Articles | Volume 16, issue 21
https://doi.org/10.5194/acp-16-13711-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-13711-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
04 Nov 2016
Research article |
| 04 Nov 2016
Extreme dust storm over the eastern Mediterranean in September 2015: satellite, lidar, and surface observations in the Cyprus region
Rodanthi-Elisavet Mamouri
CORRESPONDING AUTHOR
Cyprus University of Technology, Department of Civil Engineering and Geomatics, Limassol, Cyprus
Institute for Astronomy, Astrophysics, Space Applications and Remote Sensing, National Observatory of Athens, Athens, Greece
Albert Ansmann
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Argyro Nisantzi
Cyprus University of Technology, Department of Civil Engineering and Geomatics, Limassol, Cyprus
Stavros Solomos
Institute for Astronomy, Astrophysics, Space Applications and Remote Sensing, National Observatory of Athens, Athens, Greece
George Kallos
School of Physics, Division of Environment and Meteorology, University of Athens, Athens, Greece
Diofantos G. Hadjimitsis
Cyprus University of Technology, Department of Civil Engineering and Geomatics, Limassol, Cyprus
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Albert Ansmann, Rodanthi-Elisavet Mamouri, Julian Hofer, Holger Baars, Dietrich Althausen, and Sabur F. Abdullaev
Atmos. Meas. Tech., 12, 4849–4865, https://doi.org/10.5194/amt-12-4849-2019, https://doi.org/10.5194/amt-12-4849-2019, 2019
Guangyao Dai, Dietrich Althausen, Julian Hofer, Ronny Engelmann, Patric Seifert, Johannes Bühl, Rodanthi-Elisavet Mamouri, Songhua Wu, and Albert Ansmann
Atmos. Meas. Tech., 11, 2735–2748, https://doi.org/10.5194/amt-11-2735-2018, https://doi.org/10.5194/amt-11-2735-2018, 2018
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Rodanthi-Elisavet Mamouri and Albert Ansmann
Atmos. Meas. Tech., 10, 3403–3427, https://doi.org/10.5194/amt-10-3403-2017, https://doi.org/10.5194/amt-10-3403-2017, 2017
Moritz Haarig, Albert Ansmann, Dietrich Althausen, André Klepel, Silke Groß, Volker Freudenthaler, Carlos Toledano, Rodanthi-Elisavet Mamouri, David A. Farrell, Damien A. Prescod, Eleni Marinou, Sharon P. Burton, Josef Gasteiger, Ronny Engelmann, and Holger Baars
Atmos. Chem. Phys., 17, 10767–10794, https://doi.org/10.5194/acp-17-10767-2017, https://doi.org/10.5194/acp-17-10767-2017, 2017
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Our measurements performed with a lidar on Barbados give a vertical profile of Saharan dust, which was transported over 5000 km across the Atlantic. The new triple-wavelength depolarization technique reveals more information about the shape and size of dust, which will improve our understanding of the aging process of dust in the atmosphere and its representation in dust models. Changing properties of dust particles influence the solar radiation and the cloud properties and thus our climate.
Stavros Solomos, Albert Ansmann, Rodanthi-Elisavet Mamouri, Ioannis Binietoglou, Platon Patlakas, Eleni Marinou, and Vassilis Amiridis
Atmos. Chem. Phys., 17, 4063–4079, https://doi.org/10.5194/acp-17-4063-2017, https://doi.org/10.5194/acp-17-4063-2017, 2017
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An extreme dust storm affected Middle East and the Eastern Mediterranean in September 2015. This event was produced by a combination of meteorological and land-use properties. Analysis with remote sensing observations and modeling simulations reveals (i) transport of warm moist air from the Red and Arabian seas, (ii) formation of a thermal low over Syria, (iii) convective outflows and haboob formation (i.e. propagating dust walls), and (iv) changes in land-use and dust erodibility due to war.
Juan Antonio Bravo-Aranda, Livio Belegante, Volker Freudenthaler, Lucas Alados-Arboledas, Doina Nicolae, María José Granados-Muñoz, Juan Luis Guerrero-Rascado, Aldo Amodeo, Giusseppe D'Amico, Ronny Engelmann, Gelsomina Pappalardo, Panos Kokkalis, Rodanthy Mamouri, Alex Papayannis, Francisco Navas-Guzmán, Francisco José Olmo, Ulla Wandinger, Francesco Amato, and Martial Haeffelin
Atmos. Meas. Tech., 9, 4935–4953, https://doi.org/10.5194/amt-9-4935-2016, https://doi.org/10.5194/amt-9-4935-2016, 2016
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This work analyses the lidar polarizing sensitivity by means of the Stokes–Müller formalism and provides a new tool to quantify the systematic error of the volume linear depolarization ration (δ) using the Monte Carlo technique. Results evidence the importance of the lidar polarizing effects which can lead to systematic errors larger than 100 %. Additionally, we demonstrate that a proper lidar characterization helps to reduce the uncertainty.
Rodanthi-Elisavet Mamouri and Albert Ansmann
Atmos. Chem. Phys., 16, 5905–5931, https://doi.org/10.5194/acp-16-5905-2016, https://doi.org/10.5194/acp-16-5905-2016, 2016
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
M. Sicard, G. D'Amico, A. Comerón, L. Mona, L. Alados-Arboledas, A. Amodeo, H. Baars, J. M. Baldasano, L. Belegante, I. Binietoglou, J. A. Bravo-Aranda, A. J. Fernández, P. Fréville, D. García-Vizcaíno, A. Giunta, M. J. Granados-Muñoz, J. L. Guerrero-Rascado, D. Hadjimitsis, A. Haefele, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, R. E. Mamouri, I. Mattis, F. Molero, N. Montoux, A. Muñoz, C. Muñoz Porcar, F. Navas-Guzmán, D. Nicolae, A. Nisantzi, N. Papagiannopoulos, A. Papayannis, S. Pereira, J. Preißler, M. Pujadas, V. Rizi, F. Rocadenbosch, K. Sellegri, V. Simeonov, G. Tsaknakis, F. Wagner, and G. Pappalardo
Atmos. Meas. Tech., 8, 4587–4613, https://doi.org/10.5194/amt-8-4587-2015, https://doi.org/10.5194/amt-8-4587-2015, 2015
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In the framework of the ACTRIS summer 2012 measurement campaign (8 June–17 July 2012), EARLINET organized and performed a controlled exercise of feasibility to demonstrate its potential to perform operational, coordinated measurements and deliver products in near-real time. The paper describes the measurement protocol and discusses the delivery of real-time and near-real-time lidar-derived products.
M. Abdelkader, S. Metzger, R. E. Mamouri, M. Astitha, L. Barrie, Z. Levin, and J. Lelieveld
Atmos. Chem. Phys., 15, 9173–9189, https://doi.org/10.5194/acp-15-9173-2015, https://doi.org/10.5194/acp-15-9173-2015, 2015
V. Amiridis, E. Marinou, A. Tsekeri, U. Wandinger, A. Schwarz, E. Giannakaki, R. Mamouri, P. Kokkalis, I. Binietoglou, S. Solomos, T. Herekakis, S. Kazadzis, E. Gerasopoulos, E. Proestakis, M. Kottas, D. Balis, A. Papayannis, C. Kontoes, K. Kourtidis, N. Papagiannopoulos, L. Mona, G. Pappalardo, O. Le Rille, and A. Ansmann
Atmos. Chem. Phys., 15, 7127–7153, https://doi.org/10.5194/acp-15-7127-2015, https://doi.org/10.5194/acp-15-7127-2015, 2015
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LIVAS is a 3-D multi-wavelength global aerosol and cloud optical database optimized for future space-based lidar end-to-end simulations of realistic atmospheric scenarios as well as retrieval algorithm testing activities. The global database is based on CALIPSO observations at 532nm, while for the conversion at 355nm EARLINET data are utilized.
V. Vakkari, E. J. O'Connor, A. Nisantzi, R. E. Mamouri, and D. G. Hadjimitsis
Atmos. Meas. Tech., 8, 1875–1885, https://doi.org/10.5194/amt-8-1875-2015, https://doi.org/10.5194/amt-8-1875-2015, 2015
R. E. Mamouri and A. Ansmann
Atmos. Chem. Phys., 15, 3463–3477, https://doi.org/10.5194/acp-15-3463-2015, https://doi.org/10.5194/acp-15-3463-2015, 2015
A. Nisantzi, R. E. Mamouri, A. Ansmann, and D. Hadjimitsis
Atmos. Chem. Phys., 14, 12155–12165, https://doi.org/10.5194/acp-14-12155-2014, https://doi.org/10.5194/acp-14-12155-2014, 2014
R. E. Mamouri and A. Ansmann
Atmos. Meas. Tech., 7, 3717–3735, https://doi.org/10.5194/amt-7-3717-2014, https://doi.org/10.5194/amt-7-3717-2014, 2014
G. Pappalardo, L. Mona, G. D'Amico, U. Wandinger, M. Adam, A. Amodeo, A. Ansmann, A. Apituley, L. Alados Arboledas, D. Balis, A. Boselli, J. A. Bravo-Aranda, A. Chaikovsky, A. Comeron, J. Cuesta, F. De Tomasi, V. Freudenthaler, M. Gausa, E. Giannakaki, H. Giehl, A. Giunta, I. Grigorov, S. Groß, M. Haeffelin, A. Hiebsch, M. Iarlori, D. Lange, H. Linné, F. Madonna, I. Mattis, R.-E. Mamouri, M. A. P. McAuliffe, V. Mitev, F. Molero, F. Navas-Guzman, D. Nicolae, A. Papayannis, M. R. Perrone, C. Pietras, A. Pietruczuk, G. Pisani, J. Preißler, M. Pujadas, V. Rizi, A. A. Ruth, J. Schmidt, F. Schnell, P. Seifert, I. Serikov, M. Sicard, V. Simeonov, N. Spinelli, K. Stebel, M. Tesche, T. Trickl, X. Wang, F. Wagner, M. Wiegner, and K. M. Wilson
Atmos. Chem. Phys., 13, 4429–4450, https://doi.org/10.5194/acp-13-4429-2013, https://doi.org/10.5194/acp-13-4429-2013, 2013
Alkistis Papetta, Franco Marenco, Maria Kezoudi, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Holger Baars, Ioana Elisabeta Popovici, Philippe Goloub, Stéphane Victori, and Jean Sciare
Atmos. Meas. Tech., 17, 1721–1738, https://doi.org/10.5194/amt-17-1721-2024, https://doi.org/10.5194/amt-17-1721-2024, 2024
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We propose a method to determine depolarization parameters using observations from a reference instrument at a nearby location, needed for systems where a priori knowledge of cross-talk parameters is not available. It uses three-parameter equations to compare VDR between two co-located lidars at dust and molecular layers. It can be applied retrospectively to existing data acquired during campaigns. Its application to Cimel CE376 corrected VDR bias at high- and low-depolarizing layers.
Sofía Gómez Maqueo Anaya, Dietrich Althausen, Matthias Faust, Holger Baars, Bernd Heinold, Julian Hofer, Ina Tegen, Albert Ansmann, Ronny Engelmann, Annett Skupin, Birgit Heese, and Kerstin Schepanski
Geosci. Model Dev., 17, 1271–1295, https://doi.org/10.5194/gmd-17-1271-2024, https://doi.org/10.5194/gmd-17-1271-2024, 2024
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Mineral dust aerosol particles vary greatly in their composition depending on source region, which leads to different physicochemical properties. Most atmosphere–aerosol models consider mineral dust aerosols to be compositionally homogeneous, which ultimately increases model uncertainty. Here, we present an approach to explicitly consider the heterogeneity of the mineralogical composition for simulations of the Saharan atmospheric dust cycle with regard to dust transport towards the Atlantic.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
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An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
EGUsphere, https://doi.org/10.5194/egusphere-2024-140, https://doi.org/10.5194/egusphere-2024-140, 2024
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Aerosols contribute to the largest uncertainties in climate change predictions. Especially absorbing aerosols propose difficulties in our understanding. The eastern Mediterranean is a hot spot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during the A-LIFE field experiment to characterize aerosols and aerosol mixtures. We extend current classification and separation schemes and compare different classification schemes.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
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EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
G. Giannarakis, I. Tsoumas, S. Neophytides, C. Papoutsa, C. Kontoes, and D. Hadjimitsis
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLVIII-1-W2-2023, 1379–1384, https://doi.org/10.5194/isprs-archives-XLVIII-1-W2-2023-1379-2023, https://doi.org/10.5194/isprs-archives-XLVIII-1-W2-2023-1379-2023, 2023
M. Tzouvaras, S. Alatza, M. Prodromou, C. Theocharidis, K. Fotiou, A. Argyriou, C. Loupasakis, A. Apostolakis, Z. Pittaki, M. Kaskara, C. Kontoes, and D. Hadjimitsis
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLVIII-1-W2-2023, 1581–1587, https://doi.org/10.5194/isprs-archives-XLVIII-1-W2-2023-1581-2023, https://doi.org/10.5194/isprs-archives-XLVIII-1-W2-2023-1581-2023, 2023
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
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For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Henriette Gebauer, Athena Augusta Floutsi, Moritz Haarig, Martin Radenz, Ronny Engelmann, Dietrich Althausen, Annett Skupin, Albert Ansmann, Cordula Zenk, and Holger Baars
EGUsphere, https://doi.org/10.5194/egusphere-2023-2305, https://doi.org/10.5194/egusphere-2023-2305, 2023
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Sulfate aerosol from the volcanic eruption at Las Palmas in 2021 was observed over Cabo Verde. The impact of the eruption was observable even 1500 km away from the emission source and led to an extraordinary strong pollution in the lowermost atmosphere above Cabo Verde. We characterized the aerosol burden based on lidar and sun photometer observations. We compared the volcanic case to the typical background conditions (reference case) to quantify the volcanic pollution.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
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The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Akriti Masoom, Ilias Fountoulakis, Stelios Kazadzis, Ioannis-Panagiotis Raptis, Anna Kampouri, Basil E. Psiloglou, Dimitra Kouklaki, Kyriakoula Papachristopoulou, Eleni Marinou, Stavros Solomos, Anna Gialitaki, Dimitra Founda, Vasileios Salamalikis, Dimitris Kaskaoutis, Natalia Kouremeti, Nikolaos Mihalopoulos, Vassilis Amiridis, Andreas Kazantzidis, Alexandros Papayannis, Christos S. Zerefos, and Kostas Eleftheratos
Atmos. Chem. Phys., 23, 8487–8514, https://doi.org/10.5194/acp-23-8487-2023, https://doi.org/10.5194/acp-23-8487-2023, 2023
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We analyse the spatial and temporal aerosol spectral optical properties during the extreme wildfires of August 2021 in Greece and assess their effects on air quality and solar radiation quantities related to health, agriculture, and energy. Different aerosol conditions are identified (pure smoke, pure dust, dust–smoke together); the largest impact on solar radiation quantities is found for cases with mixed dust–smoke aerosols. Such situations are expected to occur more frequently in the future.
Ulla Wandinger, Athena Augusta Floutsi, Holger Baars, Moritz Haarig, Albert Ansmann, Anja Hünerbein, Nicole Docter, David Donovan, Gerd-Jan van Zadelhoff, Shannon Mason, and Jason Cole
Atmos. Meas. Tech., 16, 2485–2510, https://doi.org/10.5194/amt-16-2485-2023, https://doi.org/10.5194/amt-16-2485-2023, 2023
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We introduce an aerosol classification model that has been developed for the Earth Clouds, Aerosols and Radiation Explorer (EarthCARE). The model provides a consistent description of microphysical, optical, and radiative properties of common aerosol types such as dust, sea salt, pollution, and smoke. It is used for aerosol classification and assessment of radiation effects based on the synergy of active and passive observations with lidar, imager, and radiometer of the multi-instrument platform.
Athena Augusta Floutsi, Holger Baars, Ronny Engelmann, Dietrich Althausen, Albert Ansmann, Stephanie Bohlmann, Birgit Heese, Julian Hofer, Thomas Kanitz, Moritz Haarig, Kevin Ohneiser, Martin Radenz, Patric Seifert, Annett Skupin, Zhenping Yin, Sabur F. Abdullaev, Mika Komppula, Maria Filioglou, Elina Giannakaki, Iwona S. Stachlewska, Lucja Janicka, Daniele Bortoli, Eleni Marinou, Vassilis Amiridis, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Boris Barja, and Ulla Wandinger
Atmos. Meas. Tech., 16, 2353–2379, https://doi.org/10.5194/amt-16-2353-2023, https://doi.org/10.5194/amt-16-2353-2023, 2023
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DeLiAn is a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio) and the Ångström exponent. The data collection is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarization lidar measurements and currently covers two wavelengths, 355 and 532 nm, for 13 aerosol categories ranging from basic aerosol types to mixtures.
