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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 16, 1081-1104, 2016
https://doi.org/10.5194/acp-16-1081-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
01 Feb 2016
Size distribution and optical properties of mineral dust aerosols transported in the western Mediterranean
C. Denjean1,2, F. Cassola3, A. Mazzino3, S. Triquet1, S. Chevaillier1, N. Grand1, T. Bourrianne4, G. Momboisse4, K. Sellegri5, A. Schwarzenbock5, E. Freney5, M. Mallet6, and P. Formenti1 1Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR-CNRS 7583, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
2Leibniz Institute for Tropospheric Research (TROPOS), Permoserstraße 15, Leipzig, Germany
3Department of Physics and INFN, Genoa, Italy
4Centre National de Recherches Météorologiques (CNRM), Météo-France, Toulouse, France
5Laboratoire de Météorologie Physique (LaMP), CNRS/Université Blaise Pascal, Clermont-Ferrand, France
6Laboratoire d'Aérologie (LA), Université de Toulouse, CNRS, Toulouse, France
Abstract. This study presents in situ aircraft measurements of Saharan mineral dust transported over the western Mediterranean basin in June–July 2013 during the ChArMEx/ADRIMED (the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region) airborne campaign. Dust events differing in terms of source region (Algeria, Tunisia and Morocco), time of transport (1–5 days) and height of transport were sampled. Mineral dust were transported above the marine boundary layer, which conversely was dominated by pollution and marine aerosols. The dust vertical structure was extremely variable and characterized by either a single layer or a more complex and stratified structure with layers originating from different source regions. Mixing of mineral dust with pollution particles was observed depending on the height of transport of the dust layers. Dust layers carried a higher concentration of pollution particles below 3 km above sea level (a.s.l.) than above 3 km a.s.l., resulting in a scattering Ångström exponent up to 2.2 below 3 km a.s.l. However, the optical properties of the dust plumes remained practically unchanged with respect to values previously measured over source regions, regardless of the altitude. Moderate absorption of light by the dust plumes was observed with values of aerosol single scattering albedo at 530 nm ranging from 0.90 to 1.00. Concurrent calculations from the aerosol chemical composition revealed a negligible contribution of pollution particles to the absorption properties of the dust plumes that was due to a low contribution of refractory black carbon in regards to the fraction of dust and sulfate particles. This suggests that, even in the presence of moderate pollution, likely a persistent feature in the Mediterranean, the optical properties of the dust plumes could be assumed similar to those of native dust in radiative transfer simulations, modelling studies and satellite retrievals over the Mediterranean. Measurements also showed that the coarse mode of mineral dust was conserved even after 5 days of transport in the Mediterranean, which contrasts with the gravitational depletion of large particles observed during the transport of dust plumes over the Atlantic. Simulations with the WRF mesoscale meteorological model highlighted a strong vertical turbulence within the dust layers that could prevent deposition of large particles during their atmospheric transport. This has important implications for the dust radiative effects due to surface dimming, atmospheric heating and cloud formation. The results presented here add to the observational data set necessary for evaluating the role of mineral dust on the regional climate and rainfall patterns in the western Mediterranean basin and understanding their atmospheric transport at global scale.

Citation: Denjean, C., Cassola, F., Mazzino, A., Triquet, S., Chevaillier, S., Grand, N., Bourrianne, T., Momboisse, G., Sellegri, K., Schwarzenbock, A., Freney, E., Mallet, M., and Formenti, P.: Size distribution and optical properties of mineral dust aerosols transported in the western Mediterranean, Atmos. Chem. Phys., 16, 1081-1104, https://doi.org/10.5194/acp-16-1081-2016, 2016.
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Short summary
This study investigates the size distribution, chemical composition, and optical properties of Saharan mineral dust transported over the western Mediterranean using in situ measurements collected from aircraft. Their variability due to altitude, time of transport, and mixing rate with pollution particles are discussed. We found moderate light absorption of the dust plumes even in the presence of pollution particles and the persistence of large dust particles after transport in the Mediterranean.
This study investigates the size distribution, chemical composition, and optical properties of...
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