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Volume 16, issue 3
Atmos. Chem. Phys., 16, 1747-1760, 2016
https://doi.org/10.5194/acp-16-1747-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 1747-1760, 2016
https://doi.org/10.5194/acp-16-1747-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 15 Feb 2016

Research article | 15 Feb 2016

Secondary organic aerosol formation from isoprene photooxidation during cloud condensation–evaporation cycles

L. Brégonzio-Rozier et al.
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Altieri, K. E., Seitzinger, S. P., Carlton, A. G., Turpin, B. J., Klein, G. C., and Marshall, A. G.: Oligomers formed through in-cloud methylglyoxal reactions: Chemical composition, properties, and mechanisms investigated by ultra-high resolution FT-ICR mass spectrometry, Atmos. Environ., 42, 1476–1490, 2008.
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Benkelberg, H. J., Hamm, S., and Warneck, P.: Henry's law coefficients for aqueous solutions of acetone, acetaldehyde and acetonitrile, and equilibrium constants for the addition compounds of acetone and acetaldehyde with bisulfite, J. Atmos. Chem., 20, 17–34, 1995.
Betterton, E. A. and Hoffmann, M. R.: Henry's law constants of some environmentally important aldehydes, Environ. Sci. Technol., 22, 1415–1418, 1988.
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The impact of cloud events on isoprene secondary organic aerosol (SOA) formation has been studied from an isoprene/ NOx/light system in an atmospheric simulation chamber. aqSOA formation can be linked to water soluble volatile organic compounds' dissolution in the aqueous phase and to further aqueous phase reactions. Cloud-induced SOA formation is experimentally demonstrated in this study, thus highlighting the importance of aqueous multiphase systems in atmospheric SOA formation estimations.
The impact of cloud events on isoprene secondary organic aerosol (SOA) formation has been...
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