Yun He, Zhenping Yin, Albert Ansmann, Fuchao Liu, Longlong Wang, Dongzhe Jing, and Huijia Shen
Atmos. Meas. Tech., 16, 1951–1970, https://doi.org/10.5194/amt-16-1951-2023, https://doi.org/10.5194/amt-16-1951-2023, 2023
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With the AERONET database, this study derives dust-related conversion factors at oceanic sites used in the POLIPHON method, which can convert lidar-retrieved dust extinction to ice-nucleating particle (INP)- and cloud condensation nuclei (CCN)-relevant parameters. The particle linear depolarization ratio in the AERONET aerosol inversion product is used to identify dust data points. The derived conversion factors can be applied to inverse 3-D global distributions of dust-related INPCs and CCNCs.
Kevin Ohneiser, Albert Ansmann, Jonas Witthuhn, Hartwig Deneke, Alexandra Chudnovsky, Gregor Walter, and Fabian Senf
Atmos. Chem. Phys., 23, 2901–2925, https://doi.org/10.5194/acp-23-2901-2023, https://doi.org/10.5194/acp-23-2901-2023, 2023
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This study shows that smoke layers can reach the tropopause via the self-lofting effect within 3–7 d in the absence of pyrocumulonimbus convection if the
aerosol optical thickness is larger than approximately 2 for a longer time period. When reaching the stratosphere, wildfire smoke can sensitively influence the stratospheric composition on a hemispheric scale and thus can affect the Earth’s climate and the ozone layer.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
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Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
Eleni Drakaki, Vassilis Amiridis, Alexandra Tsekeri, Antonis Gkikas, Emmanouil Proestakis, Sotirios Mallios, Stavros Solomos, Christos Spyrou, Eleni Marinou, Claire L. Ryder, Demetri Bouris, and Petros Katsafados
Atmos. Chem. Phys., 22, 12727–12748, https://doi.org/10.5194/acp-22-12727-2022, https://doi.org/10.5194/acp-22-12727-2022, 2022
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State-of-the-art atmospheric dust models have limitations in accounting for a realistic dust size distribution (emission, transport). We modify the parameterization of the mineral dust cycle by including particles with diameter >20 μm, as indicated by observations over deserts. Moreover, we investigate the effects of reduced settling velocities of dust particles. Model results are evaluated using airborne and spaceborne dust measurements above Cabo Verde.
Albert Ansmann, Kevin Ohneiser, Alexandra Chudnovsky, Daniel A. Knopf, Edwin W. Eloranta, Diego Villanueva, Patric Seifert, Martin Radenz, Boris Barja, Félix Zamorano, Cristofer Jimenez, Ronny Engelmann, Holger Baars, Hannes Griesche, Julian Hofer, Dietrich Althausen, and Ulla Wandinger
Atmos. Chem. Phys., 22, 11701–11726, https://doi.org/10.5194/acp-22-11701-2022, https://doi.org/10.5194/acp-22-11701-2022, 2022
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For the first time we present a systematic study on the impact of wildfire smoke on ozone depletion in the Arctic (2020) and Antarctic stratosphere (2020, 2021). Two major fire events in Siberia and Australia were responsible for the observed record-breaking stratospheric smoke pollution. Our analyses were based on lidar observations of smoke parameters (Polarstern, Punta Arenas) and NDACC Arctic and Antarctic ozone profiles as well as on Antarctic OMI satellite observations of column ozone.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Kevin Ohneiser, Albert Ansmann, Bernd Kaifler, Alexandra Chudnovsky, Boris Barja, Daniel A. Knopf, Natalie Kaifler, Holger Baars, Patric Seifert, Diego Villanueva, Cristofer Jimenez, Martin Radenz, Ronny Engelmann, Igor Veselovskii, and Félix Zamorano
Atmos. Chem. Phys., 22, 7417–7442, https://doi.org/10.5194/acp-22-7417-2022, https://doi.org/10.5194/acp-22-7417-2022, 2022
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We present and discuss 2 years of long-term lidar observations of the largest stratospheric perturbation by wildfire smoke ever observed. The smoke originated from the record-breaking Australian fires in 2019–2020 and affects climate conditions and even the ozone layer in the Southern Hemisphere. The obvious link between dense smoke occurrence in the stratosphere and strong ozone depletion found in the Arctic and in the Antarctic in 2020 can be regarded as a new aspect of climate change.
Goutam Choudhury, Albert Ansmann, and Matthias Tesche
Atmos. Chem. Phys., 22, 7143–7161, https://doi.org/10.5194/acp-22-7143-2022, https://doi.org/10.5194/acp-22-7143-2022, 2022
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Lidars provide height-resolved type-specific aerosol properties and are key in studying vertically collocated aerosols and clouds. In this study, we compare the aerosol number concentrations derived from spaceborne lidar with the in situ flight measurements. Our results show a reasonable agreement between both datasets. Such an agreement has not been achieved yet. It shows the potential of spaceborne lidar in studying aerosol–cloud interactions, which is needed to improve our climate forecasts.
Igor Veselovskii, Qiaoyun Hu, Albert Ansmann, Philippe Goloub, Thierry Podvin, and Mikhail Korenskiy
Atmos. Chem. Phys., 22, 5209–5221, https://doi.org/10.5194/acp-22-5209-2022, https://doi.org/10.5194/acp-22-5209-2022, 2022
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A remote sensing method based on fluorescence lidar measurements can detect and quantify the smoke content in the upper troposphere and inside cirrus clouds. Based on two case studies, we demonstrate that the fluorescence lidar technique provides the possibility to estimate the smoke surface area concentration within freshly formed cirrus layers. This value was used in a smoke ice nucleating particle parameterization scheme to predict ice crystal number concentrations in cirrus generation cells.
Michaël Sicard, Carmen Córdoba-Jabonero, María-Ángeles López-Cayuela, Albert Ansmann, Adolfo Comerón, María-Paz Zorzano, Alejandro Rodríguez-Gómez, and Constantino Muñoz-Porcar
Atmos. Chem. Phys., 22, 1921–1937, https://doi.org/10.5194/acp-22-1921-2022, https://doi.org/10.5194/acp-22-1921-2022, 2022
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This paper completes the companion paper of Córdoba-Jabonero et al. (2021). We estimate the total direct radiative effect produced by mineral dust particles during the June 2019 mega-heatwave at two sites in Spain and Germany. The results show that the dust particles in the atmosphere contribute to cooling the surface (less radiation reaches the surface) and that the heatwave (parametrized by high surface and air temperatures) contributes to reducing this cooling.
Jerónimo Escribano, Enza Di Tomaso, Oriol Jorba, Martina Klose, Maria Gonçalves Ageitos, Francesca Macchia, Vassilis Amiridis, Holger Baars, Eleni Marinou, Emmanouil Proestakis, Claudia Urbanneck, Dietrich Althausen, Johannes Bühl, Rodanthi-Elisavet Mamouri, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 22, 535–560, https://doi.org/10.5194/acp-22-535-2022, https://doi.org/10.5194/acp-22-535-2022, 2022
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We explore the benefits and consistency in adding lidar dust observations in a dust optical depth assimilation. We show that adding lidar data to a dust optical depth assimilation has valuable benefits and the dust analysis improves. We discuss the impact of the narrow satellite footprint of the lidar dust observations on the assimilation.
Moritz Haarig, Albert Ansmann, Ronny Engelmann, Holger Baars, Carlos Toledano, Benjamin Torres, Dietrich Althausen, Martin Radenz, and Ulla Wandinger
Atmos. Chem. Phys., 22, 355–369, https://doi.org/10.5194/acp-22-355-2022, https://doi.org/10.5194/acp-22-355-2022, 2022
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The irregular shape of dust particles makes it difficult to treat them correctly in optical models. Atmospheric measurements of dust optical properties are therefore of great importance. The present study increases the space of observed parameters from 355 and 532 nm towards 1064 nm, which is of special importance for large dust particles. The lidar ratio influenced by mineralogy and the depolarization ratio influenced by shape are measured for the first time at all three wavelengths.
Martin Radenz, Johannes Bühl, Patric Seifert, Holger Baars, Ronny Engelmann, Boris Barja González, Rodanthi-Elisabeth Mamouri, Félix Zamorano, and Albert Ansmann
Atmos. Chem. Phys., 21, 17969–17994, https://doi.org/10.5194/acp-21-17969-2021, https://doi.org/10.5194/acp-21-17969-2021, 2021
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This study brings together long-term ground-based remote-sensing observations of mixed-phase clouds at three key locations of aerosol–cloud interactions in the Northern and Southern Hemisphere midlatitudes. The findings contribute several new aspects on the nature of the excess of supercooled liquid clouds in the Southern Hemisphere, such as a long-term lidar-based estimate of ice-nucleating particle profiles as well as the effects of boundary layer coupling and gravity waves on ice formation.
Sebastian Düsing, Albert Ansmann, Holger Baars, Joel C. Corbin, Cyrielle Denjean, Martin Gysel-Beer, Thomas Müller, Laurent Poulain, Holger Siebert, Gerald Spindler, Thomas Tuch, Birgit Wehner, and Alfred Wiedensohler
Atmos. Chem. Phys., 21, 16745–16773, https://doi.org/10.5194/acp-21-16745-2021, https://doi.org/10.5194/acp-21-16745-2021, 2021
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The work deals with optical properties of aerosol particles in dried and atmospheric states. Based on two measurement campaigns in the rural background of central Europe, different measurement approaches were compared with each other, such as modeling based on Mie theory and direct in situ or remote sensing measurements. Among others, it was shown that the aerosol extinction-to-backscatter ratio is relative humidity dependent, and refinement with respect to the model input parameters is needed.
Kevin Ohneiser, Albert Ansmann, Alexandra Chudnovsky, Ronny Engelmann, Christoph Ritter, Igor Veselovskii, Holger Baars, Henriette Gebauer, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, and Marion Maturilli
Atmos. Chem. Phys., 21, 15783–15808, https://doi.org/10.5194/acp-21-15783-2021, https://doi.org/10.5194/acp-21-15783-2021, 2021
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The highlight of the lidar measurements during the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition of the German icebreaker Polarstern (October 2019–October 2020) was the detection of a persistent, 10 km deep Siberian wildfire smoke layer in the upper troposphere and lower stratosphere (UTLS) from about 7–8 km to 17–18 km height that could potentially have impacted the record-breaking ozone depletion over the Arctic in the spring of 2020.
Ronny Engelmann, Albert Ansmann, Kevin Ohneiser, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, Marion Maturilli, Igor Veselovskii, Cristofer Jimenez, Robert Wiesen, Holger Baars, Johannes Bühl, Henriette Gebauer, Moritz Haarig, Patric Seifert, Ulla Wandinger, and Andreas Macke
Atmos. Chem. Phys., 21, 13397–13423, https://doi.org/10.5194/acp-21-13397-2021, https://doi.org/10.5194/acp-21-13397-2021, 2021
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A Raman lidar was operated aboard the icebreaker Polarstern during MOSAiC and monitored aerosol and cloud layers in the central Arctic up to 30 km height. The article provides an overview of the spectrum of aerosol profiling observations and shows aerosol–cloud interaction studies for liquid-water and ice clouds. A highlight was the detection of a 10 km deep wildfire smoke layer over the North Pole up to 17 km height from the fire season of 2019, which persisted over the whole winter period.
Carmen Córdoba-Jabonero, Albert Ansmann, Cristofer Jiménez, Holger Baars, María-Ángeles López-Cayuela, and Ronny Engelmann
Atmos. Meas. Tech., 14, 5225–5239, https://doi.org/10.5194/amt-14-5225-2021, https://doi.org/10.5194/amt-14-5225-2021, 2021
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An experimental assessment of a polarized micro-pulse lidar (P-MPL) in comparison to reference lidars is presented regarding the retrieval of aerosol optical properties. The evaluation is focused on both the optimally determined overlap function and volume linear depolarization ratio. A P-MPL overlap must be regularly estimated to derive suitable aerosol products (backscatter, extinction, and particle depolarization ratio). This methodology can be easily applied to other P-MPL systems.
Hannes J. Griesche, Kevin Ohneiser, Patric Seifert, Martin Radenz, Ronny Engelmann, and Albert Ansmann
Atmos. Chem. Phys., 21, 10357–10374, https://doi.org/10.5194/acp-21-10357-2021, https://doi.org/10.5194/acp-21-10357-2021, 2021
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Heterogeneous ice formation in Arctic mixed-phase clouds under consideration of their surface-coupling state is investigated. Cloud phase and macrophysical properties were determined by means of lidar and cloud radar measurements, the coupling state, and cloud minimum temperature by radiosonde profiles. Above −15 °C cloud minimum temperature, surface-coupled clouds are more likely to contain ice by a factor of 2–6. By means of a literature survey, causes of the observed effects are discussed.
Albert Ansmann, Kevin Ohneiser, Rodanthi-Elisavet Mamouri, Daniel A. Knopf, Igor Veselovskii, Holger Baars, Ronny Engelmann, Andreas Foth, Cristofer Jimenez, Patric Seifert, and Boris Barja
Atmos. Chem. Phys., 21, 9779–9807, https://doi.org/10.5194/acp-21-9779-2021, https://doi.org/10.5194/acp-21-9779-2021, 2021
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We present retrievals of tropospheric and stratospheric height profiles of particle mass, volume, surface area concentration of wildfire smoke layers, and related cloud condensation nuclei (CCN) and ice-nucleating particle (INP) concentrations. The new analysis scheme is applied to ground-based lidar observations of stratospheric Australian smoke over southern South America and to spaceborne lidar observations of tropospheric North American smoke.
Carmen Córdoba-Jabonero, Michaël Sicard, María-Ángeles López-Cayuela, Albert Ansmann, Adolfo Comerón, María-Paz Zorzano, Alejandro Rodríguez-Gómez, and Constantino Muñoz-Porcar
Atmos. Chem. Phys., 21, 6455–6479, https://doi.org/10.5194/acp-21-6455-2021, https://doi.org/10.5194/acp-21-6455-2021, 2021
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The particular pathway of dust outbreaks defines the aerosol scenario and short-wave (SW) dust direct radiative effect (DRE). The synergetic use of POLIPHON method with continuous P-MPL measurements allows SW DRE of coarse (Dc) and fine (Df) dust particles to be evaluated separately. A dust-induced cooling effect is found, and despite Dc usually being dominant in intense dust events, the Df contribution to the total DRE can be significant, being higher at the top of atmosphere than on surface.
Ville Vakkari, Holger Baars, Stephanie Bohlmann, Johannes Bühl, Mika Komppula, Rodanthi-Elisavet Mamouri, and Ewan James O'Connor
Atmos. Chem. Phys., 21, 5807–5820, https://doi.org/10.5194/acp-21-5807-2021, https://doi.org/10.5194/acp-21-5807-2021, 2021
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The depolarization ratio is a valuable parameter for aerosol categorization from remote sensing measurements. Here, we introduce particle depolarization ratio measurements at the 1565 nm wavelength, which is substantially longer than previously utilized wavelengths and enhances our capabilities to study the wavelength dependency of the particle depolarization ratio.
Cristofer Jimenez, Albert Ansmann, Ronny Engelmann, David Donovan, Aleksey Malinka, Jörg Schmidt, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 20, 15247–15263, https://doi.org/10.5194/acp-20-15247-2020, https://doi.org/10.5194/acp-20-15247-2020, 2020
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A novel lidar method to study cloud microphysical properties (of liquid water clouds) and to study aerosol–cloud interaction (ACI) is developed and presented in this paper. In Part 1, the theoretical framework including an error analysis is given together with an overview of the aerosol information that the same lidar system can obtain. The ACI concept based on aerosol and cloud information is also explained. Applications of the proposed approach to lidar measurements are presented in Part 2.
