospheric Concentrations.
Sub-report 2.1A of Synthesis and Assessment Product 2.1 by the U.S. Climate
Change Science Program and the Subcommittee on Global Change Research,
Department of Energy, Office of Biological & Environmental Research,
Washington, D.C., USA, 154 pp., 2007.
Dufresne, J.-L., Foujols, M.-A., Denvil, S., Caubel, A., Marti, O., Aumont,
O., Balkanski, Y., Bekki, S., Bellenger, H., Benshila, R., Bony, S., Bopp,
L., Braconnot, P., Brockmann, P., Cadule, P., Cheruy, F., Codron, F., Cozic,
A., Cugnet, D., de Noblet, N., Duvel, J.-P., Ethé, C., Fairhead, L.,
Fichefet, T., Flavoni, S., Friedlingstein, P., Grandpeix, J.-Y., Guez, L.,
Guilyardi, E., Hauglustaine, D., Hourdin, F., Idelkadi, A., Ghattas, J.,
Joussaume, S., Kageyama, M., Krinner, G., Labetoulle, S., Lahellec, A.,
Lefebvre, M.-P., Lefevre, F., Levy, C., Li, Z. X., Lloyd, J., Lott, J.,
Madec, G., Mancip, M., Marchand, M., Masson, S., Meurdesoif, Y., Mignot, J.,
Musat, I., Parouty, S., Polcher, J., Rio, C., Schulz, M., Swingedouw, D.,
Szopa, S., Talandier, C., Terray, P., Viovy, N., and Vuichard, N.: Climate
change projections using the IPSL-CM5 Earth System Model: from CMIP3 to
CMIP5, Clim. Dynam., 40, 2123–2165, 2013.
EEA (Environmental Protection Agency): Air quality in Europe – 2013 report,
available at:
http://www.eea.europa.eu/publications/air-quality-in-europe-2013 (last
access: 30 September 2015), 2013.
Engardt, M., Bergstrom, R., and Andersson, C.: Climate and emission changes
contributing to changes in near-surface ozone in Europe over the coming
decades: Results from model studies, Ambio, 38, 452–458,
https://doi.org/10.1579/0044-7447-38.8.452, 2009.
GEA: Global Energy Assessment – Toward a Sustainable Future, Cambridge
University Press, Cambridge, UK and New York, NY, USA and the International
Institute for Applied Systems Analysis, Laxenburg, Austria, 2012.
Geels, C., Andersson, C., Hänninen, O., Lansø, A. S., Schwarze, P. E.,
Skjøth, C. A., and Brandt, J.: Future Premature Mortality Due to O3,
Secondary Inorganic Aerosols and Primary PM in Europe – Sensitivity to
Changes in Climate, Anthropogenic Emissions, Population and Building Stock,
Int. J. Environ. Res. Public Health, 12, 2837–2869, 2015.
Gidhagen, L., Engardt, M., Lövenheim, B., and Johansson, C.: Modeling
effects of climate change on air quality and population exposure in urban
planning scenarios, Adv. Meteorol., 2012, 240894, https://doi.org/10.1155/2012/240894,
2012.
Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P. I., and Geron,
C.: Estimates of global terrestrial isoprene emissions using MEGAN (Model of
Emissions of Gases and Aerosols from Nature), Atmos. Chem. Phys., 6,
3181–3210, https://doi.org/10.5194/acp-6-3181-2006, 2006.
Giorgi, F., Coppola, E., Solmon, F., Mariotti, L., Sylla, M. B., Bi, X.,
Elguindi, N., Diro, G. T., Nair, V., Giuliani, G., Turuncoglu, U. U.,
Cozzini, S., Güttler, L., O'Brien, T. A., Tawfik, A. B., Shalaby, A.,
Zakey, A. S., Steiner, A. L., Stordal, F., Sloan, L. C., and Brankovic, C.:
RegCM4: model description and preliminary tests over multiple CORDEX domains,
Clim. Res., 52, 7–29, 2012.
Hauglustaine, D. A., Hourdin, F., Jourdain, L., Filiberti, M.-A., Walters,
S., Lamarque, J. F., and Holland, E. A.: Interactive chemistry in the
Laboratoire de Meteorologie Dynamique general circulation model: Description
and background tropospheric chemistry evaluation, J. Geophys. Res., 190,
D04314, https://doi.org/10.1029/2003JD003957, 2004.
