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Volume 16, issue 16 | Copyright
Atmos. Chem. Phys., 16, 10489-10500, 2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 22 Aug 2016

Research article | 22 Aug 2016

Tropospheric ozone variability during the East Asian summer monsoon as observed by satellite (IASI), aircraft (MOZAIC) and ground stations

Sarah Safieddine1,a, Anne Boynard1, Nan Hao2, Fuxiang Huang3, Lili Wang4, Dongsheng Ji4, Brice Barret5, Sachin D. Ghude6, Pierre-François Coheur7, Daniel Hurtmans7, and Cathy Clerbaux1,7 Sarah Safieddine et al.
  • 1Sorbonne Universités, UPMC Univ. Paris 06, Université Versailles St-Quentin, CNRS/INSU, LATMOS-IPSL, Paris, France
  • 2German Aerospace Center (DLR), Remote Sensing Technology Institute (IMF), Oberpfaffenhofen, Germany
  • 3National Satellite Meteorological Center, China Meteorological Administration, Beijing, China
  • 4LAPC, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, China
  • 5Laboratoire d'Aérologie, Observatoire Midi-Pyrénées, Université Paul Sabatier, CNRS, Toulouse, France
  • 6Indian Institute of Tropical Meteorology, Pashan Rd., Pune-411 008, India
  • 7Spectroscopie de l'Atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles (U.L.B.), Brussels, Belgium
  • anow at: Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA

Abstract. Satellite measurements from the thermal Infrared Atmospheric Sounding Interferometer (IASI), aircraft data from the MOZAIC/IAGOS project, as well as observations from ground-based stations, are used to assess the tropospheric ozone (O3) variability during the East Asian Summer Monsoon (EASM). Six years 2008–2013 of IASI data analysis reveals the ability of the instrument to detect the onset and the progression of the monsoon seen by a decrease in the tropospheric 0–6km O3 column due to the EASM, and to reproduce this decrease from one year to the other. The year-to-year variability is found to be mainly dependent on meteorology. Focusing on the period of May-August 2011, taken as an example year, IASI data show clear inverse relationship between tropospheric 0–6km O3 on one hand and meteorological parameters such as cloud cover, relative humidity and wind speed, on the other hand. Aircraft data from the MOZAIC/IAGOS project for the EASM of 2008–2013 are used to validate the IASI data and to assess the effect of the monsoon on the vertical distribution of the tropospheric O3 at different locations. Results show good agreement with a correlation coefficient of 0.73 (12%) between the 0–6km O3 column derived from IASI and aircraft data. IASI captures very well the inter-annual variation of tropospheric O3 observed by the aircraft data over the studied domain. Analysis of vertical profiles of the aircraft data shows a decrease in the tropospheric O3 that is more important in the free troposphere than in the boundary layer and at 10–20°N than elsewhere. Ground station data at different locations in India and China show a spatiotemporal dependence on meteorology during the monsoon, with a decrease up to 22ppbv in Hyderabad, and up to 5ppbv in the North China Plain.

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The Asian Summer Monsoon has implication on the weather and climate system as well as pollutants concentration over the monsoon regions leading to effects on the global air quality. Our results, combining satellite, aircraft and ground station data, show that tropospheric ozone, decrease during the period May–August over East and South Asia due to the Monsoon. The magnitude of this drop depends largely on meteorology and geographic location.
The Asian Summer Monsoon has implication on the weather and climate system as well as pollutants...