Cristofer Jimenez, Albert Ansmann, Ronny Engelmann, David Donovan, Aleksey Malinka, Patric Seifert, Robert Wiesen, Martin Radenz, Zhenping Yin, Johannes Bühl, Jörg Schmidt, Boris Barja, and Ulla Wandinger
Atmos. Chem. Phys., 20, 15265–15284, https://doi.org/10.5194/acp-20-15265-2020, https://doi.org/10.5194/acp-20-15265-2020, 2020
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Part 2 presents the application of the dual-FOV polarization lidar technique introduced in Part 1. A lidar system was upgraded with a second polarization telescope, and it was deployed at the southernmost tip of South America. A comparison with alternative remote sensing techniques and the evaluation of the aerosol–cloud–wind relation in a convective boundary layer in pristine marine conditions are presented in two case studies, demonstrating the potential of the approach for ACI studies.
Ourania Soupiona, Alexandros Papayannis, Panagiotis Kokkalis, Romanos Foskinis, Guadalupe Sánchez Hernández, Pablo Ortiz-Amezcua, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Papagiannopoulos, Stefanos Samaras, Silke Groß, Rodanthi-Elisavet Mamouri, Lucas Alados-Arboledas, Aldo Amodeo, and Basil Psiloglou
Atmos. Chem. Phys., 20, 15147–15166, https://doi.org/10.5194/acp-20-15147-2020, https://doi.org/10.5194/acp-20-15147-2020, 2020
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51 dust events over the Mediterranean from EARLINET were studied regarding the aerosol geometrical, optical and microphysical properties and radiative forcing. We found δp532 values of 0.24–0.28, LR532 values of 49–52 sr and AOT532 of 0.11–0.40. The aerosol mixing state was also examined. Depending on the dust properties, intensity and solar zenith angle, the estimated solar radiative forcing ranged from −59 to −22 W m−2 at the surface and from −24 to −1 W m−2 at the TOA (cooling effect).
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Hannes J. Griesche, Patric Seifert, Albert Ansmann, Holger Baars, Carola Barrientos Velasco, Johannes Bühl, Ronny Engelmann, Martin Radenz, Yin Zhenping, and Andreas Macke
Atmos. Meas. Tech., 13, 5335–5358, https://doi.org/10.5194/amt-13-5335-2020, https://doi.org/10.5194/amt-13-5335-2020, 2020
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In summer 2017, the research vessel Polarstern performed cruise PS106 to the Arctic north of Svalbard. In the frame of the cruise, remote-sensing observations of the atmosphere were performed on Polarstern to continuously monitor aerosol and clouds above the vessel. In our study, we present the deployed instrumentation and applied data analysis methods and provide case studies of the aerosol and cloud observations made during the cruise. Statistics of low-cloud occurrence are presented as well.
Nikolaos Papagiannopoulos, Giuseppe D'Amico, Anna Gialitaki, Nicolae Ajtai, Lucas Alados-Arboledas, Aldo Amodeo, Vassilis Amiridis, Holger Baars, Dimitris Balis, Ioannis Binietoglou, Adolfo Comerón, Davide Dionisi, Alfredo Falconieri, Patrick Fréville, Anna Kampouri, Ina Mattis, Zoran Mijić, Francisco Molero, Alex Papayannis, Gelsomina Pappalardo, Alejandro Rodríguez-Gómez, Stavros Solomos, and Lucia Mona
Atmos. Chem. Phys., 20, 10775–10789, https://doi.org/10.5194/acp-20-10775-2020, https://doi.org/10.5194/acp-20-10775-2020, 2020
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Volcanic and desert dust particles affect human activities in manifold ways; consequently, mitigation tools are important. Their early detection and the issuance of early warnings are key elements in the initiation of operational response procedures. A methodology for the early warning of these hazards using European Aerosol Research Lidar Network (EARLINET) data is presented. The tailored product is investigated during a volcanic eruption and mineral dust advected in the eastern Mediterranean.
Julian Hofer, Albert Ansmann, Dietrich Althausen, Ronny Engelmann, Holger Baars, Khanneh Wadinga Fomba, Ulla Wandinger, Sabur F. Abdullaev, and Abduvosit N. Makhmudov
Atmos. Chem. Phys., 20, 9265–9280, https://doi.org/10.5194/acp-20-9265-2020, https://doi.org/10.5194/acp-20-9265-2020, 2020
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For the first time, a dense data set of particle extinction-to-backscatter ratios (lidar ratios), depolarization ratios, and backscatter- and extinction-related Ångström exponents for a Central Asian site are presented. The observations were performed with a continuously running multiwavelength polarization Raman lidar at Dushanbe, Tajikistan, during an 18-month campaign. The found optical properties reflect the large range of occurring aerosol mixtures.
Kevin Ohneiser, Albert Ansmann, Holger Baars, Patric Seifert, Boris Barja, Cristofer Jimenez, Martin Radenz, Audrey Teisseire, Athina Floutsi, Moritz Haarig, Andreas Foth, Alexandra Chudnovsky, Ronny Engelmann, Félix Zamorano, Johannes Bühl, and Ulla Wandinger
Atmos. Chem. Phys., 20, 8003–8015, https://doi.org/10.5194/acp-20-8003-2020, https://doi.org/10.5194/acp-20-8003-2020, 2020
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Unique lidar observations of a strong perturbation in stratospheric aerosol conditions in the Southern Hemisphere caused by the extreme Australian bushfires in 2019–2020 are presented. One of the main goals of this article is to provide the CALIPSO and Aeolus spaceborne lidar science teams with basic input parameters (lidar ratios, depolarization ratios) for a trustworthy documentation of this record-breaking event.
Athena Augusta Floutsi, Holger Baars, Martin Radenz, Moritz Haarig, Zhenping Yin, Patric Seifert, Cristofer Jimenez, Ulla Wandinger, Ronny Engelmann, Boris Barja, Felix Zamorano, and Albert Ansmann
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-453, https://doi.org/10.5194/acp-2020-453, 2020
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Julian Hofer, Albert Ansmann, Dietrich Althausen, Ronny Engelmann, Holger Baars, Sabur F. Abdullaev, and Abduvosit N. Makhmudov
Atmos. Chem. Phys., 20, 4695–4711, https://doi.org/10.5194/acp-20-4695-2020, https://doi.org/10.5194/acp-20-4695-2020, 2020
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For the first time, continuous, vertically resolved long-term aerosol measurements were conducted with a state-of-the-art multiwavelength lidar over a Central Asian site. Such observations are urgently required in efforts to predict future climate and environmental conditions and to support spaceborne remote sensing (ground truth activities).
Elina Giannakaki, Panos Kokkalis, Eleni Marinou, Nikolaos S. Bartsotas, Vassilis Amiridis, Albert Ansmann, and Mika Komppula
Atmos. Meas. Tech., 13, 893–905, https://doi.org/10.5194/amt-13-893-2020, https://doi.org/10.5194/amt-13-893-2020, 2020
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A new method, called ElEx, is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. Comparisons with both Raman lidar profiles during nightime and sun photometer daytime aerosol optical depth observations demonstrate the potential of the ElEx methodology.
Johannes Bühl, Patric Seifert, Martin Radenz, Holger Baars, and Albert Ansmann
Atmos. Meas. Tech., 12, 6601–6617, https://doi.org/10.5194/amt-12-6601-2019, https://doi.org/10.5194/amt-12-6601-2019, 2019
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In the present paper, we present a novel remote-sensing technique for the measurement of ice crystal number concentrations in clouds. The fall velocity of ice crystals measured with values from cloud radar and a radar wind profiler is used in order to derive information about ice crystal size and number concentration. In contrast to existing methods based on the combination of lidar and cloud radar, the present method can also be used in optically thick clouds.
Albert Ansmann, Rodanthi-Elisavet Mamouri, Johannes Bühl, Patric Seifert, Ronny Engelmann, Julian Hofer, Argyro Nisantzi, James D. Atkinson, Zamin A. Kanji, Berko Sierau, Mihalis Vrekoussis, and Jean Sciare
Atmos. Chem. Phys., 19, 15087–15115, https://doi.org/10.5194/acp-19-15087-2019, https://doi.org/10.5194/acp-19-15087-2019, 2019
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For the first time, a closure study of the relationship between the ice-nucleating particle concentration (INPC) and ice crystal number concentration (ICNC) in altocumulus and cirrus layers, solely based on ground-based active remote sensing, is presented. The closure studies were conducted in Cyprus. A focus was on altocumulus and cirrus layers which developed in pronounced Saharan dust layers. The closure studies show that heterogeneous ice nucleation can play a dominant role in ice formation.
Holger Baars, Albert Ansmann, Kevin Ohneiser, Moritz Haarig, Ronny Engelmann, Dietrich Althausen, Ingrid Hanssen, Michael Gausa, Aleksander Pietruczuk, Artur Szkop, Iwona S. Stachlewska, Dongxiang Wang, Jens Reichardt, Annett Skupin, Ina Mattis, Thomas Trickl, Hannes Vogelmann, Francisco Navas-Guzmán, Alexander Haefele, Karen Acheson, Albert A. Ruth, Boyan Tatarov, Detlef Müller, Qiaoyun Hu, Thierry Podvin, Philippe Goloub, Igor Veselovskii, Christophe Pietras, Martial Haeffelin, Patrick Fréville, Michaël Sicard, Adolfo Comerón, Alfonso Javier Fernández García, Francisco Molero Menéndez, Carmen Córdoba-Jabonero, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Daniele Bortoli, Maria João Costa, Davide Dionisi, Gian Luigi Liberti, Xuan Wang, Alessia Sannino, Nikolaos Papagiannopoulos, Antonella Boselli, Lucia Mona, Giuseppe D'Amico, Salvatore Romano, Maria Rita Perrone, Livio Belegante, Doina Nicolae, Ivan Grigorov, Anna Gialitaki, Vassilis Amiridis, Ourania Soupiona, Alexandros Papayannis, Rodanthi-Elisaveth Mamouri, Argyro Nisantzi, Birgit Heese, Julian Hofer, Yoav Y. Schechner, Ulla Wandinger, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 15183–15198, https://doi.org/10.5194/acp-19-15183-2019, https://doi.org/10.5194/acp-19-15183-2019, 2019
Carlos Toledano, Benjamín Torres, Cristian Velasco-Merino, Dietrich Althausen, Silke Groß, Matthias Wiegner, Bernadett Weinzierl, Josef Gasteiger, Albert Ansmann, Ramiro González, David Mateos, David Farrel, Thomas Müller, Moritz Haarig, and Victoria E. Cachorro
Atmos. Chem. Phys., 19, 14571–14583, https://doi.org/10.5194/acp-19-14571-2019, https://doi.org/10.5194/acp-19-14571-2019, 2019
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Ground-based sun photometers have been used to analyze the properties of long-range transported Saharan dust over Barbados. The measurements were carried out as part of the Saharan Aerosol Long-Range Transport and Aerosol–Cloud-Interaction Experiment (SALTRACE), carried out in the Caribbean in 2013. A variety of instruments, ground-based and airborne, were used in this research. In this paper, the sun photometer data are presented and related to data collected from other co-located instruments.
Moritz Haarig, Adrian Walser, Albert Ansmann, Maximilian Dollner, Dietrich Althausen, Daniel Sauer, David Farrell, and Bernadett Weinzierl
Atmos. Chem. Phys., 19, 13773–13788, https://doi.org/10.5194/acp-19-13773-2019, https://doi.org/10.5194/acp-19-13773-2019, 2019
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Aerosol particles are necessary in forming a cloud droplet. In order to improve studies of cloud formation, the aerosol load and type below a cloud has to be measured without disturbing the cloud. The lidar is a perfect tool for this purpose, as it provides a vertical profile of the aerosol particles from the ground. We validated the lidar retrieval of cloud-relevant aerosol properties like particle number concentrations with airborne in situ measurements in the Saharan Air Layer at Barbados.
Zhenping Yin, Albert Ansmann, Holger Baars, Patric Seifert, Ronny Engelmann, Martin Radenz, Cristofer Jimenez, Alina Herzog, Kevin Ohneiser, Karsten Hanbuch, Luc Blarel, Philippe Goloub, Gaël Dubois, Stephane Victori, and Fabrice Maupin
Atmos. Meas. Tech., 12, 5685–5698, https://doi.org/10.5194/amt-12-5685-2019, https://doi.org/10.5194/amt-12-5685-2019, 2019
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A new shipborne Sun–sky–lunar photometer was validated through comparisons with collocated MICROTOPS II and multiwavelength Raman polarization lidar measurements during two trans-Atlantic cruises. A full diurnal cycle of mixed dust–smoke episode was captured by both the shipborne photometer and lidar. The coefficient of determination for the linear regression between MICROTOPS II and the shipborne photometer was 0.993 for AOD at 500 nm based on the entire dataset.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Ioannis Binietoglou, Albert Ansmann, Ulla Wandinger, Julian Hofer, John Yorks, Edward Nowottnick, Abduvosit Makhmudov, Alexandros Papayannis, Aleksander Pietruczuk, Anna Gialitaki, Arnoud Apituley, Artur Szkop, Constantino Muñoz Porcar, Daniele Bortoli, Davide Dionisi, Dietrich Althausen, Dimitra Mamali, Dimitris Balis, Doina Nicolae, Eleni Tetoni, Gian Luigi Liberti, Holger Baars, Ina Mattis, Iwona Sylwia Stachlewska, Kalliopi Artemis Voudouri, Lucia Mona, Maria Mylonaki, Maria Rita Perrone, Maria João Costa, Michael Sicard, Nikolaos Papagiannopoulos, Nikolaos Siomos, Pasquale Burlizzi, Rebecca Pauly, Ronny Engelmann, Sabur Abdullaev, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 11743–11764, https://doi.org/10.5194/acp-19-11743-2019, https://doi.org/10.5194/acp-19-11743-2019, 2019
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To increase accuracy and validate satellite-based products, comparison with ground-based reference observations is required. To do this, we present evaluation activity of EARLINET for the qualitative and quantitative assessment of NASA's CATS lidar operating aboard the International Space Station (ISS) while identified discrepancies are discussed. Better understanding CATS performance and limitations provides a valuable basis for scientific studies implementing the satellite-based lidar system.
Albert Ansmann, Rodanthi-Elisavet Mamouri, Julian Hofer, Holger Baars, Dietrich Althausen, and Sabur F. Abdullaev
Atmos. Meas. Tech., 12, 4849–4865, https://doi.org/10.5194/amt-12-4849-2019, https://doi.org/10.5194/amt-12-4849-2019, 2019
Eleni Marinou, Matthias Tesche, Athanasios Nenes, Albert Ansmann, Jann Schrod, Dimitra Mamali, Alexandra Tsekeri, Michael Pikridas, Holger Baars, Ronny Engelmann, Kalliopi-Artemis Voudouri, Stavros Solomos, Jean Sciare, Silke Groß, Florian Ewald, and Vassilis Amiridis
Atmos. Chem. Phys., 19, 11315–11342, https://doi.org/10.5194/acp-19-11315-2019, https://doi.org/10.5194/acp-19-11315-2019, 2019
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We assess the feasibility of ground-based and spaceborne lidars to retrieve profiles of cloud-relevant aerosol concentrations and ice-nucleating particles. The retrieved profiles are in good agreement with airborne in situ measurements. Our methodology will be applied to satellite observations in the future so as to provide a global 3D product of cloud-relevant properties.
Andreas Foth, Thomas Kanitz, Ronny Engelmann, Holger Baars, Martin Radenz, Patric Seifert, Boris Barja, Michael Fromm, Heike Kalesse, and Albert Ansmann
Atmos. Chem. Phys., 19, 6217–6233, https://doi.org/10.5194/acp-19-6217-2019, https://doi.org/10.5194/acp-19-6217-2019, 2019
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In this study, we present the vertical aerosol distribution in the pristine region of the southern tip of South America determined by ground-based and spaceborne lidar observations. Most aerosol load is contained within the planetary boundary layer up to about 1200 m. The free troposphere is characterized by a very low aerosol concentration but a frequent occurrence of clouds. Lofted aerosol layers were rarely observed and, when present, were characterized by very low optical thicknesses.
Stavros Solomos, Abdelgadir Abuelgasim, Christos Spyrou, Ioannis Binietoglou, and Slobodan Nickovic
Geosci. Model Dev., 12, 979–988, https://doi.org/10.5194/gmd-12-979-2019, https://doi.org/10.5194/gmd-12-979-2019, 2019
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In this research we developed a time-dependent dust source map for NMME-DREAM v1.0 model based on the MODIS Normalized Digital Vegetation Index (NDVI). Areas with NDVI < 0.1 are classified as active dust sources. The new modeling system is tested for the analysis of dust particle dispersion over SW Asia using a mesoscale model grid increment of 0.1° × 0.1° km for a period of 1 year. Simulated AOD increased compared to the static dust source approach and there was an increase in dust loads.