Jacob, D., Petersen, J., Eggert, B., Alias, A., Christensen, O. B., Bouwer,
L. M., Braun, A., Colette, A., Déqué, M., Georgievski, G.,
Georgopoulou, E., Gobiet, A., Menut, L., Nikulin, G., Haensler, A.,
Hempelmann, N., Jones, C., Keuler, K., Kovats, S., Kroner, N., Kotlarski, S.,
Kriegsmann, A., Martin, E., van Meijgaard, E., Moseley, C., Pfeifer, S.,
Preuschmann, S., Radermacher, C., Radtke, K., Rechid, D., Rounsevell, M.,
Samuelsson, P., Somot, S., Soussana, J.-F., Teichmann, C., Valentini, R.,
Vautard, R., Weber, B., and Yiou, P.: EURO-CORDEX: new high-resolution
climate change projections for European impact research, Reg. Environ.
Change, 14, 563–578, https://doi.org/10.1007/s10113-013-0499-2, 2014.
Jacob, D. J. and Winner, D. A.: Effect of climate change on air quality,
Atmos. Environ., 43, 51–63, 2009.
Jerrett, M., Finkelstein, M. M., Brook, J. R., Arain, M.A., Kanaroglou, P.,
Stieb, D. M., Gilbert, N. L., Verma, D., Finkelstein, N., Chapman, K. R., and
Sears, M. R.: A cohort study of traffic-related air pollution and mortality
in Toronto, Ontario, Canada, Environ. Health Persp., 117, 772–777, 2009.
Johnson, C. E., Collins, W. J., Stevenson, D. S., and Derwent, R. G.: The
relative roles of climate and emissions changes on future oxidant
concentrations, J. Geophys. Res., 104, 18631–18645, 1999.
Kahnert, M.: Variational data analysis of aerosol species in a regional CTM:
background error covariance constraint and aerosol optical observation
operators, Tellus B, 60, 753–770, 2008.
Katragkou, E., Zanis, P., Kioutsioukis, I., Tegoulias, I., Melas, D.,
Krüger, B. C., and Coppola, E.: Future climate change impacts on summer
surface ozone from regional climate-air quality simulations over Europe, J.
Geophys. Res., 116, D22307, https://doi.org/10.1029/2011JD015899, 2011.
Ketzel, M., Omstedt, G., and Johansson, C.: Estimation and validation of
PM2.5/PM10 exhaust and non-exhaust emission factors for practical
street pollution modeling, Atmos. Environ., 41, 9370–9385, 2007.
Klimont, Z., Kupiainen, K., Heyes, C., Cofala, J., Rafaj, P.,
Höglund-Isaksson, L., Borken, J., Schöpp, W., Winiwarter, W.,
Purohit, P., Bertok, I., and Sander, R.: ECLIPSE V4a: global emission data
set developed with the GAINS model for the period 2005 to 2050, Key features
and principal data sources, available at:
http://eccad.sedoo.fr/eccad_extract_interface/JSF/page_login.jsf (last
access: 30 September 2015), 2013.
Lacressonniere, G., Peuch, V.-H., Vautard, R., Arteta, J., Déqué, M.,
Joly, M., Josse, B., Marécal, V., and Saint-Martin, D.: European air
quality in the 2030s and 2050s: Impacts of global regional emission trends
and of climate change, Atmos. Environ., 92, 348–358, 2014.
Lamarque, J.-F., Bond, T. C., Eyring, V., Granier, C., Heil, A., Klimont, Z.,
Lee, D., Liousse, C., Mieville, A., Owen, B., Schultz, M. G., Shindell, D.,
Smith, S. J., Stehfest, E., Van Aardenne, J., Cooper, O. R., Kainuma, M.,
Mahowald, N., McConnell, J. R., Naik, V., Riahi, K., and van Vuuren, D. P.:
Historical (1850–2000) gridded anthropogenic and biomass burning emissions
of reactive gases and aerosols: methodology and application, Atmos. Chem.
Phys., 10, 7017–7039, https://doi.org/10.5194/acp-10-7017-2010, 2010.
Langner, J., Bergström, R., and Pleijel, K.: European scale modeling of
sulfur, oxidised nitrogen and photochemical oxidants. Model development and
evaluation for the 1994 growing season, Swedish Meteorological and
Hydrological Institute, RMK No. 82, 71 pp. (with errata), 1998.
