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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 15, issue 12
Atmos. Chem. Phys., 15, 6745–6765, 2015
https://doi.org/10.5194/acp-15-6745-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: The Pan European Gas-Aerosols Climate Interaction Study...

Atmos. Chem. Phys., 15, 6745–6765, 2015
https://doi.org/10.5194/acp-15-6745-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 18 Jun 2015

Research article | 18 Jun 2015

Formation of highly oxidized multifunctional compounds: autoxidation of peroxy radicals formed in the ozonolysis of alkenes – deduced from structure–product relationships

T. F. Mentel et al.

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AR by Thomas Mentel on behalf of the Authors (08 May 2015)  Author's response    Manuscript
ED: Publish subject to technical corrections (23 May 2015) by Urs Baltensperger
AR by Thomas Mentel on behalf of the Authors (26 May 2015)  Author's response    Manuscript
Publications Copernicus
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Short summary
We studied a series of cycloalkenes and methyl-substituted alkenes in order to elucidate the structural pre-requisites and chemical pathways to the recently discovered class of highly oxidized molecules ELVOC (Ehn et al., Nature, 2014). ELVOC may totally change the view on (parts of) the mechanism of SOA formation. We present results which support recent observations of H shifts from C-H to peroxy radicals, highlighting the pivotal role of peroxyradicals in organic atmospheric chemistry.
We studied a series of cycloalkenes and methyl-substituted alkenes in order to elucidate the...
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