Cristofer Jimenez, Albert Ansmann, Ronny Engelmann, Moritz Haarig, Jörg Schmidt, and Ulla Wandinger
Atmos. Meas. Tech., 12, 1077–1093, https://doi.org/10.5194/amt-12-1077-2019, https://doi.org/10.5194/amt-12-1077-2019, 2019
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We propose an extended formalism for a full instrumental characterization of a three-channel lidar system, allowing the retrieval of highly accurate linear depolarization profiles. The results obtained at several depolarizing scenarios, the good agreement with the retrievals of a second collocated calibrated lidar system, and the long-term stability of the calibration parameters corroborate the potential and robustness of the new technique.
Evagoras Evagorou, Christodoulos Mettas, Athos Agapiou, Kyriacos Themistocleous, and Diofantos Hadjimitsis
Adv. Geosci., 45, 397–407, https://doi.org/10.5194/adgeo-45-397-2019, https://doi.org/10.5194/adgeo-45-397-2019, 2019
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Freely and open distributed optical satellite images used to obtain bathymetric data for shallow waters based on timeseries analysis of multispectral Sentinel-2 datasets. The ratio transform algorithm was implemented for twelve monthly images covering a year. Bathymetric maps were generated and compared with LIDAR measurements. The results showed that bathymetry can be obtained from satellite data within a Root Mean Square Error while more accurate results were generated during the summer.
Thomas Dimopoulos, Hristos Tyralis, Nikolaos P. Bakas, and Diofantos Hadjimitsis
Adv. Geosci., 45, 377–382, https://doi.org/10.5194/adgeo-45-377-2018, https://doi.org/10.5194/adgeo-45-377-2018, 2018
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The paper examines a machine learning algorithm (Random Forests) in comparison with Multivariate Linear Regression, for a data-set of 3500 transactions of residential apartments in Nicosia District in Cyprus. The methodology suggested, indicated high accuracy of the Random Forests Method, that can be applied in automated valuation models and CAMA systems.
Maroula N. Alverti, Kyriakos Themistocleous, Phaedon C. Kyriakidis, and Diofantos G. Hadjimitsis
Adv. Geosci., 45, 305–320, https://doi.org/10.5194/adgeo-45-305-2018, https://doi.org/10.5194/adgeo-45-305-2018, 2018
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The scientific objective is to find a simple understandable model linking human smart characteristics to a group of socio-demographic and urban environment indices, applied to the case of Limassol Urban Complex, Cyprus. The results reveal that the human smart characteristics are significantly correlated with demographic dynamics and built infrastructure characteristics. For instance creativity and open-mindedness appear in most densely urban areas.
Christos Stathopoulos, George Galanis, Nikolaos S. Bartsotas, and George Kallos
Adv. Geosci., 45, 289–294, https://doi.org/10.5194/adgeo-45-289-2018, https://doi.org/10.5194/adgeo-45-289-2018, 2018
Albert Ansmann, Holger Baars, Alexandra Chudnovsky, Ina Mattis, Igor Veselovskii, Moritz Haarig, Patric Seifert, Ronny Engelmann, and Ulla Wandinger
Atmos. Chem. Phys., 18, 11831–11845, https://doi.org/10.5194/acp-18-11831-2018, https://doi.org/10.5194/acp-18-11831-2018, 2018
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Extremely large light extinction coefficients of 500 Mm-1, about 20 times higher than after the Pinatubo volcanic eruptions in 1991, were observed by EARLINET lidars in the stratosphere over central Europe from 21 to 22 August, 2017. This paper provides an overview based on ground-based (lidar, AERONET) and satellite (MODIS, OMI) remote sensing.
Moritz Haarig, Albert Ansmann, Holger Baars, Cristofer Jimenez, Igor Veselovskii, Ronny Engelmann, and Dietrich Althausen
Atmos. Chem. Phys., 18, 11847–11861, https://doi.org/10.5194/acp-18-11847-2018, https://doi.org/10.5194/acp-18-11847-2018, 2018
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The worldwide only triple-wavelength polarization/Raman lidar was used to measure optical, microphysical, and morphological properties of aged Canadian wildfire smoke occurring in the troposphere and stratosphere over Leipzig, Germany, in August 2017. A strong contrast between the tropospheric and stratospheric smoke properties was found.
Carmen Córdoba-Jabonero, Michaël Sicard, Albert Ansmann, Ana del Águila, and Holger Baars
Atmos. Meas. Tech., 11, 4775–4795, https://doi.org/10.5194/amt-11-4775-2018, https://doi.org/10.5194/amt-11-4775-2018, 2018
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The high potential of the MPLNET polarized Micro-Pulse LiDAR (P-MPL) is demonstrated in synergy with the POLIPHON (POlarization-LIdar PHOtometer Networking) method to retrieve the vertical separation of both the optical and mass features of the dust, smoke and pollen components mixed with other aerosols. This synergetic procedure can be easily applied to the worldwide MPLNET lidar systems and to space-borne lidars: the ongoing NASA CALIPSO/CALIOP and the forthcoming ESA EarthCARE/ATLID.
Antonis Gkikas, Vincenzo Obiso, Carlos Pérez García-Pando, Oriol Jorba, Nikos Hatzianastassiou, Lluis Vendrell, Sara Basart, Stavros Solomos, Santiago Gassó, and José Maria Baldasano
Atmos. Chem. Phys., 18, 8757–8787, https://doi.org/10.5194/acp-18-8757-2018, https://doi.org/10.5194/acp-18-8757-2018, 2018
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The present study investigates the direct radiative effects (DREs), induced during 20 intense Mediterranean desert dust outbreaks, based on regional short-term numerical simulations of the NMMB-MONARCH model: more specifically, (i) the DREs and their associated impacts on temperature and surface sensible and latent heat fluxes, (ii) the feedbacks on dust AOD and dust emissions, and (iii) the possible improvements in short-term forecasts (up to 84 h) of temperature and radiation.
Dimitra Mamali, Eleni Marinou, Jean Sciare, Michael Pikridas, Panagiotis Kokkalis, Michael Kottas, Ioannis Binietoglou, Alexandra Tsekeri, Christos Keleshis, Ronny Engelmann, Holger Baars, Albert Ansmann, Vassilis Amiridis, Herman Russchenberg, and George Biskos
Atmos. Meas. Tech., 11, 2897–2910, https://doi.org/10.5194/amt-11-2897-2018, https://doi.org/10.5194/amt-11-2897-2018, 2018
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The paper's scope is to evaluate the performance of in situ atmospheric aerosol instrumentation on board unmanned aerial vehicles (UAVs) and the performance of algorithms used to calculate the aerosol mass from remote sensing instruments by comparing the two independent techniques to each other. Our results indicate that UAV-based aerosol measurements (using specific in situ and remote sensing instrumentation) can provide reliable ways to determine the aerosol mass throughout the atmosphere.
Guangyao Dai, Dietrich Althausen, Julian Hofer, Ronny Engelmann, Patric Seifert, Johannes Bühl, Rodanthi-Elisavet Mamouri, Songhua Wu, and Albert Ansmann
Atmos. Meas. Tech., 11, 2735–2748, https://doi.org/10.5194/amt-11-2735-2018, https://doi.org/10.5194/amt-11-2735-2018, 2018
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The presented calibration method grants access to quality approved automated atmospheric water vapor profiles from lidar measurements. This method uses the Raman lidar data from the water vapor and nitrogen channels and additional data from sun photometer and GDAS. The retrieved water vapor profiles agree well with respective profiles from radio soundings. The paper describes this method and shows results from the CyCARE (Cyprus Cloud Aerosol and Rain Experiment) campaign in 2015–2017.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Aristeidis K. Georgoulias, Stavros Solomos, Stelios Kazadzis, Julien Chimot, Huizheng Che, Georgia Alexandri, Ioannis Binietoglou, Vasiliki Daskalopoulou, Konstantinos A. Kourtidis, Gerrit de Leeuw, and Ronald J. van der A
Atmos. Chem. Phys., 18, 1337–1362, https://doi.org/10.5194/acp-18-1337-2018, https://doi.org/10.5194/acp-18-1337-2018, 2018
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We provide a 3-D climatology of desert dust aerosols over South and East Asia, based on 9 years of CALIPSO observations and an EARLINET methodology. The results provide the horizontal, vertical and seasonal distribution of dust aerosols over SE Asia along with the change in dust transport pathways. The dataset is unique for its potential applications, including evaluation and assimilation activities in atmospheric simulations and the estimation of the climatic impact of dust aerosols.
Sebastian Düsing, Birgit Wehner, Patric Seifert, Albert Ansmann, Holger Baars, Florian Ditas, Silvia Henning, Nan Ma, Laurent Poulain, Holger Siebert, Alfred Wiedensohler, and Andreas Macke
Atmos. Chem. Phys., 18, 1263–1290, https://doi.org/10.5194/acp-18-1263-2018, https://doi.org/10.5194/acp-18-1263-2018, 2018
Alexandra Tsekeri, Anton Lopatin, Vassilis Amiridis, Eleni Marinou, Julia Igloffstein, Nikolaos Siomos, Stavros Solomos, Panagiotis Kokkalis, Ronny Engelmann, Holger Baars, Myrto Gratsea, Panagiotis I. Raptis, Ioannis Binietoglou, Nikolaos Mihalopoulos, Nikolaos Kalivitis, Giorgos Kouvarakis, Nikolaos Bartsotas, George Kallos, Sara Basart, Dirk Schuettemeyer, Ulla Wandinger, Albert Ansmann, Anatoli P. Chaikovsky, and Oleg Dubovik
Atmos. Meas. Tech., 10, 4995–5016, https://doi.org/10.5194/amt-10-4995-2017, https://doi.org/10.5194/amt-10-4995-2017, 2017
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The Generalized Aerosol Retrieval from Radiometer and Lidar Combined data algorithm (GARRLiC) and the LIdar-Radiometer Inversion Code (LIRIC) provide the opportunity to study the aerosol vertical distribution by combining ground-based lidar and sun-photometric measurements. Here, we utilize the capabilities of both algorithms for the characterization of Saharan dust and marine particles, along with their mixtures, in the south-eastern Mediterranean.
Albert Ansmann, Franziska Rittmeister, Ronny Engelmann, Sara Basart, Oriol Jorba, Christos Spyrou, Samuel Remy, Annett Skupin, Holger Baars, Patric Seifert, Fabian Senf, and Thomas Kanitz
Atmos. Chem. Phys., 17, 14987–15006, https://doi.org/10.5194/acp-17-14987-2017, https://doi.org/10.5194/acp-17-14987-2017, 2017
Julian Hofer, Dietrich Althausen, Sabur F. Abdullaev, Abduvosit N. Makhmudov, Bakhron I. Nazarov, Georg Schettler, Ronny Engelmann, Holger Baars, K. Wadinga Fomba, Konrad Müller, Bernd Heinold, Konrad Kandler, and Albert Ansmann
Atmos. Chem. Phys., 17, 14559–14577, https://doi.org/10.5194/acp-17-14559-2017, https://doi.org/10.5194/acp-17-14559-2017, 2017
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The Central Asian Dust Experiment provides unprecedented data on vertically resolved aerosol optical properties over Central Asia from continuous 18-month polarization Raman lidar observations in Dushanbe, Tajikistan. Central Asia is affected by climate change (e.g. glacier retreat) but in a large part missing vertically resolved aerosol measurements, which would help to better understand transport of dust and pollution aerosol across Central Asia and their influence on climate and health.
Moritz Haarig, Albert Ansmann, Josef Gasteiger, Konrad Kandler, Dietrich Althausen, Holger Baars, Martin Radenz, and David A. Farrell
Atmos. Chem. Phys., 17, 14199–14217, https://doi.org/10.5194/acp-17-14199-2017, https://doi.org/10.5194/acp-17-14199-2017, 2017
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The depolarization ratio and the backscatter coefficient of marine particles are correlated with the relative humidity. The measurements were performed under atmospheric conditions with a multi-wavelength lidar system in pure marine conditions over Barbados in February 2014. For RH < 50 % the sea salt particles have a cubic-like shape resulting in an enhanced depolarization ratio of up to 0.15. This agrees with model results of cubic sea salt. The extinction enhancement f(RH) factor was derived.
Franziska Rittmeister, Albert Ansmann, Ronny Engelmann, Annett Skupin, Holger Baars, Thomas Kanitz, and Stefan Kinne
Atmos. Chem. Phys., 17, 12963–12983, https://doi.org/10.5194/acp-17-12963-2017, https://doi.org/10.5194/acp-17-12963-2017, 2017
Rodanthi-Elisavet Mamouri and Albert Ansmann
Atmos. Meas. Tech., 10, 3403–3427, https://doi.org/10.5194/amt-10-3403-2017, https://doi.org/10.5194/amt-10-3403-2017, 2017
Moritz Haarig, Albert Ansmann, Dietrich Althausen, André Klepel, Silke Groß, Volker Freudenthaler, Carlos Toledano, Rodanthi-Elisavet Mamouri, David A. Farrell, Damien A. Prescod, Eleni Marinou, Sharon P. Burton, Josef Gasteiger, Ronny Engelmann, and Holger Baars
Atmos. Chem. Phys., 17, 10767–10794, https://doi.org/10.5194/acp-17-10767-2017, https://doi.org/10.5194/acp-17-10767-2017, 2017
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Our measurements performed with a lidar on Barbados give a vertical profile of Saharan dust, which was transported over 5000 km across the Atlantic. The new triple-wavelength depolarization technique reveals more information about the shape and size of dust, which will improve our understanding of the aging process of dust in the atmosphere and its representation in dust models. Changing properties of dust particles influence the solar radiation and the cloud properties and thus our climate.
Panagiotis G. Kosmopoulos, Stelios Kazadzis, Michael Taylor, Eleni Athanasopoulou, Orestis Speyer, Panagiotis I. Raptis, Eleni Marinou, Emmanouil Proestakis, Stavros Solomos, Evangelos Gerasopoulos, Vassilis Amiridis, Alkiviadis Bais, and Charalabos Kontoes
Atmos. Meas. Tech., 10, 2435–2453, https://doi.org/10.5194/amt-10-2435-2017, https://doi.org/10.5194/amt-10-2435-2017, 2017
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We study the impact of dust on solar energy using remote sensing data in conjunction with synergistic modelling and forecasting techniques. Under high aerosol loads, we found great solar energy losses of the order of 80 and 50% for concentrated solar power and photovoltaic installations, respectively. The 1-day forecast presented an overall accuracy within 10% in direct comparison to the real conditions under high energy potential, optimising the efficient energy planning and policies.
Johannes Bühl, Patric Seifert, Ronny Engelmann, Julia Fruntke, and Albert Ansmann
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-230, https://doi.org/10.5194/acp-2017-230, 2017
Revised manuscript not accepted
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Vertical air motion is a key driver of physical processes in clouds. The stability of clouds and the process of ice formation have been shown to depend critically on vertical air motions. However, observations of vertical air motions and ice formation in clouds are rare. This motivated us in the Up- and downdraft in Drop and Ice Nucleation Experiment (UDINE) to deliver a comprehensive statistics, connecting remote-sensing observations of vertical motions and ice formation.
Eleni Marinou, Vassilis Amiridis, Ioannis Binietoglou, Athanasios Tsikerdekis, Stavros Solomos, Emannouil Proestakis, Dimitra Konsta, Nikolaos Papagiannopoulos, Alexandra Tsekeri, Georgia Vlastou, Prodromos Zanis, Dimitrios Balis, Ulla Wandinger, and Albert Ansmann
Atmos. Chem. Phys., 17, 5893–5919, https://doi.org/10.5194/acp-17-5893-2017, https://doi.org/10.5194/acp-17-5893-2017, 2017
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We provide a 3D multiyear analysis on the evolution of Saharan dust over Europe, using a dust product retrieved from the CALIPSO satellite and using EARLINET methods. The results reveal for the first time the 9-year 3D seasonal patterns of dust over its transport paths from the Sahara towards the Mediterranean. The dataset is unique with respect to its potential applications, including the evaluation of dust models and the estimation of ice nuclei concentration profiles from space.
