Articles | Volume 15, issue 14
https://doi.org/10.5194/acp-15-7819-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-7819-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
16 Jul 2015
Research article |
| 16 Jul 2015
Changing shapes and implied viscosities of suspended submicron particles
Y. Zhang
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
M. S. Sanchez
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Department of Chemical Engineering, University of São Paulo, São Paulo, Brazil
C. Douet
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Department of Energy and Environment, National Institute of Applied Science of Lyon, Villeurbanne, France
Y. Wang
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
School of Public Health, Harvard University, Boston, Massachusetts, USA
A. P. Bateman
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Z. Gong
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
M. Kuwata
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Earth Observatory of Singapore, School of Physical and Mathematical Sciences, College of Sciences, Nanyang Technological University, Singapore, Singapore
L. Renbaum-Wolff
Department of Chemistry, University of British Columbia, Vancouver, British Columbia, Canada
B. B. Sato
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Department of Chemical Engineering, Federal University of Sao Carlos, Sao Carlos, São Paulo, Brazil
P. F. Liu
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
A. K. Bertram
Department of Chemistry, University of British Columbia, Vancouver, British Columbia, Canada
F. M. Geiger
CORRESPONDING AUTHOR
Department of Chemistry, Northwestern University, Evanston, Illinois, USA
S. T. Martin
CORRESPONDING AUTHOR
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA
Department of Earth and Planetary Sciences, Harvard University, Cambridge, Massachusetts, USA
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- Influence of relative humidity on cyclohexene SOA formation from OH photooxidation S. Liu et al. 10.1016/j.chemosphere.2019.05.131
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- Profiling Aerosol Liquid Water Content Using a Polarization Lidar W. Tan et al. 10.1021/acs.est.9b07502
- Viscosity and phase state of aerosol particles consisting of sucrose mixed with inorganic salts Y. Song et al. 10.5194/acp-21-10215-2021
- Multiphase chemistry in the troposphere: It all starts … and ends … with gases B. Finlayson‐Pitts 10.1002/kin.21305
- Influence of Functional Groups on the Viscosity of Organic Aerosol N. Rothfuss & M. Petters 10.1021/acs.est.6b04478
- Models for the bead mobility technique: A droplet-based viscometer M. Sellier et al. 10.1080/02786826.2019.1599320
- Viscous organic aerosol particles in the upper troposphere: diffusivity-controlled water uptake and ice nucleation? D. Lienhard et al. 10.5194/acp-15-13599-2015
- Diffusion of Organic Molecules as a Function of Temperature in a Sucrose Matrix (a Proxy for Secondary Organic Aerosol) K. Kiland et al. 10.1021/acs.jpclett.9b02182
- Substrate colonization by an emulsion drop prior to spreading S. Borkar & A. Ramachandran 10.1038/s41467-021-26015-2
- The secondary formation of organosulfates under interactions between biogenic emissions and anthropogenic pollutants in summer in Beijing Y. Wang et al. 10.5194/acp-18-10693-2018
- Challenges and Opportunities in Molecular-Level Indoor Surface Chemistry and Physics Y. Liu et al. 10.1016/j.xcrp.2020.100256
- Predicting the influence of particle size on the glass transition temperature and viscosity of secondary organic material M. Petters & S. Kasparoglu 10.1038/s41598-020-71490-0
- Humidity Dependence of the Condensational Growth of α-Pinene Secondary Organic Aerosol Particles Y. Qin et al. 10.1021/acs.est.1c01738
- Factors controlling the evaporation of secondary organic aerosol from α‐pinene ozonolysis T. Yli‐Juuti et al. 10.1002/2016GL072364
- Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter P. Liu et al. 10.1021/acscentsci.7b00452
- The viscosity of atmospherically relevant organic particles J. Reid et al. 10.1038/s41467-018-03027-z
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Short summary
The present work estimates the viscosity of submicron organic particles while they are still suspended as an aerosol without further post-processing techniques that can possibly alter the properties of semi-volatile materials. Results imply that atmospheric particles, at least those similar to the ones of this study and for low- to middle-RH regimes, can reach equilibrium or react rather slowly with the surrounding gas phase on time scales even longer than the residence time in the atmosphere.
The present work estimates the viscosity of submicron organic particles while they are still...
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