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Volume 16, issue 15
Atmos. Chem. Phys., 16, 10241-10261, 2016
https://doi.org/10.5194/acp-16-10241-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 10241-10261, 2016
https://doi.org/10.5194/acp-16-10241-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 12 Aug 2016

Research article | 12 Aug 2016

Atmospheric salt deposition in a tropical mountain rainforest at the eastern Andean slopes of south Ecuador – Pacific or Atlantic origin?

Sandro Makowski Giannoni1, Katja Trachte1, Ruetger Rollenbeck1, Lukas Lehnert1, Julia Fuchs2, and Joerg Bendix1 Sandro Makowski Giannoni et al.
  • 1Laboratory for Climatology and Remote Sensing (LCRS), Institute of Physical Geography, Department of Geography, Philipps-Universitaet, Marburg, Germany
  • 2Laboratory of Climatology, Institute of Physical Geography, Department of Geography, Ruhr-Universitaet, Bochum, Germany

Abstract. Sea salt (NaCl) has recently been proven to be of the utmost importance for ecosystem functioning in Amazon lowland forests because of its impact on herbivory, litter decomposition and, thus, carbon cycling. Sea salt deposition should generally decline as distance from its marine source increases. For the Amazon, a negative east–west gradient of sea salt availability is assumed as a consequence of the barrier effect of the Andes Mountains for Pacific air masses. However, this generalized pattern may not hold for the tropical mountain rainforest in the Andes of southern Ecuador. To analyse sea salt availability, we investigated the deposition of sodium (Na+) and chloride (Cl), which are good proxies of sea spray aerosol. Because of the complexity of the terrain and related cloud and rain formation processes, sea salt deposition was analysed from both, rain and occult precipitation (OP) along an altitudinal gradient over a period between 2004 and 2009. To assess the influence of easterly and westerly air masses on the deposition of sodium and chloride over southern Ecuador, sea salt aerosol concentration data from the Monitoring Atmospheric Composition and Climate (MACC) reanalysis data set and back-trajectory statistical methods were combined. Our results, based on deposition time series, show a clear difference in the temporal variation of sodium and chloride concentration and Na+Cl ratio in relation to height and exposure to winds. At higher elevations, sodium and chloride present a higher seasonality and the Na+Cl ratio is closer to that of sea salt. Medium- to long-range sea salt transport exhibited a similar seasonality, which shows the link between our measurements at high elevations and the sea salt synoptic transport. Although the influence of the easterlies was predominant regarding the atmospheric circulation, the statistical analysis of trajectories and hybrid receptor models revealed a stronger impact of the north equatorial Atlantic, Caribbean, and Pacific sea salt sources on the atmospheric sea salt concentration in southern Ecuador. The highest concentration in rain and cloud water was found between September and February when air masses originated from the north equatorial Atlantic, the Caribbean Sea and the equatorial Pacific. Together, these sources accounted for around 82.4% of the sea salt budget over southern Ecuador.

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We have analysed the atmospheric deposition of sodium and chloride and its emission sources in a tropical mountain forest characterized by a very complex terrain in the south of Ecuador. We found that, given the special location of the study area in a topographic depression in the Andes and thanks to the seasonal shifts in the atmospheric synoptic circulation, the contribution of additional sea salt sources might in part alleviate the scarcity of salt seen in other forests in the western Amazon.
We have analysed the atmospheric deposition of sodium and chloride and its emission sources in a...
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