Jann Schrod, Daniel Weber, Jaqueline Drücke, Christos Keleshis, Michael Pikridas, Martin Ebert, Bojan Cvetković, Slobodan Nickovic, Eleni Marinou, Holger Baars, Albert Ansmann, Mihalis Vrekoussis, Nikos Mihalopoulos, Jean Sciare, Joachim Curtius, and Heinz G. Bingemer
Atmos. Chem. Phys., 17, 4817–4835, https://doi.org/10.5194/acp-17-4817-2017, https://doi.org/10.5194/acp-17-4817-2017, 2017
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In this paper we present data of ice-nucleating particles (INPs) from a 1-month campaign in the Eastern Mediterranean using unmanned aircraft systems (UASs, drones) and offline sampling with subsequent laboratory analysis. To our knowledge, this is the first time INPs were measured onboard a UAS. We find that INP concentrations were 1 magnitude higher aloft than at the ground, highlighting that surface-based measurement of INP may only be of limited significance for the situation at cloud level.
Stavros Solomos, Albert Ansmann, Rodanthi-Elisavet Mamouri, Ioannis Binietoglou, Platon Patlakas, Eleni Marinou, and Vassilis Amiridis
Atmos. Chem. Phys., 17, 4063–4079, https://doi.org/10.5194/acp-17-4063-2017, https://doi.org/10.5194/acp-17-4063-2017, 2017
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An extreme dust storm affected Middle East and the Eastern Mediterranean in September 2015. This event was produced by a combination of meteorological and land-use properties. Analysis with remote sensing observations and modeling simulations reveals (i) transport of warm moist air from the Red and Arabian seas, (ii) formation of a thermal low over Syria, (iii) convective outflows and haboob formation (i.e. propagating dust walls), and (iv) changes in land-use and dust erodibility due to war.
Evangelia Diapouli, Manousos I. Manousakas, Stergios Vratolis, Vasiliki Vasilatou, Stella Pateraki, Kyriaki A. Bairachtari, Xavier Querol, Fulvio Amato, Andrés Alastuey, Angeliki A. Karanasiou, Franco Lucarelli, Silvia Nava, Giulia Calzolai, Vorne L. Gianelle, Cristina Colombi, Célia Alves, Danilo Custódio, Casimiro Pio, Christos Spyrou, George B. Kallos, and Konstantinos Eleftheriadis
Atmos. Chem. Phys., 17, 3673–3685, https://doi.org/10.5194/acp-17-3673-2017, https://doi.org/10.5194/acp-17-3673-2017, 2017
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This study examined the contribution of two natural sources (long-range transport of African dust and sea salt) to the airborne particulate matter concentrations, in 5 southern European cities (Porto, Barcelona, Milan, Florence, Athens). The results demonstrated that natural sources are often expressed with high-intensity events, leading even to exceedances of the EU air quality standards. This effect was more pronounced in the case of African dust intrusions in the eastern Mediterranean area.
Christos S. Zerefos, Kostas Eleftheratos, John Kapsomenakis, Stavros Solomos, Antje Inness, Dimitris Balis, Alberto Redondas, Henk Eskes, Marc Allaart, Vassilis Amiridis, Arne Dahlback, Veerle De Bock, Henri Diémoz, Ronny Engelmann, Paul Eriksen, Vitali Fioletov, Julian Gröbner, Anu Heikkilä, Irina Petropavlovskikh, Janusz Jarosławski, Weine Josefsson, Tomi Karppinen, Ulf Köhler, Charoula Meleti, Christos Repapis, John Rimmer, Vladimir Savinykh, Vadim Shirotov, Anna Maria Siani, Andrew R. D. Smedley, Martin Stanek, and René Stübi
Atmos. Chem. Phys., 17, 551–574, https://doi.org/10.5194/acp-17-551-2017, https://doi.org/10.5194/acp-17-551-2017, 2017
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The paper makes a convincing case that the Brewer network is capable of detecting enhanced SO2 columns, as observed, e.g., after volcanic eruptions. For this reason, large volcanic eruptions of the past decade have been used to detect and forecast SO2 plumes of volcanic origin using the Brewer and other ground-based networks, aided by satellite, trajectory analysis calculations and modelling.
Alexandra Tsekeri, Vassilis Amiridis, Franco Marenco, Athanasios Nenes, Eleni Marinou, Stavros Solomos, Phil Rosenberg, Jamie Trembath, Graeme J. Nott, James Allan, Michael Le Breton, Asan Bacak, Hugh Coe, Carl Percival, and Nikolaos Mihalopoulos
Atmos. Meas. Tech., 10, 83–107, https://doi.org/10.5194/amt-10-83-2017, https://doi.org/10.5194/amt-10-83-2017, 2017
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The In situ/Remote sensing aerosol Retrieval Algorithm (IRRA) provides vertical profiles of aerosol optical, microphysical and hygroscopic properties from airborne in situ and remote sensing measurements. The algorithm is highly advantageous for aerosol characterization in humid conditions, employing the ISORROPIA II model for acquiring the particle hygroscopic growth. IRRA can find valuable applications in aerosol–cloud interaction schemes and in validation of active space-borne sensors.
Josef Gasteiger, Silke Groß, Daniel Sauer, Moritz Haarig, Albert Ansmann, and Bernadett Weinzierl
Atmos. Chem. Phys., 17, 297–311, https://doi.org/10.5194/acp-17-297-2017, https://doi.org/10.5194/acp-17-297-2017, 2017
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To study aerosol transport in the Saharan Air Layer (SAL) from Africa to the Caribbean, we combine advanced optical models of Saharan aerosols with Stokes settling and two hypotheses about the occurrence of vertical mixing. By testing our hypotheses with lidar and in situ profiles measured near the top of the transported SAL, we find strong evidence that vertical mixing occurs in the SAL over the Atlantic with significant consequences for size distribution of the transported Saharan aerosols.
Juan Antonio Bravo-Aranda, Livio Belegante, Volker Freudenthaler, Lucas Alados-Arboledas, Doina Nicolae, María José Granados-Muñoz, Juan Luis Guerrero-Rascado, Aldo Amodeo, Giusseppe D'Amico, Ronny Engelmann, Gelsomina Pappalardo, Panos Kokkalis, Rodanthy Mamouri, Alex Papayannis, Francisco Navas-Guzmán, Francisco José Olmo, Ulla Wandinger, Francesco Amato, and Martial Haeffelin
Atmos. Meas. Tech., 9, 4935–4953, https://doi.org/10.5194/amt-9-4935-2016, https://doi.org/10.5194/amt-9-4935-2016, 2016
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This work analyses the lidar polarizing sensitivity by means of the Stokes–Müller formalism and provides a new tool to quantify the systematic error of the volume linear depolarization ration (δ) using the Monte Carlo technique. Results evidence the importance of the lidar polarizing effects which can lead to systematic errors larger than 100 %. Additionally, we demonstrate that a proper lidar characterization helps to reduce the uncertainty.
Silke Groß, Josef Gasteiger, Volker Freudenthaler, Thomas Müller, Daniel Sauer, Carlos Toledano, and Albert Ansmann
Atmos. Chem. Phys., 16, 11535–11546, https://doi.org/10.5194/acp-16-11535-2016, https://doi.org/10.5194/acp-16-11535-2016, 2016
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Dual-wavelength depolarization sensitive Raman lidar measurements were used to characterize the optical properties of the dust loaded convective boundary layer over the Caribbean. Furthermore we derived the dust volume fraction and dust mass concentration within the convective boundary layer.
Moritz Haarig, Ronny Engelmann, Albert Ansmann, Igor Veselovskii, David N. Whiteman, and Dietrich Althausen
Atmos. Meas. Tech., 9, 4269–4278, https://doi.org/10.5194/amt-9-4269-2016, https://doi.org/10.5194/amt-9-4269-2016, 2016
Johannes Bühl, Patric Seifert, Alexander Myagkov, and Albert Ansmann
Atmos. Chem. Phys., 16, 10609–10620, https://doi.org/10.5194/acp-16-10609-2016, https://doi.org/10.5194/acp-16-10609-2016, 2016
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We probe thin layered clouds with remote sensing instruments from ground in order to get insight into atmospheric processes like the formation of rain or snow. We think that the findings of our work can be used to improve climate and weather simulations. The present paper presents a new technique that can be used to detect the shape, fall speed and mass of ice particles falling from layered clouds. With such information the impact of cloud ice, e.g., on the lifetime of a cloud, can be estimated.
Rodanthi-Elisavet Mamouri and Albert Ansmann
Atmos. Chem. Phys., 16, 5905–5931, https://doi.org/10.5194/acp-16-5905-2016, https://doi.org/10.5194/acp-16-5905-2016, 2016
Ronny Engelmann, Thomas Kanitz, Holger Baars, Birgit Heese, Dietrich Althausen, Annett Skupin, Ulla Wandinger, Mika Komppula, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Ina Mattis, Holger Linné, and Albert Ansmann
Atmos. Meas. Tech., 9, 1767–1784, https://doi.org/10.5194/amt-9-1767-2016, https://doi.org/10.5194/amt-9-1767-2016, 2016
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The atmospheric science community demands for autonomous and quality-assured vertically resolved measurements of aerosol and cloud properties. For this purpose, a portable lidar called Polly
was developed at TROPOS in 2003. This lidar type was continuously improved with gained experience from EARLINET, worldwide field campaigns, and institute collaborations within the last 10 years. We present recent changes to the setup of our portable multiwavelength Raman and polarization lidar PollyXT.
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
Anatoli Chaikovsky, Oleg Dubovik, Brent Holben, Andrey Bril, Philippe Goloub, Didier Tanré, Gelsomina Pappalardo, Ulla Wandinger, Ludmila Chaikovskaya, Sergey Denisov, Jan Grudo, Anton Lopatin, Yana Karol, Tatsiana Lapyonok, Vassilis Amiridis, Albert Ansmann, Arnoud Apituley, Lucas Allados-Arboledas, Ioannis Binietoglou, Antonella Boselli, Giuseppe D'Amico, Volker Freudenthaler, David Giles, María José Granados-Muñoz, Panayotis Kokkalis, Doina Nicolae, Sergey Oshchepkov, Alex Papayannis, Maria Rita Perrone, Alexander Pietruczuk, Francesc Rocadenbosch, Michaël Sicard, Ilya Slutsker, Camelia Talianu, Ferdinando De Tomasi, Alexandra Tsekeri, Janet Wagner, and Xuan Wang
Atmos. Meas. Tech., 9, 1181–1205, https://doi.org/10.5194/amt-9-1181-2016, https://doi.org/10.5194/amt-9-1181-2016, 2016
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This paper presents a detailed description of LIRIC (LIdar-Radiometer Inversion Code) algorithm for simultaneous processing of coincident lidar and radiometric observations for the retrieval of the aerosol concentrations. As the lidar/radiometric input data we use measurements from European Aerosol Research Lidar Network (EARLINET) lidars and collocated sun-photometers of Aerosol Robotic Network (AERONET). The LIRIC software package was implemented and tested at a number of EARLINET stations.
A. Skupin, A. Ansmann, R. Engelmann, P. Seifert, and T. Müller
Atmos. Chem. Phys., 16, 1863–1876, https://doi.org/10.5194/acp-16-1863-2016, https://doi.org/10.5194/acp-16-1863-2016, 2016
M. Jähn, D. Muñoz-Esparza, F. Chouza, O. Reitebuch, O. Knoth, M. Haarig, and A. Ansmann
Atmos. Chem. Phys., 16, 651–674, https://doi.org/10.5194/acp-16-651-2016, https://doi.org/10.5194/acp-16-651-2016, 2016
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Large eddy simulations (LESs) are performed for the area of the Caribbean island Barbados to investigate island effects on boundary layer modification, cloud generation and vertical mixing of aerosols. Incoming Saharan dust layers are analyzed and effects of layer thinning, subsidence and turbulent downward transport become apparent, which are sensitive to atmospheric stability and wind shear. Comparisons of LES model output with lidar data systems are made to validate the modeling results.
M. Sicard, G. D'Amico, A. Comerón, L. Mona, L. Alados-Arboledas, A. Amodeo, H. Baars, J. M. Baldasano, L. Belegante, I. Binietoglou, J. A. Bravo-Aranda, A. J. Fernández, P. Fréville, D. García-Vizcaíno, A. Giunta, M. J. Granados-Muñoz, J. L. Guerrero-Rascado, D. Hadjimitsis, A. Haefele, M. Hervo, M. Iarlori, P. Kokkalis, D. Lange, R. E. Mamouri, I. Mattis, F. Molero, N. Montoux, A. Muñoz, C. Muñoz Porcar, F. Navas-Guzmán, D. Nicolae, A. Nisantzi, N. Papagiannopoulos, A. Papayannis, S. Pereira, J. Preißler, M. Pujadas, V. Rizi, F. Rocadenbosch, K. Sellegri, V. Simeonov, G. Tsaknakis, F. Wagner, and G. Pappalardo
Atmos. Meas. Tech., 8, 4587–4613, https://doi.org/10.5194/amt-8-4587-2015, https://doi.org/10.5194/amt-8-4587-2015, 2015
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In the framework of the ACTRIS summer 2012 measurement campaign (8 June–17 July 2012), EARLINET organized and performed a controlled exercise of feasibility to demonstrate its potential to perform operational, coordinated measurements and deliver products in near-real time. The paper describes the measurement protocol and discusses the delivery of real-time and near-real-time lidar-derived products.
S. Groß, V. Freudenthaler, K. Schepanski, C. Toledano, A. Schäfler, A. Ansmann, and B. Weinzierl
Atmos. Chem. Phys., 15, 11067–11080, https://doi.org/10.5194/acp-15-11067-2015, https://doi.org/10.5194/acp-15-11067-2015, 2015
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In June and July 2013 dual-wavelength lidar measurements were performed in Barbados to study long-range transported Saharan dust across the Atlantic Ocean and investigate transport-induced changes. The focus of our measurements is the intensive optical properties, the lidar ratio and the particle linear depolarization ratio. While the lidar ratio shows no differences compared to the values of fresh Saharan dust, the particle linear depolarization ratio shows slight differences.
J. Schmidt, A. Ansmann, J. Bühl, and U. Wandinger
Atmos. Chem. Phys., 15, 10687–10700, https://doi.org/10.5194/acp-15-10687-2015, https://doi.org/10.5194/acp-15-10687-2015, 2015
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M. Simmel, J. Bühl, A. Ansmann, and I. Tegen
Atmos. Chem. Phys., 15, 10453–10470, https://doi.org/10.5194/acp-15-10453-2015, https://doi.org/10.5194/acp-15-10453-2015, 2015
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The paper combines remote sensing observations and detailed cloud modeling. It was shown that the main features of the observations could be captured which allows one to perform sensitivity studies. Those show that the liquid phase is mainly determined by the dynamical parameters of the model, whereas the ice phase is dominated by microphysical parameters such as ice nuclei number and ice particle shape.
J. Bühl, R. Leinweber, U. Görsdorf, M. Radenz, A. Ansmann, and V. Lehmann
Atmos. Meas. Tech., 8, 3527–3536, https://doi.org/10.5194/amt-8-3527-2015, https://doi.org/10.5194/amt-8-3527-2015, 2015
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Case studies of combined vertical-velocity measurements of Doppler lidar, cloud radar and wind profiler are presented. The measurements were taken at the Meteorological Observatory, Lindenberg, Germany. Synergistic products are presented that are derived from the vertical-velocity measurements of the three instruments: a comprehensive classification mask of vertically moving atmospheric targets and the terminal fall velocity of water droplets and ice crystals corrected for vertical air motion.
M. Abdelkader, S. Metzger, R. E. Mamouri, M. Astitha, L. Barrie, Z. Levin, and J. Lelieveld
Atmos. Chem. Phys., 15, 9173–9189, https://doi.org/10.5194/acp-15-9173-2015, https://doi.org/10.5194/acp-15-9173-2015, 2015
V. Amiridis, E. Marinou, A. Tsekeri, U. Wandinger, A. Schwarz, E. Giannakaki, R. Mamouri, P. Kokkalis, I. Binietoglou, S. Solomos, T. Herekakis, S. Kazadzis, E. Gerasopoulos, E. Proestakis, M. Kottas, D. Balis, A. Papayannis, C. Kontoes, K. Kourtidis, N. Papagiannopoulos, L. Mona, G. Pappalardo, O. Le Rille, and A. Ansmann
Atmos. Chem. Phys., 15, 7127–7153, https://doi.org/10.5194/acp-15-7127-2015, https://doi.org/10.5194/acp-15-7127-2015, 2015
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LIVAS is a 3-D multi-wavelength global aerosol and cloud optical database optimized for future space-based lidar end-to-end simulations of realistic atmospheric scenarios as well as retrieval algorithm testing activities. The global database is based on CALIPSO observations at 532nm, while for the conversion at 355nm EARLINET data are utilized.
