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Volume 16, issue 19
Atmos. Chem. Phys., 16, 12551–12565, 2016
https://doi.org/10.5194/acp-16-12551-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: Regional transport and transformation of air pollution in...

Atmos. Chem. Phys., 16, 12551–12565, 2016
https://doi.org/10.5194/acp-16-12551-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 07 Oct 2016

Research article | 07 Oct 2016

Distribution and sources of air pollutants in the North China Plain based on on-road mobile measurements

Yi Zhu1, Jiping Zhang2, Junxia Wang1, Wenyuan Chen1, Yiqun Han1, Chunxiang Ye3, Yingruo Li1, Jun Liu1, Limin Zeng1, Yusheng Wu1, Xinfeng Wang4, Wenxing Wang4, Jianmin Chen4, and Tong Zhu1,5 Yi Zhu et al.
  • 1State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, 100871 Beijing, China
  • 2Institute of Atmospheric Physics, Chinese Academy of Sciences, 100029 Beijing, China
  • 3School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
  • 4Environment Research Institute, School of Environmental Science and Engineering, Shandong University, 250100 Ji'nan, China
  • 5The Beijing Innovation Center for Engineering Science and Advanced Technology, Peking University, Beijing, China

Abstract. The North China Plain (NCP) has been experiencing severe air pollution problems with rapid economic growth and urbanisation. Many field and model studies have examined the distribution of air pollutants in the NCP, but convincing results have not been achieved, mainly due to a lack of direct measurements of pollutants over large areas. Here, we employed a mobile laboratory to observe the main air pollutants in a large part of the NCP from 11 June to 15 July 2013. High median concentrations of sulfur dioxide (SO2) (12 ppb), nitrogen oxides (NOx) (NO + NO2; 452 ppb), carbon monoxide (CO) (956 ppb), black carbon (BC; 5.5 µg m−3) and ultrafine particles (28 350 cm−3) were measured. Most of the high values, i.e. 95 percentile concentrations, were distributed near large cities, suggesting the influence of local emissions. In addition, we analysed the regional transport of SO2 and CO, relatively long-lived pollutants, based on our mobile observations together with wind field and satellite data analyses. Our results suggested that, for border areas of the NCP, wind from outside this area would have a diluting effect on pollutants, while south winds would bring in pollutants that have accumulated during transport through other parts of the NCP. For the central NCP, the concentrations of pollutants were likely to remain at high levels, partly due to the influence of regional transport by prevalent south–north winds over the NCP and partly by local emissions.

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With five repeated experiments using a mobile laboratory, we obtained the spatial distribution of major air pollutants over the surface of the North China Plain (NCP). All the pollutants were at high levels, with pollutant peak values in nearby major cities and along transport routes. With simulated wind fields, we identified the prevalent transport routes of air pollutants on different parts of the NCP, reflecting the transport of air pollution between megacities and surrounding regions.
With five repeated experiments using a mobile laboratory, we obtained the spatial distribution...
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