Langner, J., Bergström, R., and Foltescu, V.: Impact of climate change on
surface ozone and deposition of sulphur and nitrogen in Europe, Atmos.
Environ., 39, 1129–1141, 2005.
Langner, J., Engardt, M., Baklanov, A., Christensen, J. H., Gauss, M., Geels,
C., Hedegaard, G. B., Nuterman, R., Simpson, D., Soares, J., Sofiev, M.,
Wind, P., and Zakey, A.: A multi-model study of impacts of climate change on
surface ozone in Europe, Atmos. Chem. Phys., 12, 10423–10440,
https://doi.org/10.5194/acp-12-10423-2012, 2012a.
Langner, J., Engardt, M., and Andersson, C.: European summer surface ozone
1990–2100, Atmos. Chem. Phys., 12, 10097–10105,
https://doi.org/10.5194/acp-12-10097-2012, 2012b.
Lattuati, M.: Contribution a l'etude du bilan de l'ozone tropospherique a
l'interface de l'Europe et de l'Atlantique Nord: modelisation lagrangienne et
mesures en altitude, PhD thesis, Universite P. M. Curie, Paris, France, 1997.
Lauwaet, D., Viaene, P., Brisson, E., van Lipzig, N.P.M., van Noije, T.,
Strunk, A., Van Looy, S., Veldeman, N., Blyth, L., De Ridder, K., and
Janssen, S.: The effect of climate change and emission scenarios on ozone
concentrations over Belgium: a high-resolution model study for policy
support, Atmos. Chem. Phys., 14, 5893–5904, https://doi.org/10.5194/acp-14-5893-2014,
2014.
Lepeule, J., Laden, F., Dockery, D., and Schwartz, J.: Chronic exposure to
fine particles and mortality: an extended follow-up of the Harvard Six Cities
study from 1974 to 2009, Environ. Health Persp., 120, 965–970, 2012.
Liao, H., Chen, W.-T., and Seinfeld, J. H.: Role of climate change in global
predictions of future tropospheric ozone and aerosols, J. Geophys. Res., 111,
D12304, https://doi.org/10.1029/2005JD006852, 2006.
Likhvar, V., Pascal, M., Markakis, K., Colette, A., Hauglustaine, D., Valari,
M., Klimont, Z., Medina, S., and Kinney, P.: A multi-scale health impact
assessment of air pollution over the 21st century, Sci. Total. Environ., 514,
439–449, 2015.
Markakis, K., Valari, M., Colette, A., Sanchez, O., Perrussel, O., Honore,
C., Vautard, R., Klimont, Z., and Rao, S.: Air quality in the mid-21st
century for the city of Paris under two climate scenarios; from the regional
to local scale, Atmos. Chem. Phys., 14, 7323–7340,
https://doi.org/10.5194/acp-14-7323-2014, 2014.
Markakis, K., Valari, M., Perrussel, O., Sanchez, O., and Honore, C.:
Climate-forced air-quality modeling at the urban scale: sensitivity to model
resolution, emissions and meteorology, Atmos. Chem. Phys., 15, 7703–7723,
https://doi.org/10.5194/acp-15-7703-2015, 2015.
Megaritis, A. G., Fountoukis, C., Charalampidis, P. E., Denier van der Gon,
H. A. C., Pilinis, C., and Pandis, S. N.: Linking climate and air quality
over Europe: effects of meteorology on PM2.5 concentrations, Atmos.
Chem. Phys., 14, 10283–10298, https://doi.org/10.5194/acp-14-10283-2014, 2014.
Menut, L., Schmechtig, C., and Marticorena, B.: Sensitivity of the
sandblasting fluxes calculations to the soil size distribution accuracy, J.
Atmos. Ocean. Tech., 22, 1875–1884, 2005.
Menut, L., Bessagnet, B., Khvorostyanov, D., Beekmann, M., Blond, N.,
Colette, A., Coll, I., Curci, G., Foret, G., Hodzic, A., Mailler, S., Meleux,
F., Monge, J.-L., Pison, I., Siour, G., Turquety, S., Valari, M., Vautard,
R., and Vivanco, M. G.: CHIMERE 2013: a model for regional atmospheric
composition modelling, Geosci. Model Dev., 6, 981–1028,
https://doi.org/10.5194/gmd-6-981-2013, 2013.