A. Nisantzi, R. E. Mamouri, A. Ansmann, G. L. Schuster, and D. G. Hadjimitsis
Atmos. Chem. Phys., 15, 7071–7084, https://doi.org/10.5194/acp-15-7071-2015, https://doi.org/10.5194/acp-15-7071-2015, 2015
V. Vakkari, E. J. O'Connor, A. Nisantzi, R. E. Mamouri, and D. G. Hadjimitsis
Atmos. Meas. Tech., 8, 1875–1885, https://doi.org/10.5194/amt-8-1875-2015, https://doi.org/10.5194/amt-8-1875-2015, 2015
R. E. Mamouri and A. Ansmann
Atmos. Chem. Phys., 15, 3463–3477, https://doi.org/10.5194/acp-15-3463-2015, https://doi.org/10.5194/acp-15-3463-2015, 2015
A. Nisantzi, R. E. Mamouri, A. Ansmann, and D. Hadjimitsis
Atmos. Chem. Phys., 14, 12155–12165, https://doi.org/10.5194/acp-14-12155-2014, https://doi.org/10.5194/acp-14-12155-2014, 2014
R. E. Mamouri and A. Ansmann
Atmos. Meas. Tech., 7, 3717–3735, https://doi.org/10.5194/amt-7-3717-2014, https://doi.org/10.5194/amt-7-3717-2014, 2014
G. Pappalardo, A. Amodeo, A. Apituley, A. Comeron, V. Freudenthaler, H. Linné, A. Ansmann, J. Bösenberg, G. D'Amico, I. Mattis, L. Mona, U. Wandinger, V. Amiridis, L. Alados-Arboledas, D. Nicolae, and M. Wiegner
Atmos. Meas. Tech., 7, 2389–2409, https://doi.org/10.5194/amt-7-2389-2014, https://doi.org/10.5194/amt-7-2389-2014, 2014
T. Kanitz, A. Ansmann, A. Foth, P. Seifert, U. Wandinger, R. Engelmann, H. Baars, D. Althausen, C. Casiccia, and F. Zamorano
Atmos. Meas. Tech., 7, 2061–2072, https://doi.org/10.5194/amt-7-2061-2014, https://doi.org/10.5194/amt-7-2061-2014, 2014
F. Dahlkötter, M. Gysel, D. Sauer, A. Minikin, R. Baumann, P. Seifert, A. Ansmann, M. Fromm, C. Voigt, and B. Weinzierl
Atmos. Chem. Phys., 14, 6111–6137, https://doi.org/10.5194/acp-14-6111-2014, https://doi.org/10.5194/acp-14-6111-2014, 2014
A. Skupin, A. Ansmann, R. Engelmann, H. Baars, and T. Müller
Atmos. Meas. Tech., 7, 701–712, https://doi.org/10.5194/amt-7-701-2014, https://doi.org/10.5194/amt-7-701-2014, 2014
A. Baklanov, K. Schlünzen, P. Suppan, J. Baldasano, D. Brunner, S. Aksoyoglu, G. Carmichael, J. Douros, J. Flemming, R. Forkel, S. Galmarini, M. Gauss, G. Grell, M. Hirtl, S. Joffre, O. Jorba, E. Kaas, M. Kaasik, G. Kallos, X. Kong, U. Korsholm, A. Kurganskiy, J. Kushta, U. Lohmann, A. Mahura, A. Manders-Groot, A. Maurizi, N. Moussiopoulos, S. T. Rao, N. Savage, C. Seigneur, R. S. Sokhi, E. Solazzo, S. Solomos, B. Sørensen, G. Tsegas, E. Vignati, B. Vogel, and Y. Zhang
Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, https://doi.org/10.5194/acp-14-317-2014, 2014
V. Amiridis, U. Wandinger, E. Marinou, E. Giannakaki, A. Tsekeri, S. Basart, S. Kazadzis, A. Gkikas, M. Taylor, J. Baldasano, and A. Ansmann
Atmos. Chem. Phys., 13, 12089–12106, https://doi.org/10.5194/acp-13-12089-2013, https://doi.org/10.5194/acp-13-12089-2013, 2013
U. S. Nair, Y. Wu, C. D. Holmes, A. Ter Schure, G. Kallos, and J. T. Walters
Atmos. Chem. Phys., 13, 10143–10157, https://doi.org/10.5194/acp-13-10143-2013, https://doi.org/10.5194/acp-13-10143-2013, 2013
J. Wagner, A. Ansmann, U. Wandinger, P. Seifert, A. Schwarz, M. Tesche, A. Chaikovsky, and O. Dubovik
Atmos. Meas. Tech., 6, 1707–1724, https://doi.org/10.5194/amt-6-1707-2013, https://doi.org/10.5194/amt-6-1707-2013, 2013
C. Spyrou, G. Kallos, C. Mitsakou, P. Athanasiadis, C. Kalogeri, and M. J. Iacono
Atmos. Chem. Phys., 13, 5489–5504, https://doi.org/10.5194/acp-13-5489-2013, https://doi.org/10.5194/acp-13-5489-2013, 2013
G. Pappalardo, L. Mona, G. D'Amico, U. Wandinger, M. Adam, A. Amodeo, A. Ansmann, A. Apituley, L. Alados Arboledas, D. Balis, A. Boselli, J. A. Bravo-Aranda, A. Chaikovsky, A. Comeron, J. Cuesta, F. De Tomasi, V. Freudenthaler, M. Gausa, E. Giannakaki, H. Giehl, A. Giunta, I. Grigorov, S. Groß, M. Haeffelin, A. Hiebsch, M. Iarlori, D. Lange, H. Linné, F. Madonna, I. Mattis, R.-E. Mamouri, M. A. P. McAuliffe, V. Mitev, F. Molero, F. Navas-Guzman, D. Nicolae, A. Papayannis, M. R. Perrone, C. Pietras, A. Pietruczuk, G. Pisani, J. Preißler, M. Pujadas, V. Rizi, A. A. Ruth, J. Schmidt, F. Schnell, P. Seifert, I. Serikov, M. Sicard, V. Simeonov, N. Spinelli, K. Stebel, M. Tesche, T. Trickl, X. Wang, F. Wagner, M. Wiegner, and K. M. Wilson
Atmos. Chem. Phys., 13, 4429–4450, https://doi.org/10.5194/acp-13-4429-2013, https://doi.org/10.5194/acp-13-4429-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The radiative impact of biomass burning aerosols on dust emissions over Namibia and the long-range transport of smoke observed during the Aerosols, Radiation and Clouds in southern Africa (AEROCLO-sA) campaign
Extending the wind profile beyond the surface layer by combining physical and machine learning approaches
Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories
Measurement report: Hygroscopicity of size-selected aerosol particles in the heavily polluted urban atmosphere of Delhi: impacts of chloride aerosol
An observation-constrained estimation of brown carbon aerosol direct radiative effects
The Puy de Dôme ICe Nucleation Intercomparison Campaign (PICNIC): comparison between online and offline methods in ambient air
Optical properties and simple forcing efficiency of the organic aerosols and black carbon emitted by residential wood burning in rural central Europe
Particle phase state and aerosol liquid water greatly impact secondary aerosol formation: insights into phase transition and its role in haze events
Measurement report: Nocturnal subsidence behind the cold front enhances surface particulate matter in plains regions: observations from the mobile multi-lidar system
Increase in precipitation scavenging contributes to long-term reductions of light-absorbing aerosol in the Arctic
Sea spray emissions from the Baltic Sea: comparison of aerosol eddy covariance fluxes and chamber-simulated sea spray emissions
Attribution of aerosol particle number size distributions to major sources using a 11-year-long urban dataset
Higher absorption enhancement of black carbon in summer shown by 2-year measurements at the high-altitude mountain site of Pic du Midi Observatory in the French Pyrenees
Variations of the atmospheric polycyclic aromatic hydrocarbon concentrations, sources, and health risk and the direct medical costs of lung cancer around the Bohai Sea against a background of pollution prevention and control in China
Introducing the novel concept of cumulative concentration roses for studying the transport of ultrafine particles from an airport to adjacent residential areas
Significant spatial gradients in new particle formation frequency in Greece during summer
Impact of desert dust on new particle formation events and the cloud condensation nuclei budget in dust-influenced areas
Active thermokarst regions contain rich sources of ice-nucleating particles
Examining the vertical heterogeneity of aerosols over the Southern Great Plains
Drivers controlling black carbon temporal variability in the lower troposphere of the European Arctic
Efficient droplet activation of ambient black carbon particles in sub-urban environment
Opinion: The strength of long-term comprehensive observations to meet multiple grand challenges in different environments and in the atmosphere
Contribution of fluorescent primary biological aerosol particles to low-level Arctic cloud residuals
Measurement report: Size-resolved mass concentration of equivalent black carbon-containing particles larger than 700 nm and their role in radiation
Aerosol absorption using in situ filter-based photometers and ground-based sun photometry in the Po Valley urban atmosphere
Aerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds
Aircraft ice-nucleating particle and aerosol composition measurements in the western North American Arctic
Mechanisms controlling giant sea salt aerosol size distributions along a tropical orographic coastline
New particle formation leads to enhanced cloud condensation nuclei concentrations on the Antarctic Peninsula
Mixing state and effective density of aerosol particles during the Beijing 2022 Olympic Winter Games
Tropospheric sulfate from Cumbre Vieja volcano at Las Palmas, transported towards Cabo Verde – lidar measurements of aerosol extinction, backscatter and depolarization at 355, 532 and 1064 nm
Measurement report: Shipborne observations of black carbon aerosols in the western Arctic Ocean during summer and autumn 2016–2020: boreal fire impacts
Quantified effect of seawater biogeochemistry on the temperature dependence of sea spray aerosol fluxes
Annual cycle of aerosol properties over the central Arctic during MOSAiC 2019–2020 – light-extinction, CCN, and INP levels from the boundary layer to the tropopause
3D assimilation and radiative impact assessment of aerosol black carbon over the Indian region using aircraft, balloon, ground-based, and multi-satellite observations
Measurement Report: A comparison of ice-nucleating particle and cloud condensation nuclei sources and properties during autumn at contrasting marine and terrestrial locations
Evaluation of aerosol- and gas-phase tracers for identification of transported biomass burning emissions in an industrially influenced location in Texas, USA
Physicochemical characterization and source apportionment of Arctic ice-nucleating particles observed in Ny-Ålesund in autumn 2019
Cyclones enhance the transport of sea spray aerosols to the high atmosphere in the Southern Ocean
Impact of 2020 COVID-19 lockdowns on particulate air pollution across Europe
New particle formation in the tropical free troposphere during CAMP2Ex: statistics and impact of emission sources, convective activity, and synoptic conditions
Explaining apparent particle shrinkage related to new particle formation events in western Saudi Arabia does not require evaporation
Investigation of the effects of the Greek extreme wildfires of August 2021 on air quality and spectral solar irradiance
Characterization of dust-related new particle formation events based on long-term measurement in the North China Plain
Airborne investigation of black carbon interaction with low-level, persistent, mixed-phase clouds in the Arctic summer
The variation in the particle number size distribution during the rainfall: wet scavenging and air mass changing
Opinion: New directions in atmospheric research offered by research infrastructures combined with open and data-intensive science
Characterization of size-segregated particles' turbulent flux and deposition velocity by eddy correlation method at an Arctic site
Vertical distribution of black carbon and its mixing state in the urban boundary layer in summer
Insights into the size-resolved dust emission from field measurements in the Moroccan Sahara
Cyrille Flamant, Jean-Pierre Chaboureau, Marco Gaetani, Kerstin Schepanski, and Paola Formenti
Atmos. Chem. Phys., 24, 4265–4288, https://doi.org/10.5194/acp-24-4265-2024, https://doi.org/10.5194/acp-24-4265-2024, 2024
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In the austral dry season, the atmospheric composition over southern Africa is dominated by biomass burning aerosols and terrigenous aerosols (so-called mineral dust). This study suggests that the radiative effect of biomass burning aerosols needs to be taken into account to properly forecast dust emissions in Namibia.
Boming Liu, Xin Ma, Jianping Guo, Renqiang Wen, Hui Li, Shikuan Jin, Yingying Ma, Xiaoran Guo, and Wei Gong
Atmos. Chem. Phys., 24, 4047–4063, https://doi.org/10.5194/acp-24-4047-2024, https://doi.org/10.5194/acp-24-4047-2024, 2024
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Accurate wind profile estimation, especially for the lowest few hundred meters of the atmosphere, is of great significance for the weather, climate, and renewable energy sector. We propose a novel method that combines the power-law method with the random forest algorithm to extend wind profiles beyond the surface layer. Compared with the traditional algorithm, this method has better stability and spatial applicability and can be used to obtain the wind profiles on different land cover types.
Gabriela R. Unfer, Luiz A. T. Machado, Paulo Artaxo, Marco A. Franco, Leslie A. Kremper, Mira L. Pöhlker, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 3869–3882, https://doi.org/10.5194/acp-24-3869-2024, https://doi.org/10.5194/acp-24-3869-2024, 2024
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Amazonian aerosols and their interactions with precipitation were studied by understanding them in a 3D space based on three parameters that characterize the concentration and size distribution of aerosols. The results showed characteristic arrangements regarding seasonal and diurnal cycles, as well as when interacting with precipitation. The use of this 3D space appears to be a promising tool for aerosol population analysis and for model validation and parameterization.
Anil Kumar Mandariya, Ajit Ahlawat, Mohammed Haneef, Nisar Ali Baig, Kanan Patel, Joshua Apte, Lea Hildebrandt Ruiz, Alfred Wiedensohler, and Gazala Habib
Atmos. Chem. Phys., 24, 3627–3647, https://doi.org/10.5194/acp-24-3627-2024, https://doi.org/10.5194/acp-24-3627-2024, 2024
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The current study explores the temporal variation of size-selected particle hygroscopicity in Delhi for the first time. Here, we report that the high volume fraction contribution of ammonium chloride to aerosol governs the high aerosol hygroscopicity and associated liquid water content based on the experimental data. The episodically high ammonium chloride present in Delhi's atmosphere could lead to haze and fog formation under high relative humidity in the region.
Yueyue Cheng, Chao Liu, Jiandong Wang, Jiaping Wang, Zhouyang Zhang, Li Chen, Dafeng Ge, Caijun Zhu, Jinbo Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 3065–3078, https://doi.org/10.5194/acp-24-3065-2024, https://doi.org/10.5194/acp-24-3065-2024, 2024
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Brown carbon (BrC), a light-absorbing aerosol, plays a pivotal role in influencing global climate. However, assessing BrC radiative effects remains challenging because the required observational data are hardly accessible. Here we develop a new BrC radiative effect estimation method combining conventional observations and numerical models. Our findings reveal that BrC absorbs up to a third of the sunlight at 370 nm that black carbon does, highlighting its importance in aerosol radiative effects.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
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Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Andrea Cuesta-Mosquera, Kristina Glojek, Griša Močnik, Luka Drinovec, Asta Gregorič, Martin Rigler, Matej Ogrin, Baseerat Romshoo, Kay Weinhold, Maik Merkel, Dominik van Pinxteren, Hartmut Herrmann, Alfred Wiedensohler, Mira Pöhlker, and Thomas Müller
Atmos. Chem. Phys., 24, 2583–2605, https://doi.org/10.5194/acp-24-2583-2024, https://doi.org/10.5194/acp-24-2583-2024, 2024
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This study evaluated the air pollution and climate impacts of residential-wood-burning particle emissions from a rural European site. The authors investigate the optical and physical properties that connect the aerosol emissions with climate by evaluating atmospheric radiative impacts via simple-forcing calculations. The study contributes to reducing the lack of information on the understanding of the optical properties of air pollution from anthropogenic sources.
Xiangxinyue Meng, Zhijun Wu, Jingchuan Chen, Yanting Qiu, Taomou Zong, Mijung Song, Jiyi Lee, and Min Hu
Atmos. Chem. Phys., 24, 2399–2414, https://doi.org/10.5194/acp-24-2399-2024, https://doi.org/10.5194/acp-24-2399-2024, 2024
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Our study revealed that particles predominantly exist in a semi-solid or solid state during clean winter days with RH below 30 %. However, a non-liquid to a liquid phase transition occurred when the aerosol liquid water (ALW) mass fraction surpassed 15 % (dry mass) at transition RH thresholds ranging from 40 % to 60 %. We also provide insights into the increasingly important roles of particle phase state variation and ALW in secondary particulate growth during haze formation in Beijing, China.
