Articles | Volume 16, issue 15
https://doi.org/10.5194/acp-16-10299-2016
https://doi.org/10.5194/acp-16-10299-2016
Research article
 | 
15 Aug 2016
Research article |  | 15 Aug 2016

Uptake of gaseous formaldehyde by soil surfaces: a combination of adsorption/desorption equilibrium and chemical reactions

Guo Li, Hang Su, Xin Li, Uwe Kuhn, Hannah Meusel, Thorsten Hoffmann, Markus Ammann, Ulrich Pöschl, Min Shao, and Yafang Cheng

Related authors

Measurement Report: Wintertime new particle formation in the rural area of the North China Plain – influencing factors and possible formation mechanism
Juan Hong, Min Tang, Qiaoqiao Wang, Nan Ma, Shaowen Zhu, Shaobin Zhang, Xihao Pan, Linhong Xie, Guo Li, Uwe Kuhn, Chao Yan, Jiangchuan Tao, Ye Kuang, Yao He, Wanyun Xu, Runlong Cai, Yaqing Zhou, Zhibin Wang, Guangsheng Zhou, Bin Yuan, Yafang Cheng, and Hang Su
Atmos. Chem. Phys., 23, 5699–5713, https://doi.org/10.5194/acp-23-5699-2023,https://doi.org/10.5194/acp-23-5699-2023, 2023
Short summary
Reactive uptake coefficients for multiphase reactions determined by a dynamic chamber system
Guo Li, Hang Su, Meng Li, Uwe Kuhn, Guangjie Zheng, Lei Han, Fengxia Bao, Ulrich Pöschl, and Yafang Cheng
Atmos. Meas. Tech., 15, 6433–6446, https://doi.org/10.5194/amt-15-6433-2022,https://doi.org/10.5194/amt-15-6433-2022, 2022
Short summary
Bimodal distribution of size-resolved particle effective density: results from a short campaign in a rural environment over the North China Plain
Yaqing Zhou, Nan Ma, Qiaoqiao Wang, Zhibin Wang, Chunrong Chen, Jiangchuan Tao, Juan Hong, Long Peng, Yao He, Linhong Xie, Shaowen Zhu, Yuxuan Zhang, Guo Li, Wanyun Xu, Peng Cheng, Uwe Kuhn, Guangsheng Zhou​​​​​​​, Pingqing Fu, Qiang Zhang, Hang Su, and Yafang Cheng
Atmos. Chem. Phys., 22, 2029–2047, https://doi.org/10.5194/acp-22-2029-2022,https://doi.org/10.5194/acp-22-2029-2022, 2022
Short summary
Reactive nitrogen around the Arabian Peninsula and in the Mediterranean Sea during the 2017 AQABA ship campaign
Nils Friedrich, Philipp Eger, Justin Shenolikar, Nicolas Sobanski, Jan Schuladen, Dirk Dienhart, Bettina Hottmann, Ivan Tadic, Horst Fischer, Monica Martinez, Roland Rohloff, Sebastian Tauer, Hartwig Harder, Eva Y. Pfannerstill, Nijing Wang, Jonathan Williams, James Brooks, Frank Drewnick, Hang Su, Guo Li, Yafang Cheng, Jos Lelieveld, and John N. Crowley
Atmos. Chem. Phys., 21, 7473–7498, https://doi.org/10.5194/acp-21-7473-2021,https://doi.org/10.5194/acp-21-7473-2021, 2021
Short summary
Multifactor colorimetric analysis on pH-indicator papers: an optimized approach for direct determination of ambient aerosol pH
Guo Li, Hang Su, Nan Ma, Guangjie Zheng, Uwe Kuhn, Meng Li, Thomas Klimach, Ulrich Pöschl, and Yafang Cheng
Atmos. Meas. Tech., 13, 6053–6065, https://doi.org/10.5194/amt-13-6053-2020,https://doi.org/10.5194/amt-13-6053-2020, 2020
Short summary