Nenes, A., Pilinis, C., and Pandis, S.: ISORROPIA: A new thermodynamic model
for inorganic multicomponent atmospheric aerosols, Aquat. Geochem., 4,
123–152, 1998.
Nolte, C. G., Gilliland, A. B., Hogrefe, C., and Mickley, L. J.: Linking
global to regional models to assess future climate impacts on surface ozone
levels in the United States, J. Geophys. Res., 113, D14307,
https://doi.org/10.1029/2007JD008497, 2008.
Omstedt, G., Bringfelt, B., and Johansson, C.: A model for vehicle-induced
non-tailpipe emissions of particles along Swedish roads, Atmos. Environ., 39,
6088–6097, 2005.
Pascal, M., Corso, M., Chanel, O., Declecq, C., Badaloni, C., Cesaroni, G.,
Henschel, S., Maister, K., Haluza, D., Martin-Olmedo, P., and Medina S.:
Assessing the public health impact of urban air pollution in 25 European
cities: results of the Aphekom project, Sci. Total Environ., 449, 390–400,
2013.
Prather, M., Gauss, M., Berntsen, T., Isaksen, I., Sundet, J., Bey, I.,
Brasseur, G., Dentener, F., Derwent, R., Stevenson, D., Grenfell, L.,
Hauglustaine, D., Horowitz, L., Jacob, D., Mickley, L., Lawrence, M., von
Kuhlmann, R., Muller, J.-F., Pitari, G., Rogers, H., Johnson, M., van Weele,
M., and Wild, O.: Fresh air in the 21st century?, Geophys. Res. Lett., 30,
1100, https://doi.org/10.1029/2002GL016285, 2003.
REVIHAAP: Review of evidence on health aspects of air pollution – REVIHAAP
Project, available at:
http://www.euro.who.int/en/health-topics/environment-and-health/air-quality/publications/2013/review-of-evidence-on-health-aspects-of-air-pollution-revihaap-project-final-technical-report
(last access: 30 September 2015), 2013.
Riahi, K., Rao, S., Krey, V., Cho, C., Chirkov, V., Fischer, G., Kindermann,
G., Nakicenovic, N., and Rafaj, P.: RCP 8.5-A scenario of comparatively high
greenhouse gas emissions, Climatic Change, 109, 33–57, 2011.
Robertson, L., Langner, J., and Engardt, M.: An Eulerian limited-area
atmospheric transport model, J. Appl. Meteorol., 38, 190–210, 1999.
Seinfeld, J. H. and Pandis, S. N.: Atmospheric Chemistry and Physics: From
Air Pollution to Climate Change, 2nd Edn., John Wiley and Sons, Hoboken, NJ,
2006.
Skamarock, W. C. and Klemp, J. B.: A time-split non-hydrostatic atmospheric
model, J. Comput. Phys., 227, 3465–3485, 2008.
Sillman, S. and He, D.: Some theoretical results concerning O3-NOx-VOC
chemistry and NOx-VOC indicators, J. Geophys. Res., 107, 4659,
https://doi.org/10.1029/2001JD001123, 2002.
Sillman, S., Vautard, R., Menut, L., and Kley, D.: O3-NOX-VOC sensitivity and
NOX-VOC indicators in Paris: Results from models and Atmospheric Pollution
over the Paris Area (ESQUIF) measurements, J. Geophys. Res., 108, 8563,
https://doi.org/10.1029/2002JD001561, 2003.
Simpson, D., Benedictow, A., Berge, H., Bergström, R., Emberson, L. D.,
Fagerli, H., Flechard, C. R., Hayman, G. D., Gauss, M., Jonson, J. E.,
Jenkin, M. E., Nyíri, A., Richter, C., Semeena, V. S., Tsyro, S.,
Tuovinen, J.-P., Valdebenito, Á., and Wind, P.: The EMEP MSC-W chemical
transport model – technical description, Atmos. Chem. Phys., 12, 7825–7865,
https://doi.org/10.5194/acp-12-7825-2012, 2012.