Yiming Wang, Haolin Wang, Yujie Qin, Xinqi Xu, Guowen He, Nanxi Liu, Shengjie Miao, Xiao Lu, Haichao Wang, and Shaojia Fan
Atmos. Chem. Phys., 24, 2267–2285, https://doi.org/10.5194/acp-24-2267-2024, https://doi.org/10.5194/acp-24-2267-2024, 2024
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We conducted a vertical measurement of winter PM2.5 using a mobile multi-lidar system in four cities. Combined with the surface PM2.5 data, the ERA5 reanalysis data, and GEOS-Chem simulations during Dec 2018–Feb 2019, we found that transport nocturnal PM2.5 enhancement by subsidence (T-NPES) events widely occurred with high frequencies in plains regions in eastern China but happened less often in basin regions like Xi’an and Chengdu. We propose a conceptual model of the T-NPES events.
Dominic Heslin-Rees, Peter Tunved, Johan Ström, Roxana Cremer, Paul Zieger, Ilona Riipinen, Annica M. L. Ekman, Konstantinos Eleftheriadis, and Radovan Krejci
Atmos. Chem. Phys., 24, 2059–2075, https://doi.org/10.5194/acp-24-2059-2024, https://doi.org/10.5194/acp-24-2059-2024, 2024
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Light-absorbing atmospheric particles (e.g. black carbon – BC) exert a warming effect on the Arctic climate. We show that the amount of particle light absorption decreased from 2002 to 2023. We conclude that in addition to reductions in emissions of BC, wet removal plays a role in the long-term reduction of BC in the Arctic, given the increase in surface precipitation experienced by air masses arriving at the site. The potential impact of biomass burning events is shown to have increased.
Julika Zinke, Ernst Douglas Nilsson, Piotr Markuszewski, Paul Zieger, Eva Monica Mårtensson, Anna Rutgersson, Erik Nilsson, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 1895–1918, https://doi.org/10.5194/acp-24-1895-2024, https://doi.org/10.5194/acp-24-1895-2024, 2024
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We conducted two research campaigns in the Baltic Sea, during which we combined laboratory sea spray simulation experiments with flux measurements on a nearby island. To combine these two methods, we scaled the laboratory measurements to the flux measurements using three different approaches. As a result, we derived a parameterization that is dependent on wind speed and wave state for particles with diameters 0.015–10 μm. This parameterization is applicable to low-salinity waters.
Máté Vörösmarty, Philip K. Hopke, and Imre Salma
EGUsphere, https://doi.org/10.5194/egusphere-2024-316, https://doi.org/10.5194/egusphere-2024-316, 2024
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The World Health Organization identified the ultrafine particles, which make up most of the particle number concentrations, as a potential risk factor for humans. The sources of particle numbers are very different from those of the particulate matter mass. We performed source apportionment of size segregated particle number concentrations over the diameter range of 6–1000 nm in Budapest for 11 full years. Six source types were identified, characterised, and quantified.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
Atmos. Chem. Phys., 24, 1801–1824, https://doi.org/10.5194/acp-24-1801-2024, https://doi.org/10.5194/acp-24-1801-2024, 2024
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At a French high-altitude site, where many complex interactions between black carbon (BC), radiation, clouds and snow impact climate, 2 years of refractive BC (rBC) and aerosol optical and microphysical measurements have been made. We observed strong seasonal rBC properties variations, with an enhanced absorption in summer compared to winter. The combination of rBC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the rBC light absorption seasonality.
Wenwen Ma, Rong Sun, Xiaoping Wang, Zheng Zong, Shizhen Zhao, Zeyu Sun, Chongguo Tian, Jianhui Tang, Song Cui, Jun Li, and Gan Zhang
Atmos. Chem. Phys., 24, 1509–1523, https://doi.org/10.5194/acp-24-1509-2024, https://doi.org/10.5194/acp-24-1509-2024, 2024
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This is the first report of long-term atmospheric PAH monitoring around the Bohai Sea. The results showed that the concentrations of PAHs in the atmosphere around the Bohai Sea decreased from June 2014 to May 2019, especially the concentrations of highly toxic PAHs. This indicates that the contributions from PAH sources changed to a certain extent in different areas, and it also led to reductions in the related health risk and medical costs following pollution prevention and control.
Julius Seidler, Markus N. Friedrich, Christoph K. Thomas, and Anke C. Nölscher
Atmos. Chem. Phys., 24, 137–153, https://doi.org/10.5194/acp-24-137-2024, https://doi.org/10.5194/acp-24-137-2024, 2024
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Here, we study the transport of ultrafine particles (UFPs) from an airport to two new adjacent measuring sites for 1 year. The number of UFPs in the air and the diurnal variation are typical urban. Winds from the airport show increased number concentrations. Additionally, considering wind frequencies, we estimate that, from all UFPs measured at the two sites, 10 %–14 % originate from the airport and/or other UFP sources from between the airport and site.
Andreas Aktypis, Christos Kaltsonoudis, David Patoulias, Panayiotis Kalkavouras, Angeliki Matrali, Christina N. Vasilakopoulou, Evangelia Kostenidou, Kalliopi Florou, Nikos Kalivitis, Aikaterini Bougiatioti, Konstantinos Eleftheriadis, Stergios Vratolis, Maria I. Gini, Athanasios Kouras, Constantini Samara, Mihalis Lazaridis, Sofia-Eirini Chatoutsidou, Nikolaos Mihalopoulos, and Spyros N. Pandis
Atmos. Chem. Phys., 24, 65–84, https://doi.org/10.5194/acp-24-65-2024, https://doi.org/10.5194/acp-24-65-2024, 2024
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Extensive continuous particle number size distribution measurements took place during two summers (2020 and 2021) at 11 sites in Greece for the investigation of the frequency and the spatial extent of new particle formation. The frequency during summer varied from close to zero in southwestern Greece to more than 60 % in the northern, central, and eastern regions. The spatial variability can be explained by the proximity of the sites to coal-fired power plants and agricultural areas.
Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Fernando Rejano, Andrea Casans, Gloria Titos, Francisco José Olmo, Lubna Dada, Simo Hakala, Tareq Hussein, Katrianne Lehtipalo, Pauli Paasonen, Antti Hyvärinen, Noemí Pérez, Xavier Querol, Sergio Rodríguez, Nikos Kalivitis, Yenny González, Mansour A. Alghamdi, Veli-Matti Kerminen, Andrés Alastuey, Tuukka Petäjä, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 23, 15795–15814, https://doi.org/10.5194/acp-23-15795-2023, https://doi.org/10.5194/acp-23-15795-2023, 2023
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Here we present the first study of the effect of mineral dust on the inhibition/promotion of new particle formation (NPF) events in different dust-influenced areas. Unexpectedly, we show that the occurrence of NPF events is highly frequent during mineral dust outbreaks, occurring even during extreme dust outbreaks. We also show that the occurrence of NPF events during mineral dust outbreaks significantly affects the potential cloud condensation nuclei budget.
Kevin R. Barry, Thomas C. J. Hill, Marina Nieto-Caballero, Thomas A. Douglas, Sonia M. Kreidenweis, Paul J. DeMott, and Jessie M. Creamean
Atmos. Chem. Phys., 23, 15783–15793, https://doi.org/10.5194/acp-23-15783-2023, https://doi.org/10.5194/acp-23-15783-2023, 2023
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Ice-nucleating particles (INPs) are important for the climate due to their influence on cloud properties. To understand potential land-based sources of them in the Arctic, we carried out a survey near the northernmost point of Alaska, a landscape connected to the permafrost (thermokarst). Permafrost contained high concentrations of INPs, with the largest values near the coast. The thermokarst lakes were found to emit INPs, and the water contained elevated concentrations.
Yang Wang, Chanakya Bagya Ramesh, Scott E. Giangrande, Jerome Fast, Xianda Gong, Jiaoshi Zhang, Ahmet Tolga Odabasi, Marcus Vinicius Batista Oliveira, Alyssa Matthews, Fan Mei, John E. Shilling, Jason Tomlinson, Die Wang, and Jian Wang
Atmos. Chem. Phys., 23, 15671–15691, https://doi.org/10.5194/acp-23-15671-2023, https://doi.org/10.5194/acp-23-15671-2023, 2023
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We report the vertical profiles of aerosol properties over the Southern Great Plains (SGP), a region influenced by shallow convective clouds, land–atmosphere interactions, boundary layer turbulence, and the aerosol life cycle. We examined the processes that drive the aerosol population and distribution in the lower troposphere over the SGP. This study helps improve our understanding of aerosol–cloud interactions and the model representation of aerosol processes.
Stefania Gilardoni, Dominic Heslin-Rees, Mauro Mazzola, Vito Vitale, Michael Sprenger, and Radovan Krejci
Atmos. Chem. Phys., 23, 15589–15607, https://doi.org/10.5194/acp-23-15589-2023, https://doi.org/10.5194/acp-23-15589-2023, 2023
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Models still fail in reproducing black carbon (BC) temporal variability in the Arctic. Analysis of equivalent BC concentrations in the European Arctic shows that BC seasonal variability is modulated by the efficiency of removal by precipitation during transport towards high latitudes. Short-term variability is controlled by synoptic-scale circulation patterns. The advection of warm air from lower latitudes is an effective pollution transport pathway during summer.
Ping Tian, Dantong Liu, Kang Hu, Yangzhou Wu, Mengyu Huang, Hui He, Jiujiang Sheng, Chenjie Yu, Dawei Hu, and Deping Ding
EGUsphere, https://doi.org/10.5194/egusphere-2023-2744, https://doi.org/10.5194/egusphere-2023-2744, 2023
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The results here thus provide direct evidence of efficient droplet activation of BC, and the CCN activation fraction of BC was higher than all-particle suggested the higher CCN activity of BC though its hygroscopicity is lower. Our research reveals that the evolution of BC's hygroscopicity and its CCN activation properties through atmospheric aging can be effectively characterized by the photochemical age.
Markku Kulmala, Anna Lintunen, Hanna Lappalainen, Annele Virtanen, Chao Yan, Ekaterina Ezhova, Tuomo Nieminen, Ilona Riipinen, Risto Makkonen, Johanna Tamminen, Anu-Maija Sundström, Antti Arola, Armin Hansel, Kari Lehtinen, Timo Vesala, Tuukka Petäjä, Jaana Bäck, Tom Kokkonen, and Veli-Matti Kerminen
Atmos. Chem. Phys., 23, 14949–14971, https://doi.org/10.5194/acp-23-14949-2023, https://doi.org/10.5194/acp-23-14949-2023, 2023
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To be able to meet global grand challenges, we need comprehensive open data with proper metadata. In this opinion paper, we describe the SMEAR (Station for Measuring Earth surface – Atmosphere Relations) concept and include several examples (cases), such as new particle formation and growth, feedback loops and the effect of COVID-19, and what has been learned from these investigations. The future needs and the potential of comprehensive observations of the environment are summarized.
Gabriel Pereira Freitas, Ben Kopec, Kouji Adachi, Radovan Krejci, Dominic Heslin-Rees, Karl Espen Yttri, Alun Hubbard, Jeffrey M. Welker, and Paul Zieger
EGUsphere, https://doi.org/10.5194/egusphere-2023-2600, https://doi.org/10.5194/egusphere-2023-2600, 2023
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Bioaerosols can participate in ice formation within clouds. In the Arctic, where global warming manifests most, they may become increasingly more important as their sources are prevailing for a longer period of the year. We have directly measured bioaerosols within clouds for a full year at an Arctic mountain site using a novel combination of cloud particle sampling and single-particle techniques. We show that bioaerosols act as cloud seeds and may influence the presence of ice within clouds.
Weilun Zhao, Ying Li, Gang Zhao, Song Guo, Nan Ma, Shuya Hu, and Chunsheng Zhao
Atmos. Chem. Phys., 23, 14889–14902, https://doi.org/10.5194/acp-23-14889-2023, https://doi.org/10.5194/acp-23-14889-2023, 2023
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Studies have concentrated on particles containing black carbon (BC) smaller than 700 nm because of technical limitations. In this study, BC-containing particles larger than 700 nm (BC>700) were measured, highlighting their importance to total BC mass and absorption. The contribution of BC>700 to the BC direct radiative effect was estimated, highlighting the necessity to consider the whole size range of BC-containing particles in the model estimation of BC radiative effects.
Alessandro Bigi, Giorgio Veratti, Elisabeth Andrews, Martine Collaud Coen, Lorenzo Guerrieri, Vera Bernardoni, Dario Massabò, Luca Ferrero, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 23, 14841–14869, https://doi.org/10.5194/acp-23-14841-2023, https://doi.org/10.5194/acp-23-14841-2023, 2023
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Atmospheric particles include compounds that play a key role in the greenhouse effect and air toxicity. Concurrent observations of these compounds by multiple instruments are presented, following deployment within an urban environment in the Po Valley, one of Europe's pollution hotspots. The study compares these data, highlighting the impact of ground emissions, mainly vehicular traffic and biomass burning, on the absorption of sun radiation and, ultimately, on climate change and air quality.
Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li, Wenche Aas, Chris Lunder, Radovan Krejci, Julie Thérèse Pasquier, Jan Henneberger, Robert Oscar David, Christoph Ritter, Claudia Mohr, Paul Zieger, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13941–13956, https://doi.org/10.5194/acp-23-13941-2023, https://doi.org/10.5194/acp-23-13941-2023, 2023
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Low-altitude clouds play a key role in regulating the climate of the Arctic, a region that suffers from climate change more than any other on the planet. We gathered meteorological and aerosol physical and chemical data over a year and utilized them for a parameterization that help us unravel the factors driving and limiting the efficiency of cloud droplet formation. We then linked this information to the sources of aerosol found during each season and to processes of cloud glaciation.
Alberto Sanchez-Marroquin, Sarah L. Barr, Ian T. Burke, James B. McQuaid, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 13819–13834, https://doi.org/10.5194/acp-23-13819-2023, https://doi.org/10.5194/acp-23-13819-2023, 2023
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The sources and concentrations of ice-nucleating particles (INPs) in the Arctic are still poorly understood. Here we report aircraft-based INP concentrations and aerosol composition in the western North American Arctic. The concentrations of INPs and all aerosol particles were low. The aerosol samples contained mostly sea salt and dust particles. Dust particles were more relevant for the INP concentrations than sea salt. However, dust alone cannot account for all of the measured INPs.
Katherine L. Ackerman, Alison D. Nugent, and Chung Taing
Atmos. Chem. Phys., 23, 13735–13753, https://doi.org/10.5194/acp-23-13735-2023, https://doi.org/10.5194/acp-23-13735-2023, 2023
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Sea salt aerosol is an important marine aerosol that may be produced in greater quantities in coastal regions than over the open ocean. This study observed these particles along the windward coastline of O'ahu, Hawai'i, to understand how wind and waves influence their production and dispersal. Overall, wave heights were the strongest variable correlated with changes in aerosol concentrations, while wind speeds played an important role in their horizontal dispersal and vertical mixing.
Jiyeon Park, Hyojin Kang, Yeontae Gim, Eunho Jang, Ki-Tae Park, Sangjong Park, Chang Hoon Jung, Darius Ceburnis, Colin O'Dowd, and Young Jun Yoon
Atmos. Chem. Phys., 23, 13625–13646, https://doi.org/10.5194/acp-23-13625-2023, https://doi.org/10.5194/acp-23-13625-2023, 2023
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We measured the number size distribution of 2.5–300 nm particles and cloud condensation nuclei (CCN) number concentrations at King Sejong Station on the Antarctic Peninsula continuously from 1 January to 31 December 2018. During the pristine and clean periods, 97 new particle formation (NPF) events were detected. For 83 of these, CCN concentrations increased by 2 %–268 % (median 44 %) following 1 to 36 h (median 8 h) after NPF events.
Aodong Du, Jiaxing Sun, Hang Liu, Weiqi Xu, Wei Zhou, Yuting Zhang, Lei Li, Xubing Du, Yan Li, Xiaole Pan, Zifa Wang, and Yele Sun
Atmos. Chem. Phys., 23, 13597–13611, https://doi.org/10.5194/acp-23-13597-2023, https://doi.org/10.5194/acp-23-13597-2023, 2023
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We characterized the impacts of emission controls on particle mixing state and density during the Beijing Olympic Winter Games using a SPAMS in tandem with a DMA and an AAC. OC and sulfate-containing particles increased, while those from primary emissions decreased. The effective particle densities increased and varied largely for different particles, highlighting the impacts of aging and formation processes on the changes of particle density and mixing state.
