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Volume 16, issue 16
Atmos. Chem. Phys., 16, 10501–10519, 2016
https://doi.org/10.5194/acp-16-10501-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 10501–10519, 2016
https://doi.org/10.5194/acp-16-10501-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 22 Aug 2016

Research article | 22 Aug 2016

Satellite observations of stratospheric hydrogen fluoride and comparisons with SLIMCAT calculations

Jeremy J. Harrison et al.
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Boone, C. D., Walker, K. A., and Bernath, P. F.: Version 3 Retrievals for the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS), in: The Atmospheric Chemistry Experiment ACE at 10: A Solar Occultation Anthology, edited by: Bernath, P. F., A. Deepak Publishing, Hampton, Virginia, USA, 103–127, available at: http://www.ace.uwaterloo.ca/publications/2013/Version3.5retreivals2013.pdf (last access: 16 August 2016), 2013.
Brown, A. T., Chipperfield, M. P., Boone, C., Wilson, C., Walker, K. A., and Bernath, P. F.: Trends in atmospheric halogen containing gases since 2004, J. Quant. Spectrosc. Ra., 112, 2552–2566, 2011.
Brown, A. T., Chipperfield, M. P., Richards, N. A. D., Boone, C., and Bernath, P. F.: Global stratospheric fluorine inventory for 2004–2009 from Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) measurements and SLIMCAT model simulations, Atmos. Chem. Phys., 14, 267–282, https://doi.org/10.5194/acp-14-267-2014, 2014.
Chipperfield, M. P.: Multiannual simulations with a three-dimensional chemical transport model, J. Geophys. Res., 104, 1781–1805, https://doi.org/10.1029/98jd02597, 1999.
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HF, the dominant stratospheric fluorine reservoir, results from the atmospheric degradation of anthropogenic species such as CFCs, HCFCs, and HFCs. All are strong greenhouse gases, and CFCs and HCFCs deplete stratospheric ozone. We report the comparison of HF global distributions and trends measured by the ACE-FTS and HALOE satellite instruments with the output of SLIMCAT, a chemical transport model. The global HF trends reveal a slowing down in the rate of increase of HF since the 1990s.
HF, the dominant stratospheric fluorine reservoir, results from the atmospheric degradation of...
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