Sjödin, A., Ekström, M., and Hammarström, U.: Implementation and
Evaluation of the ARTEMIS Road Model for Sweden's International Reporting
Obligations on Air Emissions, in Proceedings of the 2nd Conference
Environment & Transport including the 15th Conference of Transport &
Air Pollution, Vol. 1, 375–382, Reims, France, June 2006.
Strandberg, G., Bärring, L., Hansson, U., Jansson, C., Jones, C.,
Kjellström, E., Kolax, M., Kupiainen, M., Nikulin, G., Samuelsson, P.,
Ullerstig, A., and Wang, S.: CORDEX scenarios for Europe from the Rossby
Centre regional climate model RCA4. SMHI reports, RMK 116. ISSN 0347-2116,
2014.
Szopa, S. and Hauglustaine, D.: Relative impacts of worldwide tropospheric
ozone changes and regional emission modifications on European surface-ozone
levels, C. R. Geosci., 339, 709–720, 2007.
Szopa, S., Balkanski, Y., Schulz, M., Bekki, S., Cugnet, D., Fortems-Cheiney,
A., Turquety, S., Cozic, A., Deandreis, C., Hauglustaine, D., Idelkadi, A.,
Lathiere, J., Lefevre, F., Marchand, M., Vuolo, R., Yan, N., and Dufresne,
J.-L.: Aerosol and ozone changes as forcing for climate evolution between
1850 and 2100, Clim. Dynam., 40, 2223–2250, 2013.
Valari, M. and Menut, L.: Does an Increase in Air Quality Models' Resolution
Bring Surface Ozone Concentrations Closer to Reality?, J. Atmos. Ocean.
Tech., 25, 1955–1968, 2008.
Vautard, R., Honoré, C., Beekmann, M., and Rouil, L.: Simulation of ozone
during the August 2003 heat wave and emission control scenarios, Atmos.
Environ., 39, 2957–2967, 2005.
Vautard R., Builtjes, P. H. J., Thunis, P., Cuvelier, C., Bedogni, M.,
Bessagnet, B., Honore, C., Moussiopoulos, N., Pirovano, G., Schaap, M.,
Stern, R., Tarasson, L., and Wind, P.: Evaluation and intercomparison of
Ozone and PM10 simulations by several chemistry transport models over
four European cities within the CityDelta project, Atmos. Environ., 41,
173–188, 2007.
Vautard, R., Gobiet, A., Sobolowski, S., Kjellström, E., Stegehuis, A.,
Watkiss, P., Mendlik, T., Landgren, O., Nikulin, G., Teichmann, C., and
Jacob, D.: The European climate under a 2 °C global warming,
Environ. Res. Lett., 9, 034006, https://doi.org/10.1088/1748-9326/9/3/034006, 2014.
Watson, L., Lacressonnière, G., Gauss, M., Engardt, M., Andersson, C.,
Josse, B., Marécal, V., Nyiri, A., Sobolowski, S., Siour, G., and
Vautard, R.: The impact of meteorological forcings on gas phase air
pollutants over Europe, Atmos. Environ., 119, 240–257, 2015.
Yttri, K. E., Simpson, D., Nøjgaard, J. K., Kristensen, K., Genberg, J.,
Stenström, K., Swietlicki, E., Hillamo, R., Aurela, M., Bauer, H.,
Offenberg, J. H., Jaoui, M., Dye, C., Eckhardt, S., Burkhart, J. F., Stohl,
A., and Glasius, M.: Source apportionment of the summer time carbonaceous
aerosol at Nordic rural background sites, Atmos. Chem. Phys., 11,
13339–13357, https://doi.org/10.5194/acp-11-13339-2011, 2011.
Zanis, P., Katragkou, E., Tegoulias, I., Poupkou, A., Melas, D., Huszar, P.,
and Giorgi, F.: Evaluation of near surface ozone in air quality simulations
forced by a regional climate model over Europe for the period 1991–2000,
Atmos. Environ., 45, 6489–6500, 2011.
Short summary
The overall climate benefit at both cities and pollutants is −2 to −10 % depending on metric. Over the city of Paris local mitigation of NOx emissions increases future ozone due to titration inhibition. Climate is the most influential factor for maximum ozone in Paris, which is particularly interesting from a health impact perspective. Over urban areas with major regional contribution (e.g. Stockholm) the bias due to coarse emission inventory may lead to policy misclassification.
The overall climate benefit at both cities and pollutants is −2 to −10 % depending on metric....
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