Henriette Gebauer, Athena Augusta Floutsi, Moritz Haarig, Martin Radenz, Ronny Engelmann, Dietrich Althausen, Annett Skupin, Albert Ansmann, Cordula Zenk, and Holger Baars
EGUsphere, https://doi.org/10.5194/egusphere-2023-2305, https://doi.org/10.5194/egusphere-2023-2305, 2023
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Sulfate aerosol from the volcanic eruption at Las Palmas in 2021 was observed over Cabo Verde. The impact of the eruption was observable even 1500 km away from the emission source and led to an extraordinary strong pollution in the lowermost atmosphere above Cabo Verde. We characterized the aerosol burden based on lidar and sun photometer observations. We compared the volcanic case to the typical background conditions (reference case) to quantify the volcanic pollution.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
EGUsphere, https://doi.org/10.5194/egusphere-2023-2315, https://doi.org/10.5194/egusphere-2023-2315, 2023
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Black carbon aerosols (BC) play important roles in Arctic climate change, yet they are not well understood because of limited observational facts. We observed BC mass concentrations (mBC) in the Western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high BC events in the Arctic Ocean.
Karine Sellegri, Theresa Barthelmeß, Jonathan Trueblood, Antonia Cristi, Evelyn Freney, Clémence Rose, Neill Barr, Mike Harvey, Karl Safi, Stacy Deppeler, Karen Thompson, Wayne Dillon, Anja Engel, and Cliff Law
Atmos. Chem. Phys., 23, 12949–12964, https://doi.org/10.5194/acp-23-12949-2023, https://doi.org/10.5194/acp-23-12949-2023, 2023
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The amount of sea spray emitted to the atmosphere depends on the ocean temperature, but this dependency is not well understood, especially when ocean biology is involved. In this study, we show that sea spray emissions are increased by up to a factor of 4 at low seawater temperatures compared to moderate temperatures, and we quantify the temperature dependence as a function of the ocean biogeochemistry.
Albert Ansmann, Kevin Ohneiser, Ronny Engelmann, Martin Radenz, Hannes Griesche, Julian Hofer, Dietrich Althausen, Jessie M. Creamean, Matthew C. Boyer, Daniel A. Knopf, Sandro Dahlke, Marion Maturilli, Henriette Gebauer, Johannes Bühl, Cristofer Jimenez, Patric Seifert, and Ulla Wandinger
Atmos. Chem. Phys., 23, 12821–12849, https://doi.org/10.5194/acp-23-12821-2023, https://doi.org/10.5194/acp-23-12821-2023, 2023
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The 1-year MOSAiC (2019–2020) expedition with the German ice breaker Polarstern was the largest polar field campaign ever conducted. The Polarstern, with our lidar aboard, drifted with the pack ice north of 85° N for more than 7 months (October 2019 to mid-May 2020). We measured the full annual cycle of aerosol conditions in terms of aerosol optical and cloud-process-relevant properties. We observed a strong contrast between polluted winter and clean summer aerosol conditions.
Nair Krishnan Kala, Narayana Sarma Anand, Mohanan R. Manoj, Srinivasan Prasanth, Harshavardhana S. Pathak, Thara Prabhakaran, Pramod D. Safai, Krishnaswamy K. Moorthy, and Sreedharan K. Satheesh
Atmos. Chem. Phys., 23, 12801–12819, https://doi.org/10.5194/acp-23-12801-2023, https://doi.org/10.5194/acp-23-12801-2023, 2023
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We present a 3D data set of aerosol black carbon over the Indian mainland by assimilating data from surface, aircraft, and balloon measurements, along with multi-satellite observations. Radiative transfer computations using height-resolved aerosol absorption show higher warming in the free troposphere and will have large implications for atmospheric stability. This data set will help reduce the uncertainty in aerosol radiative effects in climate model simulations over the Indian region.
Elise K. Wilbourn, Larissa Lacher, Carlos Guerrero, Hemanth S. K. Vepuri, Kristina Höhler, Jens Nadolny, Ottmar Möhler, and Naruki Hiranuma
EGUsphere, https://doi.org/10.5194/egusphere-2023-1456, https://doi.org/10.5194/egusphere-2023-1456, 2023
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Ambient ice and cloud particles were measured at terrestrial and temperate marine sites. Ice particles were more abundant in the former site while the fraction of ice particles relative to total ambient particles was higher in the latter site. We found continental and biogenic materials as a major source of ice particles in the terrestrial site. A positive correlation was found for ice and cloud particle concentrations in the marine site, implying they originate from the same source.
Sujan Shrestha, Shan Zhou, Manisha Mehra, Meghan Guagenti, Subin Yoon, Sergio L. Alvarez, Fangzhou Guo, Chun-Ying Chao, James H. Flynn III, Yuxuan Wang, Robert J. Griffin, Sascha Usenko, and Rebecca J. Sheesley
Atmos. Chem. Phys., 23, 10845–10867, https://doi.org/10.5194/acp-23-10845-2023, https://doi.org/10.5194/acp-23-10845-2023, 2023
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We evaluated different methods for assessing the influence of long-range transport of biomass burning (BB) plumes at a coastal site in Texas, USA. We show that the aerosol composition and optical properties exhibited good agreement, while CO and acetonitrile trends were less specific for assessing BB source influence. Our results demonstrate that the network of aerosol optical measurements can be useful for identifying the influence of aged BB plumes in anthropogenically influenced areas.
Guangyu Li, Elise K. Wilbourn, Zezhen Cheng, Jörg Wieder, Allison Fagerson, Jan Henneberger, Ghislain Motos, Rita Traversi, Sarah D. Brooks, Mauro Mazzola, Swarup China, Athanasios Nenes, Ulrike Lohmann, Naruki Hiranuma, and Zamin A. Kanji
Atmos. Chem. Phys., 23, 10489–10516, https://doi.org/10.5194/acp-23-10489-2023, https://doi.org/10.5194/acp-23-10489-2023, 2023
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In this work, we present results from an Arctic field campaign (NASCENT) in Ny-Ålesund, Svalbard, on the abundance, variability, physicochemical properties, and potential sources of ice-nucleating particles (INPs) relevant for mixed-phase cloud formation. This work improves the data coverage of Arctic INPs and aerosol properties, allowing for the validation of models predicting cloud microphysical and radiative properties of mixed-phase clouds in the rapidly warming Arctic.
Jun Shi, Jinpei Yan, Shanshan Wang, Shuhui Zhao, Miming Zhang, Suqing Xu, Qi Lin, Hang Yang, and Siying Dai
Atmos. Chem. Phys., 23, 10349–10359, https://doi.org/10.5194/acp-23-10349-2023, https://doi.org/10.5194/acp-23-10349-2023, 2023
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An underway aerosol-monitoring system was used to determine the Na+ concentration during different cyclone periods in the Southern Ocean in order to assess the potential effects of cyclones on sea spray aerosol (SSA) emissions. It was estimated that more than 23 % of SSAs were transported upwards during cyclone periods. Vertically transported SSAs can be regarded as an important source of CCN and hence have an effect on climate in the middle and high latitudes of the Southern Hemisphere.
Jean-Philippe Putaud, Enrico Pisoni, Alexander Mangold, Christoph Hueglin, Jean Sciare, Michael Pikridas, Chrysanthos Savvides, Jakub Ondracek, Saliou Mbengue, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Laurent Poulain, Dominik van Pinxteren, Hartmut Herrmann, Andreas Massling, Claus Nordstroem, Andrés Alastuey, Cristina Reche, Noemí Pérez, Sonia Castillo, Mar Sorribas, Jose Antonio Adame, Tuukka Petaja, Katrianne Lehtipalo, Jarkko Niemi, Véronique Riffault, Joel F. de Brito, Augustin Colette, Olivier Favez, Jean-Eudes Petit, Valérie Gros, Maria I. Gini, Stergios Vratolis, Konstantinos Eleftheriadis, Evangelia Diapouli, Hugo Denier van der Gon, Karl Espen Yttri, and Wenche Aas
Atmos. Chem. Phys., 23, 10145–10161, https://doi.org/10.5194/acp-23-10145-2023, https://doi.org/10.5194/acp-23-10145-2023, 2023
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Many European people are still exposed to levels of air pollution that can affect their health. COVID-19 lockdowns in 2020 were used to assess the impact of the reduction in human mobility on air pollution across Europe by comparing measurement data with values that would be expected if no lockdown had occurred. We show that lockdown measures did not lead to consistent decreases in the concentrations of fine particulate matter suspended in the air, and we investigate why.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Simo Hakala, Ville Vakkari, Heikki Lihavainen, Antti-Pekka Hyvärinen, Kimmo Neitola, Jenni Kontkanen, Veli-Matti Kerminen, Markku Kulmala, Tuukka Petäjä, Tareq Hussein, Mamdouh I. Khoder, Mansour A. Alghamdi, and Pauli Paasonen
Atmos. Chem. Phys., 23, 9287–9321, https://doi.org/10.5194/acp-23-9287-2023, https://doi.org/10.5194/acp-23-9287-2023, 2023
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Things are not always as they first seem in ambient aerosol measurements. Observations of decreasing particle sizes are often interpreted as resulting from particle evaporation. We show that such observations can counterintuitively be explained by particles that are constantly growing in size. This requires one to account for the previous movements of the observed air. Our explanation implies a larger number of larger particles, meaning more significant effects of aerosols on climate and health.
Akriti Masoom, Ilias Fountoulakis, Stelios Kazadzis, Ioannis-Panagiotis Raptis, Anna Kampouri, Basil E. Psiloglou, Dimitra Kouklaki, Kyriakoula Papachristopoulou, Eleni Marinou, Stavros Solomos, Anna Gialitaki, Dimitra Founda, Vasileios Salamalikis, Dimitris Kaskaoutis, Natalia Kouremeti, Nikolaos Mihalopoulos, Vassilis Amiridis, Andreas Kazantzidis, Alexandros Papayannis, Christos S. Zerefos, and Kostas Eleftheratos
Atmos. Chem. Phys., 23, 8487–8514, https://doi.org/10.5194/acp-23-8487-2023, https://doi.org/10.5194/acp-23-8487-2023, 2023
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We analyse the spatial and temporal aerosol spectral optical properties during the extreme wildfires of August 2021 in Greece and assess their effects on air quality and solar radiation quantities related to health, agriculture, and energy. Different aerosol conditions are identified (pure smoke, pure dust, dust–smoke together); the largest impact on solar radiation quantities is found for cases with mixed dust–smoke aerosols. Such situations are expected to occur more frequently in the future.
Xiaojing Shen, Junying Sun, Huizheng Che, Yangmei Zhang, Chunhong Zhou, Ke Gui, Wanyun Xu, Quan Liu, Junting Zhong, Can Xia, Xinyao Hu, Sinan Zhang, Jialing Wang, Shuo Liu, Jiayuan Lu, Aoyuan Yu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 8241–8257, https://doi.org/10.5194/acp-23-8241-2023, https://doi.org/10.5194/acp-23-8241-2023, 2023
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New particle formation (NPF) events occur when the dust episodes' fade is analysed based on long-term measurement of particle number size distribution. Analysis shows that the observed formation and growth rates are approximately 50 % of and 30 % lower than those of other NPF events. As a consequence of the uptake of precursor gases on mineral dust, the physical and chemical properties of submicron particles, as well as the ability to be cloud condensation nuclei, can be changed.
Marco Zanatta, Stephan Mertes, Olivier Jourdan, Regis Dupuy, Emma Järvinen, Martin Schnaiter, Oliver Eppers, Johannes Schneider, Zsófia Jurányi, and Andreas Herber
Atmos. Chem. Phys., 23, 7955–7973, https://doi.org/10.5194/acp-23-7955-2023, https://doi.org/10.5194/acp-23-7955-2023, 2023
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Black carbon (BC) particles influence the Arctic radiative balance. Vertical measurements of black carbon were conducted during the ACLOUD campaign in the European Arctic to study the interaction of BC with clouds. This study shows that clouds influence the vertical variability of BC properties across the inversion layer and that multiple activation and transformation mechanisms of BC may occur in the presence of low-level, persistent, mixed-phase clouds.
Guangdong Niu, Ximeng Qi, Liangduo Chen, Lian Xue, Shiyi Lai, Xin Huang, Jiaping Wang, Xuguang Chi, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 23, 7521–7534, https://doi.org/10.5194/acp-23-7521-2023, https://doi.org/10.5194/acp-23-7521-2023, 2023
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The reported below-cloud wet-scavenging coefficients (BWSCs) are much higher than theoretical data, but the reason remains unclear. Based on long-term observation, we find that air mass changing during rainfall events causes the overestimation of BWSCs. Thus, the discrepancy in BWSCs between observation and theory is not as large as currently believed. To obtain reasonable BWSCs and parameterizations from field observations, the effect of air mass changes needs to be considered.
Andreas Petzold, Ulrich Bundke, Anca Hienola, Paolo Laj, Cathrine Lund Myhre, Alex Vermeulen, Angeliki Adamaki, Werner Kutsch, Valerie Thouret, Damien Boulanger, Markus Fiebig, Markus Stocker, Zhiming Zhao, and Ari Asmi
EGUsphere, https://doi.org/10.5194/egusphere-2023-1423, https://doi.org/10.5194/egusphere-2023-1423, 2023
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The atmosphere-centred European environmental research infrastructures ACTRIS, IAGOS and ICOS can assume a leading role in atmospheric sciences thanks to their capacities for acquisition and reporting of long-term and high-quality observational data. We elaborate on the novel research opportunities which evolve from the combination of open access to data, data interoperability and tools and technologies offered by data-intensive science through the European Open Science Cloud.
Antonio Donateo, Gianluca Pappaccogli, Daniela Famulari, Mauro Mazzola, Federico Scoto, and Stefano Decesari
Atmos. Chem. Phys., 23, 7425–7445, https://doi.org/10.5194/acp-23-7425-2023, https://doi.org/10.5194/acp-23-7425-2023, 2023
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This work aims to measure the turbulent fluxes and the dry deposition velocity for size-segregated particles (from ultrafine to quasi-coarse range) at an Arctic site (Svalbard). Aiming to characterize the effect of surface properties on dry deposition, continuous observations were performed from the coldest months (on snow surface) to the snow melting period and throughout the summer (snow-free surface). A data fit of the deposition velocity as a function of particle diameters will be provided.
Hang Liu, Xiaole Pan, Shandong Lei, Yuting Zhang, Aodong Du, Weijie Yao, Guiqian Tang, Tao Wang, Jinyuan Xin, Jie Li, Yele Sun, Junji Cao, and Zifa Wang
Atmos. Chem. Phys., 23, 7225–7239, https://doi.org/10.5194/acp-23-7225-2023, https://doi.org/10.5194/acp-23-7225-2023, 2023
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We provide the average vertical profiles of black carbon (BC) concentration, size distribution and coating thickness at different times of the day in an urban area based on 112 vertical profiles. In addition, it is found that BC in the residual layer generally has a thicker coating, higher absorption enhancement and hygroscopicity than on the surface. Such aged BC could enter into the boundary layer and influence the BC properties in the early morning.
Cristina González-Flórez, Martina Klose, Andrés Alastuey, Sylvain Dupont, Jerónimo Escribano, Vicken Etyemezian, Adolfo Gonzalez-Romero, Yue Huang, Konrad Kandler, George Nikolich, Agnesh Panta, Xavier Querol, Cristina Reche, Jesús Yus-Díez, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 7177–7212, https://doi.org/10.5194/acp-23-7177-2023, https://doi.org/10.5194/acp-23-7177-2023, 2023
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Atmospheric mineral dust consists of tiny mineral particles that are emitted by wind erosion from arid regions. Its particle size distribution (PSD) affects its impact on the Earth's system. Nowadays, there is an incomplete understanding of the emitted dust PSD and a lot of debate about its variability. Here, we try to address these issues based on the measurements performed during a wind erosion and dust emission field campaign in the Moroccan Sahara within the framework of FRAGMENT project.
Cited articles
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Levy, R. C., Remer, L. A., Kleidman, R. G., Mattoo, S., Ichoku, C., Kahn, R., and Eck, T. F.: Global evaluation of the Collection 5 MODIS dark-target aerosol products over land, Atmos. Chem. Phys., 10, 10399–10420, https://doi.org/10.5194/acp-10-10399-2010, 2010.
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