Related subject area

Subject: Gases | Research Activity: Laboratory Studies | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Extension, development, and evaluation of the representation of the OH-initiated dimethyl sulfide (DMS) oxidation mechanism in the Master Chemical Mechanism (MCM) v3.3.1 framework
Lorrie Simone Denise Jacob, Chiara Giorio, and Alexander Thomas Archibald
Atmos. Chem. Phys., 24, 3329–3347, https://doi.org/10.5194/acp-24-3329-2024,https://doi.org/10.5194/acp-24-3329-2024, 2024
Short summary
On the potential use of highly oxygenated organic molecules (HOMs) as indicators for ozone formation sensitivity
Jiangyi Zhang, Jian Zhao, Yuanyuan Luo, Valter Mickwitz, Douglas Worsnop, and Mikael Ehn
Atmos. Chem. Phys., 24, 2885–2911, https://doi.org/10.5194/acp-24-2885-2024,https://doi.org/10.5194/acp-24-2885-2024, 2024
Short summary
Oxygenated organic molecules produced by low-NOx photooxidation of aromatic compounds: contributions to secondary organic aerosol and steric hindrance
Xi Cheng, Yong Jie Li, Yan Zheng, Keren Liao, Theodore K. Koenig, Yanli Ge, Tong Zhu, Chunxiang Ye, Xinghua Qiu, and Qi Chen
Atmos. Chem. Phys., 24, 2099–2112, https://doi.org/10.5194/acp-24-2099-2024,https://doi.org/10.5194/acp-24-2099-2024, 2024
Short summary
Impact of temperature on the role of Criegee intermediates and peroxy radicals in dimer formation from β-pinene ozonolysis
Yiwei Gong, Feng Jiang, Yanxia Li, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 167–184, https://doi.org/10.5194/acp-24-167-2024,https://doi.org/10.5194/acp-24-167-2024, 2024
Short summary
Atmospheric impact of 2-methylpentanal emissions: kinetics, photochemistry, and formation of secondary pollutants
María Asensio, Sergio Blázquez, María Antiñolo, José Albaladejo, and Elena Jiménez
Atmos. Chem. Phys., 23, 14115–14126, https://doi.org/10.5194/acp-23-14115-2023,https://doi.org/10.5194/acp-23-14115-2023, 2023
Short summary

Cited articles

Andreae, M. O. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Global Biogeochem. Cy., 15, 955–966, 2001.
Ayers, G. P., Gillett, R. W., Granek, H., deServes, C., and Cox, R. A.: Formaldehyde production in clean marine air, Geophys. Res. Lett., 24, 401–404, 1997.
Batterman, S., Padmanabham, I., and Milne, P.: Effective gas-phase diffusion coefficients in soils at varying water content measured using a one-flow sorbent based technique, Environ. Sci. Technol., 30, 770–778, 1996.
Behnke, W., George, C., Scheer, V., and Zetzsch, C.: Production and decay of ClNO2, from the reaction of gaseous N2O5 with NaCl solution: Bulk and aerosol experiments, J. Geophys. Res.-Atmos., 102, 3795–3804, 1997.
Brunauer, S., Emmett, P. H., and Teller, E.: Adsorption of Gases in Multimolecular Layers, J. Am. Chem. Soc., 60, 309–319, https://doi.org/10.1021/ja01269a023, 1938.
Download
Short summary
Indoor and outdoor formaldehyde (HCHO) are both of considerable concern because of its health effects and its role in atmospheric chemistry. The heterogeneous reactions between gaseous HCHO with soils can pose important impact on both HCHO budget and soil ecosystem. Our results confirms that HCHO uptake by soil is a complex process involving both adsorption/desorption and chemical reactions. Soil and soil-derived airborne particles can either act as a source or a sink for HCHO.
Altmetrics
Final-revised paper
Preprint